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Rare earth-doped mixed Ni-Cu-Zn ferrites as an effective photocatalytic agent for active degradation of Rhodamine B dye

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Journal of Rare Earths 2024年第3期42卷 488-496,I0003页

作者： s.apnil.a.jadhav sandeep B.somvanshi sudarshan s.Gawali Kranti Zakde K.M.jadhav Department of Physics Dr.Babasaheb Ambedkar Marathwada UniversityAurangabad431004MaharashtraIndia school of Materials Engineering Purdue UniversityWest Lafayette 47906USA University Department of Basic and Applied sciences MGM UniversityAurangabad431003MaharashtraIndia

In this study, a series of Gd^(3+)-doped mixed Ni-Cu-Zn ferrites with composition of Zn_(0.5)Ni_(0.3)Cu_(0.2)Fe_(2-x)Gd_(x)O_(4)(x = 0, 0.025, 0.05, 0.075, 0.1) was prepared using self-ignition sol-gel method. The prepared nanoparticles with an average size ranging from 22 to 26 nm show a single-phase cubic structure belonging to the spinel matrix. A rise in the Gd^(3+)concentration leads to an increase in crystallite size and lattice parameter. In Fourier transform infrared spectra, two main absorption bands belonging to the spinel structure are observed. The high-frequency bands(v_(1)) represent the tetrahedral complex, while the lowfrequency bands(v_(2)) signify the octahedral complex. The optical bandgap of the nanoferrites is found within the range of 2.91 to 2.41 eV, depending on their size. The magnetic characteristics of the material,such as saturation magnetization and coercivity are significantly altered with the concentration of Gd^(3+)in the solution. Using Rhodamine B(RhB) as a model organic pollutant, an in-depth investigation of the photocatalytic activity of the compounds was carried out. The present outcomes show that adding an adequate amount of Gd^(3+)significantly enhances the number of hydroxyl radicals produced by the ferrite,in turn, increasing the photocatalytic activity of the material. Mechanism elucidated by scavenger studies reveals that ·OH and holes are the primary reactive radicals responsible for the degradation *** photocatalysts show an insignificant performance loss in five consecutive cycles. Thus, it is concluded that these photocatalysts are highly suitable for the remediation of dye-contaminated wastewater.

关键词： Gd^(3+)substitution spinel ferrite structural properties Magnetic properties Photocatalysis Rare earths

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Influence of cerium ions on structure-dependent magnetic properties of Ba-sr M-type hexaferrite nanocrystals

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Journal of Rare Earths 2024年第2期42卷 364-372,I0005页

作者： Ram A.Pawar sunil M.Patange P.M.Dighe sher singh Meena Abdullah GAl-sehemi Mehboobali Pannipara santosh s.jadhav Department of Physics ArtsCommerce and Science CollegeAhmednagar413711MaharashtraIndia Department of Physics Shri Krishna MahavidyalayaGunjotiDistOsmanabad413606MaharashtraIndia Padmashri Vikhe Patil College of Arts Science and CommercePravaranagarA/P.Loni(Kd)Tal.RahataDistAhmednagar413713MaharashtraIndia solid state Physics Division Bhabha Atomic Research CentreMumbai400085MaharashtraIndia Department of Chemistry King Khalid UniversityAbha61413Saudi Arabia Department of Physics D.S.M's ArtsCommerce and Science CollegeJintur431509MaharashtraIndia

