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Structure characterization of the oxide film on FGH96 superalloy powders with various oxidation degrees

International Journal of Minerals,Metallurgy and Materials 2024年第9期31卷 2037-2047页

作者： Yang liu Yufeng liu sha Zhang lin Zhang Peng Zhang shaorong Zhang Na liu Zhou li Xuanhui Qu Beijing Advanced Innovation Center for Materials Genome Engineering Institute for Advanced Materials and TechnologyUniversity of Science and Technology BeijingBeijing 100083China Institute of Materials Intelligent Technology Liaoning Academy of MaterialsShenyang 110004China Science and Technology on Advanced High Temperature Structural Materials Laboratory AECC Beijing Institute of Aeronautical MaterialsBeijing 100095China

The structure of the oxide film on FGH96 alloy powders significantly influences the mechanical properties of *** this study,FGH96 alloy powders with various oxygen contents were investigated using high-resolution transmission electron microscopy and atomic probe technology to elucidate the structure evolution of the oxide *** dispersive spectrometer analysis revealed the presence of two distinct components in the oxide film of the alloy powders:amorphous oxide layer covering the γ matrix and amorphous oxide particles above the *** alloying elements within the oxide layer showed a laminated distribution,with Ni,Co,Cr,and Al/Ti,which was attributed to the decreasing oxygen equilibrium pressure as oxygen diffused from the surface into the γ *** the other hand,Ti enrichment was observed in the oxide particles caused by the oxidation and decomposition of the carbide *** analysis of the oxide film with oxygen contents of 140,280,and 340 ppm showed similar element distributions,while the thickness of the oxide film varies approximately at 9,14,and 30 nm,*** findings provide valuable insights into the structural analysis of the oxide film on FGH96 alloy powders.

关键词： Ni-based superalloys surface structure oxide layer thickness oxidation behavior element distribution

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Synergistic Brønsted Base/Photoredox-Catalyzed Three-Component Coupling with Malonates to Synthesize δ-Hydroxy Esters and δ-Keto Esters

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Chinese Journal of Chemistry 2024年第9期42卷 957-962页

作者： Ting li Wei Wang Ming Dong Zhije Zhang sha Yu Zhengchu Chen Siping Wei Dong Yi Green Pharmaceutical Technology Key Laboratory of Luzhou City Central Nervous System Drug Key Laboratory of Sichuan ProvinceSchoolof PharmacySouthwestMedicalUniversityLuzhouSichuan 646000China Nuclear Medicine and Molecular Imaging Key Laboratory of Sichuan Province LuzhouSichuan 646000China

Multicomponent alkene 1,2-dicarbofunctionalizations(DCFs)have emerged as a powerful strategy to rapidly incorporate both two carbon subunits across one C-C double bond in one step for enhancing molecular complexity and *** the best of our knowledge,there is only one report on photoredox-catalyzed three-component DCFs with malonates through the radical−radical cross-coupling,while photoredox-catalyzed radical-polar crossover(RPC)-type DCFs with malonates were still ***,we describe a redox-neutral RPC-type 1,2-dialkylation of styrenes with malonates and aldehydes through the synergistic Brønsted base/photoredox catalysis *** transition-metal-free strategy provides an efficient and clean approach to a broad variety ofδ-hydroxy esters and also features exceptionally mild conditions,wide compatibility of substrate scope and functional groups,and high atomic ***,three-component 1,2-alkylacylation from the same starting materials was achieved in one-pot manner through such RPC-type coupling and subsequent two-electron oxidation process,providing a set ofδ-keto esters of interest in pharmaceutical research.

