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On a Nonlocal Problem Modelling Ohmic Heating in Planar Domains

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Acta Mathematica Sinica,English Series 2013年第3期29卷 523-534页

作者： Fei LIANG qi lin liu Yu Xiang LI School of Mathematics and Physics Xi'an University of Science and Technology Xi'an 710054 P. R. China Department of Mathematics Anhui Science and Technology University Fengyang 233100 P. R. China Department of Mathematics Southeast University Nanjing 210096 P. R. China

In this paper, we consider the nonlocal problem of the formand the associated nonlocal stationary problemwhere λ is a positive parameter. For Ω to be an annulus, we prove that the nonlocal stationary problem has a unique solution if and only if λ 〈 2｜Ω｜2, and for λ = 2｜Ω｜2, the solution of the nonlocal parabolic problem grows up globally to infinity as t→∞.

关键词： Nonlocal elliptic problems nonlocal parabolic problems blow-up in infinite time

Hybrid pedestrian positioning system using wearable inertial sensors and ultrasonic ranging

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Defence Technology（防务技术） 2024年第3期33卷 327-338页

作者： lin qi Yu liu Chuanshun Gao Tao Feng Yue Yu School of Communication and Information Engineering Chongqing University of Posts and TelecommunicationsChongqing 400065China Department of Land Surveying and Geo-Informatics The Hong Kong Polytechnic UniversityHong Kong 999077China

Pedestrian positioning system(PPS)using wearable inertial sensors has wide applications towards various emerging fields such as smart healthcare,emergency rescue,soldier positioning,*** performance of traditional PPS is limited by the cumulative error of inertial sensors,complex motion modes of pedestrians,and the low robustness of the multi-sensor collaboration *** paper presents a hybrid pedestrian positioning system using the combination of wearable inertial sensors and ultrasonic ranging(H-PPS).A robust two nodes integration structure is developed to adaptively combine the motion data acquired from the single waist-mounted and foot-mounted node,and enhanced by a novel ellipsoid constraint *** addition,a deep-learning-based walking speed estimator is proposed by considering all the motion features provided by different nodes,which effectively reduces the cumulative error originating from inertial ***,a comprehensive data and model dual-driven model is presented to effectively combine the motion data provided by different sensor nodes and walking speed estimator,and multi-level constraints are extracted to further improve the performance of the overall *** results indicate that the proposed H-PPS significantly improves the performance of the single PPS and outperforms existing algorithms in accuracy index under complex indoor scenarios.

关键词： Pedestrian positioning system Wearable inertial sensors Ultrasonic ranging Deep-learning Data and model dual-driven

Triclosan-conjugated,Lipase-responsive Polymeric Micelles for Eradication of Staphylococcal Biofilms

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Chinese Journal of Polymer Science 2024年第6期42卷 718-728页

作者： Yan-qiang Huang Yuan-Feng Li Yong liu lin-qi Shi Guangxi Technology Innovation Cooperation Base of Prevention and Control Pathogenic Microbes with Drug Resistance Youjiang Medical University for NationalitiesBaise533000China Translational Medicine Laboratory the First Affiliated Hospital of Wenzhou Medical UniversityWenzhou325035China Wenzhou Institute University of Chinese Academy of SciencesWenzhou325001China State Key Laboratory of Medicinal Chemical Biology Key Laboratory of Functional Polymer Materials of Ministry of Educationand Institute of Polymer ChemistryCollege of ChemistryNankai UniversityTianjin300071China

Bacterial biofilms present a significant challenge in treating drug-resistant infections,necessitating the development of innovative *** this study,we introduce triclosan-conjugated,lipase-responsive polymeric micelles designed to exploit biofilm properties and serve as a responsive drug delivery *** micelles were created using an amphiphilic block polymer synthesized via ring-opening polymerization ofε-caprolactone(CL)and triclosan-containing cyclic trimethylene carbonate(MTC-Tri).Poly(ethylene glycol)(PEG-OH)acted as the macro-initiator,resulting in micelles with a PEG shell that facilitated their penetration into bacterial *** important advantage of our micelles lies in their interaction with local bacterial lipases within *** lipases triggered rapid micelle degradation,releasing triclosan in a controlled *** liberated triclosan effectively eliminated bacteria embedded in the ***,the triclosan-conjugated micelles displayed minimal toxicity to murine fibroblasts,indicating their biocompatibility and *** finding emphasizes the potential application of these micelles in combatting drug resistance observed in bacterial *** triclosan-conjugated,lipase-responsive polymeric micelles exhibit promising characteristics for addressing drug resistance in bacterial *** harnessing biofilm properties and implementing a responsive drug delivery system,we seek to provide an effective solution in the fight against drug-resistant bacteria.

