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High-temperature wetting behavior between slag and refractory

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Journal of Iron and Steel research International 2024年第6期31卷 1304-1319页

作者： Yong-xin Wang ya-ge Li ya-bo Gao Zhong Huang Hai-jun Zhang The State Key Laboratory of refractories and Metallurgy Wuhan University of Science and TechnologyWuhan 430081HubeiChina

Slag corrosion is one of the main factors of the damage of refractory,and its primary manifestations involve the melting of refractory in slag and the slag penetration into refractory,both of which are highly related to the wetting behavior between slag and *** high-temperature wettability could be characterized by parameters including the surface tension,adhesion work,and spreading coefficient of the slag on refractory surface,and it could be suppressed by altering the slag/refractory interface,thus resulting in an improved anti-corrosion *** this,the key knowledges of the slag corrosion,theory of wetting behavior and test of high-temperature contact angle were firstly ***,the major factors influencing the high-temperature slag wetting behavior were discussed based on the aspects of slag composition,refractory composition,and surface ***,the future research direction was proposed in this field.

关键词： High-temperature wetting refractory Slag corrosion Surface tension

Cyclic Gradient Methods for Unconstrained Optimization

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Journal of the Operations research Society of China 2024年第3期12卷 809-828页

作者： ya Zhang Cong Sun School of Science Beijing University of Posts and TelecommunicationsBeijing100876China

Gradient method is popular for solving large-scale *** this work,the cyclic gradient methods for quadratic function minimization are extended to general smooth unconstrained optimization *** with nonmonotonic line search,we prove its global ***,the proposed algorithms have sublinear convergence rate for general convex functions,and r-linear convergence rate for strongly convex *** experiments show that the proposed methods are effective compared to the state of the arts.

关键词： Gradient method Unconstrained optimization Nonmonotonic line search Global convergence

Fabricating functionally graded Fe-Cr-Co permanent magnetic alloys via laser powder bed fusion

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Journal of Iron and Steel research International 2024年第3期31卷 729-737页

作者： ya-zhou He ya-qing Hou Peng Shen Hao Zhang Dong Zhou Hang Su Central Iron and Steel research Institute Co. Ltd.Beijing 100081China Material Digital r&D Center China Iron and Steel Research Institute Group Co.Ltd.Beijing 100081China

Laser powder bed fusion(LPBF)in-situ alloying technology offers the possibility to construct gradient materials with varied structures and *** graded Fe-Cr-Co permanent magnetic alloys were fabricated by LPBF and in-situ alloying mixed powders of Fe,Cr,and Co *** effects of different Fe,Cr and Co contents on the microstructure,magnetic properties and hardness of Fe-Cr-Co alloys prepared by LPBF were *** as-built Fe-Cr-Co alloys present a single body-centered-cubic phase and have a homogeneous distribution of *** mechanical properties and magnetic properties of the compositionally graded sample show a gradient *** the increase in Cr content,the Vickers hardness of the sample increases,and the saturation magnetization of the sample *** optimal magnetic properties in an isotropic state are given as coercivity HcB=21.65 kA/m,remanence Br=0.70 T and energy product(BH)_(max)=5.35 kJ/m^(3),which are comparable to or higher than the reported magnetic properties in an isotropic state prepared by traditional powder *** in-situ alloying technology has the potential to further explore Fe-Cr-Co magnetic materials,such as those consisting of multiple or more constituent elements,and to maximize the compositional flexibility of magnetic materials.

关键词： Fe-Cr-Co alloy Laser powder bed fusion In-situ alloying Functional material Magnetic property

Anti-corrosive and highly reversible zinc metal anode enabled by the phenolic resin coating

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rare Metals 2024年第5期43卷 2115-2124页

作者： ya-Ping Wang ya-Di yang Shu-Qi Duan Li Wang Jia-Shuo Guo An-Qiang Pan School of Materials Science and Engineering Hebei University of TechnologyTianjin 300130China Key Laboratory of Special Functional Materials for Ecological Environment and Information(Hebei University of Technology).Ministry of Education Tianjin 300130China Key Laboratory for New Type of Functional Materials in Hebei Province Hebei University of TechnologyTianjin 300130China School of Materials Science and Engineering Central South UniversityChangsha 410083China

