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Channel-Feedback-Free Transmission for Downlink FD-RAn:A Radio Map Based Complex-Valued Precoding network Approach

China Communications 2024年第4期21卷 10-22页

作者： Zhao Jiwei Chen Jiacheng sun Zeyu Shi Yuhang Zhou Haibo Xuemin(Sherman)Shen School of Electronic Science and Engineering Nanjing UniversityNanjing 210023China College of Information Science and Electronic Engineering Zhejiang UniversityHangzhou 310058China Department of Mathematics and Theories Peng Cheng LaboratoryShenzhen 518000China Department of Electrical and Computer Engineering University of WaterlooWaterlooOntarioN2L 3G1Canada

As the demand for high-quality services proliferates,an innovative network architecture,the fully-decoupled RAn(FD-RAn),has emerged for more flexible spectrum resource utilization and lower network ***,with the decoupling of uplink base stations and downlink base stations in FDRAn,the traditional transmission mechanism,which relies on real-time channel feedback,is not suitable as the receiver is not able to feedback accurate and timely channel state information to the *** paper proposes a novel transmission scheme without relying on physical layer channel ***,we design a radio map based complex-valued precoding network(RMCPnet)model,which outputs the base station precoding based on user *** comprises multiple subnets,with each subnet responsible for extracting unique modal features from diverse input ***,the multimodal embeddings derived from these distinct subnets are integrated within the information fusion layer,culminating in a unified *** also develop a specific RMCPnet training algorithm that employs the negative spectral efficiency as the loss *** evaluate the performance of the proposed scheme on the public DeepMIMO dataset and show that RMCPnet can achieve 16%and 76%performance improvements over the conventional real-valued neural network and statistical codebook approach,respectively.

关键词： beamforming complex neural networks deep learning FD-RAn

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Hybrid perovskite shows temperature-dependent photoluminescence and dielectric response triggered by halogen substitution

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结构化学 2024年第6期43卷 28-33页

作者： Xiao-Tong sun Hao-Fei ni Yi Zhang Da-Wei Fu Ordered Matter Science Research Center Jiangsu Key Laboratory for Science and Applications of Molecular FerroelectricsSoutheast UniversityNanjing211189People's Republic of China Institute for Science and Applications of Molecular Ferroelectrics Key Laboratory of the Ministry of Education for Advanced Catalysis MaterialsZhejiang Normal UniversityJinhua321004People's Republic of China

Materials exhibiting dielectric switching response and photoluminescence(PL)are promising for sensors and information *** previous research,we synthesized a series of materials with red or green PL and dielectric switching capabilities by incorporating luminescent metal halides into organic ammonium ***,effective modification to synthesize organic-inorganic hybrid materials with dielectric switching response and orange PL continues to be a challenge in the respective *** PL materials are valuable for switching and sensors,and most orange light sources are derived from rare earth elements,making them harder to *** have successfully synthesized two organic-inorganic hybrid materials([CMPD]PbBr3(1)and[BMPD]PbBr3(2),CMPD=n-ClCH2-n-methylpiperidine,BMPD=n-BrCH2-n-methylpiperidine)that exhibit both orange PL and dielectric switching *** Cl in compound 1 is substituted by Br in compound 2,the phase transition temperature of the compound is elevated by 45 *** compounds exhibit captivating orange light emission when exposed to ultraviolet *** research provides insights into exploring multifunctional materials with orange PL and dielectric switching response and provides proof for halogen substitution strategies to design materials with higher phase transition temperatures.

关键词： Dielectric switching Photoluminescence Orange

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High Temperature Iron Ethylene Polymerization Catalysts Bearing n,n,n'-2-(1-(2,4-Dibenzhydryl-6-fluorophenylimino)ethyl)-6-(1-(arylphenylimino)ethyl)pyridines

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Chinese Journal of Polymer Science 2024年第2期42卷 188-201,I0007页

作者： Chantsalnyam Bariashir qiu-Yue Zhang Bayasgalan Ulambayar Gregory A.Solan Tong-Ling Liang Wen-Hua sun Institute of Chemistry and Chemical Technology Mongolian Academy of SciencesUlaanbaatar13330Mongolia Key Laboratory of Engineering Plastics and Beijing national Laboratory for Molecular Science Institute of ChemistryChinese Academy of SciencesBeijing100190China Department of Chemistry University of LeicesterUniversity RoadLeicesterLE17RHUK State Key Laboratory for Oxo Synthesis and Selective Oxidation Lanzhou Institute of Chemical PhysicsChinese Academy of SciencesLanzhou730000China

