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Self-healing Hydrogelsand Underlying Reversible Intermolecular Interactions

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Chinese Journal of Polymer Science 2021年第10期39卷 1246-1261,I0005页

作者： Meng Wu qiong-Yao peng Lin-Bo Han Hong-Bo Zeng Department of Chemical&Materials Engineering University of AlbertaEdmontonAlberta T6G 1H9Canada College of Health Science and Environmental Engineering Shenzhen Technology UniversityShenzhen 518118China

Self-healing hydrogels have attracted growing attention over the past decade due to their biomimetic structure,biocompatibility,as well as enhanced lifespan and reliability,thereby have been widely used in various biomedical,electrical and environmental engineering *** feature article has reviewed our recent progress in self-healing hydrogels derived from mussel-inspired interactions,multiple hydrogen-bonding functional groups such as 2-ureido-4[1H]-pyrimidinohe(UPy),dynamic covalent bonds(eg,Schiff base reactions and boronic ester bonds).The underlying molecular basics of these interactions,hydrogel preparation principles,and corresponding performances and applications are *** underlying reversible intermolecular interaction mechanisms in these hydrogels were investigated using nanomechanical techniques such as surface forces apparatus(SFA)and atomic force microscopy(AFM),providing fundamental insights into the self-healing mechanisms of the *** remaining challenging issues and perspectives in this rapidly developing research area are also discussed.

关键词： Self-healing hydrogels Mussel-inspired Interaction Multiple hydrogen-bonding Dynamic covalent bonds Intermolecular forces

Disturbance effects on community structure of Ficus tinctoria fig wasps in Xishuangbanna, China： Implications for the fig/fig wasp mutualism

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Insect Science 2009年第5期16卷 417-424页

作者： Wen-Juan Ma Da-Rong Yang Yan-qiong peng Xishuangbanna Tropical Botanical Garden Chinese Academy of Sciences Kunming Graduate School of the Chinese Academy ofSciences Beijing China

Fig trees are important components of tropical forests, because their fruits are eaten by so many vertebrates, but they depend on pollinating fig wasps to produce mature fruits. Disturbance to habitat structure can have a major impact on insect diversity and com- position, potentially reducing fruit yields. We investigated the impact of habitat disturbance on the fig wasp community associated with male figs ofFicus tinctoria in Xishuangbanna, China. The community comprised one pollinator species Liporrhopalum gibbosae and six non-pollinating wasp species： Sycoscapter sp. 1, Philotrypesis ravii, Philotrypesis sp. 1, Neosycophila omeomorpha, Sycophila sp.1, and Walkerella sp.1. More disturbed areas were characterized by higher temperatures, less shade, and more vehicle noise. The response of the fig wasp community was complex, with no simple relationship between intensity of disturbance and pollinator abundance. However, the sex ratios （proportion of male progeny） of pollinators increased significantly in more disturbed areas. We conclude that potential changes in fig wasp community composition brought about by disturbance, are unpredictable, with unclear consequences for tropical rainforest biodiversity.

关键词： disturbance Ficus tinctoria fig/fig wasp mutualism wasp community

Enhanced and asymmetric signatures of hybridization at climatic margins: Evidence from closely related dioecious fig species

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Plant Diversity 2024年第2期46卷 181-193页

作者： Jian-Feng Huang Clive T.Darwell Yan-qiong peng CAS Key Laboratory of Tropical Forest Ecology Xishuangbanna Tropical Botanical GardenChinese Academy of SciencesMengla 666303China National Center for Genetic Engineering and Biotechnology(BIOTEC) 113 Thailand Science ParkPhahonyothin RoadKhlong NuengKhlong LuangPathum Thani 12120Thailand

Hybridization plays a significant role in biological evolution. However, it is not clear whether ecological contingency differentially influences likelihood of hybridization, particularly at ecological margins where parental species may exhibit reduced fitnesses. Moreover, it is unknown whether future ecosystem change will increase the prevalence of hybridization. Ficus heterostyla and F. squamosa are closely related species co-distributed from southern Thailand to southwest China where hybridization, yielding viable seeds, has been documented. As a robust test of ecological factors driving hybridization, we investigated spatial hybridization signatures based on nuclear microsatellites from extensive population sampling across a widespread contact range. Both species showed high population differentiation and strong patterns of isolation by distance. Admixture estimates exposed asymmetric interspecific gene *** of hybridization increase significantly towards higher latitude zones, peaking at the northern climatic margins. Geographic variation in reproductive phenology combined with ecologically challenging marginal habitats may promote this phenomenon. Our work is a first systematic evaluation of such patterns in a comprehensive, latitudinally-based clinal context, and indicates that tendency to hybridize appears strongly influenced by environmental conditions. Moreover, that future climate change scenarios will likely alter and possibly augment cases of hybridization at ecosystem scales.

