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Ion emission from warm dense matter produced by irradiation with a soft x-ray free-electron laser

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Matter and Radiation at Extremes 2024年第1期9卷 71-84页

作者： Josef Krása Tomás Burian Vera Hájková Jaromír Chalupský Šimon Jelínek Katerina Frantálová michal Krupka Zuzana Kuglerová Sushil Kumar Singh Vojtech Vozda Ludek Vysín michalŠmíd Pablo Perez-Martin Marion Kühlman Juan Pintor Jakub Cikhardt Matthias Dreimann Dennis Eckermann Felix rosenthal Sam M.Vinko Alessandro Forte Thomas Gawne Thomas Campbell Shenyuan Ren YuanFeng Shi Trevor Hutchinson Oliver Humphries Thomas Preston Mikako Makita Motoaki Nakatsutsumi Xiayun Pan Alexander Köhler Marion Harmand Sven Toleikis Katerina Falk Libor Juha Department of Radiation and Chemical Physics Institute of PhysicsCzech Academy of SciencesNa Slovance 218221 Prague 8Czech Republic Laser Plasma Department Institute of Plasma PhysicsCzech Academy of SciencesZa Slovankou 318200 Prague 8Czech Republic Department of Surface and Plasma Science Faculty of Mathematics and PhysicsCharles University in PragueV Holesovi ckách 218000 Prague 8Czech Republic Department of Physical Electronics Faculty of Nuclear Science and Engineering PhysicsCzech Technical University in PragueV Holesovi ckách 218000 Prague 8Czech Republic Helmholtz-Zentrum Dresden-Rossendorf Bautzner Landstraße 40001328 DresdenGermany DESY Photon Science Notkestraße 85D-22607 HamburgGermany Institut de Minéralogie de Physique des Matériaux et de CosmochimieUMR 7590–UPMC/CNRS/IRD/MNHNSorbonne Université4 place Jussieu75005 ParisFrance Department of Physics Faculty of Electrical EngineeringCzech Technical University in PragueTechnická216627 Prague 6Czech Republic Center for Soft Nanoscience University of MünsterBusso-Peus-Straße 10D-48149 MünsterGermany Department of Physics Clarendon LaboratoryUniversity of OxfordParks RoadOxford OX13PUUnited Kingdom Central Laser Facility STFC Rutherford Appleton LaboratoryDidcot OX110QXUnited Kingdom Lawrence Livermore National Laboratory 7000 East AvenueLivermoreCalifornia 94550USA European XFEL GmbH Holzkoppel 4D-22869 SchenefeldGermany Technische Universität Dresden 01062 DresdenGermany

We report on an experiment performed at the FLASH2 free-electron laser(FEL)aimed at producing warm dense matter via soft x-ray isochoric heating.In the experiment,we focus on study of the ions emitted during the soft x-ray ablation process using time-of-flight electron multipliers and a shifted Maxwell–Boltzmann velocity distribution model.We find that most emitted ions are thermal,but that some impurities chemisorbed on the target surface,such as protons,are accelerated by the electrostatic field created in the plasma by escaped electrons.The morphology of the complex crater structure indicates the presence of several ion groups with varying temperatures.We find that the ion sound velocity is controlled by the ion temperature and show how the ion yield depends on the FEL radiation attenuation length in different materials.

关键词： electrostatic emitted chemi

Rice-wheat comparative genomics:Gains and gaps

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The Crop Journal 2024年第3期12卷 656-669页

作者： Akila Wijerathna-Yapa Ruchi Bishnoi Buddhini Ranawaka Manu Maya Magar Hafeez Ur Rehman Swati G.Bharad michal T.Lorenc Vinita Ramtekey Sasha Gohar Charu Lata Md.Harun-Or-Rashid Maryam Razzaq Muhammad Sajjad Bhoja *** School of Agriculture and Food Sustainability The University of QueenslandSt LuciaQLD 4072Australia ARC Centre of Excellence for Plant Success in Nature and Agriculture The University of QueenslandSt LuciaQLD 4072Australia Department of Genetics and Plant Breeding College of AgricultureUmmedganj-KotaAgriculture UniversityKotaRajasthan 324001India Centre for Agriculture and the Bioeconomy Queensland University of Technology(QUT)2 George StreetBrisbaneQLD 4000Australia UWA School of Agriculture and Environment The University of Western Australia35 Stirling HighwayCrawleyWA 6009Australia Nepal Agriculture Research Council KhumaltarLalitpurNepal Department of Agronomy University of AgricultureFaisalabad 38040Pakistan Department of Agricultural Botany Dr Panjabrao Deshmukh Krishi VidyapeethAkola 444104MaharashtraIndia ICAR-Indian Institute of Seed Science MauUttar Pradesh 275103India School of Natural Sciences Macquarie UniversityMacquarie ParkNSW 2109Australia ICAR-Indian Institute of Wheat and Barley Research Flowrdale 54642ShimlaIndia International Maize and Wheat Improvement Center(CIMMYT)Bangladesh Office Gulshan-2Dhaka 1212Bangladesh Center for Seed Science University of AgricultureFaisalabad 38000Pakistan Department of Biosciences COMSATS University IslamabadPark RoadTarlai KalanIslamabad 45550Pakistan CGIAR’s Excellence in Breeding(EiB)Platform/Accelerated Breeding Initiative International Maize and Wheat Improvement Center(CIMMYT)El Batán 56237Mexico

