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Insights into the mechanism of multiple Cu-doped Co Fe_(2)O_(4)nanocatalyst activated peroxymonosulfate for efficient degradation of Rhodamine b

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Journal of Environmental Sciences 2024年第3期137卷 382-394页

作者： Yuanmin Mo Xiaoping zhang School of Environment&Energy South China University of TechnologyGuangzhou Higher Education Mega CentreGuangzhou 510006China The Key Laboratory of Pollution Control and Ecosystem Restoration in Industry Clusters of Ministry of Education Guangzhou 510006China Guangdong Provincial Key Laboratory of Solid Wastes Pollution Control and Recycling Guangzhou 510006China Guangdong Provincial Engineering and Technology Research Center for Environmental Risk Prevention and Emergency Disposal Guangzhou 510006China

The multiple metal catalyst as a promising nanomaterial has shown excellent activity in the peroxymonosulfate(PMS)activation for pollutant ***,the role of special sites and in-depth understanding of the PMS activation mechanism are not fully *** this study,a Cu-doped CoFe_(2)O_(4)nanocatalyst(0.5CCF)was synthesized by a sol-gel and calcination method,and used for PMS activation to remove Rhodamine b(Rhb).The results showed that the Cu doping obviously enhanced the catalytic performance of CoFe_(2)O_(4),with 99.70%of Rhb removed by 0.5CCF while 74.91%in the CoFe_(2)O_(4)within 15 *** on the X-ray photoelectron spectroscopy and electrochemical analysis,this could be ascribed to the more low valence of Co and Fe species generated on the 0.5CCF and faster electron transfers occurred in the 0.5CCF due to the Cu *** addition,Cu doping could provide more reaction sites for the 0.5CCF to activate PMS for Rhb *** metal species and the surface hydroxyl were the reaction sites of PMS activation,and the surface hydroxyl played an important role in surface-bound reactive species *** the PMS activation,the Cu not only activated PMS to produce reactive oxygen species(ROS),but also regenerated Co^(2+)and Fe^(2+)to accelerate the PMS *** non-radical of ^(1)O_(2)was the main ROS with a 99.35%of contribution rate,and the SO_(5)^(·–)self-reaction was its major *** study provides a new insight to enhance the PMS activation performance of multiple metal catalysts by Cu doping in wastewater treatment.

关键词： Cu-doped CoFe_(2)O_(4)nanocatalyst PMS activation Mechanism Rhodamine b removal

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A SINGULAR DIRICHLET PRObLEM FOR THE MONGE-AMPÈRE TYPE EQUATION

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Acta Mathematica Scientia 2024年第5期44卷 1965-1983页

作者： Zhijun zhang bo zhang School of Mathematics and Information Science Yantai UniversityYantai264005China

We consider the singular Dirichlet problem for the Monge-Ampère type equation{\rm det}\D^2 u=b(x)g(-u)(1+|\nabla u|^2)^{q/2},\u<0,\x\in\Omega,\u|_{\partial\Omega}=0,whereΩis a strictly convex and bounded smooth doma... 详细信息

We consider the singular Dirichlet problem for the Monge-Ampère type equation{\rm det}\D^2 u=b(x)g(-u)(1+|\nabla u|^2)^{q/2},\ubounded smooth domain inℝn,q∈[0,n+1),g∈C∞(0,∞)is positive and strictly decreasing in(0,∞)with\lim\limits_{s\rightarrow 0^+}g(s)=\infty,and b∈C∞(Ω)is positive inΩ.We obtain the existence,nonexistence and global asymptotic behavior of the convex solution to such a problem for more general b and *** approach is based on the Karamata regular variation theory and the construction of suitable sub-and super-solutions.

关键词： Monge-Ampère equation a singular boundary value problem the unique convex solution global asymptotic behavior

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Distributed velocity-free formation tracking control for clustered UAVs under virtual leader-follower framework

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Science China(Technological Sciences) 2024年第5期67卷 1538-1552页

作者： zhang ZhaoYu DUAN Haibin School of Automation Science and Electrical Engineering Beihang UniversityBeijing100083China

The collective formation control problem of a cluster of rotorcraft unmanned aerial vehicles(UAVs)is investigated in this *** consensus tracking towards formation centroid with following UAVs forming a predefined configuration around the leader is considered as the *** prior studies,the information of the central reference trajectory,which is deemed as a virtual leader in the leader-follower topology,is not directly accessible for partial nodes through the communication ***,a novel distributed formation tracking control scheme is ***,a decentralized saturation observer is employed to estimate the reference acceleration signal of the virtual *** the absence of linear velocity measurement,two sliding manifolds are proposed by introducing the relative discrepancy terms of position and *** a smooth saturation operator in the form of a sigmoid function is applied to generate the command force ***,under the dilemma of constrained capabilities of the airborne sensors equipped on the rotorcrafts,the angular velocity is difficult to *** cascaded auxiliary attitude error systems are established on each rotorcraft system to synthesize the rotating torque with no need to require the angular velocity *** to the strong coupling and nonlinearity of the rotorcraft UAV system,the command angular velocity and the derivatives of command input are hard to *** a continuous nonlinear differentiator is proposed to work with the difficulties in deriving the explicit expression of system ***,a detailed stability analysis is conducted progressively on the angular control loop,reference trajectory observer loop,and the position control loop.A simulation scheme for a cluster of four rotorcraft UAVs tracking sinusoidal trajectory are presented and the formation control results are proven advantageous in comparison with the control protocol in previous literature.

