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Topological feature engineering for machine learning based halide perovskite materials design

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npj Computational Materials 2022年第1期8卷 1943-1950页

作者： D.Vijay Anand Qiang Xu JunJie Wee Kelin Xia tze chien sum Division of Mathematical Sciences School of Physical and Mathematical SciencesNanyang Technological UniversitySingapore637371Singapore Division of Physics&Applied Physics School of Physical and Mathematical SciencesNanyang Technological UniversitySingapore637371Singapore

Accelerated materials development with machine learning(ML)assisted screening and high throughput experimentation for new photovoltaic materials holds the key to addressing our grand energy ***-driven ML is envisaged as a decisive enabler for new perovskite materials ***,its full potential can be severely curtailed by poorly represented molecular descriptors(or fingerprints).Optimal descriptors are essential for establishing effective mathematical representations of quantitative structure-property *** we reveal that our persistent functions(PFs)based learning models offer significant accuracy advantages over traditional descriptor based models in organic-inorganic halide perovskite(OIHP)materials design and have similar performance as deep learning *** multiscale simplicial complex approach not only provides a more precise representation for OIHP structures and underlying interactions,but also has better transferability to ML *** results demonstrate that advanced geometrical and topological invariants are highly efficient feature engineering approaches that can markedly improve the performance of learning models for molecular data ***,new structure-property relationships can be established between our invariants and *** anticipate that our molecular representations and featurization models will transcend the limitations of conventional approaches and lead to breakthroughs in perovskite materials design and discovery.

关键词： perovskite halide invariants

Origins of the long-range exciton diffusion in perovskite nanocrystal films: photon recycling vs exciton hopping

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Light(Science & Applications) 2021年第1期10卷 41-49页

作者： David Giovanni Marcello Righetto Qiannan Zhang Jia Wei Melvin Lim Sankaran Ramesh tze chien sum Division of Physics and Applied Physics School of Physical and Mathematical SciencesNanyang Technological University(NTU)21 Nanyang LinkSingapore 637371Singapore Energy Research Institute@NTU(ERI@N) Interdisciplinary Graduate SchoolNanyang Technological University50 Nanyang AvenueS2-B3a-01Singapore 639798Singapore

The outstanding optoelectronic performance of lead halide perovskites lies in their exceptional carrier diffusion *** the perovskite material dimensionality is reduced to exploit the quantum confinement effects,the disruption to the perovskite lattice,often with insulating organic ligands,raises new questions on the charge diffusion ***,we report direct imaging of>1μm exciton diffusion lengths in CH3NH3PbBr3 perovskite nanocrystal(PNC)***,the resulting exciton mobilities in these PNC films can reach 10±2cm^(2)V^(-1) s^(-1),,which is counterintuitively several times higher than the carrier mobility in 3D perovskite *** show that this ultralong exciton diffusion originates from both efficient inter-NC exciton hopping(via Forster energy transfer)and the photon recycling process with a smaller yet significant ***,our study not only sheds new light on the highly debated origins of the excellent exciton diffusion in PNC films but also highlights the potential of PNCs for optoelearonic applications.

关键词： properties. perovskite diffusion

Targeting c-Myc as a novel approach for hepatocellular carcinoma

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World Journal of Hepatology 2010年第1期2卷 16-20页

作者： chien-Ru Liu Chun-Nin Lee tze-Sian Chan H Eugene Liu Department of Medicine Taipei City Hospital Department of Medicine Wanfang HospitalTaipei Medical University Department of Medicine Department of Lab- oratory Medicineand Graduate Institute of Clinical MedicineTaipei Medical University

Hepatocelluar carcinoma(HCC) is the most lethal cancer in the *** HCC over-express c-Myc,which plays a critical role in regulating cellular growth,differentiation and apoptosis in both normal and neoplastic cells. c-Myc is among the most frequently overexpressed genes in human *** of c-Myc in hepatic cells leads to development of hepatocellular ***,we review the current progress in understanding physiologic function and regulation of c-Myc as well as its role in hepatic carcinogenesis and discuss the association of c-Myc activation in chronic hepatitis B infection and the upregulation of HIF-1/*** also explore the possibility of treating HCC by inhibiting c-Myc and examine the pros and cons of such an *** this strategy is currently not available in clinics,with recent advances in better drug design,pharmacokinetics and pharmacogenetics,inhibition of c-Myc might become a novel therapy for HCC in the future.

