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Coupled Ferroelectricity and Correlated States in a Twisted Quadrilayer MoS_(2) Moiré Superlattice

Chinese Physics Letters 2023年第4期40卷 68-73页

作者：吴帆帆李璐徐巧玲刘乐袁亚龙赵交交黄智恒昝晓洲 Kenji Watanabe takashi taniguchi 时东霞冼乐德杨威杜罗军张广宇 Beijing National Laboratory for Condensed Matter Physics and Institute of PhysicsChinese Academy of SciencesBeijing 100190China School of Physical Sciences University of Chinese Academy of SciencesBeijing 100049China Songshan Lake Materials Laboratory Dongguan 523808China College of Physics and Electronic Engineering Center for Computational SciencesSichuan Normal UniversityChengdu 610068China Research Center for Functional Materials National Institute for Materials Science1-1 NamikiTsukuba 305-0044Japan International Center for Materials Nanoarchitectonics National Institute for Materials Science1-1 NamikiTsukuba 305-0044Japan

Moiré superlattices have emerged as a highly controllable quantum platform for exploration of various fascinating phenomena,such as Mott insulator states,ferroelectric order,unconventional superconductivity and orbital *** remarkable progress has been achieved,current research in moiré physics has mainly focused on the single species properties,while the coupling between distinct moiré quantum phenomena remains *** we demonstrate,for the first time,the strong coupling between ferroelectricity and correlated states in a twisted quadrilayer MoS2moiré superlattice,where the twist angles are controlled in sequence to be ~57°,~0°,and ~-57°.Correlated insulator states are unambiguously established at moiré band filling factors v = 1,2,3 of twisted quadrilayer MoS_(2).Remarkably,ferroelectric order can occur at correlated insulator states and disappears quickly as the moiré band filling deviates from the integer fillings,providing smoking gun evidences of the coupling between ferroelectricity and correlated *** results demonstrate the coupling between different moiré quantum properties and will hold great promise for new moiré physics and applications.

关键词： ferroelectric quantum twisted

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Epitaxial growth of trilayer graphene moiré superlattice

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Chinese Physics B 2023年第7期32卷 510-514页

作者：袁亚龙褚衍邦胡成田金朋刘乐吴帆帆季怡汝赵交交黄智恒昝晓洲杜罗军 Kenji Watanabe takashi taniguchi 时东霞史志文杨威张广宇 Beijing National Laboratory for Condensed Matter Physics and Institute of Physics Chinese Academy of Sciences(CAS)Beijing 100190China School of Physical Sciences University of Chinese Academy of SciencesBeijing 100190China Key Laboratory of Artificial Structures and Quantum Control(Ministry of Education) School of Physics and AstronomyShanghai Jiao Tong UniversityShanghai 200240China Collaborative Innovation Center of Advanced Microstructures Nanjing 210093China Research Center for Functional Materials National Institute for Materials Science1-1 NamikiTsukuba 305-0044Japan International Center for Materials Nanoarchitectonics National Institute for Materials Science1-1 NamikiTsukuba 305-0044Japan Songshan Lake Materials Laboratory Dongguan 523808China

The graphene-based moiré superlattice has been demonstrated as an exciting system for investigating strong correlation phenomenon. However, the fabrication of such moiré superlattice mainly relies on transfer technology. Here, we report the epitaxial growth of trilayer graphene(TLG) moiré superlattice on hexagonal boron nitride(h BN) by a remote plasma-enhanced chemical vapor deposition method. The as-grown TLG/h BN shows a uniform moiré pattern with a period of ~ 15 nm by atomic force microscopy(AFM) imaging, which agrees with the lattice mismatch between graphene and h BN. By fabricating the device with both top and bottom gates, we observed a gate-tunable bandgap at charge neutral point(CNP) and displacement field tunable satellite resistance peaks at half and full fillings. The resistance peak at half-filling indicates a strong electron–electron correlation in our grown TLG/h BN superlattice. In addition, we observed quantum Hall states at Landau level filling factors ν = 6, 10, 14,..., indicating that our grown trilayer graphene has the ABC stacking order. Our work suggests that epitaxy provides an easy way to fabricate stable and reproducible two-dimensional strongly correlated electronic materials.