关键词： distributed formation control unmanned rotorcraft clusters velocity-free tracking nonlinear differentiator

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Enhanced charge separation by incomplete calcination modified co-doped TiO_(2)nanoparticle for isothiazolinone photocatalytic degradation

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Nano Research 2024年第6期17卷 4834-4843页

作者： Zhiren Guo Xiao zhang Xinyuan Li Chang Cui Zilei zhang Hansheng Li Dongxiang zhang Jinying Li Xiyan Xu Jiatao zhang School of Chemistry and Chemical Engineering Beijing Institute of TechnologyBeijing 102488China Department of Chemistry MSU-BIT UniversityShenzhen 517182Chin

Photocatalytic oxidation techniques are promising for degradation of the highly ecotoxic and refractory isothiazolinone bactericides in relevant industrial ***,low charge separation and directional transport efficiency under solar light radiation restrain their practical ***,we report a nanostructured photocatalyst doped with Gd and b in TiO_(2)with carbon incorporation and defect formation through incomplete *** specific surface area,grain size,and hydrophilicity of TiO_(2)are improved,which is beneficial for the interfacial reaction between the photocatalyst and *** reduction of the bandgap,the broadening of the photo-absorption range,and the retarded electron-hole recombination promote the photocatalytic performance due to the improved oxygen vacancies based on the electron distribution *** difference in partial density of states(ΔPDOS)between the current catalyst and raw TiO_(2)indicates that the co-doping of Gd and b with incomplete calcination changes the electronic hybridization of conduction band and valence band near the Fermi level,and affects the band gap *** improved charge separation and directional transport efficiency and benefited the formation of main active species,including•OH and O_(2)•−,for the pollutant *** rate of photocatalytic removal of benzisothiazolinone(bIT)by the current photocatalyst reaches 1.25 h^(−1),being 4.31 times that of TiO_(2).The current work offers a constructive approach to the design and synthesis of nanostructured photocatalysts for the photocatalytic degradation of refractory organic pollutants.

关键词： TiO_(2)nanoparticle charge separation oxygen vacancies electron distribution modification photocatalytic degradation

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THE SUPERCLOSENESS OF THE FINITE ELEMENT METHOD FOR A SINGULARLY PERTURbED CONVECTION-DIFFUSION PRObLEM ON A bAKHVALOV-TYPE MESH IN 2D

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Acta Mathematica Scientia 2024年第4期44卷 1572-1593页

作者： Chunxiao zhang Jin zhang School of Mathematics and Statistics Shandong Normal UniversityJinan 250014China

For singularly perturbed convection-diffusion problems,supercloseness analysis of the finite element method is still open on bakhvalov-type meshes,especially in the case of *** difficulties arise from the width of the mesh in the layer adjacent to the transition point,resulting in a suboptimal estimate for *** analysis techniques cannot handle these difficulties *** fill this gap,here a novel interpolation is designed delicately for the smooth part of the solution,bringing about the optimal supercloseness result of almost order 2 under an energy norm for the finite element *** theoretical result is uniform in the singular perturbation parameterεand is supported by the numerical experiments.

关键词： singularly perturbed convection-diffusion finite element method supercloseness bakhvalov-type mesh

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Near-surface wind field characteristics of the desert-oasis transition zone in Dunhuang,China

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Journal of Arid Land 2024年第5期16卷 654-667页

作者： PAN Jiapeng zhang Kecun AN Zhishan zhang Yu Key Laboratory of Desert and Desertification&Dunhuang Gobi and Desert Ecology and Environment Research Station Northwest Institute of Eco-Environment and ResourcesChinese Academy of SciencesLanzhou 730000China University of Chinese Academy of Sciences Beijing 100049China

