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Arsenic and fluoride co-enrichment of groundwater in the loess areas and associated human health risks:A case study of Dali County in the Guanzhong Basin

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China Geology 2024年第3期7卷 445-459页

作者： Rui-ping Liu Fei Liu hua-qing chen Yu-ting Yang hua Zhu You-ning Xu Jian-gang Jiao Refaey M El-Wardany Xi'an Center China Geological SurveyMinistry of Natural ResourcesXi'an 710054China Observation and Research Station of Environmental Geology of Typical Mines in Shaanxi Province MNRXi'an 710054China Key Laboratory for Geo-hazards in Loess Area MNRXi'an 710054China Dalian Ocean and Fishery Comprehensive Administration Supervision Lochus Dalian 116000China Pingliang City Development and Reform Commission Pingliang 744000China School of Earth Science and Resources Chang’an UniversityXi'an 710054China Faculty of Science Al-Azhar UniversityAssiut 71524Egypt

This study aims to reveal the occurrence and origin of typical groundwater with high arsenic and fluoride concentrations in the loess area of the Guanzhong Basin—a Neogene faulted *** findings are as follows:(1)Groundwater samples with high arsenic and fluoride concentrations collected from the loess area and the terraces of the Weihe River accounted for 26%and 30%,respectively,of the total samples,with primary hydrochemical type identified as HCO_(3)-*** karst and sand areas exhibit relatively high groundwater quality,serving as preferred sources for water *** is recommended that local governments fully harness groundwater in these areas;(2)groundwater with high arsenic and fluoride concentrations in the loess area and the alluvial plain of rivers in Dali County is primarily distributed within the Guanzhong Basin,which represents the drainage zone of groundwater;(3)arsenic and fluoride in groundwater originate principally from natural and anthropogenic sources;(4)the human health risk assessments reveal that long-term intake of groundwater with high arsenic and fluoride concentrations pose cancer or non-cancer risks,which are more serious to kids compared to *** study provides a theoretical basis for the prevention and treatment of groundwater with high arsenic and fluoride concentrations in loess areas.

关键词： Arsenic Fluoride Groundwater Cancer risk Kid and adult Human health risk assessment Hydrogeological survey engineering Environmental geological survey engineering Loess areas

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Synthesis and characterization ofα-{3-[(2,3-dihydroxy) propoxy]propyl}-ω-butylpolydimethylsiloxanes

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Chinese Chemical Letters 2009年第6期20卷 729-732页

作者： Xiao Li Zhan Zhen huan Luo qing hua Zhang Bi chen Feng Qiu chen Department of Chemical and Biochemical Engineering. Zhejiang University Hangzhou 310027 China

Hydrosilylation has been carried out between Si-H terminated polydimethylsiloxanes with narrow molecular weight distribution and protected 3-allyloxy-l,2-propanediol, and after subsequently alcoholyzed, α-{3-[（2,3-dihydroxy）propoxy]propyl}-ω- butyl-polydimethylsiloxanes with varying number of （（Si（CH3）2-O） unit were obtained. At each step, the produced compounds were carefully characterized. The results showed that each step was successfully carried out and target products were achieved.

关键词： Polydimethylsiloxane Anionic ring-opening polymerization Hydrosilylation Alcoholysis

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Studies on New Additions to 5-Methoxy-2 (5H)-Furanone: 1, 4-Addition of Grignard Reagents, and 1,3-Dipolar Cycloaddition of Silyl Nitronates

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Chinese Chemical Letters 2001年第4期12卷 293-296页

作者： Zhao Yang WANG Jia Ling CUI Bao Shan DU qing hua chen Department of Chemistry Beijing Normal UniversityBeijing 100875 Dept.of Chem. South China Nor.UnivGuangzhou 510631 Present address:School of Pharm. Beijing UnivBeijing 100033

1,4-Addition reaction of Grignard's reagent to 5-methoxy-2(5H)-furanone 1 was accomplished. which provided a new possible route for synthesizing beta -alkyl-Y-alkyloxy-Y-butyrolactone. A novel concise method of prepar... 详细信息

关键词： Michael addition Grignard reagent 1 3-dipolar cycloaddition silyl nitronates.