关键词： epitaxial growth ABC-TLG/hBN moirésuperlattice electron correlations

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Intrinsic Electronic Properties of BN-Encapsulated,van der Waals Contacted MoSe_(2)Field-Effect Transistors

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Chinese Physics Letters 2023年第6期40卷 98-103页

作者：邵印江周健徐宁陈健渡邊賢司谷口尚施毅黎松林 School of Electronic Science and Engineering National Laboratory of Solid-State Microstructuresand Collaborative Innovation Center of Advanced MicrostructuresNanjing UniversityNanjing 210023China National Institute for Materials Science TsukubaIbaraki 305-0044Japan

Two-dimensional(2D)semiconductors have attracted considerable interest for their unique physical ***,we report the intrinsic cryogenic electronic transport properties in few-layer MoSe_(2)field-effect transistors(FETs)that are fully encapsulated in ultraclean hexagonal boron nitride dielectrics and are simultaneously van der Waals contacted with gold *** FETs exhibit electronically favorable channel/dielectric interfaces with low densities of interfacial traps(<1010cm^(-2)),which lead to outstanding device characteristics at room temperature,including near-Boltzmann-limit subthreshold swings(65 mV/dec),high carrier mobilities(53–68 cm^(2)·V-1·s^(-1)),and negligible scanning hystereses(<15 mV).The dependence of various contact-related parameters with temperature and carrier density is also systematically characterized to understand the van der Waals contacts between gold and MoSe_(2).The results provide insightful information about the device physics in van der Waals contacted and encapsulated 2D FETs.

关键词： hexagonal boron dielectric

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莫尔超晶格场诱导关联绝缘态的量子振荡（英文）

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Science Bulletin 2023年第11期 1127-1133页

作者：刘乐褚衍邦杨光袁亚龙吴帆帆季怡汝田金朋杨蓉 Kenji Watanabe takashi taniguchi 龙根时东霞刘健鹏沈洁吕力杨威张广宇 Beijing National Laboratory for Condensed Matter Physics and Institute of Physics Chinese Academy of Sciences School of Physical Sciences University of Chinese Academy of Sciences Songshan Lake Materials Laboratory Research Center for Functional Materials National Institute for Materials Science International Center for Materials Nanoarchitectonics National Institute for Materials Science School of Physical Sciences and Technology Shanghai Tech University Shanghai Tech Laboratory for Topological Physics Shanghai Tech University

本文报道了转角双层-双层石墨烯关联绝缘态中的量子振荡行为.作者发现价带半填充处具有谷各向异性的绝缘态会随着磁场周期性振荡,且最大振幅高达150 kΩ.此外,该绝缘态量子振荡行为可以被垂直方向的电场有效调控.振荡频率随着电场增加...

本文报道了转角双层-双层石墨烯关联绝缘态中的量子振荡行为.作者发现价带半填充处具有谷各向异性的绝缘态会随着磁场周期性振荡,且最大振幅高达150 kΩ.此外,该绝缘态量子振荡行为可以被垂直方向的电场有效调控.振荡频率随着电场增加线性减小,这表明绝缘态中存在着不断减小的费米面;从振幅变温行为中提取的有效质量随电场变化体现为非线性的行为,但总体保持在0.1me的量级.同样的量子振荡行为也出现在导带半填充处以及非石墨栅极的样品中,表明了该现象的普适性.为了解释该振荡的起源,作者根据实验中提取的与费米面相关的参数构建了反带模型,并通过计算发现能隙中的态密度会随磁场发生振荡,这与实验结果相吻合.本研究表明转角双层-双层石墨烯蕴含着丰富的关联和拓扑现象,是研究凝聚态中的关联物态极好的平台.

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Real- and momentum-indirect neutral and charged excitons in a multi-valley semiconductor

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National Science Open 2023年第4期2卷 76-85页

作者： Zhiheng Huang Yuhui Li Tao Bo Yanchong Zhao Fanfan Wu Lu Li Yalong Yuan Yiru Ji Le Liu Jinpeng Tian Yanbang Chu Xiaozhou Zan Yalin Peng Xiuzhen Li Yangkun Zhang Kenji Watanabe takashi taniguchi Zhipei Sun Wei Yang Dongxia Shi Shixuan Du Luojun Du Guangyu Zhang Beijing National Laboratory for Condensed Matter Physics Key Laboratory for Nanoscale Physics and DevicesInstitute of PhysicsChinese Academy of SciencesBeijing 100190China School of Physical Sciences University of Chinese Academy of SciencesBeijing 100190China Ningbo Institute of Materials Technology&Engineering Chinese Academy of SciencesNingbo 315201China Research Center for Functional Materials National Institute for Materials Science1-1 NamikiTsukuba 305-0044Japan International Center for Materials Nanoarchitectonics National Institute for Materials Science1-1 NamikiTsukuba 305-0044Japan Department of Electronics and Nanoengineering Aalto UniversityTietotie 3Espoo FI-02150Finland Quantum Technology Finland(QTF)Centre of Excellence Department of Applied PhysicsAalto UniversityAalto FI-00076Finland Beijing Key Laboratory for Nanomaterials and Nanodevices Beijing 100190China Songshan Lake Materials Laboratory Dongguan 523808China