The n,n,n'-ferrous chloride complexes,[2-{CMen(2,4-(CHPh)_(2)-6-FC_(6)H_(2))}-6-(CMenAr)C_(5)H_(3)n]FeCl_(2)(Ar=2,6-Me_(2)C_(6)H_(3) Fe1,2,6-Et_(2)C_(6)H_(3)Fe2,2,6-^(i)Pr_(2)C_(6)H_(3) Fe3,2,4,6-Me_(3)C_(6)H_(2) Fe4 and 2,6-Et_(2)-4-MeC_(6)H_(2) Fe5),each possessing one n-2,4-dibenzhydryl-6-fluorophenyl group,were readily synthesized from their respective unsymmetrical bis(imino)pyridines,*** identification of Fe2 highlighted the variation in the steric properties provided by the dissimilar n-aryl *** pre-treatment with either MAO or MMAO,complexes Fe1-Fe5 all displayed,at an operating temperature of 80℃,high activities for ethylene polymerization with levels falling in the order:Fe4> Fe1> Fe5> Fe2> ***,Fe4/MAO displayed the highest activity of 1.94×10^(7) g_(PE)·mol_(Fe)^(-1)·h^(-1) of the study with only a modest loss in performance at 90℃.Generally,the resulting polyethylenes were highly linear(T_(m) range:122-132℃),narrowly disperse and of low molecular weight(M_(w) range:6.73-46.04kg·mol^(-1)),with the most sterically hindered Fe3 forming the highest molecular weight polymer of the ***-group analysis by ^(1)H-and ^(13)CnMR spectroscopy revealed saturated alkyl(n-propyl and i-propyl) and unsaturated vinyl chain ends indicative of the role of both β-H elimination and chain transfer to aluminum as termination *** comparison with previou sly reported iron precatalysts with similar tridentate ligand skeletons,it is evident that the introduction of a large benzhydryl group in combination with a fluorine as the ortho-substituents of one n-aryl group has the effect of enhancing thermal stability of the iron polymerization catalyst whilst maintaining appreciable polymer molecular weight.

关键词： Iron catalyst Ethylene polymerization Linear polyethylene Fluoride effect Thermal stability

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Sludge composition and characteristics shaped microbial community and further determined process performance: A study on full-scale thermal hydrolysis-anaerobic digestion processes

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Journal of Environmental Sciences 2024年第3期137卷 96-107页

作者： Wei Liu Chenxiang sun Wei Li Tianle Li Zhan Chen Jiawei Wang Zhengran Ren Xianghua Wen School of Environment Tsinghua UniversityBeijing 100084China Jinneng Holding Group DatongShanxi 037000China Research and Development Center Beijing Drainage Group Co.Ltd.Beijing 100124China Beijing Dabeinong Science and Technology Group Co. Ltd.Beijing 100080China

Anaerobic digestion (AD) with thermal hydrolysis (TH) pretreatment is a promising process for excess sludge treatment,while there lacks of the knowledge from full-scale process about the impact of sludge composition and characteristics on microbial community and *** sludge physiochemical indices,microbial community and performance data of four full-scale TH-AD plants were characterized,and their relationships was *** four plants were operated under almost similar total organic loading rate (OLR)but their methanogenesis performance differentiate into two groups,namely superior group(SupG) and the inferior group (Inf G).In both groups,TH effectively solubilized particulate organic compounds,meanwhile raised the ammonia nitrogen (nH_(4)^(+)-n) and volatile fatty acid (VFA) *** with the Sup G,thermal hydrolyzed sludge of Inf G had higher level of VFAs,nH_(4)^(+)-n and total chemical oxygen demand (t COD),which showed higher inhibition effect on microbes,leading to a community with lower diversity,lower abundance of carbohydrate degrading functional guild,higher protein degrading one,and methanogens that adapted to limited substrates,and further declined the methane production ***,it was recommended that OLR alone was not sufficient for controlling the system in design and operation,the concentration of VFAs,nH_(4)^(+)-n and t COD should be equally *** higher concentration,together with the higher abundance of Defluviitoga and Proteiniphilum were recommended as indicators for inferior running *** results proposed that microbial communities played a role of bridge between environmental factors and performance,provided implications for engineering ecology and operational regulation for full-scale sludge TH-AD process.

