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A fast forward computational method for nuclear measurement using volumetric detection constraints

Nuclear science and Techniques 2024年第2期35卷 47-63页

作者： Qiong zhang lin-Lv lin University of Electronic science and Technology of China Chengdu 610000China

Owing to the complex lithology of unconventional reservoirs,field interpreters usually need to provide a basis for interpretation using logging simulation *** the various detection tools that use nuclear sources,the detector response can reflect various types of information of the *** Monte Carlo method is one of the primary methods used to obtain nuclear detection responses in complex ***,this requires a computational process with extensive random sampling,consumes considerable resources,and does not provide real-time response ***,a novel fast forward computational method(FFCM)for nuclear measurement that uses volumetric detection constraints to rapidly calculate the detector response in various complex environments is ***,the data library required for the FFCM is built by collecting the detection volume,detector counts,and flux sensitivity functions through a Monte Carlo ***,based on perturbation theory and the Rytov approximation,a model for the detector response is derived using the flux sensitivity function method and a one-group diffusion *** environmental perturbation is constrained to optimize the model according to the tool structure and the impact of the formation and borehole within the effective detection ***,the method is applied to a neutron porosity tool for *** various complex simulation environments,the maximum relative error between the calculated porosity results of Monte Carlo and FFCM was 6.80%,with a rootmean-square error of 0.62 *** field well applications,the formation porosity model obtained using FFCM was in good agreement with the model obtained by interpreters,which demonstrates the validity and accuracy of the proposed method.

关键词： Nuclear measurement Fast forward computation Volumetric constraints

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Indispensable gutter layers in thin-film composite membranes for carbon capture

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Green Energy & Environment 2024年第8期9卷 1220-1238页

作者： Gengyi zhang Haiqing lin Department of Chemical and Biological Engineering University at Buffalo The State University at New York

Industrial thin-film composite(TFC) membranes achieve superior gas separation properties from high-performance selective layer materials,while the success of membrane technology relies on high-performance gutter layers to achieve production scalability and low-cost manufacturing. However, the current literature predominantly focuses on the design of polymer architectures to obtain high permeability and selectivity, while the art of fabricating gutter layers is usually safeguarded by industrial manufacturers and appears lackluster to academic researchers. This is the first report aiming to provide a comprehensive and critical review of state-of-the-art gutter layer materials and their design and modification to enable TFC membranes with superior separation performance. We first elucidate the importance of the gutter layer on membrane performance through modeling and experimental results. Then various gutter layer materials used to obtain high-performance composite membranes are critically reviewed, and the strategies to improve their compatibility with the selective layer are highlighted, such as oxygen plasma treatment, polydopamine deposition, and surface grafting. Finally, we present the opportunities of the gutter layer design for practical applications.

关键词： Thin-film composite membranes Gutter layer Gas separation Carbon capture

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Deep reinforcement learning based active surge control for aeroengine compressors

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Chinese Journal of Aeronautics 2024年第7期37卷 418-438页

作者： Xinglong zhang Zhonglin lin Runmin JI Tianhong zhang College of Energy and Power Engineering Nanjing University of Aeronautics and AstronauticsNanjing 210016China school of Mechanical Engineering and Automation Fuzhou UniversityFuzhou 350108China

This study proposes an active surge control method based on deep reinforcement learning to ensure the stability of compressors when adhering to the pressure rise command across the wide operating range of an ***,the study establishes the compressor dynamic model with uncertainties,disturbances,and Close-Coupled Valve(CCV)actuator *** upon this foundation,a Partially Observable Markov Decision Process(POMDP)is defined to facilitate active surge *** address the issue of unobservability,a nonlinear state observer is designed using a finite-time high-order sliding ***,an Improved soft Actor-Critic(IsAC)algorithm is developed,incorporating prioritized experience replay and adaptive temperature parameter techniques,to strike a balance between exploration and convergence during *** addition,reasonable observation variables,error-segmented reward functions,and random initialization of model parameters are employed to enhance the robustness and generalization ***,to assess the effectiveness of the proposed method,numerical simulations are conducted,and it is compared with the fuzzy adaptive backstepping method and second-Order sliding Mode Control(sOsMC)*** simulation results demonstrate that the deep reinforcement learning based controller outperforms other methods in both tracking accuracy and ***,the proposed active surge controller can effectively ensure stable operation of compressors in the high-pressure-ratio and high-efficiency region.

