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Photothermal properties of Cu@polycarbonate composites with strong localized surface plasmon resonances

Nano Research 2024年第9期17卷 8513-8520页

作者： Fengyi Wang Jiangling He Junshan Hu Zhihui Chen Yumeng Shi qing-hua xu SZU-NUS Collaborative Innovation Center for Optoelectronic Science and Technology International Collaborative Laboratory of 2D Materials for Optoelectronics Science and Technology of Ministry of EducationInstitute of Microscale OptoelectronicsShenzhen UniversityShenzhen 518060China Department of Chemistry National University of Singapore3 Science Drive 3Singapore 117543Singapore College of Materials Science and Engineering Sichuan UniversityChengdu 610065China

Copper is relatively low cost and highly abundant compared with the well-studied noble metals such as gold and ***,the poor plasmonic and high susceptibility towards oxidation limit the study of its optical properties and applications as ***,copper nanoparticles@polycarbonate(Cu@PC)composites were prepared by using a facile one-step solvothermal *** Cu@PC composites have strong localized surface plasmon resonances(LSPR)due to that the PC shell can induce the particles to form many-particles system with different particle numbers,which not only lead to overlap and hybridize of the LSPR modes,but also shift the LSPR away from the interband transitions,and the PC layer also prevents the oxidation of Cu *** photothermal conversion efficiency of Cu@PC composites reaches 41.1%under 808 nm continuous wave(CW)laser irradiation which is higher than previously reported Cu nanomaterials that have been ***,the composites also have high photothermal ***,interfacial evaporator is prepared by assembling the Cu@PC composites on scouring sponge as light absorption layer which has>92.8%absorption in entire solar spectrum *** seawater evaporation rate is 3.177 kg·m-2·h^(-1)with a E_(evaporator)/E_(water)of *** high evaporation rate interfacial evaporator with low cost,simple,and scalable approach shows great application value in the field of photothermal evaporation.

关键词： Cu nanoparticles localized surface plasmon resonances(LSPR) photothermal interfacial evaporation

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pH-responsive metal nanoparticles as high contrast theranostic agents for selective imaging and synergistic cancer therapy

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Science China Chemistry 2024年第9期67卷 3063-3070页

作者： Sichao Tian Xiaofeng He Xiao Wu Dongxue Hu qing-hua xu Department of Chemistry National University of Singapore National University of Singapore (Suzhou) Research Institute Institute of Medicinal Plant Development Chinese Academy of Medical Sciences and Peking Union Medical College Department of Biological Sciences Faculty of Science National University of Singapore

The low signal-to-noise ratio(S/N) and single functionality of fluorescence imaging agents have limited their practical applications. Bright two-photon excitation(2PE) imaging probes are highly desirable in vivo with larger imaging depth, minor autofluorescence background, and less photodamage. Herein, we developed responsive aggregated gold nanoparticles(Au NPs)as high contrast 2PE imaging agents, capable of emitting red fluorescence upon excitation of near-infrared(NIR) laser and possessing a high signal-to-noise ratio(S/N of 2,475). By forming aggregates in situ inside tumor tissue, doxorubicin hydrochloride(DOX)-loaded mix-charged gold nanoparticles(DOX-MC-Au NPs) were utilized to act as selective fluorescence imaging probes and precise therapy agents. These high-contrast theranostic agents offer a promising potential for precise cancer imaging and therapy, which might open a new venue to multifunctional and noninvasive theranostics.

