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Revolutionizing plasmonic platform via magnetic field-assisted confined ultrafast laser deposition of high-density,uniform,and ultrafine nanoparticle arrays

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International journal of Extreme Manufacturing 2024年第3期6卷 428-438页

作者： jin Xu Lingfeng Wang peilin Yang Haoqing jiang Huai Zheng Licong An Xingtao Liu Gary j cheng School of Industrial Engineering Purdue UniversityWest LafayetteIN 47906United States of America Institute of Technological Sciences Wuhan UniversityWuhanHubei 430072People’s Republic of China

The remarkable capabilities of 2D plasmonic surfaces in controlling optical waves havegarnered significant ***,the challenge of large-scale manufacturing of uniform,well-aligned,and tunable plasmonic surfaces has hindered their *** address this,we present a groundbreaking tunable plasmonic platform design achieved throughmagnetic field(MF)assisted ultrafast laser direct deposition in *** precise control of metal nanoparticles(Nps),with cobalt(Co)serving as the model material,employing an MF,and fine-tuning ultrafast laser parameters,we have effectively converted coarse and non-uniform Nps into densely packed,uniform,and ultrafine Nps(~3 nm).This revolutionary advancement results in the creation of customizable plasmonic‘hot spots,’which play a pivotal role insurface-enhanced Raman spectroscopy(SERS)*** profound impact of this designable plasmonic platform lies in its close association with plasmonic resonance and *** the plasmonic nanostructures resonate with incident light,they generate intense local electromagnetic fields,thus vastly increasing the Raman scattering *** enhancement leads to an outstanding 2–18 fold boost in SERS performance and unparalleled sensing sensitivity down to 10^(-10)***,the plasmonic platform also demonstratesrobustness,retaining its sensing capability even after undergoing 50 cycles of rinsing andre-loading of ***,this work adheres to green manufacturing standards,making it an efficient and environmentally friendly method for customizing plasmonic‘hot spots’inSERS *** study not only achieves the formation of high-density,uniform,and ultrafine Np arrays on a tunable plasmonic platform but also showcases the profound relation betweenplasmonic resonance and energy *** outstanding results observed in SERS sensors further emphasize the immense potential of this technology for energy-relatedapplications,including photocatalysis,ph

关键词： magnetic field manipulation laser deposition metasurface SERS

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Leflunomide: A versatile additive for defect reduction, enhanced optoelectronic properties and environmental stability of perovskite films

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Nano Research 2024年第4期17卷 2628-2637页

作者： Dingyue Sun Ming peng Taijin Wang Longju Yi Shizuo Zhang Feng Liu Gary j.cheng The Institute of Technological Sciences Wuhan UniversityWuhan 430072China School of power and Mechanical Engineering Wuhan UniversityWuhan 430072China School of Industrial Engineering Purdue UniversityWest LafayetteIN 47906USA

The development of perovskite photoelectric devices with excellent performance is largely dependent on the defects in the perovskite *** address this issue,a specific drug,leflunomide(LF,C_(12)H_(9)F_(3)N_(2)O_(2)),was incorporated into the perovskite to reduce defects and improve its photoelectric *** is believed that the C=O bond on LF molecule can interact with the uncoordinated pb2+of the perovskite,thereby reducing non-radiative *** novel approach of incorporating LF into perovskite films has the potential to revolutionize the development of high-performance perovskite photoelectric *** trifluoromethyl functional(–CF_(3))group on LF can form a protective layer on the surface of the perovskite film,shielding it from water ***,LF can be utilized to alter the nucleation position of perovskite,thus minimizing the number of defects and optimizing the film ***,the LF-doped perovskite film displays low trap density and high photoelectric *** LF-doped perovskite film showed a trap density of 8.28×10^(11),which is notably lower than the 2.04×10^(12) of the perovskite film without *** responsivity and detectivity of the LF-doped perovskite photodetector were 0.771 A/W and 2.81×10^(11) jones,respectively,which are much higher than the 0.23 A/W and 1.06×10^(10) jones of the LF-undoped perovskite ***,the LF-doped photodetector maintained an initial photocurrent of 86%after 30 days of storage in air,indicating drastically increased environmental *** strongly suggests that LF is an effective additive for perovskites utilized in optoelectronic devices with high performance.