The present study is a systematic effort to investigate the structure-sensitive magnetic parameters of Ce^(3+) substituted Ba-sr hexaferrite nanocrystals chemically formulated as Ba_(0.5)sr_(0.5)Ce_(x)Fe_(12-x)O_(19) where x=0.0-0.2 with Δx=*** hexaferrite powders were prepared using the sol-gel self-ignition route and structurally characterized by means of powder X-ray diffraction and Fourier transform infrared *** creation of the M-type hexaferrite phase within the synthesized samples was revealed from the Rietveld refinement of the X-ray *** occurrence of a secondary phase of CeO_(2) was revealed within the hexaferrites for the substitution,x> *** refined X-ray diffraction data were utilized to compute the lattice parameters,X-ray density,and lattice parameter *** crystal structure plotted from the refined XRD data reveals the occupancy of the ions at different lattice *** XPs data of the hexaferrite were analyzed to confirm the oxidation states of the constituent *** nanocrystalline nature of the hexaferrites was revealed from the crystallite sizes calculated using scherer's *** analysis of FTIR spectra confirms that only a fraction of Ce^(3+)accommodated in the lattice and the remaining Ce content reside in the form of the CeO_(2) *** morphology of the hexaferrites was analyzed from the FEsEM profiles of the ferrite *** magnetic behavior study was performed by analyzing the Curie temperature,hysteresis loops,and hyperfine interactions by means of susceptibility,V.s.M,and Mossbauer spectroscopy,*** hexaferrites with increasing coercivity,decreasing saturation magnetization,and decreasing Curie temperature are reported in the *** substituted Ce^(3+)ions inhibit the grain growth and create lattice imperfections giving rise to hexaferrites with tuned magnetic parameters suitable for different applications.

关键词： Ba-sr hexaferrite Ce^(3+)substitution XPs saturation magnetization Coercivity M?ssbauer spectroscopy

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Direct-seeded Rice: Genetic Improvement of Game-Changing Traits for Better Adaption

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Rice science 2024年第4期31卷 417-433页

作者： Priyanka NEGI Jagadish RANE Rajendra sadashiv WAGH Tukaram Jayaram BHOR Dipti Digambar GODsE Priyanka jadhav C.ANILKUMAR Dasari sREEKANTH K.sAMMI REDDY sharad Ramrao GADAKH K.M.BORAIH C.B.HARIsHA P.s.BAsAVARAJ Indian Council of Agricultural Research(ICAR)-National Institute of Abiotic stress Management Baramati 413115India Mahatma Phule Krishi Vidyapeeth Rahuri 413722India ICAR-Central Institute for Arid Horticulture Bikaner 334006India ICAR-National Rice Research Institute Cuttack 753006India ICAR-Directorate of Weed Research Jabalpur 482004India Dr.Panjabrao Deshmukh Krishi Vidyapeeth Akola 444104India

The sustainability of rice production continues to be a subject of uncertainty and inquiry attributed to shifts in climatic conditions. In light of the impending climate change crisis and the high labor and water costs accompanying it, direct-seeded rice(DsR) is unquestionably one of the most practical solutions. Despite its resource and climate-friendly advantages, early maturing rice faces weed competitiveness and seedling establishment challenges. Resolving these issues is crucial for promoting its wider adoption among farmers, presenting it as a more effective sustainable rice cultivation method globally. Diverse traditional and contemporary breeding methods are employed to mitigate the limitations of the DsR approach, leveraging advanced techniques such as speed breeding and genome editing. Focusing on key traits like mesocotyl length elongation, early seedling vigor, root system architecture, and weed competitiveness holds promise for transformative improvements in DsR adaptation at a broader scale within farming communities. This review aims to summarize how these features contribute to increased crop production in DsR conditions and explore the research efforts focusing on enhancing DsR adaptation through these traits. Emphasizing the pivotal role of these game-changing traits in DsR adaptation, our analysis sheds light on their potential transformative impact and offers valuable insights for advancing DsR practices.

关键词： climate change direct-seeded rice aerobic rice early vigor trait

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均相和非均相催化微藻脂质提取和酯交换制备生物燃料的研究进展

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Chinese Journal of Catalysis 2024年第4期59卷 97-117页

作者： Vinoth Kumar Ponnumsamy Hussein E.Al-Hazmi sutha shobana Jeyaprakash Dharmaraja Dipak Ashok jadhav Rajesh Banu J Grzegorz Piechota Bartłomiej Igliński Vinod Kumar Amit Bhatnagar Kyu-Jung Chae Gopalakrishnan Kumar 高雄医科大学药物与应用化学系环境医学研究中心中国台湾高雄高雄医科大学医学研究部中国台湾高雄格但斯克理工大学土木与环境工程学院波兰纳鲁特维察格但斯克范朗大学工程与技术学院建筑绿色技术与可持续发展研究组越南胡志明市工程技术学院科学与人文系化学部印度泰米尔纳德邦韩国海洋大学海洋科学与工程学院环境工程系韩国釜山泰米尔纳德邦中央大学生命科学系印度泰米尔纳德邦 GPCHEM沼气研究与分析实验室波兰尼古拉斯哥白尼大学化学系波兰克兰菲尔德大学水与能源学院英国拉彭兰塔工业大学工程科学学院分离科学系芬兰韩国海洋大学海洋可再生能源工程专业韩国釜山延世大学土木与环境工程学院韩国首尔斯塔万格大学科学技术学院化学、生物科学与环境工程研究所挪威斯塔万格

