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Bioleaching of vanadium from stone coal vanadium ore by Bacillus mucilaginosus:Influencing factors and mechanism

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International Journal of Minerals,Metallurgy and Materials 2024年第8期31卷 1828-1838页

作者： Yingbo Dong Jinyu zan Hai Lin school of Energy and Environmental Engineering University of Science and Technology BeijingBeijing 100083China Beijing Key Laboratory on Resource-oriented Treatment of Industrial Pollutants Beijing 100083China

Vanadium and its derivatives are used in various industries,including steel,metallurgy,pharmaceuticals,and aerospace *** China has massive reserves of stone coal resources,these resources have low ***,the effective extraction and recovery of metallic vanadium from stone coal is an important way to realize the efficient resource utilization of stone coal vanadium ***,Bacillus mucilaginosus was selected as the leaching *** vanadium leaching rate reached 35.5%after 20 d of bioleaching under optimal operating *** cumulative vanadium leaching rate in the contact group reached 35.5%,which was higher than that in the noncontact group(9.3%).The metabolites of ***,such as oxalic,tartaric,citric,and malic acids,dominated in bioleaching,accounting for 73.8%of the vanadium leaching ***,during leaching,the presence of stone coal stimulated the expression of carbonic anhydrase in bacterial cells,and enzyme activity increased by 1.335-1.905 *** activity positively promoted the production of metabolite organic acids,and total organic acid content increased by 39.31 mg·L^(-1),resulting in a reduction of 2.51 in the pH of the leaching system with stone *** effect favored the leaching of vanadium from stone *** force microscopy illustrated that bacterial leaching exacerbated corrosion on the surface of stone coal beyond 10 *** study provides a clear and promising strategy for exploring the bioleaching mechanism from the perspective of microbial enzyme activity and metabolites.

关键词： Bacillus mucilaginosus stone coal vanadium ore bioleaching carbonic anhydrase organic acids

Topologically protected entanglement switching around exceptional points

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Light(science & Applications) 2024年第8期13卷 1631-1644页

作者： zan Tang Tian Chen Xing Tang Xiangdong Zhang Key Laboratory of Advanced Optoelectronic Quantum Architecture and Measurements of Ministry of Education Beijing Key Laboratory of Nanophotonics&Ultrafine Optoelectronic SystemsSchool of PhysicsBeijing Institute of Technology100081 BeijingChina

The robust operation of quantum entanglement states is crucial for applications in quantum information,computing,and communications^(1–3).However,it has always been a great challenge to complete such a task because of decoherence and ***,we propose theoretically and demonstrate experimentally an effective scheme to realize robust operation of quantum entanglement states by designing quadruple degeneracy exceptional *** encircling the exceptional points on two overlapping Riemann energy surfaces,we have realized a chiral switch for entangled states with high *** to the topological protection conferred by the Riemann surface structure,this switching of chirality exhibits strong robustness against perturbations in the encircling ***,we have experimentally validated such a scheme on a quantum walk *** work opens up a new way for the application of non-Hermitian physics in the field of quantum information.

关键词： exceptional quantum Riemann

surface wave inversion with unknown number of soil layers based on a hybrid learning procedure of deep learning and genetic algorithm

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Earthquake Engineering and Engineering Vibration 2024年第2期23卷 345-358页

作者： zan Zhou Thomas Man-Hoi Lok Wan-Huan Zhou Department of Civil and Environmental Engineering Faculty of Science and TechnologyUniversity of MacaoMacaoChina

surface wave inversion is a key step in the application of surface waves to soil velocity ***,a common practice for the process of inversion is that the number of soil layers is assumed to be known before using heuristic search algorithms to compute the shear wave velocity profile or the number of soil layers is considered as an optimization ***,an improper selection of the number of layers may lead to an incorrect shear wave velocity *** this study,a deep learning and genetic algorithm hybrid learning procedure is proposed to perform the surface wave inversion without the need to assume the number of soil ***,a deep neural network is adapted to learn from a large number of synthetic dispersion curves for inferring the layer ***,the shear-wave velocity profile is determined by a genetic algorithm with the known layer *** applying this procedure to both simulated and real-world cases,the results indicate that the proposed method is reliable and efficient for surface wave inversion.

关键词： surface wave inversion analysis shear-wave velocity profile deep neural network genetic algorithm

Adaptive Bistable stochastic Resonance Based Weak signal Reception in Additive Laplacian Noise

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China Communications 2024年第1期21卷 228-241页

作者： Jin Liu zan Li Qiguang Miao Li Yang school of Computer science and Technology Xidian UniversityXi’an 710071China state Key Laboratory of Integrated services Networks Xidian UniversityXi’an 710071China

Weak signal reception is a very important and challenging problem for communication systems especially in the presence of non-Gaussian noise,and in which case the performance of optimal linear correlated receiver degrades *** at this,a novel uncorrelated reception scheme based on adaptive bistable stochastic resonance(ABsR)for a weak signal in additive Laplacian noise is *** analyzing the key issue that the quantitative cooperative resonance matching relationship between the characteristics of the noisy signal and the nonlinear bistable system,an analytical expression of the bistable system parameters is *** this basis,by means of bistable system parameters self-adaptive adjustment,the counterintuitive stochastic resonance(sR)phenomenon can be easily generated at which the random noise is changed into a benefit to assist signal ***,it is demonstrated that approximately 8dB bit error ratio(BER)performance improvement for the ABsR-based uncorrelated receiver when compared with the traditional uncorrelated receiver at low signal to noise ratio(sNR)conditions varying from-30dB to-5dB.