关键词： Self-assembly Polymer prodrug Ring-opening polymerization Biofilm eradication Cytotoxicity

Hollow Metal-Organic Framework/MXene/Nanocellulose Composite Films for Giga/Terahertz Electromagnetic Shielding and Photothermal Conversion

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Nano-Micro Letters 2024年第9期16卷 161-179页

作者： Tian Mai Lei Chen Pei‑lin Wang qi liu Ming‑Guo Ma Research Center of Biomass Clean Utilization MOE Engineering Research Center of Forestry Biomass Materials and BioenergyBeijing Key Laboratory of Lignocellulosic ChemistryCollege of Materials Science and TechnologyBeijing Forestry UniversityBeijing 100083People’s Republic of China State Silica-Based Materials Laboratory of Anhui Province Bengbu 233000People’s Republic of China

With the continuous advancement of communication technology,the escalating demand for electromagnetic shielding interference(EMI)materials with multifunctional and wideband EMI performance has become *** the electrical and magnetic components and designing the EMI material structure have attracted extensive interest,but remain a huge ***,we reported the alternating electromagnetic structure composite films composed of hollow metal-organic frameworks/layered MXene/nanocellulose(HMN)by alternating vacuum-assisted filtration *** HMN composite films exhibit excellent EMI shielding effectiveness performance in the GHz frequency(66.8 dB at Kaband)and THz frequency(114.6 dB at 0.1-4.0 THz).Besides,the HMN composite films also exhibit a high reflection loss of 39.7 dB at 0.7 THz with an effective absorption bandwidth up to 2.1 ***,HMN composite films show remarkable photothermal conversion performance,which can reach 104.6℃under 2.0 Sun and 235.4℃under 0.8 W cm^(−2),*** unique micro-and macrostructural design structures will absorb more incident electromagnetic waves via interfacial polarization/multiple scattering and produce more heat energy via the local surface plasmon resonance *** features make the HMN composite film a promising candidate for advanced EMI devices for future 6G communication and the protection of electronic equipment in cold environments.

关键词： Metal-organic frameworks MXene Nanocellulose Electromagnetic shielding Photothermal conversion

Preparation and Application of Polymerized High Internal Phase Emulsion Monoliths for the Preconcentration and Determination of Malachite Green and Leucomalachite Green in Water Samples

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Journal of Analysis and Testing 2020年第4期4卷 264-272页

作者： Li-Ping Jiang Na Li lin-qi liu Xian Zheng Fu-You Du Gui-Hua Ruan Guangxi Key Laboratory of Electrochemical and Magnetochemical Functional Materials College of Chemistry and BioengineeringGuilin University of TechnologyGuilin 541004China College of Biological and Environmental Engineering Changsha UniversityChangsha 410022China

Polymerized high internal phase emulsion(polyHIPE)monoliths were prepared and applied as adsorbent materials for solid-phase extraction(SPE)of malachite green(MG)and leucomalachite green(LMG)from water *** polyHIPE monoliths were prepared by post-functionalization of monolithic surface with 6-aminocaproic acid(ACA)via ring opening reaction of epoxy groups in glycidyl methacrylate(GMA)-based polyHIPEs,and then applied to the preconcentration and determination of trace MG and LMG in environmental water samples by combing with high-performance liquid chromatog-raphy(HPLC).Taking MG and LMG as targets,main factors affecting SPE performance of the polyHIPE monoliths were *** the optimized conditions,the ACA-functionalized polyHIPE monoliths could effectively preconcentrate MG and LMG from 150 mL of water samples,and the recoveries of MG and LMG at three spiked levels were ranged from 84.8 to 97.4%with the relative standard deviations(RSDs)lower than 6%.The proposed method exhibited good linearity in the range of 2-200 ng mL^(-1),with low limits of detection of 17.0 and 8.7 pg mL^(-1)for MG and LMG,*** addi-tion,the prepared ACA-modified polyHIPE monolith showed good durability and stability,and it could be reused for 200 cycles without obvious losing the extraction performance.