随着化石燃料燃烧导致的二氧化碳排放不断加剧气候变化,且化石燃料储量日益减少,寻求可再生能源已成为一项紧迫的任务.其中,藻类衍生可持续燃料因具有成本优势和可运输性,在解决全球能源危机方面展现出广阔前景,备受关注.利用化学转化... 详细信息

随着化石燃料燃烧导致的二氧化碳排放不断加剧气候变化,且化石燃料储量日益减少,寻求可再生能源已成为一项紧迫的任务.其中,藻类衍生可持续燃料因具有成本优势和可运输性,在解决全球能源危机方面展现出广阔前景,备受关注.利用化学转化技术从微藻中提取脂质,并通过酯交换反应可以将其转化为脂肪酸甲酯,是生产绿色生物燃料的有效途径.这一过程涉及游离脂肪酸、磷脂和甘油三酯的提取,并且生产过程能耗低,成为满足日益增长的能源需求的一种理想解决方案.本文综述了微藻脂质提取和酯交换制备生物燃料的相关研究进展.首先,介绍了微藻脂质的提取方法,包括溶剂提取法、索氏提取法、布利格和戴耶法、超临界二氧化碳提取以及离子液体溶剂法等,并分析了各方法的优缺点.随后,重点阐述了酯交换技术在微藻脂质转化中的应用,包括酸碱催化、酶催化以及原位酯交换反应等,并探讨了这些技术的反应机理、催化剂选择、反应器设计以及生物油生产工艺等方面的研究进展.通过综述上述研究进展,为微藻脂质的生产和应用提供了理论指导.研究表明,通过优化催化剂种类、反应条件以及提取方法,可以有效提高微藻脂质的转化效率和生物油品质.同时,本文也指出了当前微藻脂质生产中面临的挑战,如微藻栽培和生长条件优化、高效转化技术的开发等.随着可持续能源日益受到重视,微藻脂质作为一种可再生能源具有巨大的发展潜力.未来研究应进一步关注微藻的规模化栽培、生长条件优化以及高效转化技术的研发,以提高微藻脂质的产量和品质.同时,应进一步推动和实现微藻生物燃料的实际应用,从而为应对气候变化和能源危机提供有效的解决方案.

关键词：微藻脂质提取酯交换催化酶催化原位技术

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Lanthanum(Ⅲ) sorption studies on poly[dibenzo-18-crown-6] and its separation from uranium(Ⅵ) and thorium(Ⅳ) in L-valine medium

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Journal of Rare Earths 2009年第5期27卷 825-829页

作者： s.R.sabale D.V.jadhav B.s.Mohite Analytical and Environmental Research Lab Department of ChemistryShivaji University

The sorption study of La(Ⅲ) was carried out on poly[dibenzo-18-crown-6] and L-valine medium. The quantitative adsorption of La(Ⅲ) was found at 1×10-2 to 1×10-5 mol/L L-valine. The various eluting agents were found efficient eluents for La(Ⅲ). The capacity of crown polymer for La(Ⅲ) was found to be 0.43 ±0.01 mmol/g. The tolerance limit of various cations and anions for La(Ⅲ) was determined. La(Ⅲ) was quantitatively separated from other metal ions in binary as well as multicomponent mixtures. The study was extended to sequential separation of La(Ⅲ), U(VI) and Th(IV). The good separation yields were obtained and had good reproducibility (±2%). The method incorporated the determination of La(Ⅲ) in real sample. The method was simple, rapid and selective.

