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Orange-red emitting sr_3LaTa_3O_(12):sm^(3+) phosphors with perovskite structure and high thermal stability for w-LEDs

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Journal of Rare Earths 2024年第3期42卷 464-472,I0002页

作者： Xiaopeng hu anlin Zhang Yufeng Du Li Zhou Changlin Li Jingjing Lian Zhequan Zou Xuan Ouyang Bin Deng Lianwu Xie Ruijin Yu College of Chemistry Biology and Environmental Engineering Xiangnan UniversityChenzhou423043China College of sciences Central South University of Forestry and TechnologyChangsha410004China College of Chemistry&Pharmacy Northwest A&F UniversityYangling712100China hunan Provincial Key Laboratory of Xiangnan Rare-Precious Metals Compounds Research and Application Xiangnan UniversityChenzhou423043China

A novel layered perovskite tantalate phosphor sr_(3)LaTa_(3)O_(12):sm^(3+)(sLTO:sm^(3+)) with orange-red emission was obtained for the first time via the solid-phase synthetic method. The phase purity, surface morphology,element distribution and luminescent properties of the sLTO:xsm^(3+)(x= 0.01 mol%-0.30 mol%) phosphors were investigated. Under 408 nm excitation, the optimum doped sLTO:0.10sm^(3+) phosphor emits orangered light at 598 nm with the highest emission peak(4G_(5/2)→6H_(7/2)). The critical energy transfer distance is 1.687 nm. The prepared sLTO:0.10sm^(3+)phosphor has excellent thermal stability with temperature quenching temperature(T_(0.5)> 500 K) and high activation energy(E_(a)= 0.25 e V). Through calculation, the chromaticity coordinates of all samples are concentrated in the orange-red area, and the color purity reaches 99%. The fabricated white light-emitting diode(w-LED) has a good correlated color temperature(5132 K), a high R_(a)(89), and the CIE chromaticity coordinates(0.340, 0.327). Consequently, the superiority of orange-red-emitting tantalate sLTO:sm^(3+) phosphors for w-LEDs is demonstrated.

关键词： Tantalate sr_(3)LaTa_(3)O_(12) sm^(3+) Luminescence LED Rare earths

Enhancing XRF sensor-based sorting of porphyritic copper ore using particle swarm optimization-support vector machine(PsO-sVM)algorithm

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International Journal of Mining science and Technology 2024年第4期34卷 545-556页

作者： Zhengyu Liu Jue Kou Zengxin Yan Peilong Wang Chang Liu Chunbao sun anlin shao Bern Klein school of Civil and Resources Engineering University of Science and TechnologyBeijing 100083China Institute of Minerals Research University of Science and TechnologyBeijing 100083China state Key Laboratory of Mineral Processing Beijing 102628China Ansteel Group Mining Co.Ltd. Anshan 114000China Norman B.Keevil Institute of Mining Engineering University of British ColumbiaVancouverBC V6T 1Z4Canada

X-ray fluorescence(XRF)sensor-based ore sorting enables efficient beneficiation of heterogeneous ores,while intraparticle heterogeneity can cause significant grade detection errors,leading to misclassifications and hindering widespread technology *** classification models are crucial to determine if actual grade exceeds the sorting threshold using localized XRF *** studies mainly used linear regression(LR)algorithms including simple linear regression(sLR),multivariable linear regression(MLR),and multivariable linear regression with interaction(MLRI)but often fell short attaining satisfactory *** study employed the particle swarm optimization support vector machine(PsO-sVM)algorithm for sorting porphyritic copper ore ***-scale results showed PsO-sVM out-performed LR and raw data(RD)models and the significant interaction effects among input features was *** poor input data quality,PsO-sVM demonstrated exceptional ***-scale sorting achieved 93.0%accuracy,0.24%grade increase,84.94%recovery rate,57.02%discard rate,and a remarkable 39.62 yuan/t net smelter return(NsR)increase compared to no *** improvements were achieved by the PsO-sVM model with optimized input combinations and highest data quality(T=10,T is XRF testing times).The unsuitability of LR methods for XRF sensor-based sorting of investigated sample is *** element selection and mineral association analysis elucidate element importance and influence mechanisms.