Excitons dominate the photonic and optoelectronic properties of a *** significant advancements exist in understanding various types of excitons,progress on excitons that are indirect in both real-and momentum-spaces is still ***,we demonstrate the real-and momentum-indirect neutral and charged excitons(including their phonon replicas)in a multi-valley semiconductor of bilayer MoS_(2),by performing electric-field/doping-density dependent *** with first-principles calculations,we uncover that the observed real-and momentum-indirect exciton involves electron/hole from K/Γvalley,solving the longstanding controversy of its momentum ***,the binding energy of real-and momentum-indirect charged exciton is extremely large(i.e.,~59 meV),more than twice that of real-and momentum-direct charged exciton(i.e.,~24 meV).The giant binding energy,along with the electrical tunability and long lifetime,endows real-and momentum-indirect excitons an emerging platform to study many-body physics and to illuminate developments in photonics and optoelectronics.

关键词： excitons real-and momentum-indirect exciton giant binding energy electrical tunability multi-valley semiconductor

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Immunological milieu in the peritoneal cavity at laparotomy for gastric cancer

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World Journal of Gastroenterology 2012年第13期18卷 1470-1478页

作者： Akira Yoneda Shinichiro Ito Seiya Susumu Mitsutoshi Matsuo Ken taniguchi Yoshitsugu Tajima Susumu Eguchi takashi Kanematsu Yasuhiro Nagata Department of Surgery Nagasaki University Graduate School of Biomedical SciencesNagasaki 852-8051Japan Department of Surgery Yamaguchi Prefectural Medical CenterYamaguchi 747-8511Japan Department of Surgery National Hospital Organization Nagasaki Medical CenterNagasaki 856-8562Japan

AIM： To investigate the immunological repertoire in the peritoneal cavity of gastric cancer patients. METHODS： The peritoneal cavity is a compartment in which immunological host-tumor interactions can occur. However, the role of lymphocytes in the peri- toneal cavity of gastric cancer patients is unclear. We observed 64 patients who underwent gastrectomy for gastric cancer and 11 patients who underwent lapa-roscopic cholecystectomy for gallstones and acted as controls. Lymphocytes isolated from both peripheral blood and peritoneal lavage were analyzed for surface markers of lymphocytes and their cytokine production by flow cytometry. CD4＋CD25h＋gh T cells isolated from the patient＇s peripheral blood were co-cultivated for 4 d with the intra-peritoneal lymphocytes, and a cytokine assay was performed. RESULTS： At gastrectomy, CCR7-CD45RA- CD8＋ effector memory T cells were observed in the peritoneal cavity. The frequency of CD4＋ CD25 h＋ghT ceils in both the peripheral blood and peritoneal cavity was elevated in patients at advanced stage [control vs stage IV in the peripheral blood： 6.89 （3.39-10.4） vs 15.34 （11.37-19.31）, P 〈 0.05, control vs stage IV in the peri- toneal cavity： 8.65 （5.28-12.0） vs 19.56 （14.81-24.32）, P 〈 0.05]. On the other hand, the suppression was restored with CD4＋ CD25h＋QhT cells from their own pe- ripheral blood. This study is the first to analyze lympho- cyte and cytokine production in the peritoneal cavity in patients with gastric cancer. Immune regulation at ad- vanced stage is reversible at the point of gastrectomy. CONCLUSION： The immunological milieu in the peri- toneal cavity of patients with advanced gastric cancer elicited a Th2 response even at gastrectomy, but this response was reversible.