The desert-oasis transition zone(DOTZ)serves as a buffer area between the desert and *** its wind field characteristics is of great significance for the prevention and control of aeolian disasters in the *** this study,we used meteorological data during 2013–2019 from the portable meteorological stations at five sites(site A on the edge of the oasis,sites b,C,and D in the DOTZ,and site O in the desert)in Dunhuang,China to analyze the near-surface wind field characteristics and their causes,as well as to reveal the key role of the DOTZ in oasis *** results showed that the mean wind speed,frequency of sand-driving wind,and directional variability of wind decreased from west to east within the DOTZ,and wind speed was significantly affected by air *** terrain influenced the prevailing winds in the region,mainly from northeast and *** some areas adjacent to the oasis were controlled by southeasterly *** indicated that the near-surface wind field characteristics of the DOTZ were caused by the combined effects of local terrain and surface hydrothermal *** site D,the annual drift potential(DP)was 24.95 vector units(VU),indicating a low wind energy environment,and the resultant drift direction(RDD)showed obvious seasonal ***,the DOTZ played an important buffering role between the desert and *** with the desert,the mean wind speed in the oasis decreased by 64.98%,and the prevailing wind direction was more *** results of this study will be useful in interpreting the aeolian activity of the DOTZ in Dunhuang.

关键词： desert-oasis transition zone near-surface wind field hydrothermal difference sand-driving wind aeolian environment Dunhuang

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Toughening additive manufactured Zr-based bulk metallic glass composites by martensite phase transformation

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Journal of Materials Science & Technology 2024年第3期170卷 95-102页

作者： Pengcheng zhang Cheng zhang Jie Pan Di Ouyang Lin Liu State Key Laboratory of Materials Processing and Die&Mould Technology School of Materials Science and EngineeringHuazhong University of Science and TechnologyWuhan 430074China

Additive manufacturing technology based on laser powder bed fusion(LPbF)offers a novel approach for fabricating bulk metallic glass(bMG)products without restriction in size and ***,the bMGs prepared by LPbF usually suffered from less plasticity and poorer fracture toughness as compared to their cast counterparts due to partial crystallization in heat-affected zones(HAZs).Since crystallization in HAZs is hard to avoid completely in LPbF bMGs,it is desirable to design a suitable alloy system,in which only ductile crystalline phase,instead of brittle intermetallics,is formed in *** unique structure could effectively increase the toughness/plasticity of the LPbF *** achieve this goal,a quaternary bMG system with a composition of Zr_(47.5)Cu_(45.5)Al_(5)Co_(2)is adopted and subjected to *** is found that nearly a single phase of b_(2)-ZrCu is precipitated in HAZs,while a fully amorphous phase is formed in molten pools(MPs).This b_(2)phase reinforced bMG composite exhibits excellent mechanical properties with enhanced plasticity and ***,it is easy to modulate the mechanical properties by altering the amount of the b_(2)phase via adjusting the laser energy ***,the best combination of strength,plasticity,and notch toughness is obtained in the bMG composite containing 27.4%b_(2)phase and 72.6%amorphous phase,which exhibits yield strength(σ_(s))of 1423 MPa,plastic strain(ε_(p))of 4.65%,and notch toughness(K_(q))of 53.9 MPa m 1/***,a notable strain-hardening is also *** improvement of plasticity/toughness and appearance of strain-hardening behavior are mainly due to the martensite phase transformation from the b_(2)phase to the Cm phase during plastic deformation(i.e.,the phase transformation-induced plasticity effect).The current work provides a guide for making advanced bMGs and bMG composites by additive manufacturing.

关键词： Laser powder bed fusion bulk metallic glass composites Phase transformation-induced plasticity Deformation mechanism

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Mechanical behaviors of mylonitic granite and granitic protomylonite in a deep ductile shear zone

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Journal of Rock Mechanics and Geotechnical Engineering 2024年第7期16卷 2663-2677页

作者： Lanbin zhang Ru zhang Li Ren Zhilong zhang Zetian zhang Dong Wang Xinzhong Wang Huijun Lu State Key Laboratory of Intelligent Construction and Healthy Operation and Maintenance of Deep Underground Engineering College of Water Resource and HydropowerSichuan UniversityChengdu610065China MOE Key Laboratory of Deep Earth Science and Engineering Sichuan UniversityChengdu610065China China Railway Eryuan Engineering Group Company Ltd.Chengdu610065China School of Architecture and Civil Engineering Xihua UniversityChengdu610065China

