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High-performance,stable CoNi LDH@Ni foam composite membrane with innovative peroxymonosulfate activation for 2,4-dichlorophenol destruction

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Journal of Environmental Sciences 2024年第7期141卷 235-248页

作者： Yu Liu Weibao Liu Xinrui Gan Jiangwei shang Xiuwen cheng College of Chemistry and Environmental Science Xinjiang Laboratory of Phase Transitions and Microstructures of Condensed Matter PhysicsYili Normal UniversityYining 835000China Key Laboratory for Environmental Pollution Prediction and Control Gansu ProvinceCollege of Earth and Environmental SciencesLanzhou UniversityLanzhou 730000China

In this study,the cobalt-nickel layered double hydroxides(CoNi LDH)were synthesized with a variety of Co/Ni mass ratio,as *** comparison,Co1Ni3LDH presented the best peroxymonosulfate(PMS)activation efficiency for 2,4-dichlorophenol ***,CoNi LDH@Nickel foam(CoNi LDH@NF)composite membrane was constructed for enhancing the stability of catalytic ***,CoNi LDH@NF-PMS system exerted high degradation efficiency of 99.22%within 90 min for 2,4-DCP when[PMS]_(0)=0.4 g/L,Co^(1)Ni^(3)LDH@NF=2 cm×2 cm(0.2 g/L),reaction temperature=298 *** the surface morphology and structure of the catalyst,it was demonstrated that the CoNi LDH@NF composite membrane possessed abundant cavity structure,good specific surface area and sufficient active ***,·OH,SO_(4)·^(-)and^(1)O_(2)played the primary role in the CoNi LDH@NF-PMS system for 2,4-DCP decomposition,which revealed the PMS activation mechanism in CoNi LDH@NF-PMS ***,this study eliminated the stability and adaptability of CoNi LDH@NF composite membrane,proposing a new theoretical basis of PMS heterogeneous catalysts selection.

关键词： CoNi LDH@NF composite membrane Peroxymonosulfate 2,4-dichlorophenol Reactive radicals

Enhancement of polymyxin B1 production by an artificial microbial consortium of Paenibacillus polymyxa and recombinant Corynebacterium glutamicum producing precursor amino acids

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Synthetic and Systems Biotechnology 2024年第1期9卷 176-185页

作者： Hui-Zhong Sun Si-Yu Wei Qiu-Man Xu Wei shang Qing Li jing-Sheng cheng Ying-jin Yuan Frontiers Science Center for Synthetic Biology and Key Laboratory of Systems Bioengineering(Ministry of Education) School of Chemical Engineering and TechnologyTianjin UniversityYaguan Road 135Jinnan DistrictTianjin300350PR China Tianjin Key Laboratory of Animal and Plant Resistance College of Life ScienceTianjin Normal UniversityBinshuixi Road 393Xiqing DistrictTianjin300387PR China Department of Pharmaceutical School of Chemical Engineering and TechnologyTianjin UniversityYaguan Road 135Jinnan DistrictTianjin300350PR China

Polymyxin B,produced by Paenibacillus polymyxa,is used as the last line of defense *** this study,exogenous mixture of precursor amino acids increased the level and proportion of polymyxin B1 in the total of polymyxin B analogs of *** CJX518-AC(PPAC)from 0.15 g/L and 61.8%to 0.33 g/L and 79.9%,*** co-culture of strain PPAC and recombinant Corynebacterium glutamicum-leu01,which produces high levels of threonine,leucine,and isoleucine,increased polymyxin B1 production to 0.64 g/*** strains PPAC and ***-leu01 simultaneously inoculated into an optimized medium with 20 g/L peptone,polymyxin B1 production was increased to 0.97 g/***,the polymyxin B1 production in the co-culture of strains PPAC and ***-leu01 increased to 2.21 g/L after optimized inoculation ratios and fermentation medium with 60 g/L *** study provides a new strategy to improve polymyxin B1 production.