关键词： Hepatocellular carcinoma c-Myc Novel therapy

Clinical correlation of gallstone disease in a Chinese population in Taiwan:Experience at Cheng Hsin General Hospital

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World Journal of Gastroenterology 2006年第8期12卷 1281-1286页

作者： Chi-Ming Liu Tao-Hsin Tung Pesus Chou Victor tze-Kai Chen Chung-Te Hsu Wu-Shyong chien Yeu-Tyng Lin Hsu-Feng Lu Hui-Chuan Shih Jorn-Hon Liu Community Medicine Research Center & Institute of Public Health National Yang-Ming University Cheng Hsin General Hospital Taipei Taiwan China Community Medicine Research Center & Institute of Public Health National Yang-Ming University Taipei TaiwanChina Cardinal Tien Hospital College of Medicine Fu-Jen Catholic University National Defence Medicine Center Taipei Taiwan China Department of Nursing Kaohsiung Military General Hospital Kaohsiung Taiwan China Faculty of Medicine School of Medicine National Yang-Ming University Cheng Hsin General Hospital TaipeiTaiwan China

AIM： TO explore the prevalence of gallstone disease （GSD） in Taiwan and condition-associated factors related to it. METHODS： We studied a total of 2386 healthy adults （1235 males and 1151 females） voluntarily admitted to Cheng Hsin General Hospital for a paid physical check-up between January 2002 and December 2002. Blood samples and ultrasound sonography results were collected. RESULTS： The overall prevalence of GSD among this study-population was 5.3%, including 1.7% （n=40） having a single stone, 2.3% （n = 55） having multiple stones, and 1.3% （n = 31） having cholecystectomy. The prevalence revealed a statistically significant increase with increasing age （P〈 0.0001）. Females exhibited a greater prevalence of multiple stones than did males （3.0% vs 1.7%, P= 0.04）. Using multiple logistic regression analysis, the following appeared to be significantly related to the prevalence of GSD： older age （40-49 years vs 〈40 years, OR= 1.63 [95% CI： 0.76-3.48], 50-59 years vs 〈40 years, OR=4.93 [95% CI： 2.43-9.99], 60-69 years vs 〈40 years, OR = 6.82 [95% CI： 3.19-14.60], ≥70 years vs 〈40 years, OR= 10.65 [95% CI： 4.78-23.73]）, higher BMI （≥27 kg/m^2 vs 〈24 kg/m^2, adjusted OR= 1.74 [95% CI： 1.04-2.88]）, and higher FPG （≥ 126 mg/dL vs 〈110 mg/dL, OR= 1.71, 95% CI： 1.01-2.96）. CONCLUSION： Older age （≥50 years）, obesity （BMI ≥ 27 kg/m^2）, and type 2 diabetes （FPG ≥126 mg/dL） are associated with the prevalence of GSD.

关键词： Cross-sectional study Gallstone disease Prevalence Risk factors

法律定性与经济分析——评兰德斯与波斯纳的《侵权法的经济结构》

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法制与社会发展 2007年第4期13卷 123-128页

作者：简资修台湾大学法律学系台湾11529

兰德斯与波斯纳的《侵权法的经济结构》是本集大成之作,但其以管制的投入产出模型去分析具自治本质的侵权法,必然是失败的。在大多数情况,兰德斯与波斯纳将防害投入仅限于物理资源,因此交易成本以及冲突活动间的价值抵换,都被排除在考... 详细信息

兰德斯与波斯纳的《侵权法的经济结构》是本集大成之作,但其以管制的投入产出模型去分析具自治本质的侵权法,必然是失败的。在大多数情况,兰德斯与波斯纳将防害投入仅限于物理资源,因此交易成本以及冲突活动间的价值抵换,都被排除在考虑之外。但问题是,前者正是制度选择的基础,而后者则是正确计算社会损失的保证,因此其模型就空空如也。其结果是:一、将侵害人的效益加入了故意侵权之分析;二、在分析各种赔偿责任制的利弊时,混淆了(事前)无责任制与(事后)个案中侵害人的无庸负责;三、在过失认定时,恰好颠倒了侵害人应适用的高低标准。漠视法律定性(基于制度分工),经济分析将无所附丽。

关键词：故意侵权过失合理人标准私法交易成本

Benign esophageal lesions: Endoscopic and pathologic features

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World Journal of Gastroenterology 2015年第4期21卷 1091-1098页

作者： Shu-Jung Tsai Ching-Chung Lin Chen-Wang Chang chien-Yuan Hung tze-Yu Shieh Horng-Yuan Wang Shou-Chuan Shih Ming-Jen Chen Division of Gastroenterology Department of Internal MedicineMackay Memorial Hospital Department of Nursing Nursing and Management Mackay Junior College of Medicine Mackay Medical College

Benign esophageal lesions have a wide spectrum of clinical and pathologic features. Understanding the endoscopic and pathologic features of esophageal lesions is essential for their detection, differential diagnosis, and management. The purpose of this review is to provide updated features that may help physicians to appropriately manage these esophageal lesions. The endoscopic features of 2997 patients are reviewed. In epithelial lesions, the frequency of occurrence was in the following order: glycogenic acanthosis, heterotopic gastric mucosa, squamous papilloma, hyperplastic polyp, ectopic sebaceous gland and xanthoma. In subepithelial lesions, the order was as follows: hemangioma, leiomyoma, dysphagia aortica and granular cell tumor. Most benign esophageal lesions can be diagnosed according to their endoscopic appearance and findings on routine biopsy, and submucosal lesions, by endoscopic resection. Management is generally based upon the confidence of diagnosis and whether the lesion causes symptoms. We suggest endoscopic resection of all granular cell tumors and squamous papillomas because, while rare, these lesions have malignant potential. Dysphagia aortica should be considered in the differential diagnosis of dysphagia in the elderly.