关键词： leflunomide additive engineering defect passivation perovskite

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Deflagration and detonation induced by shock wave focusing at different Mach numbers

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Chinese journal of Aeronautics 2024年第2期37卷 249-258页

作者： Zezhong YANG jun cheng Bo ZHANG School of Aeronautics and Astronautics Shanghai Jiao Tong UniversityShanghai 200240China

Shock wave focusing is an effective way to create a hot spot or a high-pressure and hightemperature region at a certain place,showing its unique usage in detonation initiation,which is beneficial for the development of detonation-based *** flame propagation behavior after the autoignition induced by shock wave focusing is crucial to the formation and self-sustaining of the detonation *** this study,wedge reflectors with two different angles(60°and 90°)and a planar reflector are employed,and the Mach number of incident shock waves ranging from 2.0 to 2.8 is utilized to trigger different flame propagation *** pressure transducers and the high-speed schlieren imaging system are both employed to investigate the shock-shock collision and ignition *** results reveal a total of four flame propagation modes:deflagration,DDT(Deflagration-to-Detonation Transition),unsteady detonation,and direct *** detonation wave formed in the DDT and unsteady detonation mode is only approximately 75%-85%of the Chapman-jouguet(C-j)speed;meanwhile,the directly induced detonation wave speed is close to the C-j *** waves,which are strong evidence for the existence of detonation waves,are discovered in *** usage of wedge reflectors significantly reduces the initial pressure difference ratio needed for direct detonation *** also provide a practical method for differentiating between detonation and deflagration modes,which involves contrasting the speed of the reflected shock wave with the speed of the theoretically nonreactive reflected shock *** findings should serve as a reference for the detonation initiation technique in advanced detonation propulsion engines.

关键词： Deflagration Detonation Hydrogen Ignition Shock wave focusing

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Addressable structured light system using metasurface optics and an individually addressable VCSEL array

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photonics Research 2024年第6期12卷 1129-1137页

作者： CHENYANG WU XUANLUN HUANG YIpENG jI TINGYU cheng jIAXING WANG NAN CHI SHAOHUA YU CONNIE j.CHANG-HASNAIN School of Information Science and Technology Fudan UniversityShanghai 200433China Berxel photonics Co. Ltd.Shenzhen 518071China peng cheng Laboratory Shenzhen 518055China Chinese University of Hong Kong Shenzhen 518172China

Structured-light(SL)based 3D sensors have been widely used in many *** SL is the most widely deployed among all SL sensors due to its light weight,compact size,fast video rate,and low *** transmitter(known as the dot projector)consists of a randomly patterned vertical-cavity surface-emitting laser(VCSEL)array multiplicated by a diffractive optical element(DOE)with a fixed repeated *** that the separation of any two speckles is only one known and fixed number(albeit random),there are no other known scales to cal-ibrate or ***,typical SL sensors require extensive in-factory calibrations,and the depth resolution is limited to 1 mm at-60 cm *** this paper,to the best of our knowledge,we propose a novel dot projector and a new addressable SL(ASL)3D sensor by using a regularly spaced,individually addressable VCSEL array,multiplicated by a metasurface-DOE(MDOE)into a random pattern of the *** turning on or off the VCSELs in the array provides multiple known distances between neighboring speckles,which is used as a“built-in caliper”to achieve higher accuracy of *** as a precise“vernier caliper,”the addressable VCSEL array enables fine control over speckle positions and high detection *** experimentally dem-onstrated that the proposed method can result in sub-hundred-micron level *** new concept opens new possibilities for applications such as 3D computation,facial recognition,and wearable devices.

关键词： speckle light surface

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The replication crisis and its relevance to Earth Science studies:Case studies and recommendations

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Geoscience Frontiers 2024年第4期15卷 304-314页

作者： Stephen j.puetz Kent C.Condie Kurt Sundell Nick M.W.Roberts Christopher j.Spencer Slah Boulila Qiuming cheng 475 Atkinson Dr Suite 704HonoluluHI 96814USA New Mexico Institute of Mining and Technology SocorroNM 87801USA Idaho State University PocatelloID 83209USA Geochronology and Tracers Facility British Geological SurveyKeyworthNottingham NG125GGUK Queen’s University Department of Geological Sciences and Geological EngineeringKingstonOntario K7L 3N6Canada Sorbonne Université CNRSInstitut des Sciences de la Terre ParisParisFrance State Key Laboratory of Geological processes and Mineral Resources China University of GeosciencesWuhan 430074China

