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Embedding Perovskite in Polymer Matrix Achieved Positive Temperature Response with Inversed Temperature Crystallization

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Energy & Environmental Materials 2024年第5期7卷 361-371页

作者： Meiting Peng Xue Guan Yingzhu Wu Nan zhang Qi Feng Liyong Tian Yancheng Wu Yangfan zhang Feng Gan Fuqin Deng Meilin Huang Guichuan Xing Ningbo Yi College of Textile Science and Engineering Wuyi University Institute of Applied Physics and Materials Engineering University of Macau School of Applied Physics and Materials Wuyi University Faculty of Intelligent Manufacturing Wuyi University

Organic perovskites are promising semiconductor materials for advanced photoelectric applications. Their fluorescence typically shows a negative temperature coefficient due to bandgap change and structural instability. In this study, a novel perovskite-based composite with positive sensitivity to temperature was designed and obtained based on its inverse temperature crystallization, demonstrating good flexibility and solution processability. The supercritical drying method was used to address the limitations of annealing drying in preparing high-performance perovskite. Optimizing the precursor composition proved to be an effective approach for achieving high fluorescence and structural integrity in the perovskite material. This perovskite-based composite exhibited a positive temperature sensitivity of28.563%℃-1for intensity change and excellent temperature cycling reversibility in the range of 25–40℃in an ambient environment. This made it suitable for use as a smart window with rapid response. Furthermore, the perovskite composite was found to offer temperature-sensing photoluminescence and flexible processability due to its components of perovskite-based compounds and polyethylene oxide. The organic precursor solvent could be a promising candidate for use as ink to print or write on various substrates for optoelectronic devices responding to temperature.

关键词： flexibility inversed temperature crystallization perovskite positive temperature response

Unstable evolution of railway slope under the rainfall-vibration joint action

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Journal of Mountain Science 2024年第4期21卷 1419-1431页

作者： DONG Haoyu WANG Jiading zhang Dengfei LI Lin XU Yuanjun State Key Laboratory of Continental Dynamics Department of GeologyNorthwest UniversityXi’an 710069China

Understanding the unstable evolution of railway slopes is the premise for preventing slope failure and ensuring the safe operation of ***,as two major factors affecting the stability of railway slopes,few scholars have explored the unstable evolution of railway slopes under the joint action of *** on the model test of sandy soil slope,the unstable evolution process of slope under locomotive vibration,rainfall,and rainfall-vibration joint action conditions was simulated in this *** comparing and analyzing the variation trends of soil pressure and water content of slope under these conditions,the change laws of pore pressure under the influence of vibration and rainfall were *** main control factors affecting the stability of slope structure under the joint action conditions were further *** with the slope failure phenomena under these three conditions,the causes of slope instability resulting from each leading factor were ***,according to the above conclusions,the unstable evolution of the slope under the rainfall-vibration joint action was *** test results show that the unstable evolution process of sandy soil slope,under the rainfall-vibration joint action,can be divided into:rainfall erosion cracking,vibration promotion penetrating,and slope instability sliding three *** the process of slope unstable evolution,rainfall and vibration play the roles of inducing and promoting slide *** addition,the deep cracks,which are the premise for the formation of the sliding surface,and the violent irregular fluctuation of soil pressure,which reflects the near penetration of the sliding surface,constitute the instability characteristics of the railway slope *** paper reveals the unstable evolution of sandy soil slopes under the joint action of rainfall-vibration,hoping to provide the theoretical basis for the early warning and prevention technology of railway slopes.

关键词： Rainfall vibration joint action Small scale model tests Unstable evolution process Unstable characteristics Inducing sliding and promoting sliding

Removal of Microcystin-LR in lake water sample by hydrophilic mesoporous silica composites under high-throughput MALDI-TOF MS detection platform

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Chinese Chemical Letters 2024年第5期35卷 380-385页

作者： Wantong zhang Zixing Xu Guofei Dai Zhijian Li Chunhui Deng Department of Chemistry Institute of Metabolism&Integrate Biology(IMIB)Fudan UniversityShanghai 200433China Jiangxi Key Laboratory of Organic Chemistry Jiangxi Science and Technology Normal UniversityNanchang 330013China Jiangxi Academy of Water Science and Engineering Nanchang 330029China

Microcystins(MCs),a family of cyclic heptapeptide cyanotoxins,exists in aquatic environment where cyanobacterial bloom happens,which will accumulate in aquatic organisms and transfer through the food chain to higher trophic levels,posing a health risk to both animals and human *** various MCs,Microcystin-LR(MC-LR)is worthiest studied for its strong toxicity,ubiquity and *** in this work,iminodiacetic acid(IDA)decorated magnetic mesoporous silica(mSiO_(2))nanocomposites(Fe_(3)O_(4)@mSiO_(2)-IDA)were facilely synthesized which possessed the merits of large surface area(188.21 m^(2)/g),accessible porosity(2.66 nm),excellent hydrophilicity and rapid responsiveness to magnetic *** the composites were successfully employed to the removal process of Microcystin-LR in real water samples followed by Matrix-assisted laser desorption/ionization time-of-flight mass spectrometry(MALDI-TOF MS)analysis,achieving the removal efficiency above 92.5%even after ten recycles of the *** provided a potential method for removing MC-LR in aqueous environment with high effectiveness,lower costs and less secondary contamination.