Rice and wheat provide nearly 40%of human calorie and protein requirements.They share a common ancestor and belong to the Poaceae(grass)family.Characterizing their genetic homology is crucial for developing new cultivars with enhanced traits.Several wheat genes and gene families have been characterized based on their rice orthologs.Rice–wheat orthology can identify genetic regions that regulate similar traits in both crops.Rice–wheat comparative genomics can identify candidate wheat genes in a genomic region identified by association or QTL mapping,deduce their putative functions and biochemical pathways,and develop molecular markers for marker-assisted breeding.A knowledge of gene homology facilitates the transfer between crops of genes or genomic regions associated with desirable traits by genetic engineering,gene editing,or wide crossing.

关键词： Comparative genomics Orthologs Genes Synteny Genetic engineering Molecular breeding

Impact of Si on the high-temperature oxidation of AlCr(Si)N coatings

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Journal of Materials Science & Technology 2022年第5期100卷 91-100页

作者： Nikolaus Jager Michael Meindlhumer michal Zitek Stefan Spor Hynek Hruby Farwah Nahif Jaakko Julin Martin rosenthal Jozef Keckes Christian Mitterer Rostislav Daniel Christian Doppler Laboratory for Advanced Synthesis of Novel Multifunctional Coatings at the Department of Materials Science Montanuniversität LeobenAustria voestalpine eifeler Vacotec GmbH DüsseldorfGermany Institute of Ion Beam Physics and Materials Research Helmholtz-Zentrum Dresden-RossendorfDresdenGermany Department of Physics University of JyvaskylaFinland European Synchrotron Radiation Facility GrenobleFrance Erich Schmid Institute for Materials Science Austrian Academy of SciencesAustria Department of Materials Science Montanuniversität LeobenAustria

The resistance of wear protective coatings against oxidation is crucial for their use at high temperatures.Here,three nanocomposite AlCr(Si)N coatings with a fixed Al/Cr atomic ratio of 70/30 and a varying Si-content of 0 at.%,2.5 at.% and 5 at.% were analyzed by differential scanning calorimetry,thermogravimetric analysis and X-ray in order to understand the oxidation behavior depending on their Si-content.Additionally,a partially oxidized AlCrSiN coating with 5 at.%Si on a sapphire substrate was studied across the coating thickness by depth-resolved cross-sectional X-ray nanodiffraction and scanning trans-mission electron microscopy to investigate the elemental composition,morphology,phases and residual stress evolution of the oxide scale and the non-oxidized coating underneath.The results reveal enhanced oxidation properties of the AlCr(Si)N coatings with increasing Si-content,as demonstrated by a retarded onset of oxidation to higher temperatures from 1100℃ for AlCrN to 1260℃ for the Si-containing coatings and a simultaneous deceleration of the oxidation process.After annealing of the AlCrSiN sample with5 at.%Si at an extraordinary high temperature of 1400℃ for 60 min in ambient air,three zones developed throughout the coating strongly differing in their composition and structure:(i)a dense oxide layer comprising an Al-rich and a Cr-rich zone formed at the very top,followed by(ii)a fine-grained transition zone with incomplete oxidation and(iii)a non-oxidized zone with a porous structure.The varying elemental composition of these zones is furthermore accompanied by micro-structural variations and a complex residual stress development revealed by cross-sectional X-ray nanodiffraction.The results provide a deeper understanding of the oxidation behavior of AlCr(Si)N coatings depending on their Si-content and the associated elemental,microstructural and residual stress evolution during high-temperature oxidation.