For projects near the tectonic belt,mylonite of varying metamorphic degrees may be *** matrix proportion of rock reflects its internal microscopic characteristics,thus it is beneficial for engineering geology to study the effect of the matrix proportion on the mechanical properties and rupture behaviors of *** of mylonitic granite and granitic protomylonite with varying matrix proportions were obtained from a ductile shear zone for a series of uniaxial compression and acoustic emission(AE)*** results showed that with the increase in matrix proportion,the average strength and elastic modulus of the samples increased,and the rock sample with the largest matrix proportion exhibited the maximum peak stress of 244.42 MPa,which was 45.86%greater than the average peak stress of the rock samples with the smallest matrix *** the rock samples with larger matrix proportion,their mechanical parameters exhibited greater dispersion and the large-scale appearance of AE events occurred earlier,showing a relatively gradual failure *** samples had larger accumulated AE parameter values and greater degree of *** contrast,for samples with smaller matrix proportions,the large-scale appearance of AE events occurred close to the peak stress,indicating that the occurrence of damage and fractures was centralized and *** samples had lower accumulated AE parameter values and fewer cracks after ***,for the rock samples with more matrix proportion,the average variance of the b-value was 1.1,which was lower than that of rock samples with the smallest matrix proportion(the average variance of the b-value was 3.7).Furthermore,it can be predicted that under certain stress,the failure depth around a tunnel is generally smaller when the strength of rock samples with larger matrix proportion is greater.

关键词： Mylonite Matrix proportion Mechanical properties Acoustic emission(AE) Rupture behaviors

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Characterization of Fe-containing particles in Chengdu,southwest China,using single-particle aerosol mass spectrometry

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Journal of Environmental Sciences 2024年第2期136卷 110-120页

作者： Renjiang He Junke zhang Luyao Chen Wei zhang Yingwei Xi School of Public Health Southwest Medical UniversityLuzhou 646000China Faculty of Geosciences and Environmental Engineering Southwest Jiaotong UniversityChengdu 611756China Sichuan Environmental Monitoring Center Chengdu 610074China

Single-particle aerosol mass spectrometry was used to study the characteristics of Fecontaining particles during winter in Chengdu,southwest *** mass concentrations of PM_(2.5)and PM_(10)during the study period were 64±38 and 89±49μg/m~3,respectively,and NO_(2)and particulate matter were high compared with most other regions of *** Fecontaining particles were divided into seven categories with different mass spectra,sources and aging *** highest contribution was from Fe mixed with carbonaceous components(Fe-C,23.1%)*** was more mixed with sulfate than nitrate and therefore the contribution of Fe mixed with sulfate(Fe-S,20.7%)particles was higher than that of Fe mixed with nitrate(Fe-N,12.5%)*** contributions from Fe-containing particles related to primary combustion were high in the small particle size range,whereas aged Fecontaining particles and dust-related particles were mostly found in the coarse particle size *** air masses mainly originated from the west and east of Chengdu,and the corresponding PM_(2.5)concentrations were 79±36 and 55±36μg/m~3,*** west and east air masses showed stronger contributions of Fe-containing particles related to biomass burning(Fe-b)and fossil fuel combustion(Fe-C and Fe-S)particles,*** southwest area contributed the most Fe-containing *** assessments of the effects of Fe-containing particles during heavy pollution period should pay more attention to Fe-C and Fe-S ***-reduction of Fe-containing particles should consider both local emissions and short-distance transmission from the surrounding areas.

关键词： Fe-containing particles Particle composition Potential source areas Evolution Chengdu

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Degeneration of foundation cushion species induced by ecological constraints can cause massive changes in alpine plant communities

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Science China(Life Sciences) 2024年第4期67卷 789-802页

作者： Jianguo Chen Xufang Chen Lishen Qian Yazhou zhang bo Li Honghua Shi Lu Sun Christian Schöb Hang Sun Key Laboratory for Plant Diversity and biogeography of East Asia Kunming Institute of BotanyChinese Academy of SciencesKunming 650201China University of Chinese Academy of Sciences Beijing 100049China College of Resources and Environment Yunnan Agricultural UniversityKunming 650500China Área de biodiversidad y Conservación Universidad Rey Juan CarlosMóstoles 28933Spain

Foundational cushion plants can re-organize community structures and sustain a prominent proportion of alpine biodiversity,but they are sensitive to climate *** loss of cushion species can have broad consequences for associated *** potential plant community changes with the population dynamics of cushion plants remain,however,*** eight plant communities along a climatic and community successional gradient,we assessed cushion population dynamics,the underlying ecological constraints and hence associated plant community changes in alpine communities dominated by the foundational cushion plant Arenaria *** population dynamics of Arenaria are attributed to ecological constraints at a series of life history *** functions are constrained by increasing associated beneficiary plants;subsequent seedling establishment is constrained by temperature,water and light availability,extreme climate events,and interspecific competition;strong competitive exclusion may accelerate mortality and degeneration of cushion *** with cushion dynamics,species composition,abundance and community structure gradually *** cushion plants completely degenerate,previously cushion-dominated communities shift to relatively stable communities that are overwhelmingly dominated by *** warming may accelerate the degeneration process of *** of this foundational cushion plant will possibly induce massive changes in alpine plant communities and hence ecosystem functions in alpine *** assessment of the population dynamics of foundation species is critical for an effective conservation of alpine biodiversity.

关键词： alpine ecosystem biodiversity change climate change plant community dynamics foundation species global warming population dynamics

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