关键词： Aeroengine surge Active surge control Moore-Greitzer model Deep reinforcement learning soft actor-critic Nonlinear observer

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selective photosynthesis of imines from biomass-derived aldehydes over Ni/TiO_(2)

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Rare Metals 2024年第3期43卷 1116-1124页

作者： Wu-lin Li Qing-Qing zhang lin Dong Wen-Jun zhang Li-Li lin Zu-Peng Chen Jiangsu Co-Innovation Center of Efficient Processing and Utilization of Forest Resources International Innovation Center for Forest Chemicals and MaterialsCollege of Chemical EngineeringNanjing Forestry UniversityNanjing210037China Institute of Industrial Catalysis State Key Laboratory of Green Chemistry Synthesis TechnologyCollege of Chemical EngineeringZhejiang University of TechnologyHangzhou310014China

Photocatalytic reductive amination of biomass-derived aldehydes is a desirable way to selectively upgrade biomass into value-added nitrogen-containing chemicals under mild ***,it is challenging to produce imines in high selectivity because of the undesirable side reactions caused by the activity of functional ***,we demonstrate the highly reactive and selective production of imines from biomass derived aldehydes via the photocatalytic reductive amination,using a defective TiO_(2)supported nickel *** employment of methanol as the hydrogen donor and ammonia solution as the nitrogen source avoids the use of high-pressure H_(2)and expensive amines,rendering the current catalytic process safe,economical,and environmentally *** depth investigations attribute the improved separation and transfer of photogenerated charge carriers to the presence of oxygen vacancies and decorated Ni nanoparticles,thereby accelerating the production of imines from benzaldehyde amination(conversion,95.8%;seleetivity,95.2%).Furthermore,the developed system could be easily translated to the photocatalytic conversions of various biomass derived aldehydes,which provided an example of a cost-effective and sustainable approach for the valorization of biomass derived feedstocks.

关键词： Photocatalysis Biomass derivatives Imines Reduction amination Heterogeneous catalyst

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Analysis and experimental study on resistance-increasing behavior of composite high efficiency autonomous inflow control device

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Petroleum science 2024年第2期21卷 1290-1304页

作者： Liang-Liang Dong Yu-lin zhang school of Mechatronic Engineering Southwest Petroleum UniversityChengdu610500SichuanChina state Key Laboratory of Oil and Gas Reservoir Geology and Exploitation Southwest Petroleum UniversityChengdu610500SichuanChina Oil and Gas Equipment Technology Sharing and Service Platform of Sichuan ProvinceChengdu610500SichuanChina

Bottom water coning is the main reason to reduce the recovery of horizontal bottom water reservoir. By water coning, we mean the oil-water interface changes from a horizontal state to a mound-shaped cone and breaks through to the wellbore. Autonomous inflow control device(AICD) is an important instrument maintain normal production after bottom water coning, however, the resistance increasing ability of the swirl type AICD is insufficient at present, which seriously affects the water control effect. Aiming this problem, this paper designs a multi-stage resistance-increasing and composite type AICD. The separation mechanism of oil-water two phases in this structure, the resistance form of oil-water single phase and the resistance-increasing principle of water phase are analyzed. Establishing the dual-phase multi-stage separation and resistance-increasing model, and verified by measuring the throttling pressure drop and oil-water volume fraction of the AICD, it is found that the composite type AICD has the effect of ICD and AICD at the same time, which can balance the production rate of each well section at the initial stage of production, delay the occurrence of bottom water coning. In the middle and later stages of production, water-blocking can be effectively increased to achieve water control and stable *** structural sensitivity analysis, the influence law of various structural parameters on the water control performance of composite AICD was obtained. The simulation calculation results show that,compared with the existing swirl type AICD, composite AICD has higher sensitivity to moisture content,the water phase throttling pressure drop is increased by 4.5 times on average. The composite AICD is suitable for the entire stage of horizontal well production.

关键词： Water control Flow separation Flow resistance-increasing AICD device simulation and experiment

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Materials design and preparation of ultrathin two-dimensional metal halide perovskites

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Nano Research 2024年第7期17卷 6231-6246页

作者： Xiaomin zhang sihan Zhao Junran zhang lin Wang school of Flexible Electronics(Future Technologies)and Institute of Advanced Materials Key Laboratory of Flexible ElectronicsJiangsu National Synergetic Innovation Center for Advanced MaterialsSchool of Physical and Mathematical SciencesNanjing Tech UniversityNanjing 211816China

Metal halide perovskites(MHPs)have emerged as highly promising candidates for the next generation of photonics and optoelectronic devices,owing to their prominent optical and excitonic properties,as well as the convenience of ***,ultrathin two-dimensional(2D)MHPs,which are generally prepared by exfoliation,solution growth,and chemical vapor deposition method,have attracted dramatically increasing attentions owing to their combined features of ultrathin 2D morphology and superior performance of *** the growing interest in ultrathin 2D MHPs,there is currently a lack of a comprehensive and systematic overview of the distinct advantages offered by each growth method for producing these *** review critically assesses the preliminary studies on the materials design and preparation of ultrathin ***,it explores heterostructures based on ultrathin MHPs and offers insights into the challenges and opportunities that lie ahead for this enticing class of 2D materials.