关键词： High internal phase emulsion Solid-phase extraction High-performance liquid chromatography Malachite green Leucomalachite green

Constructing high-toughness polyimide binder with robust polarity and ion-conductive mechanisms ensuring long-term operational stability of silicon-based anodes

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Journal of Energy Chemistry 2024年第6期93卷 580-591,I0014页

作者： Yongjun Kang Nanxi Dong Fangzhou liu Daolei lin Bingxue liu Guofeng Tian Shengli qi Dezhen Wu State Key Laboratory of Chemical Resource Engineering Beijing University of Chemical TechnologyBeijing 100029China ENFI R&D Institute China ENFI Engineering CorporationBeijing 100038China China Automotive Battery Research Institute Co. Ltd.Beijing 101407China Changzhou Institute of Advanced Materials Beijing University of Chemical TechnologyChangzhou 213164JiangsuChina

Silicon-based materials have demonstrated remarkable potential in high-energy-density batteries owing to their high theoretical ***,the significant volume expansion of silicon seriously hinders its utilization as a lithium-ion ***,a functionalized high-toughness polyimide(PDMI) is synthesized by copolymerizing the 4,4'-Oxydiphthalic anhydride(ODPA) with 4,4'-oxydianiline(ODA),2,3-diaminobenzoic acid(DABA),and 1,3-bis(3-aminopropyl)-tetramethyl disiloxane(DMS).The combination of rigid benzene rings and flexible oxygen groups(-O-) in the PDMI molecular chain via a rigidness/softness coupling mechanism contributes to high *** plentiful polar carboxyl(-COOH) groups establish robust bonding *** ionic transport is achieved by incorporating the flexible siloxane segment(Si-O-Si),which imparts high molecular chain motility and augments free volume holes to facilitate lithium-ion transport(9.8 × 10^(-10) cm^(2) s^(-1) vs.16 × 10^(-10) cm^(2) s~(-1)).As expected,the SiO_x@PDMI-1.5 electrode delivers brilliant long-term cycle performance with a remarkable capacity retention of 85% over 500 cycles at 1.3 A g^(-1).The well-designed functionalized polyimide also significantly enhances the electrochemical properties of Si nanoparticles ***,the assembled SiO_x@PDMI-1.5/NCM811 full cell delivers a high retention of 80% after 100 *** perspective of the binder design strategy based on polyimide modification delivers a novel path toward high-capacity electrodes for high-energy-density batteries.

关键词： Polyimide binder High toughness Robust ionic transport Silicon-based anodes Lithium-ion batteries

Effect of Preload Force on Heat Generation of Li(Ni_(0.8)Co_(0.1)Mn_(0.1))O_(2)/SiO_(x)-C System Batteries:The Discharge Process

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Journal of Thermal Science 2024年第5期33卷 1809-1825页

作者： lin Chunjing LAI Zhenxing BAI Guangli MA Biao WEI Zhen qi Chuang liu Shiqiang Key Laboratory of Advanced Manufacturing Technology for Automobile Parts Ministry of EducationChongqing University of TechnologyChongqing 400054China China Auto Research New Energy Vehicle Inspection Center(Tianjin)Co Tianjin 300300China

