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Progress of vegetation modelling and future research prospects

Science China Earth Sciences 2024年第9期67卷 2718-2738页

作者： siqi li Xu ZHANG Zhengyao LU Jian NI Jianhua LU State Key Laboratory of Tibetan Plateau Earth System Resources and Environment(TPESRE)Institute of Tibetan Plateau ResearchChinese Academy of SciencesBeijing 100101China College of Resources and Environment University of Chinese Academy of SciencesBeijing 100049China British Antarctic Survey Cambridge CB30ETUnited Kingdom Department of Physical Geography and Ecosystem Science Lund UniversityLund 22362Sweden College of life Sciences Zhejiang Normal UniversityJinhua 321004China School of Atmospheric Sciences Sun Yat-sen University and Southern Marine Science and Engineering Guangdong Laboratory(Zhuhai)Zhuhai 519082China

Terrestrial vegetation is a crucial component of the Earth system,and its changes not only represent one of the most distinct aspects of climate change but also exert significant feedback within the climate system by exchanging energy,moisture,and carbon *** quantitatively and mechanistically study climate-vegetation feedback,numerical vegetation models have been developed on the theory of ecophysiological constraints on plant functional *** models eventually can simulate vegetation distribution and succession across different spatial and temporal scales,and associated terrestrial carbon cycle processes by categorizing vegetation into biomes according different plant functional types and their associated environmental *** we review the developing history of vegetation models and provide recent advances and future *** 21st century,static vegetation models,as developed statistical models,can only simulate equilibrated characteristics of vegetation *** last several decades,Dynamic Global Vegetation Models(DGVMs)have been developed to simulate instantaneous responses of vegetation to climate change and associated dynamics,and can be coupled with Earth system models to investigate interactions among atmosphere,ocean,and *** are also widely applied to investigate the dynamics accounting for changes in the geographic distribution patterns of land surface vegetation at different spatial and temporal scales and to assess the impacts of terrestrial carbon and water fluxes and land use *** suggest that future vegetation modeling could integrate with machine learning,and explore vegetation transient response and feedback as well as impacts of process hierarchies and human activities on climate and ecosystem.

关键词： Vegetation models DGVMs Ecosystems Plant functional types Plant functional traits

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Refining the Factors Affecting N_(2)O Emissions from Upland Soils with and without Nitrogen Fertilizer Application at a Global Scale

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Advances in Atmospheric Sciences 2024年第9期41卷 1804-1820页

作者： Wenqian JIANG siqi li Yong li Meihui WANG Bo WANG Ji liU Jianlin SHEN Xunhua ZHENG State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry Institute of Atmospheric PhysicsChinese Academy of SciencesBeijing 100029China Key Laboratory for Agro-ecological Processes in Subtropical Regions Institute of Subtropical AgricultureChinese Academy of SciencesChangsha 410125China Changsha Research Station for Agricultural&Environmental Monitoring Chinese Academy of SciencesChangsha 410125China University of Chinese Academy of Sciences Beijing 100049China State Environmental Protection Key Laboratory of Formation and Prevention of the Urban Air Pollution Complex Shanghai Academy of Environment SciencesShanghai 200233China Institute of Carbon Neutrality Qilu ZhongkeJinan 251699China Hubei Province Key Laboratory for Geographical Process Analysis and Simulation Central China Normal UniversityWuhan 430079China Department of Ecohydrology Leibniz Institute of Freshwater Ecology and Inland FisheriesBerlin 12587Germany Key laboratory of Environment Change and Resources Use in Beibu Gulf Ministry of EducationNanning Normal UniversityNanning 530001China Golden Mantis school of Architecture Soochow UniversitySuzhou 215123China

Nitrous oxide(N_(2)O)is a long-lived greenhouse gas that mainly originates from agricultural *** and more studies have explored the sources,influencing factors and effective mitigation measures of N_(2)O in recent ***,the hierarchy of factors influencing N_(2)O emissions from agricultural soils at the global scale remains *** this study,we carry out correlation and structural equation modeling analysis on a global N_(2)O emission dataset to explore the hierarchy of influencing factors affecting N_(2)O emissions from the nitrogen(N)and non-N fertilized upland farming systems,in terms of climatic factors,soil properties,and agricultural *** results show that the average N_(2)O emission intensity in the N fertilized soils(17.83 g N ha^(-1)d^(-1))was significantly greater than that in the non-N fertilized soils(5.34 g N ha^(−1) d^(−1))(plimate factors and agricultural practices are the most important influencing factors on N_(2)O emission in non-N and N fertilized upland soils,*** different climatic zones,without fertilizer,the primary influence factors on soil N_(2)O emissions are soil physical properties in subtropical monsoon zone,whereas climatic factors are key in the temperate *** fertilizer,the primary influence factors for subtropical monsoon and temperate continental zones are soil physical properties,while agricultural measures are the main factors in the temperate monsoon *** enhanced agricultural practices,such as reduced N fertilizer rate combined with the addition of nitrification and urease inhibitors can potentially mitigate N_(2)O emissions by more than 60%in upland farming systems.

