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Differentiated emission control strategy based on comprehensive evaluation of multi-media pollution:Case of mercury emission control

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Journal of Environmental Sciences 2023年第1期123卷 222-234页

作者： Dongwei Lv qingru wu Daiwei Ouyang Minneng Wen Gehui Zhang Shuxiao Wang Lei Duan State Key Laboratory of Environmental Simulation and Pollution Control School of EnvironmentTsinghua UniversityBeijing 100084China State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex Beijing 100084China

In order to comprehensively evaluate the environmental impact of multi-media mercury pollution under differentiated emission control strategies in China,a literature review and case studies were carried *** human exposure to methylmercury was assessed through the dietary intake of residents in areas surrounding a typical coal-fired power plant and a zinc(Zn)smelter,located either on acid soil with paddy growth in southern China,or on alkaline soil with wheat growth in northern *** with knowledge on speciated mercury in flue gas and the fate of mercury in the wastewater or solid waste of the typical emitters applying different air pollution control devices,a simplified model was developed by estimating the incremental daily intake of methylmercury from both local and global *** indicated that air pollution control for coal-fired power plants and Zn smelters can greatly reduce health risks from mercury pollution,mainly through a reduction in global methylmercury exposure,but could unfortunately induce local methylmercury exposure by transferring more mercury from flue gas to wastewater or solid waste,then contaminating surrounding soil,and thus increasing dietary intake via ***,tightening air emission control is conducive to reducing the comprehensive health risk,while the environmental equity between local and global pollution control should be fully *** in the south tends to have higher bioconcentration factors than wheat in the north,implying the great importance of strengthening local pollution control in the south,especially for Zn smelters with higher contribution to local pollution.

关键词： Mercury emission Methylmercury Heavy metal Bioconcentration factor Estimated daily intake Health risk assessment

Mercury flows in large-scale gold production and implications for Hg pollution control

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Journal of Environmental Sciences 2018年第6期30卷 91-99页

作者： qingru wu Shuxiao Wang Mei Yang Haitao Su Guoliang Li Yi Tang Jiming Hao State Key Joint Laboratory of Environment Simulation and Pollution Control School of Environment Tsinghua University Beijing 100084 China State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex Beijing 100084 China College of Electromechanical Engineering Qingdao University of Science and Technology Qingdao 266061 China

Large-scale gold production（LSGP） is one of the five convention-related atmospheric mercury（Hg） emission sources in the Minamata Convention on Mercury. However, field experiments on Hg flows of the whole process of LSGP are limited. To identify the atmospheric Hg emission points and understand Hg emission characteristics of LSGP, Hg flows in two gold smelters were studied. Overall atmospheric Hg emissions accounted for 10%–17% of total Hg outputs and the Hg emission factors for all processes were 7.6–9.6 kg/ton. There were three dominant atmospheric Hg emission points in the studied gold smelters, including the exhaust gas of the roasting process, exhaust gas from the environmental fog collection stack and exhaust gas from the converter of the refining process. Atmospheric Hg emissions from the roasting process only accounted for 16%–29% of total emissions and the rest were emitted from the refining process. The overall Hg speciation profile（gaseous elemental Hg/gaseous oxidized Hg/particulate-bound Hg） for LSGP was 34.1/57.1/8.8. The dominant Hg output byproducts included waste acid, sulfuric acid and cyanide leaching residue. Total Hg outputs from these three byproducts were 80% in smelter A and 84% in smelter B. Our study indicated that previous atmospheric Hg emissions from large-scale gold production might have been *** emission control in LSGP is not especially urgent in China compared to other significant emission sources（e.g., cement plants）. Instead, LSGP is a potential Hg release source due to the high Hg output proportions to acid and sludge.