Lithium-ion batteries(LIBs)undergo various degradation phenomena such as material decomposition,structural change and uneven lithium ion distribution during long-term cycles,which would affect their performance and *** order to improve the performance of the LIBs during their life cycle,preload force is preset when the batteries are *** preload forces will in turn affect the cycle life and heat generation of the *** order to address this issue,this work carries out charge/discharge cycle tests on a NCM811 battery under different preload *** calorimetry tests are performed to investigate the battery heat generation under different states of health(SOHs)and preload *** on the test results,an empirical prediction model for heat generation power as a function of SOH is *** show that when the preload force is 5 N·m,the battery capacity decreases in the slowest rate and the average heat generation power is the *** in peaks of the incremental capacity curve can be used to characterize the loss of lithium at the electrode,which in turn characterizes the change of heat generation power of the *** average heat generation power is mainly affected by the SOH,going through a period of trough with the decrease of the SOH and continuing to increase after crossing the critical *** general,these findings emphasize the relationship between preload force,SOH and heat generation power,which is helpful for the judgment of optimal preload to improve the efficiency of LIBs.

关键词： lithium ion battery cyclic aging preload force heat generation characteristic

Ferrihydrite transformation impacted by coprecipitation of lignin:Inhibition or facilitation?

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Journal of Environmental Sciences 2024年第5期139卷 23-33页

作者： lin liu Zhihui Yang Weichun Yang Wen Jiang qi Liao Mengying Si Feiping Zhao School of Metallurgy and Environment Central South UniversityChangsha 410083China Chinese National Engineering Research Center for Control&Treatment of Heavy Metal Pollution(CNERC-CTHMP) Changsha 410083China

Lignin is a common soil organic matter that is present in soils,but its effect on the transformation of ferrihydrite(Fh)remains *** matter is generally assumed to inhibit Fh ***,lignin can reduce Fh to Fe(Ⅱ),in which Fe(Ⅱ)-catalyzed Fh transformation ***,the effects of lignin on Fh transformation were investigated at 75℃ as a function of the lignin/Fh mass ratio(0-0.2),pH(4-8)and aging time(0-96 hr).The results of Fh-lignin samples(mass ratios=0.1)aged at different pH values showed that for Fh-lignin the time of Fh transformation into secondary crystalline minerals was significantly shortened at pH 6 when compared with pure Fh,and the Fe(Ⅱ)-accelerated transformation of Fh was strongly dependent on *** pH 6,at low lignin/Fh mass ratios(0.05-0.1),the time of secondary mineral formation decreased with increasing lignin *** high lignosulfonate-content material(lignin:Fh=0.2),Fh did not transform into secondary minerals,indicating that lignin content plays a major role in Fh *** addition,lignin affected the pathway of Fh transformation by inhibiting goethite formation and facilitating hematite *** effect of coprecipitation of lignin on Fh transformation should be useful in understanding the complex iron and carbon cycles in a soil environment.

关键词： Ferrihydrite transformation Lignin Hematite Goethite Fe(Ⅱ)-catalyzed Reactive Fe(Ⅲ)species

Devolatilization of high viscous fluids with high gravity technology

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Chinese Journal of Chemical Engineering 2024年第7期71卷 249-257页

作者： Jibing qi Youzhi liu Yandong liu Taiyuan University Taiyuan 030032China Shanxi Province Key Laboratory of Higee-Oriented Chemical Engineering North University of ChinaTaiyuan 030051China

Volatile organic compounds(VOCs)are generally toxic and harmful substances that can cause health and environmental *** removal of VOCs from polymers has become a key *** effective devolatilization to remove VOCs from high viscous fluids such as polymer is necessary and is of great *** this study,the devolatilization effect of a rotating packed bed(RPB)was studied by using polydimethylsiloxane as the viscous fluid and acetone as the *** devolatilization rate and liquid phase volume(KLa)have been *** results indicated that the optimum conditions were the high-gravity factor of 60,liquid flow rate of 10 L·h^(-1),and vacuum degree of 0.077 *** dimensionless correlation of KLa was established,and the deviations between predicted and experimental values were less than±28%.The high-gravity technology will result in lower mass transfer resistance in the devolatilization process,enhance the mass transfer process of acetone,and improve the removal effect of *** work provides a promising path for the removal of volatiles from polymers in combination with high-gravity *** can provide the basis for the application of RPB in viscous fluids.

关键词： High-gravity technology Devolatilization rate High viscous fluid Volatile organic compounds(VOCs)