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Chemical Activation of S/li2S in li-S Batteries by a Bidirectional Organic Redox Mediator

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Chemical Research in Chinese Universities 2024年第5期40卷 927-934页

作者： li Chengqiu ZHOU Chaoyong MEI Shilin YAO Changjiang State Key Laboratory of Explosion Science and Safety Protection School of Mechatronical EngineeringBeijing Institute of TechnologyBeijing100081P.R.China Xi’an Safty Energy Technology Co. Ltd.Xi’an710299P.R.China

The energy density and lifespan of prototype li-S batteries under high sulfur loading and lean electrolyte have been mainly restricted by the incomplete interconversion between insulating S8 and *** introduction of an electrocatalyst has been preserved as an effective way to breakthrough the bottleneck of the interconversion ***,we demonstrate a novel bidirectional redox mediator,insoluble dithiobisphthalimide(DTPI),as the electrocatalyst for both S8 reduction and li2S *** to the dual-functional role of both electron/li^(+)donor and acceptor,DTPI can efficiently accelerate the redox reactions during charge/discharge and significantly alleviate the incomplete conversion of sulfur ***,the li-S batteries with DTPI deliver superior specific capacity and cycling stability in comparison with those without ***,the redox mediator is scalable for synthesis and the DTPI-based 5 A·h pouch cell delivers a specific discharge capacity of around 870 mA·h·g^(−1) at 0.1 C(1 C=1675 mA/g)without capacity fading over 80 *** bidirectional catalysis mechanism has been studied through theoretical calculation and ex-situ characterization of the cathode *** work approves the effectiveness of bidirectional organic redox mediator in the construction of practical li-S batteries.

关键词： lithium-sulfur battery(LSB) Dithiobisphthalimide(DTPI) Organic redox mediator Interconversion

“突出自主学习能力,强化师范素质培养”的教学改革理论与实践

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湘南学院学报 2012年第2期33卷 71-73页

作者：李儒新李群英侯广斌湘南学院体育系湖南郴州423000

对培养体育教育专业学生自主学习能力和不断提高师范素质的教学改革理论与实践进行了探讨.实践结果表明,构建培养体育教育专业学生自主学习能力与师范素质的新模式,打造体育教育专业培养学生自主学习和师范能力的实践平台;教学效果得到... 详细信息

对培养体育教育专业学生自主学习能力和不断提高师范素质的教学改革理论与实践进行了探讨.实践结果表明,构建培养体育教育专业学生自主学习能力与师范素质的新模式,打造体育教育专业培养学生自主学习和师范能力的实践平台;教学效果得到了校内外专家和学生的一致好评,提高了学生的师范素质和自主学习能力.

关键词：自主学习师范素质教学改革

Semi-automated detection of rangeland runoff and erosion control berms using high-resolution topography data

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International Soil and Water Conservation Research 2024年第1期12卷 217-226页

作者： li li Changjiang River Scientific Research Institute of Changjiang Water Resources Commission Wuhan430010China Research Center on Mountain Torrent&Geologic Disaster Prevention Ministry of Water ResourcesWuhan430010China University of Arizona School of Natural Resources and the EnvironmentTucsonAZ85719USA

An inventory of topographic modifications is essential to addressing their impacts on hydrological and morphological processes in human-altered ***,such inventories are generally *** study presents two workflows for semi-automatic detection of linear earthen runoff and erosion control berms in rangelands using high-resolution topographic *** workflows consist of initial object identification by applying either morphological grayscale reconstruction(MGR)or the Geomorphon(GEO)method,followed by identification refinements through filters based on objects’horizontal and vertical *** sites were selected within the Altar Valley,Arizona,in the southwestern United *** site was used for developing workflows and optimizing filter thresholds,and the other two sites were used to validate *** results showed that:1)The MGR-based workflow methodology could produce final precision and detection rates of up to 92%and 75%,respectively,and take less than 5 s for a 10.1 km^(2) site;2)The workflow based on the MGR method yielded greater identification accuracy than did the GEO workflow;3)Object length,orientation,and eccentricity were important characteristics for identifying earthen berms,and are sensitive to general channel flow direction and berm shape;4)Manual interrogation of topographic data and imagery can significantly improve identification precision *** proposed workflows will be useful for developing inventories of runoff and erosion control structures in support of sustainable rangeland management.

