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Interfacial charge redistribution to promote the catalytic activity of Vs-CoP-CoS_(2)/C n-n heterojunction for oxygen evolution

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Chinese Chemical Letters 2024年第2期35卷 611-616页

作者： Jiawen sun hui Xue Jing sun Niankun Guo Tianshan Song Yi-Ru Hao Qin Wang College of Chemistry and Chemical Engineering Inner Mongolia UniversityHohhot 010021China

Modulating surface charge redistribution based on interface and defect engineering has been considered as a resultful means to boost electrocatalytic ***,the mechanism of synergistic regulation of heterojunction and vacancy defects remains ***,a Vs-CoP-CoS_(2)/C n-n heterojunction with sulfur vacancies is successfully constructed,which manifests superior electrocatalytic activity for oxygen evolution,as demonstrated by a low overpotential of 170 mV to reach 10 mA/cm^(2).The experimental results and density functional theory calculations testify that the outstanding OER performance of Vs-CoP-CoS_(2)/C heterojunction is owed to the synergistic effect of sulfur vacancies and built-in electric field at n-n heterogeneous interface,which accelerates the electron transfer,induces the charge redistribution,and regulates the adsorption energy of active intermediates during the *** study affords a promising means to regulate the electrocatalytic performance by the construction of heterogeneous interfaces and defects,and in-depth explores the synergistic mechanisms of n-n heterojunction and vacancies.

关键词： Charge redistribution n-n Heterojunction Built-in electric field Sulfur vacancy Oxygen evolution reaction

A Comparative Study of the Power-law Relationship between the Pulse width and Energy of Precursor and Main Burst

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Research in Astronomy and Astrophysics 2024年第3期24卷 144-168页

作者： hui-Ying Deng Zhao-Yang Peng Jia-ming Chen Dan Zhu College of Physics and Electronic Information Yunnan Normal UniversityKunming 650500China

In gamma-ray burst prompt emission,there is still no consistent conclusion if the precursor and main burst share the same *** this paper,we try to study this issue based on the relationship between pulse width and energy of the precursor and main *** systematically search the light curve data observed by Swift/BAT and Fermi/GBM,and find 13 long bursts with well-structured precursors and main *** fitting the precursor light curve of each different energy channel with the Norris function,we find that there is not only a power-law relationship between precursor width and energy,but also a power-law relationship between the ratio of the rising width to the decaying width and *** comparing the relationship between the precursors and the main burst pulses,we find that the distribution of the precursors and the relationship between the power-law indices are roughly the same as those of the main *** addition,it is found that the precursor width distribution as well as the upper limit of the pulse width ratio does not exceed 1 and both are asymmetric,which are also consistent with the main *** indicate that the precursor and the main burst are indistinguishable,and the precursor and the main burst may have the same physical origin.

关键词： methods data analysis-(stars) gamma-ray burst general-shock waves

Simultaneously Improved Curing,Mechanical,Antioxidative Properties and Reduced ZnO Loading of Silica Filled NR Composites by Incorporation of Low-cost Crude Carbon Dots via Conventional Melt-milling Method

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Chinese Journal of Polymer Science 2024年第6期42卷 815-825页

作者： Chao-Ying sun Hai-Jun Ji Li-Wei Li hui Yang Xiao-Peng An Yi-Ping Chen ming-Jian Han Can Jiang Li-Qun Zhang Peng Yu Run-Guo Wang State Key Laboratory of Organic-Inorganic Composites Beijing University of Chemical TechnologyBeijing100029China School of Materials Science and Engineering Wuhan Institute of TechnologyWuhan430205China

Rubbers or elastomers play an important role in hi-tech technology and civilian daily life because of their unique and strategical ***,the rubber additives are essential components for rubbers’practical ***,developing novel multifunctional additives has attracted increasing research *** this work,low-cost crude carbon dots(CCDs)were used as multifunctional additives for natural rubber/silica system(without any additional modification)through industrial compatible melt-mixing *** results revealed that the CCDs could disperse well in the NR/silica system,and they could not only endow the rubber compound with excellent anti-aging capability due to CCDs’radical scavenging activity because of their plenty of nitrogen-containing species,but also improve the curing rate and mechanical performance of the rubber ***,the CCDs could reduce the rolling resistance of the rubber composites(tanδvalue at 7%strain of the rubber composite could be decreased by 34%),which is promising for the application of energy-saving tire ***,the addition of CCDs could effectively reduce the ZnO dosage by at least 40%in the rubber composite without deteriorating its ***,this work provides valuable guidance to develop novel cheap yet effective additives for the elastomer.