关键词： metal nanoparticles two-photon excitation high contrast imaging agents fluorescence imaging cancer therapy

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Lambda polarization at the Electron-ion collider in China

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Nuclear Science and Techniques 2023年第10期34卷 117-125页

作者： Zhaohuizi Ji Xiao-Yan Zhao Ai-Qiang Guo qing-hua xu Jin-Long Zhang Institute of Frontier and Interdisciplinary Science Shandong UniversityQingdao 266237China Institute of Modern Physics of CAS Lanzhou 730000China Southern Center for Nuclear‑Science Theory(SCNT) Institute of Modern PhysicsChinese Academy of SciencesHuizhou 516000China

Lambda polarization can be measured through its self-analyzing weak decay, making it an ideal candidate for studying spin effects in high-energy scattering. In lepton-nucleon deep inelastic scattering(DIS), Lambda polarization measurements can probe polarized parton distribution functions(PDFs) and polarized fragmentation functions(FFs). One of the most promising facilities for high-energy nuclear physics research is the proposed Electron-ion collider in China(EicC). As a next-generation facility, EicC is set to advance our understanding of nuclear physics to new heights. In this article, we study the Lambda production in electron-proton collisions at the EicC energy, in particular the reconstruction of Lambda based on the performance of the designed EicC detector. In addition, taking spontaneous transverse polarization as an example, we provide a theoretical prediction with a statistical projection based on one month of EicC data, offering valuable insights into future research prospects.

关键词： Electron-ion collider in China Lambda polarization Polarizing fragmentation functions Nucleon structure

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Flower-like Au/Ag/TiO2 nanocomposites with enhanced photocatalytic efficiency under visible light irradiation

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Science China Chemistry 2017年第4期60卷 521-527页

作者： Fei Han Xin Mao qing-hua xu Department of Chemistry National University of Singapore Singapore 117543 Singapore National University of Singapore Nanoscience & Nanotechnology Initiative (NUSNNl)-Nanocore Singapore 117576 Singapore National University of Singapore (Suzhou) Research Institute Suzhou 215123 China

Uniform flower-like TiO_2 coated Au nanostars and core-shell Au@Ag natiostars with different amounts of Ag coating were prepared through a facile method by hydrolysis of TiF_4 under an acidic *** photocatalytic capability of these flower-like nanocomposites under visible light irradiation was found to be enhanced by up to 4.7-fold compared to commercial P25 TiO_2 *** enhanced photocatalytic activity was ascribed to improved light absorption and hot electron injection from the photo-excited Au@Ag core to the TiO_2 shell.

关键词：纳米复合材料可见光照射二氧化钛纳米银光催化效率 TiO2纳米粒子金光催化性能

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Identifying the risk factors for pancreatic fistula after laparoscopic pancreaticoduodenectomy in patients with pancreatic cancer

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World Journal of Gastrointestinal Surgery 2024年第6期16卷 1609-1617页

作者： Hang xu qing-Cai Meng Jie hua Wei Wang Department of Pancreatic Surgery Fudan University Shanghai Cancer CenterShanghai 200032China Department of Oncology Shanghai Medical CollegeFudan UniversityShanghai 200032China

BACKGROUND Laparoscopic pancreaticoduodenectomy(LPD)is a surgical procedure for treating pancreatic cancer;however,the risk of complications remains high owing to the wide range of organs involved during the surgery and the difficulty of *** fistula(PF)is a major complication that not only increases the risk of postoperative infection and abdominal hemorrhage but may also cause multi-organ failure,which is a serious threat to the patient’s *** study hypothesized the risk factors for PF after *** To identify the risk factors for PF after laparoscopic pancreatoduodenectomy in patients with pancreatic *** We retrospectively analyzed the data of 201 patients admitted to the Fudan University Shanghai Cancer Center between August 2022 and August 2023 who underwent LPD for pancreatic *** the basis of the PF’s incidence(grades B and C),patients were categorized into the PF(n=15)and non-PF groups(n=186).Differences in general data,preoperative laboratory indicators,and surgery-related factors between the two groups were compared and analyzed using multifactorial logistic regression and receiver-operating characteristic(ROC)curve *** The proportions of males,combined hypertension,soft pancreatic texture,and pancreatic duct diameter≤3 mm;surgery time;body mass index(BMI);and amylase(Am)level in the drainage fluid on the first postoperative day(Am>1069 U/L)were greater in the PF group than in the non-PF group(P24.91 kg/m²[odds ratio(OR)=13.978,95%confidence interval(CI):1.886-103.581],hypertension(OR=8.484,95%CI:1.22-58.994),soft pancreatic texture(OR=42.015,95%CI:5.698-309.782),and operation time>414 min(OR=15.41,95%CI:1.63-145.674)were risk factors for the development of PF after LPD for pancreatic cancer(all P<0.05).The areas under the ROC curve for BMI,