关键词： adaptive bistable stochastic resonance additive Laplacian noise low signal to noise ratio uncorrelated reception scheme weak signal reception

Organic Brønsted Acid-Catalyzed stereoselective Cationic RAFT Polymerization:The Effect of RAFT Agents

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Chinese Journal of Polymer science 2024年第6期42卷 711-717页

作者： Zheng-Yi Zhang zan Yang Yun Liao sai-Hu Liao Key Laboratory of Molecule synthesis and Function Discovery(Fujian Province University) College of ChemistryFuzhou UniversityFuzhou350108China state Key Laboratory of Physical Chemistry of solid surfaces College of Chemistry and Chemical EngineeringXiamen UniversityXiamen361005China Beijing National Laboratory for Molecular sciences Beijing100190China

The tacticity of vinyl polymers is a key factor affecting the properties of ***,organic Brønsted acids have been demonstrated as effective catalysts for the development of highly stereoselective cationic reversible addition-fragmentation chain transfer(RAFT)polymerizations of vinyl ethers,in which the use of RAFT agents could allow the control the molecular weight and tacticity of polymer products ***,the effect of RAFT agents on the tacticity-regulation remains elusive and lacks of *** this study,we synthesized four types of RAFT agents and evaluated their influence in the stereoselective cationic polymerization of isobutyl vinyl ether in the presence of PADI as a Brønsted acid catalyst,which unveils that the Z group of RAFT agents could not only affect the polydispersity of the products,but also exert a profound effect on the *** extensive screening of the RAFT agents,high stereoregularity(isotacticity,90%m)was obtained when using dithiocarbonate ester-type RAFT agents with a benzyloxy Z group.

关键词： Bronsted acid catalysis stereoselective cationic polymerization RAFT polymerization Chain transfer agents Tacticity

Counterion-Mediated Hydrogen Bonding Making strong Polyelectrolytes pH-Responsive:Current Understanding and Perspectives

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Chinese Journal of Polymer science 2024年第9期42卷 1270-1277,I0005页

作者： Yue Huang Guang-Tao Mei zan Hua Guang-Ming Liu Hefei National Research Center for Physical sciences at the Microscale Department of Chemical PhysicsKey Laboratory of Surface and Interface Chemistry and Energy Catalysis of Anhui Higher Education InstitutesUniversity of Science and Technology of ChinaHefei230026China The Key Laboratory of Functional Molecular solids Ministry of Educationand Department of Materials ChemistrySchool of Chemistry and Materials ScienceAnhui Normal UniversityWuhu214002China

The counterion-mediated hydrogen bonding(CMHB)is related to the hydrogen bonding between bound counterions and polyelectrolyte chains in polyelectrolyte systems,where the counterions can both electrostatically bind to the charged groups of polyelectrolyte chains and act as hydrogen bond donors or acceptors to form hydrogen bonds with the hydrogen bond sites associated with polyelectrolyte chains simultaneously.A large number of literatures illustrate that strong polyelectrolytes(sPs)are insensitive to pH,which severely limmits the applications of sPs as smart ***,our studies have demonstrated that the CMHB makes sPs *** perspective discusses the mechanism of pH responsiveness of sPs and the pH-tunable properties of sPs,based on the pH-controlled CMHB *** future research directions on the pH responsiveness of sPs are also discussed *** is anticipated that the study of the pH responsiveness of sPs not only will provide a new understanding of the fundamental properties of sPs,but also will greatly expand the applications of sPs in the field of smart materials.

关键词： Counterion binding Hydrogen bond Polyelectrolyte brush Polyelectrolyte complexation

Phase-field simulation of precipitation kinetics and creep properties of Ni-Al-Cr/Ta superalloys

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science China(Technological sciences) 2024年第4期67卷 1139-1150页

作者： YANG shuaiGe ZHANG zan ZHUO JiCheng LONG HongLi LI Yongsheng National Key Laboratory of Advanced Casting Technologies MIIT Key Laboratory of Advanced Metallic and Intermetallic Materials TechnologyEngineering Research Center of Materials Behavior and DesignMinistry of EducationNanjing University of Science and TechnologyNanjing 210094China