关键词： XRF sensor-based sorting PsO-sVM algorithm Copper ore pebble Receiver operating curve(ROC) Net smelter return(NsR)

Coal/Gangue Volume Estimation with Convolutional Neural Network and separation Based on Predicted Volume and Weight

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Computers, Materials & Continua 2024年第4期79卷 279-306页

作者： Zenglun Guan Murad s.Alfarzaeai Eryi hu Taqiaden Alshmeri Wang Peng school of Mechatronic Engineering China University of Mining and TechnologyXuzhou221116China China National Coal Group Corp. Beijing100029China Information Institute Ministry of Emergency Management of the ChinaBeijing100029China school of Mechanical Engineering Sana’a UniversitySana’a31220Yemen

In the coal mining industry,the gangue separation phase imposes a key challenge due to the high visual similaritybetween coal and ***,separation methods have become more intelligent and efficient,using newtechnologies and applying different features for *** such method exploits the difference in substancedensity,leading to excellent coal/gangue ***,this study uses density differences to distinguishcoal from gangue by performing volume prediction on the *** training samples maintain a record of3-side images as input,volume,and weight as the ground truth for the *** prediction process relieson a Convolutional neural network(CGVP-CNN)model that receives an input of a 3-side image and then extractsthe needed features to estimate an approximation for the *** classification was comparatively performedvia ten different classifiers,namely,K-Nearest Neighbors(KNN),Linear support Vector Machines(Linear sVM),Radial Basis Function(RBF)sVM,Gaussian Process,Decision Tree,Random Forest,Multi-Layer Perceptron(MLP),Adaptive Boosting(AdaBosst),Naive Bayes,and Quadratic Discriminant Analysis(QDA).After severalexperiments on testing and training data,results yield a classification accuracy of 100%,92%,95%,96%,100%,100%,100%,96%,81%,and 92%,*** test reveals the best timing with KNN,which maintained anaccuracy level of 100%.Assessing themodel generalization capability to newdata is essential to ensure the efficiencyof the model,so by applying a cross-validation experiment,the model generalization was *** useddataset was isolated based on the volume values to ensure the model generalization not only on new images of thesame volume but with a volume outside the trained ***,the predicted volume values were passed to theclassifiers group,where classification reported accuracy was found to be(100%,100%,100%,98%,88%,87%,100%,87%,97%,100%),*** obtaining a classification with hi

关键词： Coal coal gangue convolutional neural network CNN object classification volume estimation separation system

Light People:*** D C Bradley(FRs)

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Light(science & Applications) 2024年第9期13卷 1704-1719页

作者： Ruidong Xia Ying hu Key Laboratory for Organic Electronics&Information Displays(KLOEID) Jiangsu-Singapore Joint Research Center for Organic/Bio Electronics&Information DisplaysInstitute of Advanced Materials(IAM)Nanjing University of Posts and Telecommunications9 Wenyuan RoadNanjing 210023China Executive Management College of CHN ENERGY North District of Future Science CityChangping DistrictNo.7 Binhe AvenueBeijing 102211China

Editorial,The invention of organic light emitting diodes(LEDs)led to enormous excitement in both academe and industry in the late 1980’***,large area solution processability,roll-to-roll printing,low cost,and environmentally friendly are some of the advantages of organic semiconductor materials,which brought a new horizon for *** with the achievement of organic solar cells,transistors,lasers,and amplifiers,this has demonstrated potential applications of organic semiconductors in displays,lighting,solar energy generation,electronics,sensing and imaging,and many aspects of *** an enlightened conversation with Light:science&Applications,*** Bradley(FRs),a pioneer in the field,shared his deep insights on past,current,and future exciting developments of organic optoelectronic materials and *** particular,he expressed his opinion on the hot topics related to organic optoelectronics research and application,such as the relationship between organic and inorganic semiconductors and the challenge of electrically pumped organic *** a successful scientist,Donal has also been co-founder of several organic optoelectronics innovation companies and research centers and a long-term academic administrator serving as a Head of Department,Centre Director,and Vice-Rector for Research at Imperial College,Head of the Mathematical,Physical,and Life sciences Division at the University of Oxford,Vice-President for Research at King Abdullah University of science and Technology and now Vice-President for Research and Innovation at NEOM U and Executive Director of the NEOM Education,Research and Innovation *** this interview,we also explore the major roles and events in Donal’s career experience from the invention of the first conjugated polymer LED in the world to the set-up of entrepreneurial companies,from Cambridge to sheffield,Imperial College,and Oxford,from the UK to overseas,and from the establishment of the Cent

关键词： companies Director Bradley

Distributed Fault-Tolerant Control of Uncertain Multi-Agent systems with Connectivity Maintenance

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Journal of systems science & Complexity 2024年第1期37卷 40-62页

作者： XING Xueyan hu Guoqiang Continental-NTU Corporate Lab Nanyang Technological UniversitySingapore 639798Singapore Continental-NTU Corporate Lab and the school of Electrical and Electronic Engineering Nanyang Technological UniversitySingapore 639798Singapore