关键词： Benign tumor Esophagus Epithelial lesions Subepith

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过失责任作为私法自治之原则

北大法律评论 2014年第1期15卷 155-173页

作者：简资修中国台湾地区"中央研究院"法律学研究所台湾大学法律学系

过失是私法赔偿之核心,但其往往不为人正确理解,以至于法律体系混乱。传统的过失罪责化,无法解释为何能力较差的行为人仍须适用强人所难的高损害赔偿责任标准。所谓＂过失客观化＂,只是回避了问题,因为其未说明为何客观化及其如何可得... 详细信息

过失是私法赔偿之核心,但其往往不为人正确理解,以至于法律体系混乱。传统的过失罪责化,无法解释为何能力较差的行为人仍须适用强人所难的高损害赔偿责任标准。所谓＂过失客观化＂,只是回避了问题,因为其未说明为何客观化及其如何可得出此客观标准。有经济分析论者,直接将能力效益化,计算出客观的过失标准,得出如＂过失罪责化＂的结果。事实上,基于损害之相互性质,损害若要移转（填补）,其必须是行为人应该而且能够预见的,否则法律即是徒生滋扰;在行为人应预见且能预见的讯息条件下,可得出一个行为标准,行为人若逾越之,即应负损害赔偿责任;损害对于行为人是否可预见,取决于其行为的危险性——愈是危险行为,愈是可预见。简言之,过失责任即是危险责任。一旦明乎此,私法的损害赔偿责任体系即清楚了：严格责任不再与过失责任决然可分;故意与过失也不再是心理之区分,而在于损害预见可能性的高低;契约法的归责事由不再与侵权法的过失有矛盾;公示制度效能为何决定了物权效力的范围;过失不可能分离于不法而在后认定;侵权损害赔偿责任是填补性的而非惩罚性的。

关键词：故意过失危险责任损害填补

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过渡金属掺杂氧化锌纳米线磁性研究(英文)

吉林师范大学学报（自然科学版） 2009年第3期30卷 23-24页

作者：邢国忠王丹丹沈子建吴涛南洋理工大学数理学院物理与应用物理系新加坡673371

一维(1D)氧化物纳米材料,如纳米线(NW)具有重要战略意义在基础科学和技术应用领域。这些新颖的纳米材料表现出卓越的物理性能。特别是氧化锌纳米线是有希望的基石对光电子和透明电子器件,并且经过渡金属掺杂可导致铁磁性。这里我们报道... 详细信息

一维(1D)氧化物纳米材料,如纳米线(NW)具有重要战略意义在基础科学和技术应用领域。这些新颖的纳米材料表现出卓越的物理性能。特别是氧化锌纳米线是有希望的基石对光电子和透明电子器件,并且经过渡金属掺杂可导致铁磁性。这里我们报道氧化锌纳米结构合成及其掺杂。对其物理性能进行了测量系统,它们表现出极大的潜在应用在电子和自旋电子学。

关键词：氧化锌纳米线自旋电子学

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中国花蝇科及蝇科三新种一新亚种

昆虫学报 1974年第1期17卷 93-97页

作者：范滋德上海昆虫研究所

本文记述中国花蝇科及蝇科三新种及一新亚种。除第二种外,各新种或新亚种模式标本均存上海昆虫研究所。花蝇科 1.黑胸拟花蝇 Calythea atra Fan新种(图1,2) 体长4.0毫米。头黑色。眼:高约为长的1(1/2),有少数很微的毛。额最狭处间额消... 详细信息

本文记述中国花蝇科及蝇科三新种及一新亚种。除第二种外,各新种或新亚种模式标本均存上海昆虫研究所。花蝇科 1.黑胸拟花蝇 Calythea atra Fan新种(图1,2) 体长4.0毫米。头黑色。眼:高约为长的1(1/2),有少数很微的毛。额最狭处间额消失,侧额如线,仅前方1/2长度内有额鬃,间额鬃长,间额及沿侧额鬃列一线黑色。头前面粉被略带银色的灰色。触角黑,第三节为第二节的1(1/2)倍,芒基部半段有很短的毳毛。侧颜裸,狭于触角第三节的宽,颜鬃长大,髭在口缘一线,口上片明显。颊高约为眼高

关键词：新亚种蝇科前背鬃前腹鬃额鬃背中鬃肛尾叶胫节腹侧片股节腿节背侧片间额中华人民共和国