关键词： ultrathin perovskites material preparation exfoliation solution growth chemical vapor deposition

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Color-kinematics duality and dual conformal symmetry for a four-loop form factor in N=4 sYM

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science China(Physics,Mechanics & Astronomy) 2024年第4期67卷 64-71页

作者： Guanda lin Gang Yang siyuan zhang CAs Key Laboratory of Theoretical Physics Institute of Theoretical PhysicsChinese Academy of SciencesBeijing 100190China school of Physical sciences University of Chinese Academy of SciencesBeijing 100049China school of Fundamental Physics and Mathematical sciences Hangzhou Institute for Advanced StudyUCASHangzhou 310024China International Centre for Theoretical Physics Asia-Pacific Beijing/Hangzhou 310024China

We obtain the integrand of full-color four-loop three-point form factor of the stress-tensor supermultiplet in N=4 sYM,based on the color-kinematics(CK)duality and generalized unitarity *** result not only manifests all dual Jacobi relations via CK duality but also contains 133 free *** suggests the constructibility of the form factor at even higher loops via CK *** also find that the planar form factor has a hidden dual conformal symmetry in the lightlike limit of the operator momentum,which is checked up to four loops.

关键词： s-matrix supersymmetric model perturbative calculations

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A bifunctional POM-based Cu-viologen complex with mixed octamolybdate clusters for rapid oxidation desulfurization and effective photogeneration of hydrogen

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Rare Metals 2024年第1期43卷 236-246页

作者： lin Yang Zhong zhang Chao-Nan zhang Xiu-Li Wang College of Chemistry and Materials Engineering Bohai UniversityJinzhou 121013China Professional Technology Innovation Center of Liaoning Province for Conversion Materials of solar Cell Bohai UniversityJinzhou 121013China

The design and synthesis of catalysts for the oxidation desulfurization and production of hydrogen are extremely important for solving environmental pollution and energy ***,a novel bifunctional [α-Mo_(8)O_(26)]^(4-)/[β-Mo_(8)O_(26)]^(4-)-based Cu-viologen complex H_(4)[Cu_(2)~ⅠCl_(2)(Hbcbpy)_(4)] [α-Mo_(8)O_(26)] [β-Mo8O_(26)]·H_(2)O(BHU-2,Hbcbpy=1-(4-carboxybenzyl)-4,4'-bipyridinium) was synthesized and characterized by single-crystal X-ray diffraction(XRD),infrared radiation spectra,powder X-ray diffraction(PXRD) and X-ray photoelectron spectroscopy(XPs) *** structural characteristic of BHU-2 is the presence of two types of octamolybdate clusters [α-Mo_(8)O_(26)]^(4-)/[β-Mo_(8)O_(26)]^(4-)and a new binuclear Cu~Ⅰ-Hbcbpy complex linked by Cl-bridges[Cu_(2)ⅠCl_(2)(Hbcbpy)_(4)]^(4+).BHU-2 as a heterogeneous catalyst exhibits excellent activities to the oxidation desulfurization and photocatalytic hydrogen *** room temperature,BHU-2 can catalyze 96% conversion of methyl phenyl sulfide with 98% selectivity,and the process obeys the pseudo-first-order reaction kinetic with the half-life of9.6 *** notorious 2-chloroethyl ethyl sulfide can achieve 99% conversion with 98% selectivity within only1 min at the presence of BHU-2,and the turnover frequency(TOF) is up to 7400 h^(-1).BHU-2 also exhibits high catalytic activity for the oxidation of other aromatic and aliphatic thioethers within short time at room ***,BHU-2 shows a high catalytic activity for visible-light-driven hydrogen evolution with an H_(2) evolution rate of 1677.85 μmol·g^(-1)·h^(-1) within 10 ***,the catalytic activities do not decrease evidently after three cycles,revealing the prominent structural stability and recyclability.