关键词： Large-scale gold production Mercury Flow analysis Emission characteristics

Mercury mass flow in iron and steel production process and its implications for mercury emission control

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Journal of Environmental Sciences 2016年第5期28卷 293-301页

作者： Fengyang Wang Shuxiao Wang Lei Zhang Hai Yang Wei Gao qingru wu Jiming Hao State Key Joint Laboratory of Environment Simulation and Pollution Control School of Environment Tsinghua UniversityBeijing 100084 China State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex Beijing 100084 China

The iron and steel production process is one of the predominant anthropogenic sources of atmospheric mercury emissions worldwide. In this study, field tests were conducted to study mercury emission characteristics and mass flows at two iron and steel plants in China. It was found that low-sulfur flue gas from sintering machines could contribute up to41% of the total atmospheric mercury emissions, and desulfurization devices could remarkably help reduce the emissions. Coal gas burning accounted for 17%–49% of the total mercury emissions, and therefore the mercury control of coal gas burning, specifically for the power plant burning coal gas to generate electricity, was significantly important. The emissions from limestone and dolomite production and electric furnaces can contribute29.3% and 4.2% of the total mercury emissions from iron and steel production. More attention should be paid to mercury emissions from these two processes. Blast furnace dust accounted for 27%–36% of the total mercury output for the whole iron and steel production process. The recycling of blast furnace dust could greatly increase the atmospheric mercury emissions and should not be conducted. The mercury emission factors for the coke oven,sintering machine and blast furnace were 0.039–0.047 g Hg/ton steel, and for the electric furnace it was 0.021 g Hg/ton steel. The predominant emission species was oxidized mercury, accounting for 59%–73% of total mercury emissions to air.

关键词： Iron and steel plant Mercury Emission characteristics Mass flow Emission control

Improved atmospheric mercury simulation using updated gas-particle partition and organic aerosol concentrations

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Journal of Environmental Sciences 2022年第9期34卷 106-118页

作者： Kaiyun Liu qingru wu Shuxiao Wang Xing Chang Yi Tang Long Wang Tonghao Liu Lei Zhang Yu Zhao Qin’geng Wang Jinsheng Chen State Key Joint Laboratory of Environment Simulation and Pollution Control School of EnvironmentTsinghua UniversityBeijing 100084China State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex Beijing 100084China Institute of Atmospheric Environment Guangdong provincial academy of environmental scienceGuangzhou 510045China China National Environmental Monitoring Centre Beijing 100012China State Key Laboratory of Pollution Control and Resource Reuse School of the EnvironmentNanjing UniversityNanjing210023China Center for Excellence in Regional Atmos.Environ. Institute of Urban EnvironmentChinese Academy of SciencesXiamen 361021China

The gaseous or particulate forms of divalent mercury(HgⅡ) significantly impact the spatial distribution of atmospheric mercury concentration and deposition flux(FLX). In the new nested-grid GEOS-Chem model, we try to modify the HgⅡ gas-particle partitioning relationship with synchronous and hourly observations at four sites in China. Observations of gaseous oxidized Hg(GOM), particulate-bound Hg(PBM), and PM 2.5 were used to derive an empirical gas-particle partitioning coefficient as a function of temperature( T) and organic aerosol(OA) concentrations under different relative humidity(RH). Results showed that with increasing RH, the dominant process of HgⅡ gas-particle partitioning changed from physical adsorption to chemical desorption. And the dominant factor of HgⅡ gas-particle partitioning changed from T to OA concentrations. We thus improved the simulated OA concentration field by introducing intermediate-volatility and semi-volatile organic compounds(I/SVOCs) emission inventory into the model framework and refining the volatile distributions of I/SVOCs according to new filed tests in the recent literatures. Finally, normalized mean biases(NMBs) of monthly gaseous element mercury(GEM), GOM, PBM, WFLX were reduced from-33%–29%, 95%–300%, 64%–261%, 117%–122% to-13%–0%,-20%–80%,-31%–50%,-17%–23%. The improved model explains 69%–98% of the observed atmospheric Hg decrease during 2013–2020 and can serve as a useful tool to evaluate the effectiveness of the Minamata Convention on Mercury.