关键词： Natural rubber Crude carbon dots Antioxidant ZnO reduction Vulcanization

Upcycling municipal solid waste to sustainable hydrogen via two-stage gasification-reforming

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Journal of Energy Chemistry 2024年第9期96卷 611-624页

作者： hui Zhou Shuzhuang sun Yikai Xu Yeshui Zhang Shouliang Yi Chunfei Wu Department of Energy and Power Engineering Tsinghua UniversityBeijing 100084China School of Chemical Engineering Zhengzhou UniversityZhengzhou 450001HenanChina Key Laboratory for Advanced Materials and Feringa Nobel Prize Scientist Joint Research Center Frontiers Science Center for Materiobiology and Dynamic ChemistrySchool of Chemistry and Molecular EngineeringEast China University of Science and TechnologyShanghai 200237China School of Engineering University of AberdeenAberdeen AB243UEUK U.S.Department of Energy National Energy Technology LaboratoryPittsburghPA 15236USA School of Chemistry and Chemical Engineering Queen’s University BelfastBelfast BT71NNUK

As global municipal solid waste(MSW)quantities continue to escalate,serious socio-environmental challenges arise,necessitating innovative ***-to-hydrogen(WTH)via two-stage gasification-reforming(TSGR)presents an emergent technology for MSW upcycling,offering to ease waste management burdens and bolster the burgeoning hydrogen *** early initiatives to advance TSGR technology,a cohesive and critical analysis of cutting-edge knowledge and strategies to enhance hydrogen production remains *** review aggregates literature on MSW upcycling to hydrogen via TSGR,with a focus on optimizing process control and catalytic *** underscores technological avenues to augment hydrogen output,curtail catalyst costs,and refine system ***,the review illuminates the potential for integrating chemical and calcium looping into TSGR processes,identifying opportunities,and pinpointing *** review concludes with a summary of the current state of techno-economic analysis for this technology,presenting outstanding challenges and future research directions,with the ultimate goal of transitioning WTH from theoretical to practical application.

关键词： Municipal solidwaste Upcycling Gasification Reforming Hydrogen

Housing vacancy identification in shrinking cities based on multi-source data:A case study of Fushun city in Northeast China

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Journal of Geographical Sciences 2024年第1期34卷 89-111页

作者： sun Hongri ZHOU Guolei LIU Yanjun FU hui JIN Yu School of Geographical Sciences Northeast Normal UniversityChangchun 130024China Northeast Institute of Geography and Agroecology CASChangchun 130102China

Urban shrinkage has attracted the attention of many geographers and urban planners in recent ***,there are fewer studies on vacant housing in shrinking ***,this study combines multi-source remote sensing images and urban building data to assess the spatiotemporal variation patterns of housing vacancy in a typical shrinking city in *** following points were obtained:(1)We developed an evaluation model to identify vacant residential buildings in shrinking cities by removing the contribution of nighttime lights from roads and non-residential buildings;(2)The residential building vacancy rate in Fushun city significantly increased from 2013 to 2020,resulting in a significant high-value clustering *** impact of urban shrinkage on vacant residential buildings was higher than that on vacant non-residential buildings;(3)The World Pop population data demonstrated consistent spatial distribution and trend of population change in Fushun with the residential building vacancy rate results,suggesting good reliability of the constructed evaluation model in this *** housing vacancies can help the local government to raise awareness of the housing vacancy problem in shrinking cities and to propose reasonable renewal strategies.

关键词： housing vacancy residential building vacancy urban shrinkage VIIRS

Elucidation of the last steps of photo-ammonification:analytical method development and mechanism elucidation

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Frontiers of Environmental Science & Engineering 2024年第8期18卷 101-106页

作者： Yingjing Miao hui Wang Chunpeng Yang Ruochun Zhang Hao Zhang Peizhe sun School of Environmental Science and Engineering Tianjin UniversityTianjin 300072China SINOPEC Research Institute of Petroleum Processing Co. Ltd.Beijing 100083China School of Earth System Science Tianjin UniversityTianjin 300072China

The mechanisms underlying the photo-ammonification of nitrogenous organic compounds(NOCs)remain unclear,partly due to the analytical challenges of small NOC *** study introduced a simple methodology for accurately and simultaneously quantifying multiple small NOCs during ammonification *** developed method employed phenyl isothiocyanate as derivatization reagents,followed by high-performance liquid chromatography analysis to measure primary and secondary amines,amides,as well as NH4+over variable photo-ammonification *** our experimental setup,vacuum ultraviolet(VUV)irradiation serves as the controlled reaction environment to simulate harsh photo-ammonification *** NOCs,including pyridine,N,N-dimethylformamide,and acrylonitrile,were chosen due to their structural diversity and environmental relevance as model *** method was able to achieve excellent nitrogen mass balance,and revealed that the last steps of photo-ammonification involved oxidation of nitrogen-adjacent carbon to amide followed by the cleavage of N-C *** novel method may also help quantitative investigation of nitrogen transformations in different environmental contexts.

