检索结果-南通市图书馆

Dual metal ions/BNQDs boost PMS activation over copper tungstate photocatalyst for antibiotic removal:Intermediate,toxicity assessment and mechanism

引用

Journal of Materials Science & Technology 2024年第3期170卷 11-24页

作者： Ruyao Chen Haiyue Zhang Yuming Dong Haifeng shi School of Science Jiangnan UniversityWuxi214122China The Key Laboratory of Synthetic and Biological Colloids Ministry of EducationJiangnan UniversityWuxi214122China National Laboratory of Solid State Microstructures Nanjing UniversityNanjing210093China

In the metal-based peroxymonosulfate(PMS)activation process,the sluggish surface redox cycle of metal ions generally hampered the efficiency of PMS activation for pollutant ***,Codoped CuWO 4/BN quantum dots(CW/Co/BNQDs)photocatalysts were developed to realize Cu^(2+)/Cu+and Co^(2+)/Co^(3+)dual ions redox cycles for PMS activation,which would facilitate the tetracycline(TC)***/4Co/2BNQDs could degrade 94.8%TC within 30 min in PMS/Vis system,and the apparent rate constant of CW/4Co/2BNQDs was 2.7 times and 1.2 times higher than those of CW and CW/4Co,*** improved TC degradation performance could be attributed to the synergetic effect between BNQDs and dual redox cycles.X-ray photoelectron spectroscopy(XPS)spectra of samples before and after the reaction demonstrated that BNQDs were beneficial for accelerating the Cu^(2+)/Cu+and Co^(2+)/Co^(3+)redox cycles in CW/4Co/2BNQDs,further boosting the activation of PMS in TC *** of different radical scavengers revealed that the SO_(4)^(·−)/·OH/h+/^(1)O_(2)reactive species participated in the PMS activation for the TC degradation *** possible TC degradation pathway and intermediate toxicity were detailed *** addition,CW/4Co/2BNQDs exhibited outstanding photocatalytic activity over five consecutive cycles,which illustrated that it was supposed to be a reliable PMS activator over antibiotic elimination for practical *** this work shed new light on constructing dual redox cycles for efficient PMS activation.

关键词： Dual redox cycles Photocatalysis Peroxymonosulfate BN quantum dots Toxicity assessment

来源：

维普期刊数据库评论

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

A low-power Bluetooth-based wireless sensor network and its global confliction-solving impact localization method

引用

Chinese Journal of Aeronautics 2024年第1期37卷 153-161页

作者： Yuanjia WANG Lei QIU Qiyun XU Liming shi College of Aerospace Engineering Nanjing University of Aeronautics and AstronauticsNanjing 210016China Department of Electrical and Electronic Engineering University of EdinburghEdinburgh EH89YLUK

During the whole service lifetime of aircraft structures with composite materials,impacts are inevitable and can usually cause severe but barely visible *** the occurrences of impact are random and unpredictable,it is a hotspot direction to develop an online impact monitoring system that can meet strict limitations of aerospace applications including small size,light weight,and low power ***(PZT)sensor,being able to generate impact response signals with no external power and cover a large-scale structure with only a small amount of them,is a promising ***,for real systems,networks with multiple nodes are normally required to monitor large-scale structures in a global way to identify any impact localization confliction,yet the existing studies are mostly evaluated with single nodes instead of ***,in this paper,based on a new low-power node designed,a Bluetooth-based digital impact monitoring PZT sensor network is proposed for the first time with its global confliction-solving impact localization *** of the system as a network are researched and analyzed on a complex real aircraft wing box for a global confliction-solving impact localization,showing a satisfying high accuracy.

关键词： Bluetooth-based low-power design Confliction-solving evaluation Complex composites Piezoelectric sensors Wireless impact monitoring network

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

Fixed-Time Gradient Flows for Solving Constrained Optimization: A Unified Approach

引用

IEEE/CAA Journal of Automatica Sinica 2024年第8期11卷 1849-1864页

作者： Xinli shi Xiangping Xu Guanghui Wen Jinde Cao School of Cyber Science and Engineering Southeast UniversityNanjing 210096China School of Mathematics Southeast UniversityNanjing 210096China