关键词： Pancreatic cancer Laparoscopy Pancreaticoduodenectomy Pancreatic fistula Risk factors Receiver-operating characteristic curve

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Polyfluorene based conjugated polymer nanoparticles for two-photon live cell imaging

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Science China Chemistry 2018年第1期61卷 88-96页

作者： Shuang Li Xiao-Fang Jiang qing-hua xu Institute of Polymer optoelectronic Materials and Devices State Key Laboratory of Luminescent Materials and Devices South China University of Technology Guangzhou 510640 China National University of Singapore (Suzhou) Research Institute Suzhou 215123 China Department of Chemistry National University of Singapore Singapore 117543 Singapore

Two-photon excitation microscopy(2 PEM) has been known as a noninvasive and powerful bio-imaging tool for studying living cells, intact tissues and living animals because of their unique advantages such as localized excitation, deep tissue penetration as well as less photo-damage. However, the major limitations that hinder its practical applications in biological systems are low two-photon absorption cross sections of conventional fluorescence probes. Conjugated polymer nanoparticles(CPNs) consisting of highly fluorescent conjugated polymers are promising fluorescent probes for 2 PEM due to their unique advantages including large two-photon absorption cross sections, high fluorescence quantum yield, good photo-stability and biocompatibility, facile chemical synthesis, tunable optical properties as well as versatile surface modifications. This account summarizes the recent efforts of our group on development of novel polyfluorene based CPNs as 2 PEM contrast agents for live cell imaging.

关键词： conjugated polymers nanoparticles two-photon absorption fluorescence microscopy bio-imaging

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Circ_0004592:An auxiliary diagnostic biomarker for gastric cancer

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World Journal of Gastrointestinal Oncology 2024年第6期16卷 2757-2768页

作者： Shan Kong Yan-hua xu Ming Zheng Shao-qing Ju Heng-Chuan Shi Department of Laboratory Medicine Jiangsu Province Official HospitalNanjing 210000Jiangsu ProvinceChina Department of Laboratory Medicine Northern Jiangsu People’s HospitalYangzhou 225000Jiangsu ProvinceChina Department of Laboratory Medicine The Affiliated Hospital of Nantong UniversityNantong 226001Jiangsu ProvinceChina

BACKGROUND Gastric cancer(GC)has a high mortality rate,and robust diagnostic biomarkers are currently ***,the clinical relevance of circular RNAs(circRNAs)as GC biomarkers remains largely *** To evaluate the potential of novel circRNA circ_0004592 in the early screening and prognosis of *** High-throughput sequencing of circRNAs was performed to screen for potential target ***_0004592 expression was examined in GC tissues,cells,and *** samples were collected from healthy subjects’patients,as well as from patients with benign lesions,precancerous lesions,and GC,whereafter the diagnostic accuracy of circ_0004592 was *** correlation between circ_0004592 levels in plasma and clinicopathological data of patients with GC was further *** Circ_0004592 was upregulated in both the tissue and plasma of patients with ***,circ_0004592 expression was higher in patients with precancerous lesions than in healthy controls while being highest in patients with *** the same patient,the postoperative plasma level of circ_0004592 was lower than that in the preoperative ***,circ_0004592 level was significantly correlated with tumor differentiation,tumor depth,and lymph node *** area under the curve(AUC)of plasma circ_0004592 exhibited high sensitivity and specificity for differentiating patients with GC from healthy *** based on circ_0004592,carcinoembryonic antigen,and cancer antigen 199 achieved a superior AUC and was highly *** Plasma circ_0004592 may represent a potential non-invasive auxiliary diagnostic biomarker for patients with GC.