关键词： Ammonification NOCs Amines Nitrogen mass balance

Cost-effective fabrication of liquid metals via a laser induced graphene stamp for highly-stretchable integrated optoelectronics

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Nano Research 2024年第8期17卷 7603-7613页

作者： Weiqi sun Li Xiang Zebang Luo hui Wang Dong Li Anlian Pan College of Materials Science and Engineering Hunan UniversityChangsha 410082China

Stretchable electronics have found widespread applications in various fields such as wearable electronics,soft robots,and *** an important promising alternative of traditional rigid conductors,liquid metals have demonstrated immense potential to provide high conductivity and stretchability for the stretchable electronic ***,limited by their fluidity and high surface tension,challenges remain in achieving liquid metal patterns with low-cost,high-precision,large-scale,and complex ***,a fabrication technique was proposed based on laser-induced graphene(LIG)stamps to enable liquid metal self-selectively adhere to *** metal patterns could thus be achieved in different designed geometries and could be transferred onto stretchable *** liquid metal patterns exhibit exceptional electrical conductivity(3.24×10^(6)S/m even under 1000%strain),high stretchability(1000%strain,maximum of 2500%),small resistance changes under significant deformations(with a quality factor of 62.5 under 1000%strain),and high resolution(down to 50μm).Utilizing the patterned liquid metals,a stretchable integrated multifunctional optoelectronic system was demonstrated,encompassing a stretchable display matrix,a pressure sensor array,a wireless powering coil,and cardiovascular sensors,which further highlight the remarkable application potential of liquid metals in optoelectronic user-interaction and advanced physiological monitoring.

关键词： liquid metal wettability selective adhesion transfer printing stretchable electronics

Weak Merging Scenario of CLASH Cluster A209

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Research in Astronomy and Astrophysics 2024年第4期24卷 174-182页

作者： Wen-Cheng Feng Heng Yu Hai-hui Zhao Xiao-Lan Hou Shu-Mei Jia Cheng-Kui Li Yu-Lin Cheng Paolo Tozzi ming sun Yong Chen Department of Physics and Institute of Theoretical Physics Nanjing Normal UniversityNanjing 210023China Key Laboratory of Particle Astrophysics Institute of High Energy PhysicsChinese Academy of SciencesBeijing 100049China Department of Astronomy Beijing Normal UniversityBeijing 100875China Department of Astronomy Yunnan UniversityKunming 650091China INAF—Osservatorio Astrofisico di Arcetri Largo E.Fermi50122 FirenzeItaly Department of Astronomy University of VirginiaP.O.Box 400325CharlottesvilleVA 22904-4325USA

We study the structural and dynamical properties of A209 based on Chandra and XMM-Newton *** obtain detailed temperature,pressure,and entropy maps with the contour binning method,and find a hot region in the NW *** X-ray brightness residual map and corresponding temperature profiles reveal a possible shock front in the NW direction and a cold front feature in the SE *** with the galaxy luminosity density map we propose a weak merger scenario.A young sub-cluster passing from the SE to NW direction could explain the optical subpeak,the intracluster medium temperature map,the X-ray surface brightness excess,and the X-ray peak offset together.

关键词： X rays:galaxies:clusters galaxies:clusters:intracluster medium galaxies:clusters:Abell 209

Centrifuge modeling of unreinforced and multi-row stabilizing piles reinforced landslides subjected to reservoir water level fluctuation

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Journal of Rock Mechanics and Geotechnical Engineering 2024年第5期16卷 1600-1614页

作者： Chenyang Zhang Yueping Yin hui Yan Sainan Zhu ming Zhang Luqi Wang Department of Civil Engineering The University of Hong KongHong KongChina China Institute of Geo-environment Monitoring BeijingChina Chongqing 107 Municipal Construction Engineering Co. Ltd.ChongqingChina Faculty of Engineering China University of GeosciencesWuhanChina School of Civil Engineering Chongqing UniversityChongqingChina

With the construction of the Three Gorges Reservoir dam,frequent reservoir landslide events have been *** recent years,multi-row stabilizing piles(MRSPs)have been used to stabilize massive reservoir landslides in *** this study,two centrifuge model tests were carried out to study the unreinforced and MRSP-reinforced slopes subjected to reservoir water level(RWL)operation,using the Taping landslide as a *** results indicate that the RWL rising can provide lateral support within the submerged zone and then produce the inward seepage force,eventually strengthening the slope ***,a rapid RWL drawdown may induce outward seepage forces and a sudden debuttressing effect,consequently reducing the effective soil normal stress and triggering partial pre-failure within the RWL fluctuation ***,partial deformation and subsequent soil structure damage generate excess pore water pressures,ultimately leading to the overall failure of the reservoir *** study also reveals that a rapid increase in the downslope driving force due to RWL drawdown significantly intensifies the lateral earth pressures exerted on the ***,the MRSPs possess a considerable reinforcement effect on the reservoir landslide,transforming the overall failure into a partial deformation and failure situated above and in front of the *** mechanical transfer behavior observed in the MRSPs demonstrates a progressive alteration in relation to RWL *** the RWL rises,the mechanical states among MRSPs exhibit a growing *** shear force transfer factor(*** ratio of shear forces on pile of the n th row to that of the first row)increases significantly with the RWL *** indicates that the mechanical states among MRSPs tend toward an enhanced *** insights gained from this study contribute to a more comprehensive understanding of the failure mechanisms of reservoir landslides and the mechanical behavior of M

关键词： Reservoir landslide Failure mechanism Multi-row stabilizing piles Mechanical behavior