The accelerated method in solving optimization problems has always been an absorbing *** on the fixedtime(FxT)stability of nonlinear dynamical systems,we provide a unified approach for designing FxT gradient flows(FxTGFs).First,a general class of nonlinear functions in designing FxTGFs is provided.A unified method for designing first-order FxTGFs is shown under Polyak-Łjasiewicz inequality assumption,a weaker condition than strong *** there exist both bounded and vanishing disturbances in the gradient flow,a specific class of nonsmooth robust FxTGFs with disturbance rejection is *** the strict convexity assumption,Newton-based FxTGFs is given and further extended to solve time-varying ***,the proposed FxTGFs are further used for solving equation-constrained ***,an FxT proximal gradient flow with a wide range of parameters is provided for solving nonsmooth composite *** show the effectiveness of various FxTGFs,the static regret analyses for several typical FxTGFs are also provided in ***,the proposed FxTGFs are applied to solve two network problems,i.e.,the network consensus problem and solving a system linear equations,respectively,from the perspective of ***,by choosing component-wisely sign-preserving functions,these problems can be solved in a distributed way,which extends the existing *** accelerated convergence and robustness of the proposed FxTGFs are validated in several numerical examples stemming from practical applications.

关键词： Consensus constrained optimization disturbance rejection linear equations fixed-time gradient flow(FxTGF).

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

Role of catalyst surface-active sites in the hydrogenation ofα,β-unsaturated aldehyde

引用

Frontiers of Chemical Science and Engineering 2024年第6期18卷 41-69页

作者： Haixiang shi Tongming Su Zuzeng Qin Hongbing Ji School of Chemistry and Chemical Engineering Guangxi Key Laboratory of Petrochemical Resource Processing and Process Intensification TechnologyGuangxi UniversityNanning 530004China Zhejiang Green Petrochemical and Light Hydrocarbon Transformation Research Institute Zhejiang University of TechnologyHangzhou 310014China

As an important technology in fine chemical production,the selective hydrogenation ofα,β-unsaturated aldehydes has attracted much attention in recent *** the process ofα,β-unsaturated aldehyde hydrogenation,a conjugated system is formed between>C=CC=O,leading to hydrogenation at both ends of the conjugated system,which competes with each other and results in more complex ***,improving the reaction selectivity is also difficult in industrial ***,many researchers have reported that surface-active sites on catalysts play a crucial role inα,β-unsaturated aldehyde *** review attempts to summarize recent advances in understanding the effects of surface-active sites(SASs)over metal catalysts for enhancing the process of *** construction strategies and roles of SASs for hydrogenation catalysts are *** attention has been given to the adsorption configuration and transformation mechanism ofα,β-unsaturated aldehydes on catalysts,which contributes to understanding the relationship between SASs and hydrogenation *** addition,recent advances in metal-supported catalysts for the selective hydrogenation ofα,β-unsaturated aldehydes to understand the role of SASs in hydrogenation are briefly ***,the opportunities and challenges will be highlighted for the future development of the precise construction of SASs.

关键词： α,β-unsaturatedd aldehydes hydrogenation active site cinnamaldehyde

来源：

维普期刊数据库评论

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Hierarchical multihead self-attention for time-series-based fault diagnosis

引用

Chinese Journal of Chemical Engineering 2024年第6期70卷 104-117页

作者： Chengtian Wang Hongbo shi Bing Song Yang Tao Key Laboratory of Smart Manufacturing in Energy Chemical Process of the Ministry of Education East China University of Science and TechnologyShanghai 200237China

Fault diagnosis is important for maintaining the safety and effectiveness of chemical *** the multivariate,nonlinear,and dynamic characteristic of chemical process,many time-series-based data-driven fault diagnosis methods have been developed in recent ***,the existing methods have the problem of long-term dependency and are difficult to train due to the sequential way of *** overcome these problems,a novel fault diagnosis method based on time-series and the hierarchical multihead self-attention(HMSAN)is proposed for chemical ***,a sliding window strategy is adopted to construct the normalized time-series ***,the HMSAN is developed to extract the time-relevant features from the time-series process *** improves the basic self-attention model in both width and *** the multihead structure,the HMSAN can pay attention to different aspects of the complicated chemical process and obtain the global dynamic ***,the multiple heads in parallel lead to redundant information,which cannot improve the diagnosis *** the hierarchical structure,the redundant information is reduced and the deep local time-related features are further ***,a novel many-to-one training strategy is introduced for HMSAN to simplify the training procedure and capture the long-term ***,the effectiveness of the proposed method is demonstrated by two chemical *** experimental results show that the proposed method achieves a great performance on time-series industrial data and outperforms the state-of-the-art approaches.