关键词： Biomarker Circular RNA Diagnosis Gastric cancer Plasma

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Escape probability for isotropic emitters near Kerr black hole with astrometric

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Communications in Theoretical Physics 2024年第5期76卷 128-133页

作者： Yu-xuan Han qing-hua Zhu qing-Guo huang CAS Key Laboratory of Theoretical Physics Institute of Theoretical PhysicsChinese Academy of SciencesBeijing 100190China School of Physical Sciences University of Chinese Academy of SciencesNo.19A Yuquan RoadBeijing 100049China Department of Physics Chongqing UniversityChongqing 401331China School of Fundamental Physics and Mathematical Sciences Hangzhou Institute for Advanced Study UCASHangzhou 310024China

The paper investigates the escape probability for isotropic emitters near a Kerr black *** propose a new approach to obtain the escape probability in a general manner,going beyond previous case-by-case *** approach is based on studies of the black hole shadow with astrometric observable and can be applied to emitters with an arbitrary 4-velocities and locations,even to the emitters outside of the equatorial *** also consider representative examples illustrating how escape probabilities vary with distance,velocity,and inclination ***,this new approach provides an effective method for studying escape probabilities near Kerr black holes.

关键词： Kerr black hole photon escape probability isotropic emitters

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On the Fekete and Szego Problem for Starlike Mappings of Order α

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Acta Mathematica Sinica,English Series 2017年第4期33卷 554-564页

作者： qing hua xu Fang FANG Tai Shun LIU College of Mathematics and Information Science JiangXi Normal University Nanchang 330022 P. R. China Department of Mathematics Huzhou University Huzhou 313000 P. R. China

Let Sα*be the familiar class of normalized starlike functions of order α in the unit disk. In this paper, we establish the Fekete and Szeg? inequality for the class Sα*, and then we generalize this result to the un... 详细信息

关键词： Fekete–Szego problem starlike mappings of order α sharp coefficient bound

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Aldehyde oxidase mediated enantioselective metabolic health risk of dinotefuran

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Science China Chemistry 2024年第6期67卷 2079-2091页

作者： Liwei xu Xinxin xu hua Kuang Chuanlai xu Xiaoling Wu State Key Laboratory of Food Science and Resources Jiangnan UniversityWuxi214122China International Joint Research Laboratory for Biointerface and Biodetection and School of Food Science and Technology Jiangnan UniversityWuxi214122China Collaborative Innovation center of Food Safety and Quality Control in Jiangsu Province Jiangnan UniversityWuxi214122China

Chiral pollutants often pose significant differential environmental health *** this study,the biotransformation of chiral dinotefuran(DIN)and its enantioselective metabolic toxicity mechanisms have been systemically ***,reversedphase chromatography-high resolution mass spectrometry was developed to quantify the content of DIN R/S chiral enantiomer with pg level sensitivity,revealing a lower elimination rate constant(K_(e))of S-DIN(0.730 h^(-1))than R-DIN(0.746 h^(-1)).Secondly,the interaction mechanism between DIN metabolism and important endogenous bioactive molecules,such as aldehyde oxidase(AOX)and neurotransmitters,was *** DIN nitro-group was converted into a guanidine group by the reducing site of nearby flavin adenine dinucleotide(FAD)in AOX with the preferred higher affinity of ***,the endogenous tryptophan(Trp)aldehyde metabolic intermediate,5-hydroxyindoleacetaldehyde(5-HIAL),provides a persistent electron donor for DIN reduction via the oxidation-catalyzed site in AOX,resulting in remarkable up-regulation of monoamine neurotransmitters such as serotonin and ***,the higher level of neurotransmitters further mediated dysregulation of oxylipin homeostasis via the serotonergic pathway,where S-DIN exhibited more pronounced liver lipid damage and environmental health risk with the accumulated lipid biomarkers,oxidized triglyceride(OxTG)and oxidized sphingomyelin(OxSM).This study elucidates the AOX-mediated enantioselectivity metabolic pathway of DIN,providing a new analytical method for chiral pollutants and paves the way for their health risk assessments.

关键词： neonicotinoid dinotefuran enantiomer aldehyde oxidase metabolomics health risk

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