关键词： Earthen berm Rangeland Grayscale morphological reconstruction Geomorphon liDAR

Perturbed low-thrust geostationary orbit transfer guidance via polynomial costate estimation

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Chinese Journal of Aeronautics 2024年第3期37卷 181-193页

作者： Zhao li Hengnian li Fanghua JIANG Junfeng li State Key Laboratory of Astronautic Dynamics Xi’an Satellite Control CenterXi’an 710043China School of Aerospace Engineering Tsinghua UniversityBeijing 100084China

This paper proposes an optimal,robust,and efficient guidance scheme for the perturbed minimum-time low-thrust transfer toward the geostationary *** Earth’s oblateness perturbation and shadow are taken into *** is difficult for a Lyapunov-based or trajectory-tracking guidance method to possess multiple characteristics at the same time,including high guidance optimality,robustness,and onboard computational *** this work,a concise relationship between the minimum-time transfer problem with orbital averaging and its optimal solution is identified,which reveals that the five averaged initial costates that dominate the optimal thrust direction can be approximately determined by only four initial modified equinoctial orbit elements after a coordinate *** on this relationship,the optimal averaged trajectories constituting the training dataset are randomly generated around a nominal averaged *** polynomial regression models are trained on the training dataset and are regarded as the costate *** the transfer,the spacecraft can obtain the real-time approximate optimal thrust direction by combining the costate estimations provided by the estimators with the current state at any ***,all these computations onboard are *** simulation results show that the proposed guidance scheme possesses extremely high guidance optimality,robustness,and onboard computational efficiency.

关键词： Low thrust Orbital transfer Trajectory optimization Guidance Indirect method Orbital averaging Machine learning Geostationary satellites

Theoretical Analysis of Cooperative Driving at Idealized Unsignalized Intersections

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Tsinghua Science and Technology 2024年第1期29卷 257-270页

作者： Shen li Jiawei Zhang Zhenwu Chen li li Department of Civil Engineering Tsinghua UniversityBeijing 100084China Department of Automation Tsinghua UniversityBeijing 100084China Shenzhen Urban Transport Planning Center Co. Ltd.Shenzhen 518000China

Cooperative driving is widely viewed as a promising method to better utilize limited road resources and alleviate traffic *** recent years,several cooperative driving approaches for idealized traffic scenarios(i.e.,uniform vehicle arrivals,lengths,and speeds)have been ***,theoretical analyses and comparisons of these approaches are *** this study,we propose a unified group-by-group zipper-style movement model to describe different approaches synthetically and evaluate their *** derive the maximum throughput for cooperative driving plans of idealized unsignalized intersections and discuss how to minimize the delay of *** obtained conclusions shed light on future cooperative driving studies.

关键词： cooperative driving connected and automated vehicles unsignalized intersection

Effects of mid-passage gap with a variable surface angle on a turbine vane endwall’s aerothermal and film cooling performances

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Chinese Journal of Aeronautics 2024年第6期37卷 20-37页

作者： Zhiyu li Kaiyuan ZHANG Zhigang li Jun li Institute of Turbomachinery Xi’an Jiaotong UniversityXi’an 710049China

The mid-passage gap is an inevitable structure in a vane passage due to turbine vanes being manufactured *** coolant from this gap is able to prevent hot mainstream ingression and provide cooling protection for the endwall.A novel idea of enlarging the endwall’s coverage area and reducing the endwall’s thermal load by applying the mid-passage gap with variable surface angles is carried out in this *** endwall’s aerothermal and film cooling performances under four mid-passage gap modes at three typical mass flow ratio conditions are numerically *** indicate that under the traditional mid-passage mode,the coolant flows into the mainstream with a perpendicular incidence angle and can’t stick to the ***,cooling failure occurs,and the endwall’s thermal load is badly *** film cooling level at the suction-side endwall is improved when applying the mid-passage gap of a 45surface angle due to the secondary vortex being *** addition,when applying the mid-passage gap of a 135surface angle,the horseshoe vortex is pushed away,and the coverage area at the pressure-side endwall is enlarged *** best film cooling performance is achieved when the upstream surface angle is 135and the downstream surface angle is 45due to the adiabatic film cooling effectiveness being increased at both the pressure-and suction-side *** the mass flow ratio is 1.5%,the coverage area is enlarged by 43%,and the area-averaged adiabatic film cooling effectiveness is increased by 37%,when compared with those under the traditional mid-passage mode.