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Asymmetric Photocatalyzed Addition of Cyclic Ammes to the Chiral 5-(l)-Menthyloxy-2(5H)-furanone

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Chinese Chemical Letters 1999年第11期10卷 889-892页

作者： Zhao Yang WANG Tian Ying JIAN qing hua chen(Department of Chemistry,Beijing Normal University, Beijing 100875) Department of Chemistry Beijing Normal University Beijing 100875 China

The benzophenone-initiated photoaddition of N-methyl ammes 2 to the chiral synthon1 proceeds in a regiospecitlc and highlyr stereocontrolled thshion to give the C-C photoadductscontaining a ne\viy stereogenic center 3a-3c. The enantiomerically pure N-C photoadducts, aminobutenolides 5a-5c have been obtained from the enantioselective photoaddition of secondary cyclicammes 4 with the chiral synthon 1 under the same conditions.

关键词： Asymmetric photocatalysed conjugate addition enantiomerically pure C-Cphotoadducts. secondary cyclic amine enantiomerically pure N-C photoaducts.

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A Novel Synthesis of Isoxazole Derivatives

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Chinese Chemical Letters 1998年第9期9卷 801-802页

作者： Jun Feng WANG Bao Shan DU qing hua chen (Department of Chemistry, Beijing Normal University, Beijing 100875) Beijing Normal Univ Dept Chem Beijing 100875 Peoples R China

The new synthetic method of isoxazole derivatives was succesfully achieved. The experimental results demonstrate that thermal decomposition reactions of nitrone could take place with yields of 41 similar to 81%, to gi... 详细信息

关键词： nitrone isoxazole

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Sn-doped induced stable 1T-WSe_(2)nanosheets entrenched on N-doped carbon with extraordinary half/full sodium/potassium storage performance

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Rare Metals 2023年第5期42卷 1557-1569页

作者： Yan-Ru Liu Ze-Wei Lei Ren-Ping Liu Xin-Ye Li Pei-Xun Xiong Yong-Jin Luo qing-hua chen Ming-Deng Wei Ling-Xing Zeng qing-Rong Qian College of Life Science Fujian Normal UniversityFuzhou350007China Engineering Research Center of Polymer Green Recycling of Ministry of Education College of Environment and ResourcesCollege of Carbon Neutral Modern IndustryFujian Normal UniversityFuzhou350007China Fujian Key Laboratory of Pollution Control and Resource Reuse Fuzhou350007China Fujian Provincial Key Laboratory of Electrochemical Energy Storage Materials Fuzhou UniversityFuzhou350002China Key Laboratory of Advanced Energy Materials Chemistry Ministry of EducationCollege of ChemistryNankai UniversityTianjin300071China

At present,there have been some reports on the application of metal phase selenide(1T-MSe_(2))in the field of energy *** this manuscript,a stable Sn-doped metal phase tungsten selenide(1T-WSe_(2)-Sn)was elaborately fabricated in situ by a simple calcination technique.N-doping was introduced by employing chitosan as precursor and nanoreactor,the Sn-doping induces 1T phase of WSe_(2)and enlarges the layer space to promote the electron/ion transport and structural *** optimized 1T-WSe_(2)-Sn electrode delivers prominent cycling lifespan(285 mAh·g^(-1)at 1.0 A·g^(-1)after 900 cycles)along with decent rate capability when applied as an anode of sodium ion batteries(SIBs).The specific capacity was determined to be of 460 mAh·g^(-1)at 0.1 A·g^(-1)after *** also displays superior capacity of 183 mAh·g^(-1)at0.5 A·g^(-1)for 200 cycles when paired with Na_(3)V_(2)(PO_(4))_(3)*** as the anode for potassium ion batteries(PIBs),it exhibits a satisfactory specific capacity of 345mAh·g^(-1)at 0.1 A·g^(-1)after 50 cycles.