关键词： Microcystin-LR Mesoporous silica Magnetic composites MALDI-TOF MS analysis

Brain-inspired multimodal approach for effluent quality prediction using wastewater surface images and water quality data

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Frontiers of Environmental Science & Engineering 2024年第3期18卷 69-82页

作者： Junchen Li Sijie Lin Liang zhang Yuheng Liu Yongzhen Peng Qing Hu School of Environment Harbin Institute of TechnologyHarbin 150090China School of Environmental Science and Engineering Southern University of Science and TechnologyShenzhen 518055China Engineering Innovation Center of SUSTech(Beijing) Southern University of Science and TechnologyBeijing 100083China Faculty of Environment and Life Beijing University of TechnologyBeijing 100124China Engineering Research Center of Intelligence Perception and Autonomous Control Ministry of EducationBeijing 100124China

Efficiently predicting effluent quality through data-driven analysis presents a significant advancement for consistent wastewater treatment *** this study,we aimed to develop an integrated method for predicting effluent COD and NH3 *** employed a 200 L pilot-scale sequencing batch reactor(SBR)to gather multimodal data from urban sewage over 40 *** we collected data on critical parameters like COD,DO,pH,NH_(3),EC,ORP,SS,and water temperature,alongside wastewater surface images,resulting in a data set of approximately 40246 *** we proposed a brain-inspired image and temporal fusion model integrated with a CNN-LSTM network(BITF-CL)using this *** innovative model synergized sewage imagery with water quality data,enhancing prediction *** a result,the BITF-CL model reduced prediction error by over 23%compared to traditional methods and still performed comparably to conventional techniques even without using DO and SS sensor ***,this research presents a cost-effective and precise prediction system for sewage treatment,demonstrating the potential of brain-inspired models.

关键词： Wastewater treatment system Water quality prediction Data driven analysis Brain-inspired model Multimodal data Attention mechanism

The raphe nuclei are the early lesion site of gastric α-synuclein propagation to the substantia nigra

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Acta Pharmaceutica Sinica B 2024年第5期14卷 2057-2076页

作者： Chenglu zhang Ruxue Bo Tiantian Zhou Naihong Chen Yuhe Yuan State Key Laboratory of Bioactive Substances and Functions of Natural Medicines Chinese Academy of Medical Sciences&Peking Union Medical College Institute of Materia MedicaBeijing 100050China

Parkinson's disease(PD)is a neurodegeneration disease withα-synuclein accumulated in the substantia nigra pars compacta(SNpc)and most of the dopaminergic neurons are lost in SNpc while patients are diagnosed with *** the pathology at an early stage contributes to the development of the disease-modifying *** the“gut–brain”hypothesis is proposed to explain the underlying mechanism,where the earlier lesioned site in the brain of gastricα-synuclein and howα-synuclein further spreads are not fully *** we report that caudal raphe nuclei(CRN)are the early lesion site of gastricα-synuclein propagating through the spinal cord,while locus coeruleus(LC)and substantia nigra pars compacta(SNpc)were further affected over a time frame of 7 ***α-synuclein propagation via CRN leads to neuron loss and disordered neuron activity,accompanied by abnormal motor and non-motor *** neuron circuits are observed among CRN,LC,and SNpc,which contribute to the venerability of dopaminergic neurons in *** results show that CRN is the key region for the gastricα-synuclein spread to the *** study provides valuable details for the“gut–brain”hypothesis and proposes a valuable PD model for future research on early PD intervention.

关键词： Raphe nuclei α-Synuclein Gastrointestinal tract Electrophysiology Locus coeruleus Substantia nigra pars compacta Parkinson's disease Spinal cord

Transition-metal-catalyzed remote meta-C-H alkylation and alkynylation of aryl sulfonic acids enabled by an indolyl template

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Chinese Chemical Letters 2024年第8期35卷 254-259页

作者： Pengfei zhang Qingxue Ma Zhiwei Jiang Xiaohua Xu Zhong Jin College of Chemistry State Key Laboratory of Elemento-organic ChemistryNankai UniversityTianjin 300071China Key Laboratory of Xinjiang Native Medicinal and Edible Plant Resource Chemistry College of Chemistry and Environmental SciencesKashi UniversityKashgar 844007China

Transition-metal-catalyzed remote sp^(2)C-H functionalization of aryl sulfonic acids was hardly ever real-ized owing to competitive ortho-C-H functionalization of aryl sulfonates and electron-deficient nature of phenyl ***,with the assistance of a practical biaryl indolyl directing template,palladium-catalyzed remote sp^(2)C-H alkylation of aryl sulfonic acids have been achieved in moderate to good yields with exclusive meta ***,remote meta-selective C-H alkynylation of aryl sulfonic acids was also accomplished with a rhodium *** meta-C-H functionalized products proved to be the superior synthetic precursors,which are difficult to access using the conventional strategy.