The precipitation kinetics ofγ'-Ni_(3)(Al,Ta)phase and creep properties of Ni-15Al-x Ta at.%superalloys are investigated by the crystal plasticity phase-field *** results show that the high Ta content brings a lower creep strain for the deceleration and steady creep stage,while the creep lifetime is *** large external strain intensifies the creep damage and shortens the creep life of Ni-15Al-3Ta at.%*** kinetics evolution and elements distribution are revealed in the quaternary Ni-10Al-8.5Cr-xT a(x=1.5 at.%,2.0 at.%,2.5 at.%)superalloys by the multi-component phase-field *** anti-phase boundary(APB)changes the coarsening mechanism ofγ'phase,and Ta promotes the precipitation ofγ'phase with an increasing volume fraction and particle *** composition difference betweenγ'andγphases increases with the rising of Ta content,the strong partitioning of Ta toγ'phase strengthens the partitioning of Ni and Cr toγmatrix,and Ta shows a superiority than Al in the lattice site occupation of L1_(2)-Ni_(3)(Al,X)*** an importantγ'phase forming element,the optimization of Ta content is essential for improving the mechanical properties of Ni-based superalloys.

关键词： Ni-Al-Ta alloys creep properties kinetics phase-field

Mechanism of interfacial effects in sodium-ion storage devices

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Nano Research 2024年第3期17卷 1313-1326页

作者： Yifan Wei Lingxing zan Huicong Xia Wenfu Yan Jia-Nan Zhang College of Materials science and Engineering Zhengzhou UniversityZhengzhou 450001China Key Laboratory of Advanced Energy Catalytic and Functional Material Preparation of Zhengzhou City Zhengzhou 450001China Key Laboratory of Chemical Reaction Engineering of shaanxi Province College of Chemistry&Chemical EngineeringYan’an UniversityYan’an 716000China state Key Laboratory of Inorganic synthesis and Preparative Chemistry and College of Chemistry Jilin UniversityChangchun 130012China

Rechargeable sodium-ion batteries(sIBs)are considered as the next-generation secondary *** performance of sIB is determined by the behavior of its electrode surface and the electrode–electrolyte interface during charging and ***,the characteristics of these surfaces and interfaces should be analyzed to realize large-scale energy storage systems with high energy density and long-cycle *** various studies have investigated the properties of electrode materials,few studies have focused on the construction of stable and efficient sIB interfaces,and even fewer have explored the mechanisms of interfacial effects;however,the strategies of regulating interfacial effects are yet to be completely ***,the results obtained thus far are insufficient to draw systematic *** present study reviews the literature on the mechanism of interfacial effects in Na+storage *** interfaces in a sodium-ion storage device include a heterogeneous interface between electrode materials,a solid electrolyte interphase,and a cathode electrolyte *** interfacial effects during the intercalation,transformation,and alloy reactions and the resulting overall battery performance were theoretically *** this review,we aim to provide a theoretical basis for optimizing the structures of electrode surface and electrode–electrolyte interface to optimize the performance of *** addition,the challenges of investigating interfacial effects and several possible helpful methods and opportunities for studying the mechanisms of interfacial effects in sIBs will be presented.

关键词： sodium-ion storage interfacial effects solid electrolyte interphase cathode electrolyte interphase

Neiguan(PC6) acupoint stimulation for preventing chemotherapy-induced nausea and vomiting: a cost-effective supplement in guideline-inconsistent chemotherapy-induced nausea and vomiting prophylaxis subgroup

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Journal of Traditional Chinese Medicine 2024年第3期44卷 581-585页

作者： YU Wenxi TANG Lina LI Hongtao WANG Yonggang sHEN zan Department of Oncology Shanghai Sixth People's Hospital Affiliated to Shanghai Jiao Tong University School of MedicineShanghai200233China

OBJECTIVE: To assess the efficacy and safety of Neiguan(PC6) acupoint acustimulation in preventing chemotherapy-induced nausea and vomiting(CINV),especially for patients with guideline-inconsistent CINV prophylaxis(GICP) due to personal reasons METHODs: From January 2021 to December 2021, 373 patients suffered from solid malignancy were recruited according to the inclusion criteria. Complete response(no emesis and no rescue medication use) rate during the overall phase(0-120 h of each chemo-cycle) was the primary assessment of CINV control. The Functional Living Index-Emesis(FLIE) questionnaire was investigated among these patients as a secondary 'quality of life' objective to assess the impact of CINV on patients' daily life by recording score of nausea and vomiting. REsULTs: With acustimulation of Neiguan(PC6) acupuncture point through a portable, noninvasive and user-friendly device, in terms of complete response rate and scores in nausea/vomiting by FLIE questionnaire, patients achieve a better outcome in highly emetogenic chemotherapy(HEC) induced CINV, especially GICP subgroup. Meanwhile, analysis also demonstrated this tendency existed in other patients with HEC/GCCP(guideline consistent CINV prophylaxis) and moderate emetogenic chemotherapy, although the difference was not significant. CONCLUsION: Considering advantages of Neiguan(PC6) acustimulation such as noninvasive, covered by medical insurance and few side effects, we believe it would be an ideal auxiliary tool in CINV control, especially in patients who receive highly emetogenic chemoprotocol and are reluctant to GCCP for economic reasons.

关键词： acupuncture acustimulation tumor chemotherapy-induced nausea and vomiting