In this paper,a distributed cooperative control protocol is presented to deal with actuator failures of multi-agent systems in the presence of connectivity *** the developed strategy,each agent can track the reference trajectory of the leader in the presence of actuator failures,disturbances and *** connectivity of the multi-agent system can always be ensured during the control *** achieve the aforementioned control objectives,a potential function is introduced to the distributed adaptive fault-tolerant control algorithm to preserve the initial connected network among the *** uncertainty of the multi-agent system,which is allowed to be described by discontinuous functions,is approximated and compensated using the fuzzy logic *** asymptotic stability of the closed-loop system is demonstrated through the use of Cellina’s approximate selection theorem of nonsmooth *** to the developed adaptive laws,the upper bound of the disturbance is allowed to be uncertain,which facilitates the implementation of the control ***,simulation results are provided to verify the effectiveness of the proposed control scheme.

关键词： Actuator failure connectivity maintenance coordination control uncertainties

Antibodies elicited by Newcastle disease virus-vectored H7N9 avian influenza vaccine are functional in activating the complement system

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Journal of Integrative Agriculture 2024年第6期23卷 2052-2064页

作者： Zenglei hu Ya huang Jiao hu Xiaoquan Wang shunlin hu Xiufan Liu Joint International Research Laboratory of Agriculture and Agri-Product safety of the Ministry of Education of China Yangzhou UniversityYangzhou 225009China Animal Infectious Disease Laboratory School of Veterinary MedicineYangzhou UniversityYangzhou 225009China Jiangsu Co-innovation Center for Prevention and Control of Important Animal Infectious Diseases and Zoonoses Yangzhou UniversityYangzhou 225009China

H7N9 subtype avian influenza virus poses a great challenge for poultry *** disease virus(NDV)-vectored H7N9 avian influenza vaccines(NDV_(vec)H7N9)are effective in disease control because they are protective and allow mass *** note,these vaccines elicit undetectable H7N9-specific hemagglutination-inhibition(HI)but high IgG antibodies in ***,the molecular basis and protective mechanism underlying this particular antibody immunity remain ***,immunization with an NDV_(vec)H7N9 induced low anti-H7N9 HI and virus neutralization titers but high levels of hemagglutinin(HA)-binding IgG antibodies in *** residues(s150,G151 and s152)in HA of H7N9 virus were identified as the dominant epitopes recognized by the NDV_(vec)H7N9 immune *** transferred NDV_(vec)H7N9 immune serum conferred complete protection against H7N9 virus infection in *** NDV_(vec)H7N9 immune serum can mediate a potent lysis of HA-expressing and H7N9 virus-infected cells and significantly suppress H7N9 virus *** activities of the serum were significantly impaired after heat-inactivation or treatment with complement inhibitor,suggesting the engagement of the complement ***,mutations in the 150-sGs-152 sites in HA resulted in significant reductions in cell lysis and virus neutralization mediated by the NDV_(vec)H7N9 immune serum,indicating the requirement of antibody-antigen binding for complement ***,antibodies induced by the NDV_(vec)H7N9 can activate antibody-dependent complement-mediated lysis of H7N9 virus-infected cells and complement-mediated neutralization of H7N9 *** findings unveiled a novel role of the complement in protection conferred by the NDV_(vec)H7N9,highlighting a potential benefit of engaging the complement system in H7N9 vaccine design.

关键词： H7N9 subtype avian influenza virus NDV vector vaccine antibody immunity complement protection

A functional gel polymer electrolyte based on PVDF-HFP/gelatin toward dendrite-free lithium metal batteries

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Nano Research 2024年第4期17卷 2790-2799页

作者： Xiaoyi hu Kangli Liu shijie Zhang Guosheng shao s.Ravi P.silva Peng Zhang state Center for International Cooperation on Designer Low-carbon and Environmental Materials(CDLCEM) School of Materials Science and EngineeringZhengzhou UniversityZhengzhou 450001China Zhengzhou Materials Genome Institute(ZMGI) ZhongyuanzhiguXingyang 450100China Nanoelectronics Center Advanced Technology InstituteUniversity of SurreyGuildfordGU27XHUK