关键词： Thermal hydrolysis Anaerobic digestion Microbial community Full-scale

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Ambient electrosynthesis of urea from carbon dioxide and nitrate over Mo_(2)C nanosheet

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Chinese Chemical Letters 2024年第8期35卷 319-323页

作者： Yue Zhang Xiaoya Fan Xun He Tingyu Yan Yongchao Yao Dongdong Zheng Jingxiang Zhao q.n.hai Cai qian Liu Luming Li Wei Chu Shengjun sun Xuping sun College of Chemistry and Chemical Engineering and Key Laboratory of Photonic and Electronic Bandgap MaterialsMinistry of EducationHarbin Normal UniversityHarbin 150025China Institute of Fundamental and Frontier Sciences University of Electronic Science and Technology of ChinaChengdu 610054China Institute for Advanced Study Chengdu UniversityChengdu 610106China College of Chemistry Chemical Engineering and Materials ScienceShandong Normal UniversityJi’nan 250014China

Electrocatalytic synthesis of urea through C-n bond formation,converting carbon dioxide(CO_(2))and ni-trate(nO_(3)^(-)),presents a promising,less energy-intensive alternative to industrial urea production *** this communication,we report the application of Mo_(2)C nanosheets-decorated carbon sheets(Mo_(2)C/C)as a highly efficient electrocatalyst for facilitating C-n coupling in ambient urea *** CO_(2)-saturated 0.2 mol/L na_(2)SO_(4)solution containing 0.05 mol/L nO_(3)^(-),the Mo_(2)C/C catalyst achieves an impres-sive urea yield of 579.13μg h^(-1)mg^(-1)with high Faradaic efficiency of 44.80%at-0.5 V versus the reversible hydrogen *** theoretical calculations reveal that the multiple Mo active sites enhance the formation of^(∗)CO and^(∗)nH_(2)intermediates and facilitate their C-n *** research propels the use of Mo_(2)C-based electrodes in electrocatalysis and accentuates the capabilities of binary metal-based catalysts in C-n coupling reactions.

关键词： Mo_(2)C Multiple active sites C-n coupling Electrocatalysis Urea synthesis Density functional theory calculation

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neural Wiskott-Aldrich syndrome protein(n-WASP)promotes distant metastasis in pancreatic ductal adenocarcinoma via activation of LOXL2

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Oncology Research 2024年第4期32卷 615-624页

作者： HYUnG sun KIM YUn sun LEE SEUnG MYUnG DOnG HYO JUnG KIM DA EUn LEE HYEOn WOOnG KAnG MYEOnG JIn KIM JOOn SEOnG PARK Department of Surgery Gangnam Severance HospitalYonsei University College of MedicineSeoulKorea Department of Surgery Graduate School of Medical ScienceBrain Korea 21 ProjectYonsei University College of MedicineSeoulKorea Gibiome Co. Ltd.Gyeonggi-doKorea

Pancreatic ductal adenocarcinoma(PDAC)is one of the most aggressive solid malignancies.A specific mechanism of its metastasis has not been *** this study,we investigated whether neural Wiskott-Aldrich syndrome protein(n-WASP)plays a role in distant metastasis of *** found that n-WASP is markedly expressed in clinical patients with *** analysis showed a notably more distant metastatic pattern in the n-WASP-high group compared to the n-WASP-low group.n-WASP was noted to be a novel mediator of epithelialmesenchymal transition(EMT)via gene expression profile *** of n-WASP in pancreatic cancer cells significantly inhibited cell invasion,migration,and *** also observed positive association of lysyl oxidase-like 2(LOXL2)and focal adhesion kinase(FAK)with the n-WASP-mediated response,wherein EMT and invadopodia function were *** n-WASP and LOXL2 depletion significantly reduced the incidence of liver and lung metastatic lesions in orthotopic mouse models of pancreatic *** results elucidate a novel role for n-WASP signaling associated with LOXL2 in EMT and invadopodia function,with respect to regulation of intercellular communication in tumor cells for promoting pancreatic cancer *** findings may aid in the development of therapeutic strategies against pancreatic cancer.

