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Accelerated reconstruction of ZIF-67 with significantly enhanced glucose detection sensitivity

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Nano Research 2024年第6期17卷 4737-4743页

作者： Huihui Jin weihao Zeng wei qian Lun Li Pengxia Ji Zhengying Li Daping He School of Information Engineering Wuhan University of TechnologyWuhan 430070China Hubei Engineering Research Center of RF-Microwave Technology and Application Wuhan University of TechnologyWuhan 430070China State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan 430070China

Research on metal-organic framework(MOF)-based non-enzymatic glucose sensors usually ignores the impact of the surface reconstruction degree of MOF on the activity of catalyzing glucose *** this work,we choose zeolitic imidazolate framework-67(ZIF-67),which is commonly used in glucose sensing,as a representative to investigate the influence of reconstruction degree on its structure and glucose catalytic *** employing the electrochemical activation strategy,the activity of ZIF-67 in catalyzing glucose gradually increased with the prolongation of the activation time,reaching the optimum after 2 h *** detection sensitivity of the activated ZIF-67 was 19 times higher than that of the initial ZIF-67,and the limit of detection(LOD)was lowered from 7 to 0.4μ*** findings demonstrate that the oxidation degree of ZIF-67 deepened rapidly with continuously activation and was basically reconstructed to CoOOH after 2 h activation,accompanied by a morphological change from cuboctahedral to ***,theoretical investigation revealed that ZIF-67 is not suitable as a stable glucose sensor electrode since the adsorbed glucose molecules hasten the dissociation of ligands and the breaking of Co-N bond in ***,our work has important implications for the rational design of next-generation MOF-based glucose sensors.

关键词： zeolitic imidazolate framework-67(ZIF-67) glucose oxidation electrochemical activation reconstruction CoOOH

Advanced Electrical Motors and Control Strategies for High-quality Servo Systems-A Comprehensive Review

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Chinese Journal of Electrical Engineering 2024年第1期10卷 63-85页

作者： Ming Cheng Jiawei Zhou wei qian Bo Wang Chenchen Zhao Peng Han School of Electrical Engineering Southeast UniversityNanjing 210096China ESTUN Automation Co. Ltd.Nanjing 211106China Ansys Inc.San JoseCA 95134USA

Recent technological advancements have propelled remarkable progress in servo systems,resulting in their extensive utilization across various high-end applications.A comprehensive review of high-quality servo system technologies,focusing specifically on electrical motor topologies and control strategies is *** terms of motor topology,this study outlines the mainstream servo motors used across different periods,as well as the latest theories and technologies surrounding contemporary servo *** terms of control strategies,two well-established approaches are presented:field-oriented control and direct torque ***,it discusses advanced control strategies employed in servo systems,such as model predictive control(MPC)and fault tolerance control,among others.

关键词： Servo system servo motor control strategy magnetic field modulation

Scalable graphene foam with ultrahigh conductivity for stabilizing Pt towards efficient hydrogen evolution

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Nano Research 2024年第8期17卷 6968-6976页

作者： Ming Zhao Meng Huang Huihui Jin Dayin He wei qian Zixin Zhang Daping He State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan 430070China Hubei Engineering Research Center of RF-Microwave Technology and Application Wuhan University of TechnologyWuhan 430070China School of Information Engineering Wuhan University of TechnologyWuhan 430070China School of Chemistry and Materials Science University of Science and Technology of ChinaHefei 230026China Sanya Science and Education Innovation Park of Wuhan University of Technology Sanya 572000China

For the carbon-based catalyst to be active and stable,especially in harsh electrochemical environments,the key is to decrease the concentration of defects and raise the degree of graphitization of the carbon ***,we develop a highly graphitized graphene foam with multiplicated structure to fabricate self-supporting Pt-based catalysts for efficient and stable hydrogen evolution reaction(HER)*** foam(GO-2850)is obtained through an ultra-high temperature treatment at 2850℃,with perfect graphene structure and extremely low defect,ensuring high electrical conductivity and corrosion ***,its multiplicated structure provides an inherently favorable environment for the dispersion of Pt nanoparticles(Pt NPs)and offers abundant channels for electrolyte infiltration during the catalytic *** a result,the as-prepared Pt/GO-2850 is far active and stable than the Pt NPs supported on commercial carbon paper(Pt/CP)counterpart toward catalyzing HER,exhibiting an outstanding activity and long-term durability(300 h@10 mA·cm^(−2))in acidic/alkaline/seawater *** can be attributed to the stronger interaction between the lower-defect GO-2850 substrate and Pt,as evidenced by characterization and theoretical *** work extends further insight into the design self-supporting catalysts of high activity and stability with promising prominent application toward green energy devices.