关键词： Polyoxometalate Metal-organic complex Viologen Oxidation desulfurization Photocatalytic hydrogen production

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Toughening additive manufactured Zr-based bulk metallic glass composites by martensite phase transformation

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Journal of Materials science & Technology 2024年第3期170卷 95-102页

作者： Pengcheng zhang Cheng zhang Jie Pan Di Ouyang lin Liu state Key Laboratory of Materials Processing and Die&Mould Technology School of Materials Science and EngineeringHuazhong University of Science and TechnologyWuhan 430074China

Additive manufacturing technology based on laser powder bed fusion(LPBF)offers a novel approach for fabricating bulk metallic glass(BMG)products without restriction in size and ***,the BMGs prepared by LPBF usually suffered from less plasticity and poorer fracture toughness as compared to their cast counterparts due to partial crystallization in heat-affected zones(HAZs).since crystallization in HAZs is hard to avoid completely in LPBF BMGs,it is desirable to design a suitable alloy system,in which only ductile crystalline phase,instead of brittle intermetallics,is formed in *** unique structure could effectively increase the toughness/plasticity of the LPBF *** achieve this goal,a quaternary BMG system with a composition of Zr_(47.5)Cu_(45.5)Al_(5)Co_(2)is adopted and subjected to *** is found that nearly a single phase of B_(2)-ZrCu is precipitated in HAZs,while a fully amorphous phase is formed in molten pools(MPs).This B_(2)phase reinforced BMG composite exhibits excellent mechanical properties with enhanced plasticity and ***,it is easy to modulate the mechanical properties by altering the amount of the B_(2)phase via adjusting the laser energy ***,the best combination of strength,plasticity,and notch toughness is obtained in the BMG composite containing 27.4%B_(2)phase and 72.6%amorphous phase,which exhibits yield strength(σ_(s))of 1423 MPa,plastic strain(ε_(p))of 4.65%,and notch toughness(K_(q))of 53.9 MPa m 1/***,a notable strain-hardening is also *** improvement of plasticity/toughness and appearance of strain-hardening behavior are mainly due to the martensite phase transformation from the B_(2)phase to the Cm phase during plastic deformation(i.e.,the phase transformation-induced plasticity effect).The current work provides a guide for making advanced BMGs and BMG composites by additive manufacturing.

关键词： Laser powder bed fusion Bulk metallic glass composites Phase transformation-induced plasticity Deformation mechanism

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Precipitation and anthropogenic activities regulate the changes of NDVI in Zhegucuo Valley on the southern Tibetan Plateau

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Journal of Mountain science 2024年第2期21卷 607-618页

作者： ZHAO Wanglin WANG Hengying zhang Huifang zhang lin school of Ecology and Environment Tibet UniversityLhasa 850000China Institute of Tibetan Plateau Research Chinese Academy of SciencesBeijing 100101China southwest survey and Planning Institute of National Forestry and Grassland Administration Kunming 650000China Monitoring Center for Ecological Environment of Xizang Autonomous Region Lhasa 850000China

Whether climate change or anthropogenic activities play a more pivotal role in regulating vegetation growth on the Tibetan Plateau is still controversial.A better understanding on grassland changes at a fine scale may provide important guidance for local government policy and grassland *** two of the most reliable satellite NDVI products(MODIs NDVI and sPOT NDVI),we evaluated the dynamic of grasslands in the Zhegucuo valley on the southern Tibetan Plateau from 2000 to 2020,and analyzed its driving factors and relative influences of climate change and anthropogenic ***,the key indicators of climate change were assumed to be precipitation and *** main results were:(1)the grassland NDVI in Zhegucuo valley did not reflect a significant temporal change during the last 21 *** variation of precipitation during the early growing season(GsP)resembled that of NDVI,and the GsP was positively correlated with *** the pixel level,the partial correlation analysis showed that 37.79%of the pixels depicted a positive relationship between GsP and NDVI,while 11.32%of the pixels showed a negative relationship between temperature during the early growing season(GsT)and NDVI.(2)In view of the spatial distribution,the areas mainly controlled by GsP were generally distributed in the southern part,while those affected by GsT stood in the eastern part,mainly around the Zhegucuo lake where most population in Cuomei County settled down.(3)Decreasing NDVI trends were mainly occurred in alpine steppe at lower elevations rather than alpine meadow at higher elevations.(4)The residual trend(REsTREND)analysis further indicated that the anthropogenic activities played a more pivotal role in regulating the annual changes of NDVI rather than climate factors in this *** studies should pay more attention on climate extremes rather than the simple temporal ***,the influence of human activities on alpine grassland needs to be accessed and fully

关键词： Anthropogenic activities Climate change Precipitation Fencing Vegetation degradation

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