关键词： N_(2)O emissions influencing factors nitrogen cycling upland farming systems

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Single-atom photo-catalysts:Synthesis,characterization,and applications

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Nano Materials Science 2024年第3期6卷 284-304页

作者： siqi li Ziwang Kan He Wang Jiaxiao Bai Yunyi liu Song liu Yingjie Wu College of Chemistry Chemical Engineering and Resource UtilizationNortheast Forestry UniversityHarbin150040China School of Medicine and Health Harbin Institute of TechnologyHarbin150001China

Single-atom catalysts(SACs)are gaining popularity in catalytic reactions due to their nearly 100%atomic utilization and defined active sites,which provide great convenience for studying the catalytic mechanism of ***,SACs still present challenges such as complex formation processes,low loading and easy agglomeration of ***,we systematically discuss the synthesis methods for SACs,including coprecipitation,impregnation,atomic layer deposition,pyrolysis and Anti-Ostwald ripening *** techniques for characterizing single-atom catalysts(SACs)are described in *** utilization of individual atoms in various photocatalytic reactions and their mechanisms of action in different reactions are *** purpose of this review is to introduce single-atom synthesis methods,characterization techniques,specific catalytic action and their applications in the direction of photocatalysis,and to provide a reference for the industrialization of photocatalytic single-atoms,which is currently impossible,in the hope of promoting further development of photocatalytic single-atoms.

关键词： Photocatalysis Single atom Catalytic mechanism

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Hypolipidemic activity and mechanism of active components of Dracocephalum moldavica L. tea

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Food Science and Human Wellness 2024年

作者： siqi li Qinyu li Na Zhang Minhui li Inner Mongolia Autonomous Region Hospital of Traditional Chinese Medicine Inner Mongolia Traditional Chinese and Mongolian Medical Research Institute Department of Pharmacy， Baotou Medical College

Hyperlipidemia is associated with many diseases and considered the main contributing factor in the development of metabolic syndrome. The traditional Mongolian medicine Dracocephalum moldavica L. (D. moldavica) is commonly consumed as a tea (non-Camellia tea) for the prevention and treatment of coronary heart disease， hypertension， atherosclerosis， and other diseases. Here， we attempted to investigate the hypolipidemic activity and mechanisms underlying the active components of D. moldavica. First， the mechanism underlying the lipid accumulation-reducing effects of the D. moldavica ethanol extract was determined using in vitro experiments， and four polar fractions were screened for activity. Then， the effect of the ethyl acetate fraction of D. moldavica (EAD) on lowering blood lipid was confirmed in vivo. The combination of network pharmacological and serum pharmacochemistry analyses showed that apigenin， luteolin， and naringenin of EAD existed in prototype form in the drug-containing serum of rats. We also determined the content of the three active ingredients in EAD. Finally， in vitro experiments showed that apigenin， luteolin， and naringenin improved oleic acid-induced lipid accumulation in HepG2 cells by regulating the PPAR signaling pathway (PPARα， CPT1， and FABP3). Our findings provide mechanistic insights and application prospects for the prevention and treatment of hypolipidemia using D. moldavica.

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Circularly polarized lasing from chiral metal-organic frameworks

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Photonics Research 2024年第8期12卷 1654-1664页

作者： DEXIANG ZHU ZHOUYUANHANG WANG XIANGYU XU WENYU DU WEI HUANG YAN KUAI BENli YU JIANZHONG ZHENG ZHIJIA HU siqi li Information Materials and Intelligent Sensing Laboratory of Anhui Province Hefei 230601China School of Physics and Optoelectronic Engineering Anhui UniversityHefei 230601China Key Laboratory of Opto-Electronic Information Acquisition and Manipulation of Ministry of Education Hefei 230601China School of Environmental Science and Engineering Nanjing Tech UniversityNanjing 211816China