The leakage of liquid electrolyte and the formation of lithium dendrites pose challenges to safety and stability of lithium metal batteries(LMBs).The appearance of gel polymer electrolyte(GPE)has obviously improved the safety of traditional ***,the limited inhibition of GPE on lithium dendrites is detrimental to the safety of ***,a kind of poly(vinylidene fluoride-co-hexafluoropropylene)(PVDF-HFP)/gelatin(GN)GPE with high ionic conductivity,high-temperature resistance,and flame-retardancy,was prepared by electrospinning and soaking *** the electrospinning network of PVDF-HFP,its affinity to liquid electrolytes,makes this GPE more beneficial to ions transport and the formation of ***,the GN with sol–gel properties,enhances the mechanical property(13.5 MPa)of HFP-GN ***,X-ray photoelectron spectroscopy(XPs)and density functional theory(DFT)suggest that the attraction of polar groups of GN to Li+can regulate the distribution of Li+and protect Li ***,the application of HFP-GN GPEs to LMBs with cathodes of LiFePO_(4) and LiCoO_(2) deliver excellent electrochemical performances:after 300 cycles,the LiFePO_(4)/HFP-GN GPE/Li battery keeps a low capacity decay rate of 0.09%at 5 C;after 400 cycles at 2 C,the LiCoO_(2)/HFP-GN GPE/Li cell retains a high capacity retention of 74%.This GPE is demonstrated for the application prospect of safe LMBs.

关键词： poly(vinylidene fluoride-co-hexafluoropropylene)(PVDF-HFP) gelatin polar groups lithium metal battery lithium dendrite

Quantitative estimation of global mean precipitation throughout the Phanerozoic era

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science China Earth sciences 2024年第5期67卷 1616-1624页

作者： Xiujuan BAO Yongyun hu Laboratory for Climate and Ocean-Atmospheric studies Department of Atmospheric and Oceanic SciencesSchool of PhysicsPeking UniversityBeijing 100871China

Quantitatively estimating the global mean precipitation(GMP)throughout Earth's history is crucial for enhancing our understanding of long-term climate evolution and the hydrological ***,currently there is no established methodology for estimating global mean ***,we present the first study that estimates GMP in the Phanerozoic *** relationship between GMP and global mean surface temperature(GMsT)is investigated by analyzing data from 23 models in the Coupled Model Intercomparison Project phase 6(CMIP6).The result reveals consistent and significant impact of temperature on precipitation,with a sensitivity range of 2–3%K^(-1).Additionally,we propose a method for accessing latitudinal variations in precipitation caused by land area distributions and paleo-Koppen climatic *** climatic belts are determined based on geological indicators such as coals,evaporites,and glacial *** GMP is thus quantitatively estimated by combining variations in GMsT,land area distributions,and paleo-koppen climatic belts,spanning from 540 Ma to the present *** quantitative GMP curve demonstrates fluctuations in GMP about 500 mm yr^(-1),with values ranging from 948 to1442 mm yr-1over the Phanerozoic *** curve aligns closely with findings derived from numerical *** presented paleoprecipitation variations facilitate a more comprehensive understanding of the interconnected geological and paleoclimatic developments.

关键词： Paleoprecipitation Paleoclimate K?ppen climatic belts Global mean precipitation Hydrological cycle

Design,preparation,and characterization of a novel ZnO/CuO/Al energetic diode with dual functionality:Logic and destruction

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Defence Technology（防务技术） 2024年第4期34卷 57-68页

作者： Jialu Yang Jiaheng hu Yinghua Ye Jianbing Xu Yan hu Ruiqi shen school of Chemistry and Chemical Engineering Nanjing University of Science and TechnologyNanjing 210094China Micro-Nano Energetic Devices Key Laboratory of MIIT Nanjing 210094China Institute of space Propulsion Nanjing University of Science and TechnologyNanjing 210094China

self-destructing chips have promising applications for securing *** paper proposes a new concept of energetic diodes for the first time,which can be used for self-destructive chips.A simple two-step electrochemical deposition method is used to prepare ZnO/CuO/Al energetic diode,in which N-type ZnO and P-type CuO are constricted to a PN *** paper comprehensively discusses the material properties,morphology,semiconductor characteristics,and exploding performances of the energetic *** results show that the energetic diode has typical rectification with a turn-on voltage of about 1.78 V and a reverse leakage current of about 3×10^(-4)*** a constant voltage of 70 V loads to the energetic diode in the forward direction for about 0.14 s or 55 V loads in the reverse direction for about 0.17 s,the loaded power can excite the energetic diode exploding and the current rises to about100 *** to the unique performance of the energetic diode,it has a double function of rectification and *** energetic diode can be used as a logic element in the normal chip to complete the regular operation,and it can release energy to destroy the chip accurately.

关键词： Energetic diode ZnO—CuO—Al thermite ZnO/CuO PN junction Electrical explosion performance self-destructing chips