关键词： Hybridization Heterospecific visitation Fig Pollinator wasp Asymmetric gene flow

Tunable and improved microwave absorption of flower-like core@shell MFe_(2)O_(4)@MoS_(2)(M=Mn,Ni and Zn)nanocomposites by defect and interface engineering

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Journal of Materials Science & Technology 2023年第8期139卷 137-146页

作者： Junxiong Xiao Xiaosi Qi Xiu Gong qiong peng Yanli Chen Ren Xie Wei Zhong College of Physics Guizhou Province Key Laboratory for Photoelectrics Technology and ApplicationGuizhou UniversityGuiyang 550025China National Laboratory of Solid State Microstructures and Jiangsu Provincial Laboratory for NanoTechnology Nanjing UniversityNanjing 210093China

Previous results revealed that the defect and/or interface had a great impact on the electromagnetic pa-rameters of *** order to understand the main physical mechanisms and effectively utilize these strategies,in this study,M Fe_(2)O_(4)and flower-like core@shell M Fe_(2)O_(4)@MoS_(2)(M=Mn,Ni,and Zn)sam-ples with different categories were elaborately designed and selectively produced in large scale through a simple two-step hydrothermal *** conducted the systematical investigation on their microstruc-tures,electromagnetic parameters and microwave absorption performances(MAPs).The obtained results revealed that the large radius of M^(2+)cation could effectively boost the concentration of oxygen vacancy in the M Fe_(2)O_(4)and M Fe_(2)O_(4)@MoS_(2)samples,which resulted in the improvement of dielectric loss capabil-ities and ***,the introduction of MoS_(2)nanosheets greatly improved the interfacial effect and enhanced the polarization loss capabilities,which also boosted the *** taking full advantage of the defect and interface,the designed M Fe_(2)O_(4)@MoS_(2)samples displayed tunable and excellent com-prehensive MAPs including strong absorption capability,wide absorption bandwidth and thin matching ***,the clear understanding of defect and interface engineering made these strategies well elaborately designed and applicable to improving MAPs.

关键词： Core@shell structure M Fe_(2)O_(4)@MoS_(2)(M=Mn,Ni and Zn) Defect and interface engineering Improved microwave absorption properties

Magnetic-dielectric synergy and interfacial engineering to design yolk-shell structured CoNi@void@C and CoNi@void@C@MoS_(2) nanocomposites with tunable and strong wideband microwave absorption

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Nano Research 2022年第7期15卷 6761-6771页

作者： Chen Li Xiaosi Qi Xiu Gong qiong peng Yanli Chen Ren Xie Wei Zhong College of Physics Guizhou Province Key Laboratory for Photoelectrics Technology and ApplicationGuizhou UniversityGuiyang 550025China National Laboratory of Solid State Microstructures and Jiangsu Provincial Laboratory for NanoTechnology Nanjing UniversityNanjing 210093China

In order to effectively utilize the magnetic-dielectric synergy and interfacial engineering,in this paper,yolk–shell structured magnetic multicomponent nanocomposites(MCNCs)including CoNi@void@C and CoNi@void@C@MoS_(2) were produced in large scale by in-situ pyrolysis of cubic CoNi Prussian blue analogs(PBAs)followed by the hydrothermal process,*** of their unique structures,excellent synergistic effect between dielectric and magnetic loss,the as-prepared CoNi@void@C and CoNi@void@C@MoS_(2) MCNCs displayed very outstanding electromagnetic wave absorption performances(EMWAPs)including strong absorption capabilities,broad absorption bandwidth and thin matching ***,the as-prepared CoNi@void@C and CoNi@void@C@MoS_(2) MCNCs well maintained the cubic configuration of CoNi PBAs even after the thermal treatment and hydrothermal *** unique structure and formed carbon layers effectively prevented the corrosion of internal CoNi alloy during the formation of MoS_(2),and CoNi@void@C@MoS_(2) MCNCs with different MoS_(2) contents could be synthesized by controlling the hydrothermal *** obtained results revealed that the EM parameters,dielectric and magnetic loss capabilities of CoNi@void@C@MoS_(2) MCNCs could be tuned by controlling hydrothermal temperature and filler loading,which made their outstanding EMWAPs could be achieved in different frequency *** account of simple process,low density and high chemical stability,our findings provided a new and effective pathway to develop the strong wideband microwave absorbers.