Circularly polarized lasers play a pivotal role in classical optics,nanophotonics,and quantum optical information processing,while their fabrication remains *** article begins with examining the interactions between stimulated emission and chiral matter,outlining a simple strategy for producing circularly polarized lasing from chiral metal-organic frameworks(MOFs),such as the zeolitic imidazolate framework(ZIF),embedded with achiral laser dyes(L∕D-ZIF?dyes).It is found that the stimulated emission threshold and intensity are influenced by the interplay between the chiral polarization of the pump light and the inherent chirality of the MOF *** further present the design of a chiral vertical-cavity surface-emitting laser(VCSEL),comprising an L∕D-ZIF?dyes solid-state film sandwiched between a high-reflectivity distributed Bragg reflector(DBR)mirror and a silver *** cavity-based lasing exhibits higher asymmetry between emitting left-handed and right-handed polarized light compared to chiral spontaneous emission(SE)and amplified spontaneous emission(ASE),with an asymmetry value glum of approximately±*** value is nearly four-fold greater than that of SE and twice that of *** findings reveal a new approach to amplify chiral signals,promoting the comprehension and application of chiral–matter interactions,and offering a simple yet effective strategy to fabricate chiral lasers.

关键词： chiral polarized lasing

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In-situ fabrication of TiO2/NH2-MIL-125（Ti） via MOF-driven strategy to promote efficient interfacial effects for enhancing photocatalytic NO removal activity

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Chinese Chemical Letters 2024年第10期35卷 415-419页

作者： Maosen Xu Pengfei Zhu Qinghong Cai Meichun Bu Chenghua Zhang Hong Wu Youzhou He Min Fu siqi li Xingyan liu Chongqing Key Laboratory of Catalysis and New Environmental Materials College of Environment and Resources Chongqing Technology and Business University School of Pharmacy North Sichuan Medical College State Key Joint Laboratory of Environment Simulation and Pollution Control School of Environment Tsinghua University

Deep oxidation of NO molecules to nitrate species by photocatalysis with virtually no toxic byproduct NO2generation is a challenging task. In this study, Ti O2in-situ grows based on NH2-MIL-125（Ti）(NM-125) not only inhibited TiO 2agglomeration, but also contacted more tightly to obtain efficient interfacial effects, thus displaying excellent photocatalytic NO removal activity（68.08%）. The formation of Ti O2is directly confirmed by characterizations such as X-ray diffraction（XRD）, transmission electron microscope（TEM）, X-ray photoelectron spectroscopy（XPS）. Meanwhile, UV–vis, photoluminescence, and photoelectrochemical analysis indicate that TiO2formation effectively improves the optical properties. Moreover,the strong electron interaction and electron transport direction between NM-125 and Ti O2are investigated by density functional theoretical（DFT） calculation. Finally, combined with the results of electron spin resonance（ESR） and in-situ FT-IR test, the intermediate processes of NO adsorption and photocatalytic oxidation reaction are discussed in depth, where the production of reactive oxygen species（ROS）under light is the key factor in the successful degradation of NO. Compared with NM-125 which can only produce·OH through photogenerated electrons since the lower valence band position, NMT-2 can directly produce·OH through photogenerated holes, thereby relieving the pressure on photogenerated electrons and producing more ROS. This study will provide reasonable guidance for the modification of NM-125 for photocatalytic removal of ppb-level NO.

关键词： NH2-MIL-125(Ti) NO removal Photocatalysis ROS TiO2

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Single-atom Pd anchored in the porphyrin-center of ultrathin 2D-MOFs as the active center to enhance photocatalytic hydrogen-evolution and NO-removal

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Chinese Chemical Letters 2024年第9期35卷 364-368页

作者： Xingyan liu Chaogang Jia Guangmei Jiang Chenghua Zhang Mingzuo Chen Xiaofei Zhao Xiaocheng Zhang Min Fu siqi li Jie Wu Yiming Jia Youzhou He Chongqing Key Laboratory of Catalysis and New Environmental Materials College of Environment and ResourcesChongqing Technology and Business UniversityChongqing 400067China School of Pharmacy North Sichuan Medical CollegeNanchong 637100China Carbon Neutrality Technology Application Research Center College of River and Ocean EngineeringChongqing Jiaotong UniversityChongqing 400074China State Key Joint Laboratory of Environment Simulation and Pollution Control School of EnvironmentTsinghua UniversityBeijing 100084China National Local Joint Engineering Research Center for Road Engineering and Disaster Prevention and Reduction Technology in Mountainous Areas China Merchants Chongqing Communications Technology Research and Design Institute Co.Ltd.Chongqing 400067China Chongqing Culture Relics and Archaeology Research Institute Chongqing 400013China