关键词： Self-attention mechanism Deep learning Chemical process Time-series Fault diagnosis

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

Reoxidation of liquid steel and evolution of inclusions during protective atmosphere electroslag remelting of Ce-containing heat-resistant stainless steel

引用

Journal of Iron and Steel Research International 2024年第8期31卷 1923-1935页

作者： Yu Zhao Cheng-bin shi shijun Wang Peng Ren Jing Li State Key Laboratory of Advanced Metallurgy University of Science and Technology Beijing(USTB)Beijing 100083China

The evolution of Ce-containing inclusions and its correlation with the reoxidation of liquid steel during protective atmosphere electroslag remelting(ESR)of heat-resistant steel were *** reoxidation of liquid steel took place during the ESR,resulting in the oxygen pickup from 0.0014 to 0.0053 wt.%.The inclusions in the consumable electrode,liquid metal pool and remelted ingot are Ce_(2)O_(2)S and Ce_(2)O,inclusions *** inclusions in the remelted ingot are originated from three ways:(I)the original inclusions from the electrode;(Il)the newly formed Ce_(2)O_(2)S and Ce_(2)O_(3) inclusions in the liquid metal pool by reoxidation remaining still in remelted ingot;(IlI)the newly generated Ce2O2S and Ce_(2)O_(3) inclusions during cooling and solidification of liquid *** relative proportions of Ce_(2)O_(3) inclusions in liquid metal pool and remelted ingot are 41% and 76.5%,*** inclusions ranging from 2 to 5μm in the remelted ingot take up 55%,followed by the inclusions smaller than 2μm(43%of total inclusions).The number proportion of the Ce_(2)0,inclusions in the liquid metal pool which were removed by floating up into slag is 1.96×10-5%.

关键词： Non-metallic inclusion Electroslag remelting Rare earth cerium Reoxidation Inclusion evolution

来源：

维普期刊数据库评论

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Quaternion-Based Adaptive Trajectory Tracking Control of a Rotor-Missile with Unknown Parameters Identification

引用

Defence Technology（防务技术） 2024年第1期31卷 375-386页

作者： Jie Zhao Zhongjiao shi Yuchen Wang Wei Wang Beijing Institute of Technology Beijing 100081China

This paper investigates the adaptive trajectory tracking control problem and the unknown parameter identification problem of a class of rotor-missiles with parametric system ***,considering the uncertainty of structural and aerodynamic parameters,the six-degree-of-freedom(6Do F) nonlinear equations describing the position and attitude dynamics of the rotor-missile are established,respectively,in the inertial and body-fixed reference ***,a hierarchical adaptive trajectory tracking controller that can guarantee closed-loop stability is proposed according to the cascade characteristics of the 6Do F ***,a memory-augmented update rule of unknown parameters is proposed by integrating all historical data of the regression *** long as the finitely excited condition is satisfied,the precise identification of unknown parameters can be ***,the validity of the proposed trajectory tracking controller and the parameter identification method is proved through Lyapunov stability theory and numerical simulations.

关键词： Rotor-missile Adaptive control Parameter identification Quaternion control

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

Diffractive neural networks with improved expressive power for gray-scale image classification

引用

Photonics Research 2024年第6期12卷 1159-1166页

作者： MINJIA ZHENG WENZHE LIU LEI shi JIAN ZI State Key Laboratory of Surface Physics Key Laboratory of Micro-and Nano-Photonic Structures(Ministry of Education)and Department of PhysicsFudan UniversityShanghai 200433China Institute for Nanoelectronic Devices and Quantum Computing Fudan UniversityShanghai 200433China Collaborative Innovation Center of Advanced Microstructures Nanjing UniversityNanjing 210093China Shanghai Research Center for Quantum Sciences Shanghai 210315China

In order to harness diffractive neural networks(DNNs)for tasks that better align with real-world computer vision requirements,the incorporation of gray scale is ***,DNNs are not powerful enough to accomplish gray-scale image processing tasks due to limitations in their expressive *** our work,we elucidate the relationship between the improvement in the expressive power of DNNs and the increase in the number of phase modulation layers,as well as the optimization of the Fresnel number,which can describe the diffraction *** demonstrate this point,we numerically trained a double-layer DNN,addressing the prerequisites for intensitybased gray-scale image ***,we experimentally constructed this double-layer DNN based on digital micromirror devices and spatial light modulators,achieving eight-level intensity-based gray-scale image classification for the MNIST and Fashion-MNIST data *** optical system achieved the maximum accuracies of 95.10%and 80.61%,respectively.