关键词： graphene foam high graphitization Pt nanoparticles hydrogen evolution reaction long-term stability

Characteristics of biomass ashes from different materials and their ameliorative effects on acid soils

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Journal of Environmental Sciences 2017年第5期29卷 294-302页

作者： Renyong Shi Jiuyu Li Jun Jiang Khalid Mehmood Yuan Liu Renkou Xu wei qian State Key Laboratory of Soil and Sustainable Agriculture Institute of Soil Science Chinese Academy of Sciences Nanjing 210008 China. University of Chinese Academy of Sciences Beijing 100049 China

The chemical characteristics,element contents,mineral compositions,and the ameliorative effects on acid soils of five biomass ashes from different materials were analyzed. The chemical properties of the ashes varied depending on the source biomass material. An increase in the concrete shuttering contents in the biomass materials led to higher alkalinity,and higher Ca and Mg levels in biomass ashes,which made them particularly good at ameliorating effects on soil acidity. However,heavy metal contents,such as Cr,Cu,and Zn in the ashes,were relatively high. The incorporation of all ashes increased soil p H,exchangeable base cations,and available phosphorus,but decreased soil exchangeable acidity. The application of the ashes from biomass materials with a high concrete shuttering content increased the soil available heavy metal contents. Therefore,the biomass ashes from wood and crop residues with low concrete contents were the better acid soil amendments.

关键词： Biomass ashes Raw materials Element composition Chemical properties Amelioration of acidic soils Available heavy metals

Restudy on Time-Evolution of SUSY Dark Matter

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Communications in Theoretical Physics 2002年第10期38卷 503-508页

作者： FENG Tai-Fu LI Xue-qian MENG Qing-wei REN Zhen-Yu Institutc of High Energy Physics Academia Sinica P.O. Box 918-4 Beijing 100039 China CCAST World Lab P.O. Box 8730 Beijing 100080 China Department of Physics Nankai University Tianjin 300071 China Department of Physics Nankai University Tianjin 300071 China Institutc of High Energy Physics Academia Sinica P.O. Box 918-4 Beijing 100039 China Department of Physics Nankai University Tianjin 300071 China

We restudy the Lee-weinberg time-evolution equation including the R-parity violation. We carefullyanalyze the intluence of the boundary conditions, equation of state, SUSY parameters, especially the R-parity violation,and other factors on the time-evolution of the SUSY cold dark matter. Our numerical results show that without Rparity violation, only two ranges 20 ＜ mx01 ＜ 30 GeV and 75 ＜ mx01 ＜ 110 GeV can be consistent with data, if30 ＜ mx01 ＜ 75 GeV, there must be at least two kinds of heavy particles contributing to the cold dark matter. However,with the R-parity violation, the heavy neutralino can be dark matter constituent, but it must decay and the R-parityviolation parameter is constrained by the present data.

关键词： SUSY dark matter, time evolution

Recent advances in nanotherapeutics for the treatment of burn wounds

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Burns & Trauma 2021年第1期9卷 220-239页

作者： Rong Huang Jun Hu wei qian Liang Chen Dinglin Zhang Department of Chemistry College of Basic MedicineThird Military Medical University(Army Medical University)Chongqing 400038China Department of Neurology Southwest HospitalThird Military Medical University(Army Medical University)Chongqing 400038China Institute of Burn Research Southwest HospitalThird Military Medical University(Army Medical University)Chongqing 400038China Department of plastic surgery Southwest HospitalThird Military Medical University(Army Medical University)Chongqing 400038China State Key Laboratory of Trauma Burn and Combined InjuryChongqing400038China

Moderate or severe burns are potentially devastating injuries that can even cause death,and many of them occur every *** prevention,anti-inflammation,pain management and administration of growth factors play key roles in the treatment of burn *** therapeutic strategies under development,such as nanotherapeutics,are promising prospects for burn wound ***,including metallic and polymeric nanoformulations,have been extensively developed to manage various types of *** human and animal studies have demonstrated that nanotherapeutics are biocompatible and effective in this ***,we provide comprehensive knowledge of and an update on the progress of various nanoformulations for the treatment of burn wounds.