Aqueous zinc-ion batteries have attracted much attention due to their high theoretical capacity,low cost high safety,and ***,challenges such as dendrite growth and side reactions severely hinder the electrochemical performance of the Zn anode,leading to low Coulombic efficiency(CE)or even short circuits Herein,phenolic resin(PF)is used as a protective coating on the surface of the zinc metal *** PF layer can greatly improve the corrosion resistance of the Zn electrode in the ***,this artificial electrode/electrolyte interphase also elevates the nucleation barrier and restrains Zn^(2+)2D diffusion,regulating the zinc deposition/dissolution *** a result,PF@Zn symmetric cells exhibit superior performance than that of bare Zn symmetric cells,achieving a stable and dendrite-free cycle of 1400 ***,the carbon nanotube MnO_(2)||PF@Zn(CNT/MnO_(2)||PF@Zn)full cell also delivers a long cycle life with a high-capacity retention of about 180.0 m Ah·g^(-1)after 1400 cycles,far exceeding that of bare Zn *** work provides a facile strategy for achieving a dendrite-free and rechargeable zinc anode.

关键词： rechargeable aqueous batteries Zn metal anode Phenolic resin Anti-corrosion

One more step to realistic CO_(2) reduction reactions——geometric structures evolutions at gas-solid interface

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rare Metals 2024年第2期43卷 849-852页

作者： ya-Qiang Xie Xin Yu Ting Wang College of the Environment and Ecology Xiamen UniversityXiamen361102China

A rational design of copper(Cu)nanocatalyst is critical to the efficient carbon dioxide(CO_(2))conversion toward C1/C2 chemical ***,the lack of actual information on the vicinal Cu interfaces hinders the intrinsic activitystructure correlation *** with atomic-scale in situ characterizations(AP-STM and synchrotron-based AP-XPS),Park and co-workers study and identify the adsorbate-driven morphological evolution of Cu nanoclusters on the Cu(997)surface,providing real-space evidence for the critical role of vicinal structures on Cu *** observed surface roughening trends caused by dissociated atomic oxygen and CO adsorbates subsequently affect the result of successive catalytic reactions to produce critical intermediates,such as carbonate and formate,during the CO_(2)reduction reaction.

关键词： reaction critical rational

Fixed-Time Anti-Disturbance Average-Tracking for Multi-Agent Systems Without Velocity Measurements

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Journal of Systems Science & Complexity 2024年第3期37卷 985-1002页

作者： LI Yuling LIU Chenglin ZHANG ya CHEN yangyang Key Laboratory of Advanced Process Control for Light Industry(Ministry of Education) Institute of AutomationJiangnan UniversityWuci 214122China School of Automation Southeast UniversityNanjing 210096China

In this paper,the authors tackle a fixed-time average-tracking problem for multi-agent systems which do not require velocity measurements and are affected by external mismatched and matched *** objective requires the considered agents with second-order dynamics to follow the average value of several time-varying reference signals,each of which is acquired by only one *** of all,the average value is estimated by using a novel distributed average estimator in a fixed ***,an original observer is created to provide estimated values in a fixed time for external mismatched and matched disturbances as well as unmeasured velocities of ***,the authors propose a novel fixed-time anti-disturbance average-tracking protocol with the aid of the observer and a sliding mode *** the end,the feasibility of theoretical analysis is illustrated by some simulation experiments.

关键词： Average-tracking control fixed-time algorithm fixed-time observer mismatched distur-bances multi-agent systems velocity measurements

Concentration-dependent effects of reductive pulmonary inhalants on ultrafine particle-induced oxidative stress:Insights for health risk assessment

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Environmental Science and Ecotechnology 2024年第3期19卷 118-124页

作者： ya-qi Yu Tong Zhu BIC-ESAT and SKL-ESPC College of Environmental Sciences and EngineeringPeking UniversityBeijing100871PR China School of Environmental Science and Engineering Qingdao UniversityQingdao266071PR China