关键词： Alkene difunctionalization Photoredox catalysis Malonates Radical reactions C-C coupling Synthetic methods Aldehydes Alkylation Multicomponentreactions

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“Steric Armor”Strategy of Blue Fluorescent Emitters against Photooxidation-Induced Degradation

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Chinese Journal of Chemistry 2024年第11期42卷 1223-1229页

作者： sha-sha Wang Jing-Rui Zhang Kuan-De Wang Hao-Ran li Peng-Hui Meng Yang Zhou Xiang Yu Ying Wei Quan-You Feng Yu-He Kan ling-Hai Xie Centre for Molecular Systems and Organic Devices(CMSOD) State Key Laboratory of Organic Electronics and Information Displays&Institute of Advanced MaterialsJiangsu National Synergetic Innovation Center for Advanced Materials(SICAM)Nanjing University of Posts&TelecommunicationsNanjingJiangsu210023 China Jiangsu Key Laboratory for Chemistry of Low-Dimensional Materials School of Chemistry and Chemical EngineeringHuaiyin Normal UniversityHuai'anJiangsu223300 China

Stability against oxygen is an important factor affecting the performance of organic semiconductor *** photooxidation stability can prolong the service life of the device and maintain the mechanical and photoelectric properties of the ***,various encapsulation methods from molecular structure to macroscopic device level are used to improve photooxidation ***,we adopted a crystallization strategy to allow 14H-spiro[dibenzo[c,h]acridine-7,9′-fluorene](SFDBA)to pack tightly to resist fluorescence decay caused by *** this case,the inert group of SFDBA acts as a“steric armor”,protecting the photosensitive group from being attacked by ***,compared with the fluorescence quenching of SFDBA powder under 2 h of sunlight,SFDBA crystal can maintain its fluorescence emission for more than 8 h under the same ***,the photoluminescence quantum yields(PLQYs)of the crystalline film is 327%higher than that of the amorphous *** shows that the crystallization strategy is an effective method to resist oxidation.

关键词： Organic semiconductor Photooxidation Spirocyclic aromatic hydrocarbons Crystal engineering Fluorescence

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RKKY interaction in helical higher-order topological insulators

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Chinese Physics B 2024年第7期33卷 587-593页

作者：金莎李健李清旭朱家骥 School of Science Chongqing University of Posts and TelecommunicationsChongqing 400065China Institute for Advanced Sciences Chongqing University of Posts and TelecommunicationsChongqing 400065China Southwest Center for Theoretical Physics Chongqing UniversityChongqing 401331Chin

We theoretically investigate the Ruderman–Kittel–Kasuya–Yosida(RKKY) interaction in helical higher-order topological insulators(HOTIs), revealing distinct behaviors mediated by hinge and Dirac-type bulk carriers. Our findings show that hinge-mediated interactions consist of Heisenberg, Ising, and Dzyaloshinskii–Moriya(DM) terms, exhibiting a decay with impurity spacing z and oscillations with Fermi energy εF. These interactions demonstrate ferromagnetic behaviors for the Heisenberg and Ising terms and alternating behavior for the DM term. In contrast, bulk-mediated interactions include Heisenberg, twisted Ising, and DM terms, with a conventional cubic oscillating decay. This study highlights the nuanced interplay between hinge and bulk RKKY interactions in HOTIs, offering insights into designs of next-generation quantum devices based on HOTIs.

关键词： magnetic impurity interactions magnetic ordering spintronics topological phases

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Detection and analysis of landslide geomorphology based on UAV vertical photogrammetry

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Journal of Mountain Science 2024年第4期21卷 1190-1214页

作者： BI Rui GAN Shu YUAN Xiping li Kun li Raobo LUO Weidong CHEN Cheng GAO sha HU lin ZHU Zhifu School of Land and Resources Engineering Kunming University of Science and TechnologyKunming 650093China Plication Engineering Research Center of Spatial Information Surveying and Mapping Technology in Plateau and Mountainous Areas Set by Universities in Yunnan Province Kunming 650093China West Yunnan University of Applied Sciences Key Laboratory of Mountain Real Scene Point Cloud Data Processing and Application for Universities in Yunnan ProvinceDali 671006China