关键词： La(Ⅲ) L-valine poly[dibenzo-18-crown-6] sorption separation rare earths

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Computer-aided diabetic retinopathy diagnostic model using optimal thresholding merged with neural network

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International Journal of Intelligent Computing and Cybernetics 2020年第3期13卷 283-310页

作者： Ambaji s.jadhav Pushpa B.Patil sunil Biradar Department of Electrical and Electronics B.L.D.E.A’s V.P.Dr.P.G.Halakatti College of Engineering and Technology(Affiliated to Visvesvaraya Technological University)VijayapurIndia Department of Ophthalmology Shri B.M.Patil Medical College and Research Center(Deemed to be University)VijayapurIndia

Purpose-Diabetic retinopathy(DR)is a central root of blindness all over the *** DR is tough to diagnose in starting stages,and the detection procedure might be time-consuming even for qualified ***,intelligent disease detection techniques are extremely acceptable for progress analysis and recognition of various ***,a computer-aided diagnosis scheme based on intelligent learning approaches is intended to propose for diagnosing DR effectively using a benchmark ***/methodology/approach-The proposed DR diagnostic procedure involves four main steps:(1)image pre-processing,(2)blood vessel segmentation,(3)feature extraction,and(4)***,the retinal fundus image is taken for pre-processing with the help of Contrast Limited Adaptive Histogram Equalization(CLAHE)and average *** the next step,the blood vessel segmentation is carried out using a segmentation process with optimized gray-level *** the blood vessels are extracted,feature extraction is done,using Local Binary Pattern(LBP),Texture Energy Measurement(TEM based on Laws of Texture Energy),and two entropy computations-shanon’s entropy,and Kapur’s *** collected features are subjected to a classifier called Neural Network(NN)with an optimized training *** the gray-level thresholding and NN is enhanced by the Modified Levy Updated-Dragonfly Algorithm(MLU-DA),which operates to maximize the segmentation accuracy and to reduce the error difference between the predicted and actual outcomes of the ***,this classification error can correctly prove the efficiency of the proposed DR detection ***-The overall accuracy of the proposed MLU-DA was 16.6%superior to conventional classifiers,and the precision of the developed MLU-DA was 22%better than LM-NN,16.6%better than PsO-NN,GWO-NN,and ***,it is concluded that the implemented MLU-DA outperformed state-of-the-art algorithms in detecting ***

关键词： Diabetic retinopathy detection Gray-level thresholding Optimal trained neural network Dragon fly algorithm Levy update Performance metrics

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Role of composition and grain size in controlling the structure sensitive magnetic properties of sm substituted nanocrystalline Co-Zn ferrites

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Journal of Rare Earths 2020年第10期38卷 1069-1075,I0002页

作者： Anil B.Mugutkar shyam K.Gore Umakant B.Tumberphale Vijaykumar V.jadhav Rajaram s.Mane sunil M.Patange sagar E.shirsath santosh s.jadhav Bahirji smarak Mahavidyalaya Basmath431512MaharashtraIndia Microwave Research Laboratory N.E.S.Science CollegeNanded431601MaharashtraIndia Dnyanopasak shikshan Mandal's Arts Commerce and Science CollegeJintur431509MaharashtraIndia Guangdong Technion Israel Institute of TechnologyShantou 515006China Department of Physics Shivaji MahavidyalayaUdgir-413517MaharashtraIndia school of Physical sciences Swami Ramanand Teerth Marathwada UniversityNanded431606MaharashtraIndia shri Krishna Mahavidyalaya Gunjoti413613MaharashtraIndia school of Materials science and Engineering University of New South WalesSydney2052NSWAustralia

The nanocrystalline samarium substituted Co-Zn ferrites with chemical formula Co0.7Zn0.3smyFe2-yO4(where y=0,0.01,0.02,0.03,0.04) were synthesized by sol-gel autocombustion *** analysis of Xray diffractograms(XRD) reveals the formation of cubic spinel *** planes indexed from XRD analyses were confirmed in the selected area electron diffraction(sAED) image of the *** nature of the particles in the ferrite samples was confirmed by *** morphology was analyzed by scanning electron microscopy(sEM).Magnetic measurements show an increase in the magnetization for x ≤*** decrease in magnetization due to spin canting is observed for x=*** coercivity depends on sm3+doping concentration,grain size and saturation *** complex permeability of the ferrites was analyzed as the function of frequency and sm3+composition(y).The real part of complex permeability varies linearly with the grain size.