关键词： AlCrSiN Nanocomposite Cathodic arc Oxidation behaviour Cross-sectional X-ray nanodiffraction

Proteomic-based evidence for adult neurogenesis in birds and mammals as indicated from cerebrospinal fluid

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Neural Regeneration Research 2022年第12期17卷 2576-2581页

作者： Eleni Voukali michal Vinkler Department of Zoology Faculty of ScienceCharles UniversityPragueCzech Republic

Adult neurogenesis is the life-long process of neural stem cell proliferation,differentiation into neurons,migration,and incorporation into the existing neuronal circuits.After decades of research,it is now widely accepted that mammals and birds retain the capacity to regenerate neurons even after their subadult ontogeny.Cerebrospinal fluid participates in the regulation of the neurogenic niches of the vertebrate brain through signaling pathways not fully elucidated.Proteomic studies of cerebrospinal fluid have the potential to allow the in-depth characterization of its molecular composition.Comparative studies help to delineate those pathways that are universally critical for the regulation of neurogenesis in adulthood.In this review,we performed literature-based data mining in studies using liquid chromatography-tandem mass spectroscopy that analyzed cerebrospinal fluid samples from healthy adult humans(Homo sapiens);mice(Mus musculus);sheep(Ovis aries);chickens(Gallus gallus);and two parrot species,the budgerigar(Melopsittacus undulatus)and cockatiel(Nymphicus hollandicus).We identified up to 911 proteins represented in cerebrospinal fluid,involved in various pathways regulating adult neurogenesis.However,only 196 proteins were common across humans,mice,and birds.Pathway components involved in nervous system development,cell migration,and axonal guidance were commonly evident in all species investigated so far.Extensive bioinformatic analysis revealed that the universally over-represented pathways involved L1 cell adhesion molecule protein interactions,cell-adhesion molecules,signals regulating extracellular matrix remodeling,regulation of insulin growth factor signaling,axonal guidance,programmed cell death,immune signaling,and post-translational modifications.Most of the reported proteins are part of extracellular vesicles enriched in cerebrospinal fluid.However,the information presently available is still highly fragmentary,and far more questions persist than are answered.Technological advances will allow c

关键词： adult neurogenesis birds cerebrospinal fluid chicken comparative proteomics human mammals mass spectrometry parrots

Decarbonylative Sonogashira cross-coupling:a fruitful marriage of alkynes with carboxylic acid electrophiles

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Organic Chemistry Frontiers 2022年第1期9卷 216-222页

作者： Chengwei Liu michal Szostak School of Chemical Engineering and Technology Yantai Nanshan UniversityLongkouYantaiShandong 265713China School of Chemistry and Materials Science Nanjing University of Information Science and Technology219 Ningliu RoadNanjingJiangsu 210044China Department of Chemistry Rutgers University73 Warren StreetNewarkNJ 07102USA

The Sonogashira cross-coupling is one of the most fundamental C–C bond-forming reactions,wherein the strategic value of an alkyne moiety has found widespread applications at the frontiers of organic chemistry,materials science and drug discovery as the cornerstone building block of chemical synthesis.Although traditional variants of Sonogashira cross-coupling involve aryl halides and pseudohalides as electrophiles,recently,tremendous advances have been made in the unconventional disconnection exploiting common carboxylic acids by a decarbonylation/transmetalation pathway.This manifold(1)permits one to take advantage of carboxylic acids as a ubiquitous class of substrates in organic synthesis that are derived from an orthogonal pool of precursors to aryl halides and pseudohalides and(2)combines the benefits of the palladium-catalyzed C(sp^(2))–C(sp)coupling of terminal alkynes with the inherent presence of the carboxylic acid moiety in pharmaceuticals,natural products and organic materials.In this highlight article,we summarize the recent progress in the decarbonylative Sonogashira cross-coupling of carboxylic acid electrophiles to produce arylalkynes and conjugated enynes as a novel avenue for chemical synthesis,whereby a large number of chemical reactions critically rely on transformations of alkynes.

关键词： coupling carbonyl moiety

Literary placemaking and narrative immersion in extended reality virtual geographic environments

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International Journal of Digital Earth 2022年第1期15卷 853-867页

作者： michal Rzeszewski Jeneen Naji Faculty of Human Geography and Planning Adam Mickiewicz University in PoznanPoznanPoland Department of Media Studies Maynooth UniversityMaynoothIreland

Virtual geographical environments(VGEs)are being used to represent our sense of place through the application of extended-reality or cross-reality(XR)technologies with a focus on technological advancement and immersion.In light of this,we propose that an expanded and interdisciplinary understanding of the concept of immersion is required to facilitate an understanding of spatial data to a broader audience.The potential of focusing on narrative immersion and literary placemaking in VGEs is discussed to evoke a stronger sense of place and a feeling of presence and belonging in users.This paper seeks to highlight the unique affordances and potentialities of XR narrative style GIS digital representations through an interdisciplinary theoretically lead analysis of outputs created by the Building City dashboards project towards the goal of expanding audiences of non-specialist stakeholders in urban planning processes.

