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Accelerated design and discovery of perovskites with high conductivity for energy applications through machine learning

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npj Computational Materials 2021年第1期7卷 797-808页

作者： Pikee priya N.R.Aluru Department of Mechanical Science and Engineering University of Illinois at Urbana-ChampaignUrbanaILUSA Beckman Institute for Advanced Science and Technology University of Illinois at Urbana-ChampaignUrbanaILUSA

We use machine learning tools for the design and discovery of ABO3-type perovskite oxides for various energy applications,using over 7000 data points from the *** demonstrate a robust learning framework for efficient and accurate prediction of total conductivity of perovskites and their classification based on the type of charge carrier at different conditions of temperature and *** evaluating a set of>100 features,we identify average ionic radius,minimum electronegativity,minimum atomic mass,minimum formation energy of oxides for all B-site,and B-site dopant ions of the perovskite as the crucial and relevant predictors for determining conductivity and the type of charge *** models are validated by predicting the conductivity of compounds absent in the training *** screen 1793 undoped and 95,832 A-site and B-site doped perovskites to report the perovskites with high conductivities,which can be used for different energy applications,depending on the type of the charge carriers.

关键词： perovskite conductivity energy

Readily available alkylbenzenes as precursors for the one-pot preparation of buta-1,3-dienes under DDQ visible-light photocatalysis in benzotrifluoride

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Organic Chemistry Frontiers 2022年第5期9卷 1395-1402页

作者： Palani Natarajan Deachen Chuskit priya Department of Chemistry&Centre for Advanced Studies in Chemistry Panjab UniversityChandigarh-160014India

Easily accessible alkylbenzenes are highly valuable starting materials and solvents in synthetic organic chemistry for the production of pharmaceuticals,plastics,synthetic rubber,dyes,etc.

关键词： alkyl visible rubber

Probing the degradation of pharmaceuticals in urine using MFC and studying their removal efficiency by UPLC-MS/MS

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Journal of Pharmaceutical Analysis 2021年第3期11卷 320-329页

作者： priya Sharma Devendra Kumar Srikanth Mutnuri Applied Environmental Biotechnology Laboratory Birla Institute of Technology&Science(BITS)Pilani403726ZuarinagarIndia Central Sophisticated Instrumentation Facility Birla Institute of Technology&Science(BITS)Pilani403726ZuarinagarIndia Department of Pharmaceutical Sciences College of PharmacyUniversity of Nebraska Medical CenterOmahaNE68198-602USA

Nutrient recovery from source-separated human urine has attracted interest as it is rich in nitrogen and phosphorus that can be utilized as ***,urine also contains pharmaceuticals,steroid hormones,*** their removal is crucial as they have detrimental effects on the environment and human *** current study focuses on investigating the degradation of pharmaceuticals using a double-chamber microbial fuel cell(MFC).Urine was spiked with four pharmaceuticals(trimethoprim,lamivudine,levofloxacin,and estrone)at a concentration of 2 mg/*** MFC was operated for 7 months in batch mode with this spiked urine as *** degradation efficiency of the MFC was studied,for which a selective liquid chromatography-tandem mass-spectrometric method was developed for the quantitation of compounds used in the spiking experiments and was validated with a lower limit of quantification of 0.39 ng/*** maximum removal rate achieved was 96%±2%.The degradation mechanism involved processes like sorption and anoxic *** voltage curve obtained showed that the presence of pharmaceuticals had an initial negative impact on power generation along with increased organic content;however,after the reactor acclimatization,increased power output was achieved with maximum organics removal at 30 h of retention *** work opens a new perspective for the anoxic biodegradation of pharmaceuticals and can be useful in future bioremediation studies.