关键词： Polymyxin Co-culture Paenibacillus polymyxa Corynebacterium glutamicum Medium optimization Metabolic precursors

兼顾市场机制的主要节能发电调度模式比较研究

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电网技术 2008年第4期32卷 78-85页

作者：尚金成河南电网电力交易中心河南省郑州市450052

首先给出了在设计节能发电调度模式(模型)及运作机制时需要遵循的一般原则;然后结合中国国情,以电网安全稳定运行及连续可靠供电为约束,以节能、环保、经济、公平为目标,从节能发电调度的纯行政命令模式(计划调控、政府宏观调控)、计划... 详细信息

首先给出了在设计节能发电调度模式(模型)及运作机制时需要遵循的一般原则;然后结合中国国情,以电网安全稳定运行及连续可靠供电为约束,以节能、环保、经济、公平为目标,从节能发电调度的纯行政命令模式(计划调控、政府宏观调控)、计划调控与市场机制相结合模式到完全市场竞争模式,设计了实施节能发电调度的7种主要模式并进行了比较研究,分析了每种模式的优缺点,设定了每种模式实现的前提条件;同时设计了节能发电调度在过渡期内的4种经济补偿机制和结算模式,并进行了比较分析。最后提出了节能发电调度由纯行政命令模式向完全市场竞争模式过渡的几种过渡方式。

关键词：节能减排电力结构调整节能发电调度调度模式市场机制计划调控替代发电利益调整经济补偿机制和谐多赢机制设计帕累托改进比较研究

兼顾市场机制与政府宏观调控的节能发电调度模式及运作机制

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电网技术 2007年第24期31卷 55-62页

作者：尚金成河南电网电力交易中心河南省郑州市450052

实施节能发电调度将引起各方利益的重大调整,解决该问题的最佳办法是采用市场机制,而目前中国电力市场还很不成熟,电力工业市场化程度还很低。本文结合中国国情提出了兼顾政府宏观调控(计划调控)与市场机制的节能发电调度模式及其运作... 详细信息

实施节能发电调度将引起各方利益的重大调整,解决该问题的最佳办法是采用市场机制,而目前中国电力市场还很不成熟,电力工业市场化程度还很低。本文结合中国国情提出了兼顾政府宏观调控(计划调控)与市场机制的节能发电调度模式及其运作机制。该模式通过对各类发电机组按能耗和污染物排放水平排序来实施优化调度,以实现节能发电调度的目标要求;同时,采用政府宏观调控与市场机制相结合的办法来平衡协调各方利益,避免采用容易引起矛盾的行政命令经济补偿手段(强行切块分割),最大程度地缓解利益调整引发的社会稳定问题。该模式以电网安全及连续可靠供电为约束,以节能、环保、经济为目标,实现了政府宏观调控与市场机制的有机结合,兼顾了各方利益,有效解决了节能发电调度引起的各方利益重大调整问题。

关键词：节能发电调度市场机制宏观调控调度模式运作机制利益调整经济补偿机制和谐多赢电力市场

主成分-聚类复合模型在水环境管理中的应用——以松花江吉林段为例

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水科学进展 2005年第4期16卷 592-595页

作者：张妍尚金城于相毅北京师范大学环境学院环境模拟与污染控制国家重点实验室北京100875 东北师范大学城市与环境科学学院吉林长春130024

以松花江吉林段5年的监测资料为依据,采用主成分分析与聚类分析的复合模型,定量诊断出水污染因子对松花江吉林段的污染贡献率,合理划分出各类水环境管理区域,并提出相应的水环境管理措施。结果表明:松花江吉林段主要污染物是挥发酚、CO... 详细信息

以松花江吉林段5年的监测资料为依据,采用主成分分析与聚类分析的复合模型,定量诊断出水污染因子对松花江吉林段的污染贡献率,合理划分出各类水环境管理区域,并提出相应的水环境管理措施。结果表明:松花江吉林段主要污染物是挥发酚、COD和氨氮,表现为有机污染和非点源污染;在水环境管理分区中,丰满-龙潭桥区域属于轻污染,为水源保护江段,龙潭桥-哨口区域属于重污染,为水环境控制江段,哨口-白旗区域属于中度污染状况,为水环境自净江段。这一工作的开展对于实施河流水环境总量控制,实现松花江吉林段水域的科学化分类管理具有一定的参考价值。

关键词：主成分分析聚类分析水环境管理松花江

Degradation of Rhodamine B by MnFe-LDH/PMS/O_(3) three-phase catalytic system: performance, mechanism and ecotoxicity studies

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Frontiers of Environmental Science & Engineering 2024年第1期18卷 111-127页