Numerous scientific fields are facing a replication crisis,where the results of a study often cannot be replicated when a new study uses independent *** issue has been particularly emphasized in psychology,health,and medicine,as incorrect results in these fields could have serious consequences,where lives might be at *** other fields have also highlighted significant replication problems,the Earth Sciences seem to be an *** paucity of Earth Science research aimed at understanding the replication crisis prompted this ***,this work aims to fill that gap by seeking to replicate geological results involving various types of *** identify and discuss 11 key variables for replicating U-pb age distributions:independent data,global sampling,proxy data,data quality,disproportionate non-random sampling,stratigraphic bias,potential filtering bias,accuracy and precision,correlating time-series segments,testing assumptions and divergent analytical methods,and analytical *** while this work primarily focuses on U-pb age distributions,most of these factors(or variations of them)also apply to other geoscience ***,some of the discussions involve time-series consisting ofεHf,δ18O-zircon,14C,10Be,marineδ13C,and marineδ*** then provide specific recommendations for minimizing adverse effects related to these factors,and in the process enhancing prospects for replicating geological results.

关键词： Replication crisis Replicability Independent data Global time-series Globality index Filtered data

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Classification of complete 3-dimensional self-shrinkers in the Euclidean space R^(4)

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Science China Mathematics 2024年第4期67卷 873-882页

作者： Qing-Ming cheng Zhi Li Guoxin Wei Department of Applied Mathematics Faculty of ScienceFukuoka UniversityFukuoka 814-0180Japan College of Mathematics and Information Science Henan Normal UniversityXinxiang 453007China School of Mathematical Sciences South China Normal UniversityGuangzhou 510631China

In this paper,we completely classify 3-dimensional complete self-shrinkers with the constant norm S of the second fundamental form and the constant f3in the Euclidean space R^(4),where hij’s are components of the sec... 详细信息

关键词： mean curvature ow self-shrinker the generalized maximum principle

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photo-cured phase change energy storage material with photo-thermal conversion, self-cleaning and electromagnetic shielding performances via the lamellar structure strengthened by segment rearrangement of dynamic disulfide bond

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journal of Materiomics 2024年第5期10卷 1049-1062页

作者： Ziyu Liu Yuhan Li jue cheng junying Zhang Key Laboratory of Carbon Fiber and Functional polymers Ministry of EducationBeijing University of Chemical TechnologyBeijing100029China

At present,phase change materials(pCMs)with single function hardly meet the needs of advanced intelligent materials in practical applications,and the multifunction integration is the current ***,photo-cured multifunctional pCMs are hampered by insufficient transparency due to adding functional fillers,such as carbon and metal *** novel strategy is necessary to overcome this ***,a photo-cured multifunctional pCM is prepared by using the design of a lamellar structure composing the photo-cured phase change polymer layer and the functional fillers *** curing of the phase change polymer is realized by the photo-induced"thiol-ene"click reaction,and reversible dynamic disulfide bonds are introduced into the pCM,which not only gives the phase change crosslinked network reprocessability,but also strengthens the interface layer by the chain rearrangement to form a stable composite *** carboxylated multiwalled carbon nanotubes(CCNTs)and silver nanowires(AgNWs),as functional fillers,give the pCM photo-thermal conversion,self-cleaning and electromagnetic shielding(EMI SE)*** phase change latent heat and photo-thermal conversion can reach 105.2 j/g and 78.5%,and the water contact angle is 142°with self-cleaning *** addition,due to the dense and well-developed conductive path formed by AgNWs layer on the pCM surface,the EMI SE effect can reach 39 dB with only 6.3%(in mass)filler content and 7.2%phase change latent heat *** far as we know,this is the first report about photo-cured pCMs with self-cleaning,photo-thermal conversion and EMI SE performances.

关键词： photo-curing phase change materials Lamellar structure Interface bonding Multifunctional integration

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Crystal structure,phase transitions,and thermodynamic properties of magnesium metavanadate(MgV_(2)O_(6))

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journal of Magnesium and Alloys 2024年第4期12卷 1449-1460页

作者： Guishang pei cheng pan Dapeng Zhong junyi Xiang Xuewei Lv College of Materials Science and Engineering Chongqing UniversityChongqing 400044China Chongqing Key Laboratory of Vanadium-Titanium Metallurgy and Advanced Materials Chongqing UniversityChongqing 400044China pangang Group Research Institute Co. Ltd.Panzhihua 617000China