High-resolution landslide images are required for detailed geomorphological analysis in complex topographic environment with steep and vertical landslide *** study proposed a vertical route planning method for unmanned aerial vehicles(UAVs),which could achieve rapid image collection based on strictly calculated route *** effectiveness of this method was verified using a DJI Mavic 2 Pro,obtaining high-resolution landslide images within the Dongchuan debris flow gully,in the Xiaojiang River Basin,Dongchuan District,Yunnan,China.A three-dimensional(3D)model was constructed by the structure-from-motion and multi-view stereo(SfM-MVS).Micro-geomorphic features were analyzed through visual interpretation,geographic information system(GIS),spatial analysis,and mathematical statistics *** results demonstrated that the proposed method could obtain comprehensive vertical information on landslides while improving measurement *** 3D model was constructed using the vertically oriented flight route to achieve centimeter-level accuracy(horizontal accuracy better than 6 cm,elevation accuracy better than 3 cm,and relative accuracy better than 3.5 cm).The UAV technology could further help understand the micro internal spatial and structural characteristics of landslides,facilitating intuitive acquisition of surface *** slope of landslide clusters ranged from 36°to 72°,with the majority of the slope facing east and *** elevation levels were relatively consistent while middle to lower elevation levels gradually decreased from left to right with significant variations in lower elevation *** the rainy season,surface runoff was abundant,and steep topography exacerbated changes in surface *** route method is suitable for unmanned aerial vehicle(UAV)landslide surveys in complex mountainous *** geomorphological analysis methods used will provide references for identifying and describing topographic

关键词： UAV Landslide Vertical route SfM-MVS Topographic features

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Improved simulation of winter wheat yield in North China Plain by using PRYM-Wheat integrated dry matter distribution coefficient

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Journal of Integrative Agriculture 2024年第4期23卷 1381-1392页

作者： Xuan li shaowen Wang Yifan Chen Danwen Zhang shanshan Yang Jingwen Wang Jiahua Zhang Yun Bai sha Zhang Research Center for Remote Sensing and Digital Earth College of Computer Science and TechnologyQingdao UniversityQingdao266071China Center for Geospatial Information Shenzhen Institute of Advanced TechnologyChinese Academy of SciencesShenzhen 518055China School of Geographical Sciences Hebei Normal UniversityShijiazhuang 050024China

The accurate simulation of regional-scale winter wheat yield is important for national food security and the balance of grain supply and demand in ***,most remote sensing process models use the“biomass×harvest index(HI)”method to simulate regional-scale winter wheat ***,spatiotemporal differences in HI contribute to inaccuracies in yield simulation at the regional ***-series dry matter partition coefficients(Fr)can dynamically reflect the dry matter partition of winter *** this study,Fr equations were fitted for each organ of winter wheat using site-scale *** equations were then coupled into a process-based and remote sensingdriven crop yield model for wheat(PRYM-Wheat)to improve the regional simulation of winter wheat yield over the North China Plain(NCP).The improved PRYM-Wheat model integrated with the fitted Fr equations(PRYM-Wheat-Fr)was validated using data obtained from provincial yearbooks.A 3-year(2000-2002)averaged validation showed that PRYM-Wheat-Fr had a higher coefficient of determination(R^(2)=0.55)and lower root mean square error(RMSE=0.94 t ha^(-1))than PRYM-Wheat with a stable HI(abbreviated as PRYM-Wheat-HI),which had R^(2) and RMSE values of 0.30 and 1.62 t ha^(-1),*** PRYM-Wheat-Fr model also performed better than PRYM-Wheat-HI for simulating yield in verification years(2013-2015).In conclusion,the PRYM-Wheat-Fr model exhibited a better accuracy than the original PRYM-Wheat model,making it a useful tool for the simulation of regional winter wheat yield.

关键词： dry matter partition remote sensing model winter wheat yield North China Plain

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A local rainfall-triggered giant landslide occurred in a region along a high-speed railway on the Qinghai‒Tibetan Plateau

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Journal of Mountain Science 2024年第9期21卷 2939-2955页

作者： li Qingpeng liU Wenhui HE Renjie YING Chunye liU Hairui DOU Zengning liU Yabing YANG sha SONG Xianteng School of Geological Engineering Qinghai UniversityXining 810016China Key Lab of Cenozoic Resource and Environment in North Margin of the Tibetan Plateau Qinghai UniversityXining 810016China College of Eco-Environmental Engineering Qinghai UniversityXining 810016China Qinghai Transportation Planning and Design Institute Co Ltd Xining 810000China Xining Center for Integrated Natural Resources Survey China Geological SurveyXining 810000QinghaiChina