作者： Ying Han Ying Yang Weibao Liu Yilong Hou Ce Wang Jiangwei shang Xiuwen cheng Key Laboratory of Pollutant Chemistry and Environmental Treatment College of Chemistry and Environmental ScienceYili Normal UniversityYining 835000China Key Laboratory for Environmental Pollution Prediction and Control of Gansu Province College of Earth and Environmental SciencesLanzhou UniversityLanzhou 730000China

This study developed a novel MnFe-LDH/PMS/O3 three-phase catalytic system to degrade the organic dye RhB, which was used to address the drawbacks of persulfate oxidation and ozonation techniques. The structure, ionic and elemental composition, specific surface area, and magnetic properties of the LDHs were investigated using a variety of physicochemical characterization tools. The results showed that MnFe-LDH had a large specific surface area, a rich crystalline phase composition, and a functional group structure. The RhB degradation rate of MnFe-LDH/PMS/O3 was 0.34 min−1, which was much higher than that of other comparative systems. RhB could be completely degraded in 10 min after optimization and had a significant effect on TOC removal. The system was found to be effective over a wide pH range. Common anions were largely unaffected and humic acid acted as an inhibitor. At the same time, the system had generally effective degradation performance for different dyes. Combined with quenching experiments and EPR, it was found that SO4•−, •OH, O_(2)•−, and 1O_(2) all participated in the reaction, and •OH contributed more. The degradation pathway of RhB was derived by LC-MS, and the T.E.S.T. evaluation found that the toxicity of the intermediate product was significantly reduced. Finally, the stability and availability of LDHs were verified using cycling experiments and metal ion leaching. This work provides a theoretical basis and data support for the synergistic catalysis of PMS/O3 and the deep treatment of dye wastewater.

关键词： Rhodamine B Layered double hydroxides Peroxymonosulfate Ozonation

Change of pore water near the freezing front during soil freezing: Migration and mechanisms

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Pedosphere 2024年第4期34卷 770-782页

作者： Yajun SHI Wei MA Lianhai ZHANG chengsong YANG Fei shang cheng CHEN State Key Laboratory of Frozen Soil Engineering Northwest Institute of Eco-Environment and ResourcesChinese Academy of SciencesLanzhou 730000China University of Chinese Academy of Sciences Beijing 100049China Department of Joint NMR Laboratory for Freeze-Thaw Processes in Soils of State Key Laboratory of Frozen Soil Engineering and Suzhou Niumag Analytical Instrument Corporation Lanzhou 730000China

The formation and growth of segregation ice dominate the frost heave during soil freezing,which is closely related to water *** analyze segregation ice during soil freezing for different soils,a freezing-thawing experiment was conducted with Lanzhou loess(LZL)and Qinghai-Tibet Plateau silty clay(QSC)using a novel layered nuclear magnetic resonance *** LZL freezing,the unfrozen water content first increased and then decreased with decreasing temperature near the freezing front,but decreased with decreasing temperature in other layers,whereas during the freezing of QSC,the unfrozen water content in different layers(including the freezing front)decreased with decreased ***,the increased liquid water near the freezing front during LZL freezing was primarily adsorbed *** addition to the temperature gradient,the squeezing action during soil freezing was another important factor affecting water migration,especially at the early stage of soil ***,which of the two factors,squeezing action and temperature gradient,was the dominant one causing water migration depended on soil *** the early stage of soil freezing,the squeezing action had a significant effect on the water migration of LZL,but no significant effect on that of ***,water accumulation of LZL near the freezing front due to squeezing action at the early stage of freezing limited the formation and growth of segregation *** study provided an improved understanding for ice segregation and water migration during soil freezing.

关键词： freezing-thawing experiment frozen soil nuclear magnetic resonance phase transition segregation ice squeezing action unfrozen water water migration

Impact of next-generation sequencing on antimicrobial treatment in immunocompromised adults with suspected infections

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World Journal of Emergency Medicine 2024年第2期15卷 105-110页

作者： Jia Li Jiazhen Luo Tao Hu Ling cheng Weiwei shang Li Yan Department of Intensive Care Unit Tongji HospitalTongji Medical CollegeHuazhong University of Science and TechnologyWuhan 430030China Department of Emergency Medicine Tongji HospitalTongji Medical CollegeHuazhong University of Science and TechnologyWuhan 430030China Tongji Medical College Huazhong University of Science and TechnologyWuhan 430030China Department of Geriatrics Tongji HospitalTongji Medical CollegeHuazhong University of Science and TechnologyWuhan 430030China