关键词： yolk-shell structure CoNi@void@C CoNi@void@C@MoS_(2) interface polarization strong wideband microwave absorbers

Defect and interface engineering in core@shell structure hollow carbon@MoS_(2)nanocomposites for boosted microwave absorption performance

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Nano Research 2022年第9期15卷 7778-7787页

Defect and interface engineering are efficient approaches to adjust the physical and chemical properties of *** order to effectively utilize these strategies for the improvement of microwave absorption properties(MAPs),in this study,we reported the synthesis of hollow carbon shells and hollow carbon@MoS_(2)nanocomposites by the template-etching and templateetching-hydrothermal methods,*** obtained results indicated that the degree of defect for hollow carbon shells and hollow carbon@MoS_(2)could be modulated by the thickness of hollow carbon shell,which effectively fulfilled the optimization of electromagnetic parameters and improvement of ***,the microstructure investigations revealed that the precursor of hollow carbon shells was encapsulated by the sheet-like MoS_(2)in high *** the introduction of MoS_(2)nanosheets acting as the shell effectively improved the interfacial effects and boosted the polarization loss capabilities,which resulted in the improvement of comprehensive *** elaborately designed hollow carbon@MoS_(2)samples displayed very outstanding MAPs including strong absorption capabilities,broad absorption bandwidth,and thin matching ***,this work provided a viable strategy to improve the MAPs of microwave absorbers by taking full advantage of their defect and interface engineering.

关键词： core@shell structure hollow carbon shells hollow carbon@MoS_(2) defect and interface engineering improved microwave absorption properties

Microstructure optimization of core@shell structured MSe_(2)/FeSe_(2)@MoSe_(2)(M=Co,Ni)flower-like multicomponent nanocomposites towards high-efficiency microwave absorption

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Journal of Materials Science & Technology 2022年第33期128卷 59-70页

作者： Jingjing Zhang Xiaosi Qi Xiu Gong qiong peng Yanli Chen Ren Xie Wei Zhong College of Physics Guizhou Province Key Laboratory for Photoelectrics Technology and ApplicationGuizhou UniversityGuiyang 550025China National Laboratory of Solid State Microstructures and Jiangsu Provincial Laboratory for NanoTechnology Nanjing UniversityNanjing 210093China

In this work,we put forward a scheme to exquisitely design and selectively synthesize the core@shell structured MSe_(2)/FeSe_(2)@MoSe_(2)(M=Co,Ni)flower-like multicomponent nanocomposites(MCNCs)through a simple two-step hydrothermal reaction on the surfaces of MFe_(2)O_4 nanospheres with the certain amounts of Mo and Se *** increasing the amounts of Mo and Se sources,the obtained core@shell structured MSe_(2)/FeSe_(2)@MoSe_(2)(M=Co,Ni)MCNCs with the enhanced content of MoSe_(2)and improved flower-like geometry morphology could be produced on a large *** obtained results revealed that the as-prepared samples displayed improved comprehensive microwave absorption properties(CMAPs)with the increased amounts of Mo and Se *** as-prepared CoSe_(2)/FeSe_(2)@MoSe_(2)and NiSe_(2)/FeSe_(2)@MoSe_(2)MCNCs with the well-defined flower-like morphology could simultaneously present the outstanding CMAPs in terms of strong absorption capability,wide absorption bandwidth,and thin matching thicknesses,which mainly originated from the conduction loss and flower-like geometry ***,the findings not only develop the very desirable candidates for high-performance microwave absorption materials but also pave a new way for optimizing the CMAPs through tailoring morphology engineering.