An increasing number of geological hazards along high-speed railways on the Qinghai‒Tibetan Plateau have occurred and have resulted in a profound influence on old infrastructure,which has attracted increasing *** landslide event that occurred on September 15,2022,in Jiujiawan village,Xining city,Qinghai Province,is a typical *** on field investigations and remote sensing interpretations,a comprehensive analysis was conducted on the ***,the potential secondary failure of the current Jiujiawan landslide was assessed using Fast Lagrangian Analysis of Continua in Three Dimensions(FLAC3D).Based on the application of the small baseline subset-interferometric synthetic aperture radar(SBAS-InSAR)technique to SAR images from February 24,2017 to September 14,2022,a significant westward horizontal deformation was found to have been formed prior to the occurrence of the *** maximum annual average deformation rate in the line of sight(LOS)direction reached-45 mm/yr,with a maximum cumulative deformation of-178 *** value was consistent with the continual increase in annual precipitation(2.51 mm/yr)prior to the occurrence of the *** accumulated precipitation before the landslide was 279.8 mm,accounting for 54.2%of the total annual precipitation,with a particularly notable surge in monthly precipitation observed during August(250.3 mm).Additionally,the occurrence of a seismic event with a magnitude of Ms 6.9 in Menyuan County,80 km away from Xining,could be a potential triggering factor to the landslide,as evidenced by an abrupt subsidence alteration observed prior to and following the *** maximum subsidence in the line of sight(LOS)direction exceeded 11 mm,exhibiting a highly consistent spatial distribution with the occurrence range of *** results suggest that the Jiujiawan landslide was likely induced by earthquake events in the early stage and heavy rainfall in the later *** FLAC3D numerical

关键词： Landslide Development characteristic Driver Mudstone Xining Basin

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Deep electrical structures of Qinzhou-Fangcheng Junction Zone in Guangxi and seismogenic environment of the 1936 lingshan M6^(3/4)earthquake

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Science China Earth Sciences 2024年第2期67卷 584-603页

作者： Bin ZHOU Chunheng YAN Yan ZHAN Xiangyu SUN sha li Xiang WEN Yajun MO Yongdong YUAN Yuan YUAN Meili HUANG Earthquake Agency of Guangxi Zhuang Autonomous Region Nanning530022China State Key Laboratory of Earthquake Dynamics Institute of GeologyChina Earthquake AdministrationBeijing100029China Guangxi Geophysical Survey Institute Liuzhou545005China

The tectonic position of the southwest section of the Qinzhou Bay-Hangzhou Bay Tectonic Junction Zone(QHTJZ)can be determined by examining the Qinzhou-Fangcheng Junction Zone(QFJZ)in *** zone is significant because it was the location of the largest earthquake ever recorded in the inland region of South China,specifically the 1936 lingshan M6^(3/4)earthquake in ***,this region serves as an optimal location for researching the origins of intraplate earthquakes in South *** study presents a display of a broadband magnetotelluric(MT)prospecting profile that traverses the Guangxi QFJZ and the lingshan earthquake zone,extending from the northwest(NW)to the southeast(SE).A resistivity structure model was generated using three-dimensional(3D)inversion technology along the *** main faults in QFJZ were analyzed in terms of their deep extension forms and tectonic *** analysis was performed by integrating the results obtained from geology,gravity,wave velocity ratio,Global Position System(GPS),and geothermal *** results showed that(1)the Dongzhong-Xiaodong fault(DXf),the eastern Fangcheng-lingshan fault(FLf2),and the eastern Hepu-Beiliu fault(HBf2)were all trans-crustal deep faults,and crust-mantle ductile shear zones developed in the deep *** electrical boundary zones,DXf and HBf2,were *** inclined towards the northwest,while HBf2 inclined towards the *** Fangchenglingshan fault(FLf)exhibits a tectonic style resembling a“flower”shape in the upper *** the deeper section,it is characterized by an electrical boundary zone that gradually slopes towards the southeast direction.(2)The Hunan-Guangxi Passive Continental Margin(HGPCM)on the NW side of DXf had a stratified resistivity structure and relatively stable Bouguer gravity anomalies,which conformed to the quasi-craton tectonic attribute of the local failure at the southeastern margin of the Yangtze Block(YB).The southeastern side of this bloc

关键词： South China Block Qinzhou-Fangcheng Junction Zone Magnetotelluric 1936 lingshan M6^(3/4)earthquake Deep seismogenic environment