关键词： process mirror limitations

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

Neural Network Robust Control Based on Computed Torque for Lower Limb Exoskeleton

引用

Chinese Journal of Mechanical Engineering 2024年第2期37卷 83-99页

作者： Yibo Han Hongtao Ma Yapeng Wang Di shi Yanggang Feng Xianzhong Li Yanjun shi Xilun Ding Wuxiang Zhang School of Mechanical Engineering and Automation Beihang UniversityBeijing 100191China Beihang Goer(WeiFang)Intelligent Robot Co. Ltd.Beihang UniversityWeifangChina Research Center of Satellite Technology Harbin Institute of TechnologyHarbinChina Beijing Xinfeng Aerospace Equipment Co. LtdBeijingChina

The lower limb exoskeletons are used to assist wearers in various scenarios such as medical and industrial *** modeling errors of the exoskeleton in different application scenarios pose challenges to the robustness and stability of its control *** Radial Basis Function(RBF)neural network is used widely to compensate for modeling *** order to solve the problem that the current RBF neural network controllers cannot guarantee the asymptotic stability,a neural network robust control algorithm based on computed torque method is proposed in this paper,focusing on trajectory *** innovatively incorporates the robust adaptive term while introducing the RBF neural network term,improving the compensation ability for modeling *** stability of the algorithm is proved by Lyapunov method,and the effectiveness of the robust adaptive term is verified by the *** wearing the exoskeleton under different walking speeds and scenarios were carried out,and the results show that the absolute value of tracking errors of the hip and knee joints of the exoskeleton are consistently less than 1.5°and 2.5°,*** proposed control algorithm effectively compensates for modeling errors and exhibits high robustness.

关键词： Lower limb exoskeleton Model compensation RBF neural network Computed torque method

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

Evicting and filling attack for linking multiple network addresses of Bitcoin nodes

引用

Cybersecurity 2024年第3期7卷 49-68页

作者： Huashuang Yang Jinqiao shi Yue Gao Xuebin Wang Yanwei Sun Ruisheng shi Dongbin Wang School of Cyberspace Security Bejing University of Posts and TelecommunicationsBeijingChina Tsinghua University Bejing 100084China Institute of Information Engineering Chinese Academy of SciencesBeijingChina

Bitcoin is a decentralized P2P *** supports users to use pseudonyms instead of network addresses to send and receive transactions at the data layer,hiding users'real network *** transaction tracing attack cuts through the network layer to directly associate each transaction with the network address that issued it,thus revealing the sender's network *** this attack can be mitigated by Bitcoin's network layer privacy *** Bitcoin protects the unlinkability of Bitcoin addresses and there may be a many-to-one relation-ship between addresses and nodes,transactions sent from the same node via different addresses are seen as com-ing from different nodes because attackers can only use addresses as node *** this paper,we proposed the evicting and flling attack to expose the correlations between addresses and cluster transactions sent from different addresses of the same *** attack exploited the unisolation of Bitcoin's incoming connection processing *** particular,an attacker can utilize the shared connection pool and deterministic connection eviction strategy to infer the correlation between incoming and evicting connections,as well as the correlation between releasing and flling *** on inferred results,different addresses of the same node with these connections can be linked together,whether they are of the same or different network *** designed a multi-step attack procedure,and set reasonable attack parameters through analyzing the factors that affect the attack effciency and *** mounted this attack on both our self-run nodes and multi-address nodes in real Bitcoin network,achieving an aver-age accuracy of 96.9% and 82%,***,we found that the attack is also applicable to Zcash,Litecoin,Dogecoin,Bitcoin Cash,and *** analyzed the cost of network-wide attacks,the application scenario,and proposed countermeasures of this attack.

关键词： Security and privacy Bitcoin Address linking

来源：

维普期刊数据库评论

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

欢迎您,

建议与咨询留下您的常用邮箱和电话号码，以便我们向您反馈解决方案和替代方法

时间限定

文献类型

馆藏选择

核心期刊

语言

文献类型

帮助

文字说明：

检索规则说明：

检索范例：

分类表

所选分类

限定检索结果

文献类型

馆藏范围

日期分布

学科分类号

主题

机构

作者

语言

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

请选择保存的检索档案：

请选择收藏分类：

通借通还

欢迎您,

建议与咨询 留下您的常用邮箱和电话号码，以便我们向您反馈解决方案和替代方法

时间限定

文献类型

馆藏选择

核心期刊

语言

文献类型

帮助

文字说明：

检索规则说明：

检索范例：

分类表

所选分类

限定检索结果

文献类型

馆藏范围

日期分布

学科分类号

主题

机构

作者

语言

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

请选择保存的检索档案： 新增检索档案 确定 取消

请选择收藏分类： 新增自定义分类 确定 取消

通借通还

建议与咨询留下您的常用邮箱和电话号码，以便我们向您反馈解决方案和替代方法

请选择保存的检索档案：

请选择收藏分类：