BACKGROUND:Prompt pathogen identification can have a substantial impact on the optimization of antimicrobial *** objective of the study was to assess the diagnostic value of next-generation sequencing(NGS)for identifying pathogen and its clinical impact on antimicrobial intervention in immunocompromised patients with suspected ***:This was a retrospective *** January and August 2020,47 adult immunocompromised patients underwent NGS testing under the following clinical conditions:1)prolonged fever and negative conventional cultures;2)new-onset fever despite empiric antimicrobial treatment;and 3)afebrile with suspected infections on *** data,including conventional microbial test results and antimicrobial treatment before and after NGS,were *** were analyzed according to documented changes in antimicrobial treatment(escalated,no change,or deescalated)after the NGS ***:The median time from hospitalization to NGS sampling was 19 *** relevant pathogens were detected via NGS in 61.7% of patients(29/47),more than half of whom suffered from fungemia(n=17),resulting in an antimicrobial escalation in 53.2% of patients(25/47)and antimicrobial de-escalation in 0.2% of patients(1/47).Antimicrobial changes were mostly due to the identification of fastidious organisms such as Legionella,Pneumocystis jirovecii,and *** the remaining three cases,NGS detected clinically relevant pathogens also detected by conventional cultures a few days *** antimicrobial treatment was subsequently adjusted according to the susceptibility test ***,NGS changed antimicrobial management in 55.3%(26/47)of patients,and conventional culture detected clinically relevant pathogens in 14.9% of the patients(7/47).CONCLUSION:With its rapid identification and high sensitivity,NGS could be a promising tool for identifying relevant pathogens and enabling rapid appropriate treatment in immunocompromised patients w

关键词： Immunocompromised patients Next-generation sequencing Antimicrobial management

Flexible capacitive pressure sensor based on interdigital electrodes with porous microneedle arrays for physiological signal monitoring

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Nanotechnology and Precision Engineering 2024年第1期7卷 18-31页

作者： Jiahui Xu Minghao Wang Minyi jin Siyan shang Chuner Ni Yili Hu Xun Sun Jun Xu Bowen Ji Le Li Yuhua cheng Gaofeng Wang School of Electronics&Information MOE Engineering Research Center of Smart Microsensors and MicrosystemsHangzhou Dianzi UniversityHangzhou 310018China Wenzhou Institute of Hangzhou Dianzi University Wenzhou 310018China Key Laboratory of Intelligent Operation and Maintenance Technology&Equipment for Urban Rail Transit of Zhejiang Province College of EngineeringInstitute of Precision Machinery and Smart StructureZhejiang Normal UniversityJinhua 321004China Institute of Guizhou Aerospace Measuring and Testing Technology Guiyang 550009China Unmanned System Research Institute Northwestern Polytechnical UniversityXi’an 710072China Research&Development Institute of Northwestern Polytechnical University in Shenzhen Shenzhen 518057China

Flexible pressure sensors have many potential applications in the monitoring of physiological signals because of their good biocompatibil-ity and ***,their relatively low sensitivity,linearity,and stability have hindered their large-scale commercial ***,aﬂexible capacitive pressure sensor based on an interdigital electrode structure with two porous microneedle arrays(MNAs)is *** porous substrate that constitutes the MNA is a mixed product of polydimethylsiloxane and *** to its porous and interdigital structure,the maximum sensitivity(0.07 kPa-1)of a porous MNA-based pressure sensor was found to be seven times higher than that of an imporous MNA pressure sensor,and it was much greater than that of aﬂat pressure sensor without a porous MNA ***-element analysis showed that the interdigital MNA structure can greatly increase the strain and improve the sensitivity of the *** addition,the porous MNA-based pressure sensor was found to have good stability over 1500 loading cycles as a result of its bilayer parylene-enhanced conductive electrode *** importantly,it was found that the sensor could accurately monitor the motion of aﬁnger,wrist joint,arm,face,abdomen,eye,and Adam’s ***,preliminary semantic recognition was achieved by monitoring the movement of the Adam’s ***,multiple pressure sensors were integrated into a 33 array to detect a spatial pressure distribu-×*** to the sensors reported in previous works,the interdigital electrode structure presented in this work improves sensitivity and stability by modifying the electrode layer rather than the dielectric layer.

关键词： Capacitive pressure sensor Microneedle array Porous PDMS Interdigital electrode