关键词： Literary placemaking immersion extended-reality(XR) virtual geographic environments(VGE) urban planning

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基于聚合物分散液晶的频率可重构贴片天线

液晶与显示 2024年第1期39卷 17-24页

作者：储怡冰项颖张文慧郝禄国江博韬陈凯高延子胡湧川 michal KOHOUT 广东工业大学信息工程学院广东广州510006 北京科技大学新材料技术研究院北京100083 Department of Organic Chemistry University of Chemistry and Technology PragueCZ-16628 PragueCzech Republic

本文设计了一种以液晶聚合物为介质基板的频率可重构天线,通过调节贴片的位置及尺寸实现天线的阻抗匹配。制备聚合物分散液晶薄膜作为天线的介质,并根据液晶与聚合物的比例分别为7∶3、6∶4、5∶5这3种不同配比以及50μm和100μm两种不... 详细信息

本文设计了一种以液晶聚合物为介质基板的频率可重构天线,通过调节贴片的位置及尺寸实现天线的阻抗匹配。制备聚合物分散液晶薄膜作为天线的介质,并根据液晶与聚合物的比例分别为7∶3、6∶4、5∶5这3种不同配比以及50μm和100μm两种不同膜的厚度来考察其效果。在电场作用下,液晶微滴会沿着电场方向重新取向排列,通过改变驱动电压的大小,实现天线的频率可重构。经过对比分析得出,液晶含量(质量分数)为70%的聚合物分散液晶薄膜具有最佳的效果,在48 V的驱动电压下实现了62 MHz的频率连续调节,天线的最大增益为3.5 dBi。该基于液晶聚合物的频率可重构贴片天线结构简单、体积小、质量轻,易于集成在各种移动设备中,发展前景广阔。

关键词：液晶聚合物频率可重构贴片天线

Decoding of Factorial Experimental Design Models Implemented in Production Process

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Computers, Materials & Continua 2022年第4期71卷 1661-1675页

作者： Borislav Savkovic Pavel Kovac Branislav Dudic michal Gregus University of Novi Sad Faculty of Technical SciencesNovi Sad 21000Serbia Comenius University in Bratislava Faculty of ManagementBratislava820054 Slovakia University Business Academy Faculty of Economics and Engineering ManagementNovi Sad 21000Serbia

The paper deals with factorial experimental design models decoding.For the ease of calculation of the experimental mathematical models,it is convenient first to code the independent variables.When selecting independent variables,it is necessary to take into account the range covered by each.A wide range of choices of different variables is presented in this paper.After calculating the regression model,its variables must be returned to their original values for the model to be easy recognized and represented.In the paper,the procedures of simple first order models,with interactions and with second order models,are presented,which could be a very complicated process.Models without and with the mutual influence of independent variables differ.The encoding and decoding procedure on a model with two independent first-order parameters is presented in details.Also,the procedure of model decoding is presented in the experimental surface roughness parameters models’determination,in the face milling machining process,using the first and second order model central compositional experimental design.The simple calculation procedure is recommended in the case study.Also,a large number of examples using mathematical models obtained on the basis of the presented methodology are presented throughout the paper.

关键词： Mathematical modeling design of experiments functions coding decoding variable regression coefficienta

Data-Driven Self-Learning Controller for Power-Aware Mobile Monitoring IoT Devices

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Computers, Materials & Continua 2022年第2期70卷 2601-2618页

作者： michal Prauzek Tereza Paterova Jaromir Konecny Radek Martinek VSB–Technical University of Ostrava Department of Cybernetics and Biomedical EngineeringOstrava70800Czech Republic

Nowadays,there is a significant need for maintenance free modern Internet of things(IoT)devices which can monitor an environment.IoT devices such as these are mobile embedded devices which provide data to the internet via Low Power Wide Area Network(LPWAN).LPWAN is a promising communications technology which allows machine to machine(M2M)communication and is suitable for smallmobile embedded devices.The paper presents a novel data-driven self-learning(DDSL)controller algorithm which is dedicated to controlling small mobile maintenance-free embedded IoT devices.The DDSL algorithm is based on a modified Q-learning algorithm which allows energy efficient data-driven behavior of mobile embedded IoT devices.The aim of the DDSL algorithm is to dynamically set operation duty cycles according to the estimation of future collected data values,leading to effective operation of power-aware systems.The presented novel solution was tested on a historical data set and compared with a fixed duty cycle reference algorithm.The root mean square error(RMSE)and measurements parameters considered for the DDSL algorithm were compared to a reference algorithm and two independent criteria(the performance score parameter and normalized geometric distance)were used for overall evaluation and comparison.The experiments showed that the novel DDSL method reaches significantly lowerRMSE while the number of transmitted data count is less than or equal to the fixed duty cycle algorithm.The overall criteria performance score is 40%higher than the reference algorithm base on static confirmation settings.

关键词： 5G and beyond wireless IoT LPWAN M2M Q-learning