关键词： Burn wounds Metal and metal oxide nanotherapeutics Polymeric nanotherapeutics Therapeutic mechanism Wound healing

New Insights into Nested Long Terminal Repeat Retrotransposons in Brassica Species

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Molecular Plant 2013年第2期6卷 470-482页

作者： Lijuan wei Meili Xiaoa Zeshan An Bi Ma Annaliese S. Mason wei qian Jiana Li Donghui Fu Chongqing Engineering Research Center for Rapeseed College of Agronomy and Biotechnology Southwest University Chongqing 400716 China School of Agriculture and Food Sciences and centre for Integrative I~egume-Research The University of Queensland 1:he Universit'y of QueenslandBrisbane 4072 Australia Key Laboratory of Crop Physiology Ecology and Genetic Breeding Ministry of Education Agronomy College Jiangxi Agricultural University Nanchang330045 China

Long terminal repeat （LTR） retrotransposons, one of the foremost types of transposons, continually change or modify gene function and reorganize the genome through bursts of dramatic proliferation. Many LTR-TEs preferen-tially insert within other LTR-TEs, but the cause and evolutionary significance of these nested LTR-TEs are not well under-stood. In this study, a total of 1.52 Gb of Brassica sequence containing 2020 bacterial artificial chromosomes （BACs） was scanned, and six bacterial artificial chromosome （BAC） clones with extremely nested LTR-TEs （LTR-TEs density： 7.24/kb） were selected for further analysis. The majority of the LTR-TEs in four of the six BACs were found to be derived from the rapid proliferation of retrotransposons originating within the BAC regions, with only a few LTR-TEs originating from the proliferation and insertion of retrotransposons from outside the BAC regions approximately 5-23 Mya. LTR-TEs also pref-erably inserted into TA-rich repeat regions. Gene prediction by Genescan identified 207 genes in the 0.84Mb of total BAC sequences. Only a few genes （3/207） could be matched to the Brassica expressed sequence tag （EST） database, indicating that most genes were inactive after retrotransposon insertion. Five of the six BACs were putatively centromeric. Hence, nested LTR-TEs in centromere regions are rapidly duplicated, repeatedly inserted, and act to suppress activity of genes and to reshuffle the structure of the centromeric sequences. Our results suggest that LTR-TEs burst and proliferate on a local scale to create nested LTR-TE regions, and that these nested LTR-TEs play a role in the formation of centromeres.

关键词： LTR retrotransposons Brassica centromere retrotransposon-rich transposon burst.

Influence of injection temperature and flow rate on mixing and stratification in small passively cooling enclosures

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Nuclear Science and Techniques 2016年第4期27卷 104-114页

作者： wei-qian Zhuo Feng-Lei Niu Jun-Chi Cai Xiao-wei Su Ying-Qiu Hu Yun-Gan Zhao Yu Yu Beijing Key Laboratory of Passive Nuclear Power Safety and Technology North China Electric Power University

Thermal mixing and stratification phenomena may occur during the loss of a coolant accident or main steam line break accident in the containment of a Passive Containment Cooling System, or in the suppression pools in BWR. However, the present study pays insufficient attention to the thermal stratification phenomena in the containment of small modular reactors(SMR). In this paper, an investigation on the mixing and thermal stratification phenomena caused by the plumes or buoyant jets in SMR containments was carried out. The experiments were both conducted under non-adiabatic and adiabatic conditions for a steel containment. In each condition, two key parameters, inlet temperature, and flow rate were tested by controlling variables to identify their influence on the thermal stratification phenomenon. The visualization experiments illustrated the jet mixing and stratification development. The experiment results were compared with the numerical computation and they reached a good agreement.

关键词：热混合被动冷却注射温度流量可视化实验分层现象机箱主蒸汽管道

In situ synthesis of porous Pt-Pd bimetallic structures for sweat glucose biosensing using dynamic hydrogen bubble template method

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Rare Metals 2024年第7期43卷 3408-3414页

作者： Yi-Wen Guo qian-Hui wei Fei wei Hao Liu Hong-Bin Zhao Dong Wang Hai-Ling Tu State Key Laboratory of Advanced Materials for Smart Sensing China GRINM Group Co.Ltd.Beijing 100088China Department of Advanced Electronic Materials GRIMAT Engineering Institute Co.Ltd.Beijing 101407China General Research Institute for Nonferrous Metals Beijing 100088China GRINM(Guangdong)Institute for Advanced Materials and Technology Foshan 528000China School of Chemical Engineering Northeast Electric Power UniversityJilin 132012China

For the practical application of sweat glucose biosensors,it is crucial to develop a method for modifying the working electrode with noble metals that ensures strong *** this study,we synthesized porous Pt-Pd bimetall... 详细信息

关键词： method bubble porous