关键词： Pancreatic cancer neural Wiskott-Aldrich syndrome protein(n-WASP)signaling Metastasis Epithelial-mesenchymal transition(EMT) Lysyl oxidase-like 2(LOXL2)

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Advancing large-scale thin-film PPLn nonlinear photonics with segmented tunable micro-heaters

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Photonics Research 2024年第8期12卷 1703-1708页

作者： XIAOTInG LI HAOCHUAn LI ZHEnZHEnG WAnG ZHAOXI CHEn FEI MA KE ZHAnG WEnZHAO sun CHEnG WAnG Department of Electrical Engineering City University of Hong Kong School of Physics Sun Yat-sen University City University of Hong Kong (Dongguan) Center of Information and Communication Technology City University of Hong Kong Shenzhen Research Institute State Key Laboratory of Terahertz and Millimeter Waves City University of Hong Kong

Thin-film periodically poled lithium niobate (TF-PPLn) devices have recently gained prominence for efficient wavelength conversion processes in both classical and quantum applications. However, the patterning and poling of TF-PPLn devices today are mostly performed at chip scales, presenting a significant bottleneck for future largescale nonlinear photonic systems that require the integration of multiple nonlinear components with consistent performance and low cost. Here, we take a pivotal step towards this goal by developing a wafer-scale TF-PPLn nonlinear photonic platform, leveraging ultraviolet stepper lithography and an automated poling process. To address the inhomogeneous broadening of the quasi-phase matching(qPM) spectrum induced by film thickness variations across the wafer, we propose and demonstrate segmented thermal optic tuning modules that can precisely adjust and align the qPM peak wavelengths in each section. Using the segmented micro-heaters, we show the successful realignment of inhomogeneously broadened multi-peak qPM spectra with up to 57% enhancement of conversion efficiency. We achieve a high normalized conversion efficiency of 3802% W-1cm-2in a 6 mm long PPLn waveguide, recovering 84% of the theoretically predicted efficiency in this device. The advanced fabrication techniques and segmented tuning architectures presented herein pave the way for wafer-scale integration of complex functional nonlinear photonic circuits with applications in quantum information processing, precision sensing and metrology, and low-noise-figure optical signal amplification.

关键词： Lithium niobate Optical amplifiers Optical parametric oscillators Optical signals Precision metrology Wavelength conversion

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Leflunomide: A versatile additive for defect reduction, enhanced optoelectronic properties and environmental stability of perovskite films

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nano Research 2024年第4期17卷 2628-2637页

作者： Dingyue sun Ming Peng Taijin Wang Longju Yi Shizuo Zhang Feng Liu Gary J.Cheng The Institute of Technological Sciences Wuhan UniversityWuhan 430072China School of Power and Mechanical Engineering Wuhan UniversityWuhan 430072China School of Industrial Engineering Purdue UniversityWest LafayetteIN 47906USA

The development of perovskite photoelectric devices with excellent performance is largely dependent on the defects in the perovskite *** address this issue,a specific drug,leflunomide(LF,C_(12)H_(9)F_(3)n_(2)O_(2)),was incorporated into the perovskite to reduce defects and improve its photoelectric *** is believed that the C=O bond on LF molecule can interact with the uncoordinated Pb2+of the perovskite,thereby reducing non-radiative *** novel approach of incorporating LF into perovskite films has the potential to revolutionize the development of high-performance perovskite photoelectric *** trifluoromethyl functional(–CF_(3))group on LF can form a protective layer on the surface of the perovskite film,shielding it from water ***,LF can be utilized to alter the nucleation position of perovskite,thus minimizing the number of defects and optimizing the film ***,the LF-doped perovskite film displays low trap density and high photoelectric *** LF-doped perovskite film showed a trap density of 8.28×10^(11),which is notably lower than the 2.04×10^(12) of the perovskite film without *** responsivity and detectivity of the LF-doped perovskite photodetector were 0.771 A/W and 2.81×10^(11) Jones,respectively,which are much higher than the 0.23 A/W and 1.06×10^(10) Jones of the LF-undoped perovskite ***,the LF-doped photodetector maintained an initial photocurrent of 86%after 30 days of storage in air,indicating drastically increased environmental *** strongly suggests that LF is an effective additive for perovskites utilized in optoelectronic devices with high performance.