关键词： WSe_(2) Sn-doped Metal phase Sodium/potassium storage

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Safflower Yellow Inhibits Progression of Hepatocellular Carcinoma by Modulating Immunological Tolerance via FAK Pathway

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Chinese Journal of Integrative Medicine 2024年第4期30卷 339-347页

作者： JI hua-feng YANG Zi-qiang HAN Jun-jun LI He-fang JIN Zhao-qing chen Wei-qing chen Fei-hua GONG Mou-chun Department of General Surgery First People's Hospital of Hangzhou Lin'an DistrictHangzhou(311300)China

Objective To explore the anti-tumor effect of safflower yellow(SY)against hepatocellular carcinoma(HCC)and the underlying potential *** An in vitro model was established by mixing Luc-Hepa1-6 cells and CD3^(+)CD8^(+)T cells,followed by adding programmed cell death protein 1(PD-1)antibody(Anti-mPD-1)with or without *** apoptosis was detected by flow cytometry and the level of inflammatory cytokines was determined by enzyme-linked immunosorbent *** protein levels of programmed cell death 1 ligand 1(PD-L1),chemokine ligand(CCL5),C-X-C motif chemokine ligand 10(CXCL10)were measured by Western *** in situ animal model was established in mice followed by treatment with anti-mPD-1 with or without *** imaging was monitored with an AniView 100 imaging *** establish the FAK-overexpressed Luc-Hepa1-6 cells,cells were transfected with adenovirus containing pcDNA3.1-FAK for 48 *** The fluorescence intensity,apoptotic rate,release of inflammatory cytokines,and CCL5/CXCL10 secretion were dramatically facilitated by anti-mPD-1(P<0.01),accompanied by an inactivation of PD-1/PD-L1 axis,which were extremely further enhanced by SY(P<0.05 or P<0.01).Increased fluorescence intensity,elevated percentage of CD3+CD8+T cells,facilitated release of inflammatory cytokines,inactivated PD-1/PD-L1 axis,and increased CCL5/CXCL10 secretion were observed in Anti-mPD-1 treated mice(P<0.01),which were markedly enhanced by SY(P<0.05 or P<0.01).Furthermore,the enhanced effects of SY on inhibiting tumor cell growth,facilitating apoptosis and inflammatory cytokine releasing,suppressing the PD-1/PD-L1 axis,and inducing the CCL5/CXCL10 secretion in Anti-mPD-1 treated mixture of Luc-Hepa1-6 cells and CD3+CD8+T cells were abolished by FAK overexpression(P<0.01).Conclusion SY inhibited the progression of HCC by mediating immunological tolerance through inhibiting FAK.

关键词： hepatocellular carcinoma safflower yellow Chinese medicine tumor microenvironment programmed cell death protein 1 focal adhesion kinase

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Photothermal properties of Cu@polycarbonate composites with strong localized surface plasmon resonances

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Nano Research 2024年第9期17卷 8513-8520页

作者： Fengyi Wang Jiangling He Junshan Hu Zhihui chen Yumeng Shi qing-hua Xu SZU-NUS Collaborative Innovation Center for Optoelectronic Science and Technology International Collaborative Laboratory of 2D Materials for Optoelectronics Science and Technology of Ministry of EducationInstitute of Microscale OptoelectronicsShenzhen UniversityShenzhen 518060China Department of Chemistry National University of Singapore3 Science Drive 3Singapore 117543Singapore College of Materials Science and Engineering Sichuan UniversityChengdu 610065China

Copper is relatively low cost and highly abundant compared with the well-studied noble metals such as gold and ***,the poor plasmonic and high susceptibility towards oxidation limit the study of its optical properties and applications as ***,copper nanoparticles@polycarbonate(Cu@PC)composites were prepared by using a facile one-step solvothermal *** Cu@PC composites have strong localized surface plasmon resonances(LSPR)due to that the PC shell can induce the particles to form many-particles system with different particle numbers,which not only lead to overlap and hybridize of the LSPR modes,but also shift the LSPR away from the interband transitions,and the PC layer also prevents the oxidation of Cu *** photothermal conversion efficiency of Cu@PC composites reaches 41.1%under 808 nm continuous wave(CW)laser irradiation which is higher than previously reported Cu nanomaterials that have been ***,the composites also have high photothermal ***,interfacial evaporator is prepared by assembling the Cu@PC composites on scouring sponge as light absorption layer which has>92.8%absorption in entire solar spectrum *** seawater evaporation rate is 3.177 kg·m^(-2)·h^(-1)with a E_(evaporator)/E_(water)of *** high evaporation rate interfacial evaporator with low cost,simple,and scalable approach shows great application value in the field of photothermal evaporation.