关键词： Film cooling Heat transfer Surface angle Mid-passagegap Turbinevane endwall

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心血管病康复护理实践与思考

中国护理管理 2021年第11期21卷 1601-1607页

作者：李庆印吴岳刘湉王诗瑜李朝晖中国医学科学院阜外医院护理部北京市100037 中国医学科学院阜外医院心脏康复中心北京市100037

回顾国内外心血管病康复护理发展历程,分析心血管病康复护理研究现状的热点和难点,选取具有特色的心血管病康复护理探索性实践研究进行阐述,并对该领域后续的发展方向进行思考与展望,旨在为国内心血管病康复护理实践提供借鉴和参考。

关键词：心脏康复护理心血管病康复护理

Failure mechanisms and surface treatment processes of thermal barrier coatings:Review

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Chinese Journal of Aeronautics 2024年第9期37卷 20-40页

作者： Hao li Shengqiang YANG Xiuhong li Wenhui li College of Mechanical and Vehicle Engineering Taiyuan University of TechnologyTaiyuan 030024China Shan.xi Province Key Laboratory of Precise Machining Taiyuan University of TechnologyTaiyuan 030024China College of Aeronautics and Astronautics Taiyuan University of TechnologyTaiyuan 030024China

Thermal Barrier Coatings(TBCs)technology is key to improving the service temperature and the productivity of aircraft *** performance and failure life of TBCs are strongly influenced by surface integrity and ***,recognizing failure mechanisms and developing effective surface treatment processes are crucial for further improving the reliability and durability of *** paper explains the primary reasons for TBC failure,emphasizing on how integrity of surface and interface influences interfacial oxidation,high-temperature erosion,and Calcium-Magnesium-Alumina-Silicate(CMAS)***,this paper completely and rigorously evaluates the research status of TBCs surface treatment processes,including the characteristics and effects of various processes,and describes the requirements and goals of pretreatment and *** addition,a potential direction for the development and application of TBCs surface treatment is suggested.

关键词： Thermal BarrierCoatings(TBCs) Failure Surface treatment processes Processing goals Mass finishing

Ultrathin organic solvent nanofiltration membrane with polydopamine-HKUST-1 interlayer for organic solvent separation

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Journal of Environmental Sciences 2024年第7期141卷 182-193页

作者： Haike li Xindong li Guozai Ouyang lijinhong Huang Lang li Wenhao li Wanfu Huang Duokun li Ganzhou Key Laboratory of Basin Pollution Simulation and Control Jiangxi University of Science and TechnologyGanzhou 341000China Innovation Center for Water Quality Security Technology at Ganjiang River Basin Jiangxi University of Science and TechnologyGanzhou 341000China School of Architecture and Design Jiangxi University of Science and TechnologyGanzhou 341000China WA School of Mines:Minerals Energy and Chemical EngineeringCurtin UniversityWA 6845Australia School of Materials Science and Engineering Tiangong UniversityTianjin 300387China

Polydopamine(PDA)and metal-organic skeleton HKUST-1 were co-deposited on the base membrane of hexamethylenediamine(HDA)-crosslinked polyetherimide(PEI)ultrafiltration membrane as the interlayer,and high-throughput organic solvent nanofiltration membrane(OSN)was prepared by interfacial polymerization and solvent activation *** polyamide(PA)layer surface roughness from 28.4 nm in PA/PEI to 78.3 nm in PA/PDA-HKUST-10.6/PEI membrane,reduced the thickness of the separation layer from 79 to 14 nm,and significantly improved the hydrophilic,thermal and mechanical *** flux of the PA/PDA-HKUST-10.6/PEI membrane in a 0.1 g/L Congo Red(CR)ethanol solution at 0.6 MPa test pressure reached 21.8 L/(m^(2)·hr)and the rejection of CR was 92.8%.Solvent adsorption test,N,N-dimethylformamide(DMF)immersion experiment,and long-term operation test in ethanol showed that the membranes had high solvent *** solvent flux test demonstrated that,under the test pressure of 0.6 MPa,the flux of different solvents ranked as follows:methanol(56.9 L/(m^(2)·hr))>DMF(39.6 L/(m^(2)·hr))>ethanol(31.2 L/(m^(2)·hr))>IPA(4.5 L/(m^(2)·hr))>N-hexane(1.9 L/(m^(2)·hr)).The ability of the membranes to retain dyes in IPA/water dyes solution was also *** flux of the membrane was 30.4 L/(m^(2)·hr)and the rejection of CR was 91.6%when the IPA concentration reached 50%.This OSN membrane-making strategy is economical,environment-friendly and efficient,and has a great application prospect in organic solvent separation systems.

关键词： Interfacial polymerization Organic solvent nanofiltration Interlayer Metal-organic frameworks Polydopamine