关键词： leflunomide additive engineering defect passivation perovskite

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Highly efficient CO_(2) capture using 2-methylimidazole aqueous solution on laboratory and pilot-scale

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Chinese Journal of Chemical Engineering 2024年第3期67卷 148-156页

作者： Kun Li Han Tang Shuangshuang Li Zixuan Huang Bei Liu Chun Deng Changyu sun Guangjin Chen State Key Laboratory of Heavy Oil Processing China University of PetroleumBeijing 102249China Zhejiang Tiandi Environmental Protection Technology Co. Ltd.Hangzhou 310012China

To date,the primary industrial carbon capture approach is still absorption using aqueous solutions of ***,to pursue a substitute for the amine-based approach to improve the CO_(2) capture efficiency and decrease the energy cost further,we report a new carbon capture approach using a 2-methylimidazole(mIm)aqueous *** properties and sorption behaviors of this approach have been experimentally *** results show that the mIm solution has higher CO_(2) absorption capacity under relatively higher equilibrium pressure(>130 kPa)and lower desorption heat than the methyldiethanolamine solution.91.6%sorption capacity of mIm solution can be recovered at 353.15 K and 80 *** selectivity for CO_(2)/n_(2) and CO_(2)/CH_(4) can reach an exceptional 7609 and 4324,***,the pilot-scale tests were also performed,and the results demonstrate that more than 98%of CO_(2) in the feed gas could be removed and cyclic absorption capacity can reach 1 mol·L^(-1).This work indicates that mIm is an excellent alternative to alkanolamines for carbon capture in the industry.

关键词： CO_(2) capture Absorption 2-Methylimidazole Separation Pilot-scale tests

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Inversion method of deflection of the vertical based on SWOT wide-swath altimeter data

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Geodesy and Geodynamics 2024年第4期15卷 419-428页

作者： Xin Liu Menghao Song Chao Li Guihua Hui Jinyun Guo Yongjun Jia Heping sun College of Geodesy and Geomatics Shandong University of Science and TechnologyQingdao 266590China Weicheng Branch of natural Resources and Planning Bureau of Weifang City Weifang 261021China national Satellite Ocean Application Service Beijing 100081China State Key Laboratoryof Geodesy and Earth's Dynamics Innovation AcademyforPrecision Measurement Science and TechnologyChinese Academy of ScienceWuhan 420071China

The deflection of the vertical(DOV)is the key information in the study of ocean gravity ***,in most areas,the precision of the prime component of DoV is significantly lower than that of the meridian *** obtain higher accuracy and resolution of ocean gravity information,researchers have proposed a novel altimeter called the wide-swath *** altimeter allows for the simultaneous acquisition of high-precision and high-resolution two-dimensional measurements of sea surface height(SSH).In this paper,the Surface Water and Ocean Topography(SWOT)mission with a wide-swath altimeter on board is selected for *** cycle of swoT sea surface height data is simulated to inverse the DOV in the Arabian Sea(45°E—80°E,0°-30°n),and the inversion results are compared with those of conventional altimeter *** results demonstrate that the difference between the meridian and prime components derived from the inversion of swoT wide-swath data is minimal,significantly outperforming the inversion results of conventional nadir altimeter *** advantage of swoT wide-swath altimeter lies in its ability to use the multi-directional geoid slope at any sea surface measurement point to invert the components in the meridian and prime *** investigate the impact of this advantage on inversion precision,this paper employs a method to calculate the gradient of the geoid in multiple directions to invert DoV *** improvement effect of calculating the gradient of the geoid in multiple directions on the precision of DoV component is *** is found that the accuracy of DoV inversion has significantly improved with the increase of geodetic gradient calculation *** addition,the effects of various errors and grid spacing in SwoT wide sea surface height data on the precision of Dov inversion are also analyzed.

关键词： SWOT Wide-swath altimeter Inversion method of Dov Multi-directional Arabian sea

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