关键词： Core@shell structure MSe_(2)/FeSe_(2)@MoSe_(2)(M=Co.Ni) multicomponent nanocomposites Flower-like geometry morphology Broad frequency bandwidth Microwave absorption

Root Endophyte Shift and Key Genera Discovery in Rice under Barnyardgrass Stress

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Rice science 2023年第2期30卷 160-170,I0040-I0048页

作者： LI Shuyan YAN Qiling WANG Jieyu JIANG Huidan LI Zuren peng qiong Long Ping Branch Graduate School of Hunan UniversityChangsha 410125China Hunan Agricultural Biotechnology Research Institute Hunan Academy of Agricultural SciencesChangsha 410125China

Despite increasing knowledge of barnyardgrass(Echinochloa crus-galli) interference with rice, relatively little is known how endophytes improve the ability of rice against barnyardgrass stress. Here, we provided a detailed temporal characterization of rice root-associated microbiomes during co-cultivation with barnyardgrass and a comparison with the microbiomes of weed-free rice plants. Alpha diversity analysis indicated that barnyardgrass had the opposite effects on endophytic bacteria and fungi in rice roots, in terms of the community diversity, richness and coverage at the rice seedling stage. Principal coordinate analysis showed that barnyardgrass had only a minor effect on the community composition of endophytes in rice roots at the rice seedling stage, but showed a significant and maximum interference at the heading stage. Rice recruited many endophytes to resist biotic stress from barnyardgrass, especially for fungi. PICRUSt(phylogenetic investigation of communities by reconstruction of unobserved states) predictive analysis indicated that 23 metabolic pathways of bacteria were overrepresented in rice. In addition, the main trophic mode of fungi was pathotroph according to FUNGuild analysis. A positive correlation between bacteria and fungi in rice roots was found via network analysis. Anaeromyxobacter, Azospira and Pseudolabrys were the vital bacteria, Phaeosphaeria and Funneliformis were the dominant fungi in maintaining the stability of the ecological network. These results provided data and a theoretical basis for the in-depth understanding of what role endophytes play in rice resistance to barnyardgrass stress and will have implications on improving the resistance of rice against biotic stress using root microbiota.

关键词： rice Echinochloa crus-galli biotic stress endophytic bacterium endophytic fungus phylogenetic investigation of communities by reconstruction of unobserved states FUNGuild test

Unexpected elastic isotropy in a black phosphorene/TiC2 van der Waals heterostructure with flexible Li-ion battery anode applications

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Nano Research 2017年第9期10卷 3136-3150页

作者： qiong peng Kangming Hu Baisheng Sa Jian Zhou Bo Wu Xianhua Hou Zhimei Sun Multiscale Computational Materials Facility College of Materials Science and Engineering Euzhou University Fuzhou 3S0100 China Key Laboratory of Eco-Materials Advanced Technology (Fuzhou University) Fujian Province University Fuzhou 350 I00 China School of Materials Science and Engineering and Center for Integrated Computational Materials Engineering International Research Institute for Multidisciplinary Science Beihang University Beijing 100191 China Guangdong Engineering Technology Research Center of Efficient Green Energy and Environmental Protection Materials School ofPhysics and Telecommunication Engineering South China Normal University Guangzhou 510006 China

Recently, flexible electrodes with biaxial/omnidirectional stretchability have attracted significant attention. However, most existing pliable electrode materials can be only stretched in one direction. In this work, an unexpected isotropic van der Waals (vdW) heterostructure is proposed, based on the assembly of two-dimensional crystals of anisotropic black phosphorene (BP) and transition metal carbide (TiC2). Using vdW-corrected density functional theory calculations, the BP/TiC2 vdW heterostructure was predicted to have excellent structural and mechanical stability, superior electrical conductivity, omnidirectional flexibility, and a high Li storage capacity. We have unraveled the physical origin of the excellent stability, as well as the Li adsorption preferences of the lithiated heterostructure, based on a three-step analysis of the stability of the Li-adsorption processes. In addition, the BP/TiC2 vdW heterostructure can also be applied as the anode material for flexible Na-ion batteries because of its high Na storage capacity and strong Na binding. However, compared with Na adsorption, the capacity is higher, and the adsorption energy is more negative for Li adsorption. Our findings provide valuable insights into the exploration of a rich variety of vdW heterostructures for next-generation flexible energy storage devices.

关键词： van der Waals heterostructure omnidirectional stretchability Li adsorption flexible anode first-principles calculations