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General and specialized metabolites in peanut roots regulate arbuscular mycorrhizal symbiosis

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Journal of Integrative Agriculture 2024年第8期23卷 2618-2632页

作者： li Cui Jianguo Wang Zhaohui Tang Zheng Zhang sha Yang Feng Guo Xinguo li Jingjing Meng Jialei Zhang Yakov Kuzyakov Shubo Wan Institute of Crop Germplasm Resources Shandong Academy of Agricultural Sciences/Scientific Observing and Experimental Station of Crop Cultivation in East ChinaMinistry of Agriculture and Rural AffairsJinan 250100China shandong Academy of Agricultural Sciences Jinan 250100China Department of Soil Science of Temperate Ecosystems Department of Agricultural Soil ScienceUniversity of GöttingenGöttingen 37077Germany Peoples Friendship University of Russia(RUDN University) Miklukho-Maklaya StMoscow 117198Russia Institute of Environmental Sciences Kazan Federal University420049 KazanRussia

Arbuscular mycorrhizae(AM)fungi form symbiotic associations with plant roots,providing nutritional benefits and promoting plant growth and defenses against various *** changes in the roots during AM fungal colonization are key to understanding the development and maintenance of these ***,we investigated metabolic changes in the roots of peanut(Arachis hypogaea L.)plants during the colonization and development of AM symbiosis,and compared them to uncolonized *** primary changes during the initial stage of AM colonization were in the contents and compositions of phenylpropanoid and flavonoid *** compounds function in signaling pathways that regulate recognition,interactions,and pre-colonization between roots and AM *** compounds decreased by 25%when the symbiosis was fully established compared to the initial colonization *** AM symbiosis was established,general metabolism strongly shifted toward the formation of lipids,amino acids,carboxylic acids,and *** compounds increased by 8.5%from the pre-symbiotic stage to well-established ***-phosphatidylcholines,which are signaling compounds,were only present in AM roots,and decreased in content after the symbiosis was *** the initial stage of AM establishment,the content of salicylic acid increased two-fold,whereas jasmonic acid and abscisic acid decreased compared to uncolonized *** jasmonic acid content decreased in roots after the symbiosis was well *** symbiosis was associated with high levels of calcium,magnesium,and D-(+)-mannose,which stimulated seedling ***,specific metabolites that favor the establishment of AM symbiosis were common in the roots,primarily during early colonization,whereas general metabolism was strongly altered when AM symbiosis was *** conclusion,specialized metabolites function as signaling compounds to establish AM *** compounds are no longe

关键词： Arachis hypogaea L. arbuscular mycorrhizae fungi metabolites symbiotic association

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Anomalous photoluminescence enhancement and resonance charge transfer in type-II 2D lateral heterostructures

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Chinese Physics B 2023年第8期32卷 465-471页

作者：赵春艳李莎莎闫勇 School of Physics Henan Key Laboratory of Photovoltaic MaterialsHenan Normal UniversityXinxiang 453007China School of Electronic Engineering Chaohu UniversityHefei 238024China

Type-Ⅱband alignment can realize the efficient charge transfer and separation at the semiconductor heterointerface,which results in photoluminescence(PL)***,several researches demonstrated great enhancement of localized PL at the interface of type-Ⅱtwo-dimensional(2D)***,the dominant physical mechanism of this enhanced PL emission has not been well *** this work,we symmetrically study the exciton dynamics of type-Ⅱlateral heterostructures of monolayer MoS_(2) and WS_(2) at room *** strong PL enhancement along the one-dimensional(1D)heterointerface is associated with the trion emission of the WS_(2) shell,while a dramatic PL quenching of neutral exciton is observed on the MoS_(2) *** enhanced quantum yield of WS2trion emission can be explained by charge-transfer-enhanced photoexcited carrier dynamics,which is facilitated by resonance hole transfer from MoS_(2) side to WS_(2) *** work sheds light on the 1D exciton photophysics in lateral heterostructures,which has the potential to lead to new concepts and applications of optoelectronic device.

关键词： lateral heterostructures resonance charge transfer MoS_(2)/WS_(2) photoluminescence enhancement band alignment

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