关键词： C-H functionalization Aryl sulfonic acid Site-selectivity Transition-metal catalysis Alkylation Alkynylation

Wireless semantic communication based on semantic matching multiple access and intent bias multiplexing

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The Journal of China Universities of Posts and Telecommunications 2024年第1期31卷 26-36页

作者： Ren Chao He Zongrui Sun Chen Li Haojin zhang Haijun University of Science and Technology Beijing Beijing 100083China Research and Development Center Sony(China)LimitedBeijing 100027China

This paper proposes a multi-access and multi-user semantic communication scheme based on semantic matching and intent deviation to address the increasing demand for wireless users and *** scheme enables flexible management of long frames,allowing each unit of bandwidth to support a higher number of *** leveraging semantic classification,different users can independently access the network through the transmission of long concatenated sequences without modifying the existing wireless communication *** overcome the potential disadvantage of incomplete semantic database matching leading to semantic intent misunderstanding,the scheme proposes using intent deviation as an *** allows different receivers to interpret the same semantic information differently,enabling multiplexing where one piece of information can serve multiple users with distinct *** results show that at a bit error rate(BER)of 0.1,it is possible to reduce the transmission by approximately 20 semantic basic units.

关键词： semantic communication multiple access multiplexing multimodal communication

Damage on intestinal barrier function and microbial detoxification of deoxynivalenol:A review

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Journal of Integrative Agriculture 2024年第8期23卷 2507-2524页

作者： Jia Chen Xinran zhang Ziqi He Dongwei Xiong Miao Long Key Laboratory of Livestock Infectious Diseases Ministry of Education/College of Animal Science and Veterinary Medicine ShenyangAgricultural UniversityShenyang 110866China

Deoxynivalenol(DON)is a mycotoxin that is produced by various species of Fusarium and is ubiquitous in food and *** low concentrations,it can cause metabolic disorders in animals and humans and,at high concentrations,it can lead to pathological changes in the *** impact of DON on human/animal health and animal productivity has thus attracted a great deal of attention around the *** causes severe damage to the intestine,including compromised intestinal barrier,mucosal damage,weakened immune function,and alterations in gut microbiota *** effects exacerbate intestinal infections and inflammation in livestock and poultry,posing adverse effects on overall ***,research into biological methods for DON detoxification is a crucial avenue for future *** includes the utilization of adsorption,enzymatic degradation,and other biological approaches to mitigate DON's impact,offering new strategies for prevention and treatment of DON-induced *** research will focus on identifying highly efficient detoxifying microorganisms or enzymes to reduce DON levels in food and feed,thereby mitigating its risks to both animals and human health.

关键词： deoxynivalenol(DON) intestinal barrier function mucus barrier immune function flora composition biological detoxification

Runoff and Infiltration responses of revegetated slopes to clipping management on the northern Loess Plateau

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International Soil and Water Conservation Research 2024年第1期12卷 171-183页

作者： Qilin He Binbin Li Fengbao zhang Nan Shen Mingyi Yang The Research Center of Soil and Water Conservation and Ecological Environment Chinese Academy of Sciences and Ministry of EducationYanglingShaanxi712100China Institute of Soil and Water Conservation Chinese Academy of Sciences and Ministry of Water ResourcesYanglingShaanxi712100China Institute of Soil and Water Conservation Northwest A&F UniversityYanglingShaanxi712100China Water and Soil Conservation Monitoring Center of Ministry of Water Resources Beijing100053China University of Chinese Academy of Sciences Beijing100049China

Large-scale vegetation restoration can reduce local watershed water yield,limit vegetation establishment and subsequent growth,and influence regional ecosystem *** management by reducing aboveground parts of grassland was gradually recommended and adopted in Grain-for-Green project management to offset these additional ***,scientific evaluation of the effectiveness of clipping management on infiltration and runoff processes is necessary for maintaining the stability of the surface water system and the sustainability of vegetation restoration in semi-arid regions.A field simulated rainfall experiment was conducted with four managed clipping grasslands(mainly bunge needlegrass and Stipa grandis),including no clipping,light clipping,heavy clipping,and complete clipping under three slope gradients(10,20,and 30°)and three rainfall intensities(60,90,and 120 mm/h)to explore the mechanism of runoff and infiltration responses to clipping using structural equation modeling and variation partitioning based on an SCS-CN *** results showed the runoff coefficient of the light clipping,heavy clipping,and complete clipping plots were 1.33,2.22,and 4.22 times that of the no clipping *** light clipping,heavy clipping,and complete clipping plots decreased the infiltration coefficients by 0%,5%,and 26%relative to the no clipping *** intensity dominated runoff and infiltration amounts,and clipping intensity's total effect was stronger than slope *** intensity and slope gradient were more influential on runoff with increasing rainfall *** mutual inhibition effect was between clipping intensity and slope gradient on *** order to maintain the sustainability of restoration,a 25-50%vegetation coverage after clipping maximizes the benefits of increasing runoff and maintaining enough soil water supply that prevents possible soil *** propose that future vegetation restoration policies should evaluate the appropriat

关键词： Runoff Infiltration Grassland clipping management SCS-CN model Structural equation model Variation partitioning