关键词： Nanocrystalline ferrites Rietveld refinement HRTEM Magnetization Coercivity Permeability

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Application and Improvements of the Wing Deformation Capture with simulation for Flapping Micro Aerial Vehicle

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Journal of Bionic Engineering 2020年第6期17卷 1096-1108页

作者： Wee-Beng Tay siddharth jadhav Jian-Lei Wang Centre for Aerodynamics&Propulsion Temasek LaboratoriesNational University of SingaporeSingapore 117411Republic of Singapore shaanxi Aerospace Flight Vehicle Design Key Laboratory School of AstronauticsNorthwestern Polytechnical UniversityXi'an 710072China

Wing deformation capture with simulation is a mixed experimental-numerical approach whereby the wing deformation during flapping is captured using high-speed cameras and used as an input for the numerical *** is an alternative approach compared to pure experiment or full fluid structure interaction *** study is an update to the previous paper by Tay et al.,which aims to address the previous *** show through thrust and vorticity contour plots that this approach can simulate Flapping Micro Aerial Vehiclex(FMAVs)with reasonable ***,we use this approach to explain the thrust improvement when an additional rib is added to the original membrane wing,which is due to longer duration for the new wing to open during the fling ***,by decreasing the number of points and frames per cycle on the wing,we can simplify and shorten the digitization *** results show that this approach is an accurate and practical alternative which can be applied to general bio-inspired research.

关键词： flapping MAV immersed boundary method wing deformation membrane wings

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Observations of NO_2 and O_3 during Thunderstorm Activity Using Visible spectroscopy

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Advances in Atmospheric sciences 1996年第3期13卷 359-374页

作者： D.B.jadhav A.L.Londhe s.Bose Indian Institute of Tropical Meteorology Dr.Homi Bhabha MargPashanPune-411008MaharashtraIndiaIndian Institute of Tropical MeteorologyDr.Homi Bhabha MargPashanPune-411008MaharashtraIndiaIndian Institute of Tropical MeteorologyDr.Homi Bhabha MargPashanPune-411008MaharashtraIndia

simultaneous observations for the total column densities of NO2,O3 and H2O were carried on using the portable spectrometer (438-450 nm and 400-450 nm) and the visible spectrometer (544.4-628 nm) during premonsoon thunderstorms and embedded hail storm activity at Pune (18°32'N & 73°51'E),*** observations confirm the fact that there is an increase in O3 and NO2 column densities during *** increase in O3 was observed following onset of thunderstorm,while the increase in NO2 was observed only after the thunder flashes *** implies that the production mechanisms for O3 and NO2 in thunderstorm are *** observed column density of NO,value (1 to 3×1017molecules cm-2) during thunderstorm activity is 10 to 30 times higher than the value (1×10th molecules cm-2) of a normal day total column *** spectrometric observations and observations of thunder flashes by electric field meter showed that 6.4×1025molecules/flash of NO2 are *** increased to-oil column density of ozone during thunderstorm period is 1.2 times higher than normal (clear) day ozone *** multiple scattering in the clouds is estimated from H2O and O2 absorption bands in the visible spectral region Considering this effect the calculated amount of ozone added in the global atmosphere due to thunderstorm activity is 0.26 to 0 52 DU,and the annual production of ozone due to thunderstorm activity is of the order of 4.02×10 molecules/year The annual NO2 production may be of the order of 2.02×1035molecules/year.

关键词： Visible spectroscopy Thunderstorm Ozone production NO2 production Atmospheric electricity Lightning flashes. Multiple scattering factor

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Facile synthesis of magnetic iron oxide nanoparticles and their characterization

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Frontiers of Materials science 2014年第2期8卷 193-198页

作者： sushilkumar A. jadhav suresh V. PATIL Department of Chemistry and NIs Center University of Torino 10125 Torino Italy Department of Chemistry K.B.P. College Pandharpur affiliated to Solapur University Solapur (MH) India

Magnetic iron oxide nanoparticles are synthesized by suitable modification of the standard synthetic procedure without use of inert atmosphere and at room temperature. The facile synthesis procedure can be easily scaled up and is of important from industrial point of view for the commercial large scale production of magnetic iron oxide nanoparticles. The synthesized nanoparticles were characterized by thermal, dynamic light scattering, scanning electron microscopy and transmission electron microscopy analyses.

关键词： iron oxide iron oxide nanoparticle co-precipitation-

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