关键词： Cytokines Gastric cancer Lymphocytes Peri-toneal cavity Regulatory T cell

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A novel animal model for in vivo study of liver cancer metastasis

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World Journal of Gastroenterology 2012年第29期18卷 3875-3882页

作者： Shinsuke Fujiwara Hikaru Fujioka Chise Tateno Ken taniguchi Masahiro Ito Hiroshi Ohishi Rie Utoh Hiromi Ishibashi takashi Kanematsu Katsutoshi Yoshizato Clinical Research Center National Hospital Organization Nagasaki Medical Center and Division of HepatologyNagasaki University Graduate School of Biomedical SciencesNagasaki 856-8652Japan Liver Research Laboratory PhoenixBio Co.LtdHiroshima 739-8511Japan Yoshizato Project CLUSTERHiroshima Prefectural Institute of Industrial Science and TechnologyHiroshima 739-8511Japan Division of Surgery Ⅱ Nagasaki University Graduate School of Biomedical SciencesNagasaki 856-8652Japan Liver Research Center Osaka City UniversityGraduate School of MedicineOsaka 532-0025Japan

AIM:To establish an animal model with human hepatocyte-repopulated liver for the study of liver cancer ***:Cell transplantation into mouse livers was conducted using alpha-fetoprotein(AFP)-producing hu-man gastric cancer cells(h-GCCs) and h-hepatocytes as donor cells in a transgenic mouse line expressing urokinase-type plasminogen activator(uPA) driven by the albumin enhancer/promoter crossed with a severe combined immunodeficient(SCID) mouse line(uPA/SCID mice).Host mice were divided into two groups(A and B).Group A mice were transplanted with h-GCCs alone,and group B mice were transplanted with h-GCCs and h-hepatocytes *** replacement index(RI),which is the ratio of transplanted h-GCCs and h-hepatocytes that occupy the examined area of a histological section,was estimated by measuring h-AFP and h-albumin concentrations in sera,respectively,as well as by immunohistochemical analyses of h-AFP and human cytokeratin 18 in histological ***:The h-GCCs successfully engrafted,repopulated,and colonized the livers of mice in group A(RI = 22.0% ± 2.6%).These mice had moderately differentiated adenocarcinomatous lesions with disrupted glandular structures,which is a characteristics feature of gastric *** serum h-AFP level reached 211.0 ± 142.2 g/mL(range,7.1-324.2 g/mL).In group B mice,the h-GCCs and h-hepatocytes independently engrafted,repopulated the host liver,and developed colonies(RI = 12.0% ± 6.8% and 66.0% ± 12.3%,respectively).h-GCC colonies also showed typical adenocarcinomatous glandular structures around the *** mice survived for the full 56 day-study and did not exhibit any metastasis of h-GCCs in the extrahepatic regions during the observational *** mice with an h-hepatocyte-repopulated liver possessed metastasized h-GCCs and therefore could be a useful humanized liver animal model for studying liver cancer metastasis in ***:A novel animal model of human liver cancer metastas

关键词： Urokinase-type plasminogen activator/severe combined immunodeficient mouse Mouse with humanized liver Liver cancer metastasis Alpha-fetoprotein-producing gastric cancer cells

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Vacuum Insulation and Achievement of 980 keV,185 A/m^2 H-Ion Beam Acceleration at JAEA for the ITER Neutral Beam Injector

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Plasma Science and Technology 2013年第2期15卷 179-183页

作者： Hiroyuki TOBARI Masaki taniguchi Mieko KASHIWAGI Masayuki DAIRAKU Naotaka UMEDA Haruhiko YAMANAKA Kazuki TSUCHIDA Jumpei TAKEMOTO Kazuhiro WATANABE takashi INOUE Keishi SAKAMOTO Japan Atomic Energy Agency (JAEA) Mukouyama 801-1 Naka Ibaraki 311-1093 Japan

Abstract Vacuum insulation of -1 MV is a common issue for the HV bushing and the accel- erator for the ITER neutral beam injector （NBI）. The HV bushing as an insulating feedthrough has a five-stage structure and each stage consists of double-layered insulators. To sustain -1 MV in vacuum, reduction of electric field at several triple points existing around the double-layered insulators is a critical issue. To reduce electric field simultaneously at these points, three types of stress ring have been developed. In a voltage holding test of a full-scale mockup equipped with these stress rings, 120% of rated voltage was sustained and the voltage holding capability required in ITER was verified. In the MeV accelerator, whose target is the acceleration of a H- ion beam of 1 MeV, 200 A/mS, the gap between the grid support was extended to suppress breakdowns triggered by electric field concentration at the edge and corner of the grid support. This modi- fication improved the voltage holding capability in vacuum, and the MeV accelerator succeeded in sustaining -1 MV stably, b-~rthermore, it appeared that the H- ions beam was deflected and a part of the beam was intercepted at the acceleration grid, This causes high heat load on the grids and breakdowns during beam acceleration. To suppress the direct interception, a new grid was designed with proper aperture displacement based on a three dimensional beam trajectory analysis, As a result, 980 keV, 185 A/ms H- ion beam acceleration has been demonstrated, which is close to the ITER requirement.