As a promising anode material for magnesium ion rechargeable batteries,magnesium metavanadate(MgV_(2)O_(6))has attracted considerable research interest in recent years.A MgV_(2)O_(6)sample was synthesized via a facile solid-state reaction by multistep-firing stoichiometric mixtures of MgO and V2O5 powder under an air *** solid-state phase transition fromα-MgV_(2)O_(6)toβ-MgV_(2)O_(6)occurred at 841 K and the enthalpy change was 4.37±0.04 kj/*** endothermic effect at 1014 K and the enthalpy change was 26.54±0.26 kj/mol,which is related to the incongruent melting ofβ-MgV_(2)O_(6).In situ XRD was performed to investigate phase transition of the as-prepared MgV_(2)O_(6)at high *** cell parameters obtained by Rietveld refinement indicated that it crystallizes in a monoclinic system with the C2/m space group,and the lattice parameters of a=9.280 A°,b=3.501 A°,c=6.731 A°,β=111.76°.The solid-state phase transition fromα-MgV_(2)O_(6)toβ-MgV_(2)O_(6)was further studied by thermal kinetics,indicating that this process is controlled first by a fibril-like mechanism and then by a spherulitic-type mechanism with an increasing heating ***,the enthalpy change of MgV_(2)O_(6)at high temperatures was measured utilizing the drop calorimetry,heat capacity was calculated and given as:Cp=208.3+0.03583T-4809000T^(−2)(298-923 K)(j mol^(−1)K^(−1)),the high-temperature heat capacity can be used to calculate Gibbs free energy of MgV_(2)O_(6)at high temperatures.

关键词： MgV_(2)O_(6) Crystal structure phase transitions Thermodynamic functions

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Two-way shape memory effect in a Ti-Zr-Nb-Ta high-temperature shape memory alloy

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Rare Metals 2024年第3期43卷 1257-1262页

作者： cheng-Yang Xiong Tuo Li jun Wang Yan Li School of Materials Science and Engineering Beihang UniversityBeijing100191China

The two-way shape memory effect in a Ti-18.5Zr-10Nb-3.5Ta high-temperature shape memory alloy was investigated.X-ray diffraction measurem ent shows that the alloy is composed of orthorhombicα"-martensite.ωphase is not found in Ti-18.5Zr-10Nb-3.5Ta alloy due to the suppressing effect of Ta ***α"-martensite laths are found in the transmission electron microscope observation;after the bending deformation,there appear a lot of *** alloy exhibits a shape memory strain of 3.8%aud a high reverse martensite transformation start temperature of 464 *** maximum two-way shape memory strain of 1.2%is obtained in the alloy with the prebending training strain of 10%.The mechanism can be ascribed to the effect of internal stress field caused by dislocations.

关键词： Ti-Zr Shape memory alloys Two-way shape memory effect

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Infiltration,runoff,and slope stability behaviors of infinite slope with macropores based on an improved Green–Ampt model

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journal of Mountain Science 2024年第7期21卷 2220-2235页

作者： LI Shanghui WU Guoxiong QUE Yun jIANG Zhenliang cheng Gaoyun College of Intelligent Construction Fuzhou University of International Studies and TradeFuzhou 350202China College of Civil Engineering Chongqing Jiao Tong UniversityChongqing 400074China Chongqing Vocational College of Architectural Engineering Chongqing 400072China College of Civil Engineering Fuzhou UniversityFuzhou 350000China Department of Civil and Environmental Engineering Hong Kong University of Science and TechnologyHong Kong 999077China T.Y.Lin International Engineering Consulting(China)Co.Ltd Chongqing 401120China

Infiltration–runoff–slope instability mechanism of macropore slope under heavy rainfall is *** paper studied its instability mechanism with an improved Green–Ampt(GA)model considering the dual-porosity(i.e.,matrix and macropore)and ponding condition,and proposed the infiltration equations,infiltration–runoff coupled model,and safety factor calculation *** show that the infiltration processes of macropore slope can be divided into three stages,and the proposed model is rational by a comparative *** wetting front depth of the traditional unsaturated slope is 17.2%larger than that of the macropore slope in the early rainfall stage and 27%smaller than that of the macropore slope in the late rainfall ***,macropores benefit the slope stability in the early rainfall but not in the *** flow does not occur initially but becomes pronounced with increasing rainfall *** equal depth of the wetting front in the two domains is regarded as the onset criteria of macropore *** analysis shows that macropore flow is delayed by increasing proportion of macropore domain(ω_(f)),whereas promoted by increasing ratio of saturated permeability coefficients between the two domains(μ).The increasing trend of ponding depth is sharp at first and then grows ***,when rainfall duration is less than 3 h,ωf andμhave no significant effect on the safety factor,whereas it decreases with increasingωf and increases with increasingμunder longer duration(≥3 h).With the increase ofω_(f),the slope maximum instability time advances by 10.5 h,and with the increase ofμ,the slope maximum instability time delays by 3.1 h.

关键词： Macropore slope Green–Ampt infiltration model Equivalent wetting front ponding response time Slope stability

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