关键词： Pharmaceuticals Urine MFC Biodegradation Liquid chromatography mass spectroscopy

Interfacial charge-transfer engineering by ionic liquid for high performance planar CH3NH3PbBr3 solar cells

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Journal of Energy Chemistry 2018年第3期27卷 748-752页

作者： Xiaojia Zheng Wei Yu Shashank priya Center for Energy Harvesting Materials and System Virginia TechBlacksburgVirginia 24061United States State Key Laboratory of Catalysis Dalian Institute of Chemical PhysicsChinese Academy of SciencesDalian National Laboratory for Clean EnergyDalian116023LiaoningChina

The energy barrier at the CH3NH3Pb Br3/TiO2interface hinders the electron transfer from CH3NH3Pb Br3to compact TiO2（cp-TiO2）.Ionic liquid（IL）,that forms dipoles pointing away from TiO2,can adjust the work function of TiO2resulting in suitable energy level for charge transfer from CH3NH3Pb Br3to *** time-resolved photoluminescence spectroscopy（TRPL）measurements confirm faster electron transfer from the CH3NH3Pb Br3film to TiO2after modification by *** cells based on IL modified cp-TiO2demonstrate efficiency of～6%,much higher than the devices（0.2%）fabricated using untreated cp-TiO2as the electron transport layer.

关键词： Perovskite solar cell Ionic liquid Interface engineering Titanium dioxide

Severe liver injury due to herbal and dietary supplements and the role of liver transplantation

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World Journal of Gastroenterology 2019年第46期25卷 6704-6712页

作者： priya Grewal Jawad Ahmad Division of Liver Diseases Icahn School of Medicine at Mount Sinai

Herbal and dietary supplements(HDS)are increasingly used worldwide for numerous,mainly unproven health *** HDS industry is poorly regulated compared to prescription medicines and most products are easily *** induced liver injury(DILI)is a well-recognized entity associated with prescription and over the counter medications and many reports have emerged of potential HDS-related *** is considerable geographic variability in the risk and severity of DILI associated with HDS but the presentation of severe liver injury is similar with a hepatocellular pattern accompanied by *** type of injury can lead to acute liver failure and the need for liver *** will often fail to mention their use of HDS,considering it natural and therefore *** physicians should understand that these products can be associated with DILI and explicitly ask about HDS use in any patient with otherwise unexplained acute liver injury.

关键词： Herbal and dietary supplements Drug induced liver injury Liver transplantation Acute liver failure Geographic variability

Synthesis and characterization of Nd^(3+)-doped Ce_(0.6)Zr_(0.4)O_(2) and its doping significance on oxygen storage capacity

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Rare Metals 2021年第1期40卷 231-236页

作者： Natesan Shanmuga priya Chandramohan Somayaji S.Kanagaraj Siddaganga Institute of Technology TumkurKarnataka 572103India Indian institute of Technology Guwahati 781039India

Cerium and cerium-based oxides are found to be an important element in three-way catalytic converter(TWC).The effective utilization of TWC is found to be reduced due to thermal loading which results in structural deformation of ceria,Doping Zr^(4+)into the rare earth element can increase the oxygen storage capacity and thermal ***,an attempt was made to study the oxygen storage capacity and thermal stability of ceria by doping Zr^(4+)and Nd^(3+).Cerium-based nanocrystallite in the composition of Ce_(0.6)Zr_(0.4-x)Nd_(1.3)xO_(2)(0≤x≤0.4)was prepared by sol-gel synthesize technique with citric acid as a gel-forming agent.X-ray diffraction(XRD)result shows that doping Nd^(3+)into ceria lattice forms homogenous solid solution of cubic fluorite structure up to 25%of substitute *** higher amount of Nd^(3+)into ceria lattice leads to the formation of Nd_(2)O_(3).Raman spectrum study confirms that oxygen storage capacity band is present in Ce_(0.6)Zr_(0.4)O2 and Ce_(0.6)Zr_(0.3)Nd_(0.13)O_(2).The oxygen storage capacity was calculated through weight loss of the sample during the second heating cycle with cyclic heating from30 to 800℃in thermogravimetric analysis(TGA).The TGA study reveals that the oxygen storage capacity of Ce_(0.6)Zr_(0.4)O2 decreases after the substitution of Nd^(3+),which is due to the larger ionic radius of Nd^(3+)compared with that of Zr4+and CeO2.