关键词： neutral beam injector (NBI) negative ion beam HV bushing vacuum insu-lation

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Synchronous coexistence of liver metastases from cecal leiomyosarcoma and rectal adenocarcinoma: A case report

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World Journal of Gastroenterology 2017年第9期23卷 1725-1734页

作者： Hideki Aoki takashi Arata Masashi Utsumi Yutaka Mushiake Tomoyoshi Kunitomo Isao Yasuhara Fumitaka taniguchi Koh Katsuda Kohji Tanakaya Hitoshi Takeuchi Rie Yamasaki Department of Surgery Iwakuni Clinical Center Department of Pathology Iwakuni Clinical Center

Multiple liver tumors represent a challenging condition for abdominal surgeons both in the selection of technique and the rarity of diagnosis. There are no case reports on co-existence of liver metastases from both intestinal leiomyosarcoma and adenocarcinoma. The patient described in this report successfully underwent resection of both primary lesions and liver metastases in combination with chemotherapy. As for the leiomyosarcoma, the primary cecal lesion was revealed more than three years after the patient's first visit. Peritoneal, lymph-node, and lung recurrences were observed afterward, and thus surgeries on those regions were performed. Pathologically, the peritoneal and lung recurrences comprised leiomyosarcoma and the lymphnode recurrence was diagnosed as adenocarcinoma. Despite newly discovered multiple lung recurrences and regional lymph-node metastases, the patient lived a normal life for 73 mo after the initial operation based on multidisciplinary therapy. He ultimately died of liver failure due to invasive lymph-node recurrence from the rectal adenocarcinoma, in addition to multiple lung recurrences from the leiomyosarcoma. Hepatic recurrence did not occur in this patient's case, which appears to be one reason for his long-term survival.

关键词： Leiomyosarcoma Chemotherapy Multiple liver tumors Liver metastasis Adenocarcinoma

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Assessment of cardiac output in liver transplantation recipients

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Hepatobiliary & Pancreatic Diseases International 2008年第4期7卷 362-366页

作者： Tomohide Hori Chiduru Yamamoto Shintaro Yagi Taku Iida Kentaro taniguchi takashi Hasegawa Koichiro Yamakado Yukinobu Hori Kan Takeda Kazuo Maruyama Shinji Uemoto Department of Hepato-Pancreato-Biliary Surgery and Transplantation Kyoto University Hospital54 Shogoinkawara- choSakyo-kuKyoto606-8507Japan Department of Hepatobiliary Pancreatic Surgery Mie University Hospital2-174 EdobashiTsu CityMie Prefecture514-8507 Japan Department of Anesthesiology and Critical Care Medicine Mie University Graduate School of Medicine2-174 EdobashiTsu CityMie Prefecture514-8507Japan Department of Radiology Mie University Graduate School of Medicine2-174 EdobashiTsu CityMie Prefecture514-8507Japan Nagoya Economic University Graduate School of Law 61-1 UchikuboInuyama City Aichi Prefecture 484-8504Japan

BACKGROUND:Liver cirrhosis causes peculiar systemic hemodynamics,and accurate evaluation of systemic hemodynamic state is important for cirrhotic recipients who underwent living donor liver transplantation(LDLT). We investigated the clinical advantages of a novel non- invasive method for measuring systemic hemodynamic parameters using indocyanine green(ICG). METHODS:Twenty-eight LDLT recipients were evaluated. Simultaneous measurements of cardiac output(CO)using Swan-Ganz catheters and pulse dye densitometry(PDD) were performed every 12 hours after LDLT.A total of 155 sets of simultaneous CO measurements were obtained. RESULTS:The CO values obtained by PDD correlated well with those obtained by the invasive catheter *** addition,none of the recipients developed any side-effects, and we verified the safety of repeated ICG *** is safe,even for repeated use over time in the same recipient. Moreover,PDD can measure the blood volume(BV).CONCLUSIONS:Since the cirrhotic systemic hemody- namics characterized by high CO and large BV remains, even after LDLT,the ability to measure CO and BV in a non-invasive,simple and real-time manner using PDD has advantages for cirrhotic LDLT recipients.

关键词： liver transplantation indocyanine green pulse dye densitometry blood volume cardiac output liver cirrhosis

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