关键词： Nested GEOS-Chem model HgⅡgas-particle partitioning Organic aerosol Atmospheric mercury Mercury deposition flux

Numerical Simulation of the Relationship between the Width of Destressed Zone and Blasthole Depth

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Engineering（科研） 2020年第4期12卷 269-279页

作者： Jiansheng Tian qingru wu Zhijun Liu School of Mechanics & Civil Engineering China University of Mining & Technology Xuzhou China

Overstress in the surrounding rock of the roadway is a key reason that causes failures of deep roadways. Destressing blasting is one of the promising techniques that could improve the supporting quality. If the depth of the pressure relief blast hole is too shallow, the surrounding rock of the roadway will be broken or even collapsed. If the pressure relief blast hole is too deep, the pressure relief area will be located in the deep part of the surrounding rock of the roadway, which cannot achieve the purpose of releasing the stress in the shallow part of the surrounding rock and cause waste of the blast hole. The width or range of the pressure relief area should just fall in the high stress area of the surrounding rock of the roadway, so the pressure relief blast hole should have a reasonable depth. In order to quantitatively describe the relationship between borehole depth and the width of the stress relief zone, numerical simulations were carried out in ANSYS according to different borehole depths. The results show that the optimal destressing effect is achieved when borehole depth is 4 m. Peak stress of and is significantly reduced by 30.51% and 49.07% after blasting. Meanwhile, the high-stress area shifts about 4.8 m from the roadside to the depth of surrounding rock, thus a 3.8 m wide stress relief zone is formed around the roadside, thus, the aim of quantizing the effects of destress blasting is achieved.

关键词： Rock Burst Deep Roadway Supporting Width of Stress Relief Zone Destress Blasting Numerical Simulation

Minamata Convention on Mercury:Chinese progress and perspectives

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National Science Review 2017年第5期4卷 677-679页

作者： Yan Lin Shuxiao Wang Eirik Hovland Steindal Hua Zhang Huan Zhong Yindong Tong Zuguang Wang Hans Fredrik Veiteberg Braaten qingru wu Thorj?rn Larssen Norwegian Institute for Water Research State Key Joint Laboratory of Environment Simulation and Pollution Control School of Environment Tsinghua University Norwegian Environment Agency State Key Laboratory of Environmental Geochemistry Institute of GeochemistryChinese Academy of Sciences State Key Laboratory of Pollution Control and Resources Reuse School of the EnvironmentNanjing University School of Environmental Science and Engineering Tianjin University School of Environment & Natural Resources Renmin University of China

Mercury(Hg)is a global threat to human and environmental health[1].To address this global issue,the Minamata Convention on Mercury(MC)was agreed upon by 128 countries on 19January *** officially ratified the MC in Aug... 详细信息

关键词： Hg Minamata Convention on Mercury:Chinese progress and perspectives

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污酸处理过程的汞流向

环境工程学报 2017年第9期11卷 4965-4970页

作者：吴清茹王书肖惠霂霖清华大学环境学院环境模拟与污染控制国家重点联合实验室北京100084 国家环境保护大气复合污染来源与控制重点实验室北京100084

污酸是有色金属生产中汞的主要输出副产物。污酸处理过程的汞污染控制直接影响有色金属冶炼行业汞向水体的排放情况。选择6家有色金属冶炼企业开展污酸处理过程的汞流向研究。研究发现,测试冶炼厂污酸汞浓度分布在0.3~90μg·m L^(-1)... 详细信息

污酸是有色金属生产中汞的主要输出副产物。污酸处理过程的汞污染控制直接影响有色金属冶炼行业汞向水体的排放情况。选择6家有色金属冶炼企业开展污酸处理过程的汞流向研究。研究发现,测试冶炼厂污酸汞浓度分布在0.3~90μg·m L^(-1)范围内。污酸渣的汞浓度为73~26 354μg·g-1;锌厂1和铜厂1硫化渣的汞浓度分别为404 218μg·g-1和10 972μg·g-1。石膏渣的汞浓度普遍低于污酸渣和硫化渣的汞浓度。污酸处理过程,汞主要进入到各种处理渣中。测试冶炼厂污酸处理过程的脱汞效率为87.2%~99.9%。相对于石灰中和法和石灰铁盐法,中和硫化法和硫化-石灰铁盐法的脱汞效果相对稳定,且对低汞污酸有较高的脱汞效率。测试冶炼厂最终排放水的汞浓度分布在0.006~0.065μg·m L^(-1)的范围内,存在部分冶炼厂超标排放的情况。

关键词：有色金属冶炼污酸处理汞流向