Single-atom catalysts were widely used to treat atmospheric pollution and alleviate energy crises through ***,how to prevent the aggregation of single atoms during the preparation and catalytic processes remained a great ***,a novel ultrathin two-dimensional porphyrin-based single-atom photocatalyst Ti-MOF(abbreviated as TMPd)obtained through a simple hydrothermal synthesis strategy was used for photocatalytic hydrogen evolution and NO removal,in which the singleatom Pd tightly anchored in the center of porphyrin to ensure single-atom Pd stable *** with most reported MOFs-based photocatalysts,the TMPd showed an excellent hydrogen evolution rate(1.32 mmol g^(-1)h^(-1))and the NO removal efficiency(62%)under visible light *** high-angle annular dark-field scanning transmission electron microscope(HAADF-STEM)and synchrotron-radiation-based X-ray absorption fine-structure spectroscopy(XAFS)proved that pd in TMPd existed in an isolated state,and the atomic force microscope(AFM)proved the ultrathin morphology of *** calculations had demonstrated that single-atom Pd could serve as the active center and more effectively achieve electron transfer,indicating that single-atom Pd played a vital role in photocatalytic hydrogen *** addition,a possible photocatalytic pathway of NO removal was proposed based on ESR and in-situ infrared spectra,in which the catalysts anchored with single-atom Pd could produce more active substances and more effectively oxidize NO to NO_(2)^(-)or NO_(3)^(-).The results suggested that coordinating single-atom metal species as the active site in the center of porphyrin could be a feasible strategy to obtain various ultrathin porphyrin-based single-atom photocatalysts to acquire excellent photocatalytic performance further.

关键词： Porphyrin-based MOFs Single-atom Pd Ultrathin 2D nanosheets Hydrogen evolution NO removal

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辽代《耶律善庆墓志》补释

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文献 2024年第1期 135-142页

作者：李思齐上海交通大学外国语学院

2018年《辽金历史与考古》上公开了一方辽代墓志,被命名为《耶律善庆墓志》。经辨认对比,《耶律善庆墓志》与内蒙古大学藏契丹小字《故侍中墓志铭》出土于同一墓葬。墓主人耶律善庆即《辽史》有载的耶律蘂奴,为辽代后期重要的政治人物。

关键词：《耶律善庆墓志》《故侍中墓志铭》仲父房耶律善庆

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基于图像识别仿生木纹的三维打印路径规划方法

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同济大学学报（自然科学版） 2024年第2期52卷 268-275页

作者：于颖白捷仁李帅帅李思齐王玉同济大学机械与能源工程学院上海201804 同济大学中德工程学院上海201804

针对传统三维打印采用的诸如网格、三角等均匀同构介观结构填充存在结构效率低、与承载零件应力场不协调等问题,受自然生长的木纹可提高木材整体性能的启发,提出基于图像识别仿生木纹的三维打印路径规划方法,旨在借鉴木材的纤维排布以... 详细信息

针对传统三维打印采用的诸如网格、三角等均匀同构介观结构填充存在结构效率低、与承载零件应力场不协调等问题,受自然生长的木纹可提高木材整体性能的启发,提出基于图像识别仿生木纹的三维打印路径规划方法,旨在借鉴木材的纤维排布以改善零件的机械性能。通过木材铣削分层,依次提取各层图像木纹并生成对应打印路径,并逐层打印出仿生木纹试件。拉伸试验结果表明:相比同质量的网格填充、三角填充、直线填充三种传统均匀同构填充试件,基于仿生木纹的非均匀异构打印试件最大拉伸载荷分别提高了115.03%、72.89%、64.39%,证明了基于仿生木纹的非均匀介观填充结构能够显著提高打印件拉伸强度。

关键词：仿生木纹介观结构图像识别路径规划三维打印

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硫氧镁泡沫水泥吸波材料的制备及性能

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建筑材料学报 2024年第4期27卷 291-298页

作者：崔宝栋刘军李思琪李瑶邓永刚沈阳理工大学材料科学与工程学院辽宁沈阳110159

采用具有优良吸波性能的铁氧体和碳化硅来改性硫氧镁水泥泡沫板,研究了铁氧体和碳化硅掺量对改性硫氧镁水泥吸波性能的影响,并通过X射线衍射及扫描电子显微镜分析了其影响机理.结果表明:在3.95~18.00 GHz目标频段下,掺加5%碳化硅改性硫... 详细信息

采用具有优良吸波性能的铁氧体和碳化硅来改性硫氧镁水泥泡沫板,研究了铁氧体和碳化硅掺量对改性硫氧镁水泥吸波性能的影响,并通过X射线衍射及扫描电子显微镜分析了其影响机理.结果表明:在3.95~18.00 GHz目标频段下,掺加5%碳化硅改性硫氧镁水泥的最低反射率出现在8.40 GHz处,为-15.9 dB;掺加15%铁氧体改性硫氧镁水泥的最低反射率出现在7.04 GHz处,为-17.3 dB;铁氧体和碳化硅按照一定比例掺加到硫氧镁水泥基体中,均表现出良好的吸波性能.

关键词：硫氧镁水泥碳化硅铁氧体吸波性能

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