关键词： Cerium oxide Sol-gel technique Thermogravimetric analysis Ionic radius Homogeneous solid solution Oxygen storage capacity

An approach towards identification of leather from leather-like polymeric material using FTIR-ATR technique

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Collagen and Leather 2023年第4期6卷 67-75页

作者： priya Narayanan Sreeram Kalarical Janardhanan Central Leather Research Institute-CSIR AdyarChennai 600020India

Leather,a by-product of the meat industry,has unique strength,elasticity,water vapor permeability,resistance to abrasion,durability,and *** the background of ISO 15115:2019,the authenticity of leather has become a subject matter of *** is a need to distinguish leather(animal origin)from other leather-like materials derived from fossil fuel(PU,faux leather,etc.)and agro-product-driven vegan materials,which are also sold in the market as *** this purpose,this work relies on the signature FTIR bands of collagen(the skin-making protein)as a starting point to distinguish between animal origin and rest.A detailed investigation of all types of materials used in lifestyle products has been carried out to assess the boundary lines of this *** is reasonably concluded that the signature AmideⅠ,Ⅱ,andⅢbands of collagen occurring at 1600,1500,and 1200 cm^(-1)could serve as the first line to distinguish against all materials other than nylon and in the case of nylon,and the Amide A band at 3200 cm^(-1),forms the basis for differentiation from *** essence,the FTIR spectra can be used as a robust,easy and unambiguous technique to distinguish leather from leather-like materials currently available on the market.

关键词： Leather Synthetic leather-like polymeric material Non-destructive Collagen FTIR-ATR

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A comprehensive review of significant researches on content based indexing and retrieval of visual information

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Frontiers of Computer Science 2013年第5期7卷 782-799页

作者： R. priya T. N. SHANMUGAM Department of Mathematics Anna University-Chennai Chennai 600 025 India

Developments in multimedia technologies have paved way for the storage of huge collections of video doc- uments on computer systems. It is essential to design tools for content-based access to the documents, so as to allow an efficient exploitation of these collections. Content based anal- ysis provides a flexible and powerful way to access video data when compared with the other traditional video analysis tech- niques. The area of content based video indexing and retrieval （CBVIR）, focusing on automating the indexing, retrieval and management of video, has attracted extensive research in the last decade. CBVIR is a lively area of research with endur- ing acknowledgments from several domains. Herein a vital assessment of contemporary researches associated with the content-based indexing and retrieval of visual information. In this paper, we present an extensive review of significant researches on CBV1R. Concise description of content based video analysis along with the techniques associated with the content based video indexing and retrieval is presented.

关键词： nultimedia information content based video retrieval (CBVR) content based video indexing and retrieval (CBVIR) shot segmentation object segmentation feature extraction indexing motion estimation querying key frame retrieval and indexing.

Continuous Mixed p-norm Control Scheme with Reweighted L_(0) norm Variable Step Size for Mitigating Power Quality Problems of Grid Coupled Solar PV Systems

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CSEE Journal of Power and Energy Systems 2023年第4期9卷 1394-1404页

作者： Pallavi Verma Avdhesh Kumar Rachana Garg priya Mahajan Delhi technological university DelhiDelhi 110085India.

In this paper,the performance of a two-stage three-phase grid coupled solar photovoltaic generating system(SPVGS)is analyzed by using a novel reweighted Lo norm variable step size continuous mixed p-norm(RLo-VSSCMPN)of a voltage source inverter(VSI)control *** efficacy of the system is determined by considering unbalanced grid voltage,DC offset,voltage sag and swell,unbalanced load and variations in solar ***-VSSCMPN is used for inverter control and it ex-tracts fundamental components of load current for generating the reference grid current with a faster convergence rate and lesser steady state *** the proposed control,harmonics in the grid current follows the IEEE-519 norm and the performance is also satisfactory under varying environmental/load *** power generated from SPvGS is transferred optimally using a DC-DC boost converter utilizing the incremental conductance(INC)maximum power point *** proposed system is simulated using MATLAB/Simulink 2018a and test results are verified experimentally using dSPACE1202 in the laboratory to ensure the validity of a novel proposed robust *** Terms-INC maximum power point tracker,power quality,reweighted LoVSSCMPN algorithm,solar PV generating system,total harmonic distortion,voltage source inverter.

关键词： INC maximum power point tracker power quality reweighted LoVSSCMPN algorithm solar PV generating system total harmonic distortion voltage source inverter.