The impact of reductive pulmonary inhalants on ultrafine particles(UFPs)-induced pulmonary oxidative stress remains a crucial consideration,yet the concentration-dependent effects of these inhalants have remained *** we synthesized composite UFPs simulating atmospheric UFPs,primarily composed of metals and *** subjected these UFPs to varying concentrations(0e7000 mM)of two reductive pulmonary inhalants,N-acetylcysteine and salbutamol,to assess their influence on oxidative potential,measured through the dithiothreitol assay(OP^(DTT)).Simultaneously,we analysed the soluble metal content of UFPs to uncover potential relationships between oxidative potential and metal *** results unveil a dual role played by these inhalants in shaping the OPDTT of composite ***,OP^(DTT) generally increased as inhalant concentrations rose from 0 to 300 ***,an intriguing reversal occurred when concentrations exceeded 500 mM,resulting in a decline in *** to untreated UFPs,these inhalants induced promotion and inhibition effects within concentration ranges of 100e500 and>1000 mM,*** no significant correlation emerged between OP^(DTT) and soluble metal content as inhalant concentrations ranged from 0 to 7000 mM,noteworthy positive correlations emerged at lower inhalant concentrations(e.g.,N-acetylcysteine at 0 e300 mM).These findings provide insights into the potential influence of reductive pulmonary inhalants on health risks associated with UFP exposure,further underscoring the need for continued research in this critical area.

关键词： Concentration-dependent effects Oxidative potential reductive pulmonary inhalants Soluble metals Simulated atmospheric ultrafine particles

An Accelerated Stochastic Mirror Descent Method

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Journal of the Operations research Society of China 2024年第3期12卷 549-571页

作者： Bo-Ou Jiang ya-Xiang Yuan LSEC ICMSECAMSSChinese Academy of SciencesBeijing100190China Department of Mathematics University of Chinese Academy of SciencesBeijing100049China

Driven by large-scale optimization problems arising from machine learning,the development of stochastic optimization methods has witnessed a huge *** types of methods have been developed based on vanilla stochastic gradient descent ***,for most algorithms,convergence rate in stochastic setting cannot simply match that in deterministic *** understanding the gap between deterministic and stochastic optimization is the main goal of this ***,we are interested in Nesterov acceleration of gradient-based *** our study,we focus on acceleration of stochastic mirror descent method with implicit regularization *** that the problem objective is smooth and convex or strongly convex,our analysis prescribes the method parameters which ensure fast convergence of the estimation error and satisfied numerical performance.

关键词： Large-scale optimization Variance reduction Mirror descent Acceleration Independent sampling Importance sampling

Astrophysical S-factor and reaction rate for 15N(p,γ)16O within the modified potential cluster model

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Chinese Physics C 2024年第4期48卷 130-145页

作者： S.B.Dubovichenko A.S.Tkachenko r.ya.kezer.shvili N.A.Burkova B.M.Yeleusheva Fesenkov Astrophysical Institute 050020 AlmatyKazakhstan New York City College of Technology City University of New YorkBrooklyn11201 New YorkUSA Graduate School and University Center City University of New York10016 New YorkUSA al-Farabi Kazakh National University 050040 AlmatyKazakhstan

We study radiative p^(15)N capture on the ground state of ^(16)O at stellar energies within the framework of a modified potential cluster model(MPCM)with forbidden states,including low-lying *** investigation of the ^(15)N(p,γ0)^(16)O reaction includes the consideration of ^(3)S_(1) resonances due to E1 transitions and the contribution of the ^(3)P_(1) scattering wave in the p+^(15)N channel due to the ^(3)P_(1)→^(3)P_(0)M1 *** calculated the astrophysical low-energy S-factor,and the extrapolated S(0)turned out to be within 34.7−40.4 keV·*** important role of the asymptotic constant(AC)for the ^(15)N(p,γ0)16O process with interfering ^(3)S_(1)(312)and ^(3)S_(1)(962)resonances is elucidated.A comparison of our calculation for the S-factor with existing experimental and theoretical data is addressed,and a reasonable agreement is *** reaction rate is calculated and compared with the existing *** has negligible dependence on the variation of AC but shows a strong impact of the interference of ^(3)S_(1)(312)and ^(3)S_(1)(962)resonances in reference to the CNO Gamow windows,especially at low *** estimate the contribution of cascade transitions to the reaction rate based on the exclusive experimental data from ***.C.85,065810(2012).The reaction rate enhancement due to the cascade transitions is observed from T_(9)>0.3 and reaches the maximum factor~1.3 at T_(9)=*** present the Gamow energy window and a comparison of rates for radiative proton capture reactions ^(12)N(p,γ)^(13)O,^(13)N(p,γ)^(14)O,^(14)N(p,γ)^(15)O,and ^(15)N(p,γ)^(16)O obtained in the framework of the MPCM and provide the temperature windows,prevalence,and significance of each process.

关键词： low and astrophysical energies p^(15)N system thermonuclear reaction rate potential cluster model CNO-cycle