关键词： Cu nanoparticles localized surface plasmon resonances(LSPR) photothermal interfacial evaporation

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Thermodynamic transport mechanism of water freezing-thawing in the vadose zone in the alpine meadow of the Tibet Plateau

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Journal of Groundwater Science and Engineering 2022年第3期10卷 302-310页

作者： Gang Qiao Feng-dan Yu Wen-ke Wang Jun Zhang hua-qing chen Key Laboratory of Groundwater and Ecology in Arid and Semi-arid CGSXi’an 710054China Observation and Research Station of Groundwater and Ecology in Yulin Shaanxi DNRYulin 719053Shaanxi ProvinceChina School of Water Conservancy and Environment Chang’an UniversityXi’an 710054China

High altitude,cold and dry climate,strong solar radiation,and high evapotranspiration intensity have created an extremely fragile ecological and geological environment on the Tibet *** the heat in the vadose zone is primarily generated by the external solar radiation energy,and evapotranspiration is contingent on the consumption of vadose heat,the intensity of evapotranspiration is associated with the intensity of solar radiation and the heat budget in the vadose ***,the spatial and temporal variation of heat budget and thermodynamic transfer process of the vadose zone in the frigid region are not clear,which hinders the revelation of the dynamic mechanism of evapotranspiration in the vadose zone in the frigid *** the moisture content of the vadose zone in the alpine regions being the research object,the paper conducts in-situ geothermal observation tests,takes meteorological characteristics into consideration,and adopts the method of geothermal gradient and numerical computation to analyse the temporal and spatial variation rule of heat budget and thermodynamic transmission process of the vadose zone in the high and cold *** results show there is a positive correlation between air temperature,ground temperature,and water content of the vadose zone in both thawing and freezing *** to the change law of geothermal gradient,the thermodynamic transfer process of the vadose zone has four stages:slow exothermic heating,fast endothermic melting,slow endothermic cooling,and fast exothermic *** the surface down,the moisture freezing rate of the vadose zone is slightly higher than the melting *** is of great significance for understanding the evapotranspiration dynamic process of the vadose zone and protecting and rebuilding the ecological and geological environment in the high and cold regions.

关键词： Freeze-thaw action Thermodynamic Evapotranspiration Moisture in the vadose zone Tibet plateau

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Escape probability for isotropic emitters near Kerr black hole with astrometric

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Communications in Theoretical Physics 2024年第5期76卷 128-133页

作者： Yu-Xuan Han qing-hua Zhu qing-Guo huang CAS Key Laboratory of Theoretical Physics Institute of Theoretical PhysicsChinese Academy of SciencesBeijing 100190China School of Physical Sciences University of Chinese Academy of SciencesNo.19A Yuquan RoadBeijing 100049China Department of Physics Chongqing UniversityChongqing 401331China School of Fundamental Physics and Mathematical Sciences Hangzhou Institute for Advanced Study UCASHangzhou 310024China

The paper investigates the escape probability for isotropic emitters near a Kerr black *** propose a new approach to obtain the escape probability in a general manner,going beyond previous case-by-case *** approach is based on studies of the black hole shadow with astrometric observable and can be applied to emitters with an arbitrary 4-velocities and locations,even to the emitters outside of the equatorial *** also consider representative examples illustrating how escape probabilities vary with distance,velocity,and inclination ***,this new approach provides an effective method for studying escape probabilities near Kerr black holes.

关键词： Kerr black hole photon escape probability isotropic emitters

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