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Green.En.rgy & En.iron.en. 2024年第7期9卷 1112-1121页

作者： Yajie Bai Zhen.uan.fang Yon. Lei Lijin. Liu Huaiquan.Zhao Hon.ye Bai Weiqian. Fan.Weidon. Shi School of Chemistry an. Chemical En.in.erin. Jiangsu University School of Chemistry Beihang University In.titute of Physics & IMn.Macron.n. Technische Universit?t Ilmenau

Photoelectrochemical n.3-reduction.PEC n.TRR） n.t on.y provides a promisin. solution.for promotin. the global n.trogen.cycle,but also con.erts n.3-to the importan. chemicals（n.3）.However,it is still a great challen.e to prepare catalysts with excellen. n.3-adsorption.activation.capacity to achieve high ***,we design.d a n.vel Fe2+～Cu2+Fe3+LDH/BiVO4（FCF-LDH/BVO） catalyst with syn.rgistic effect of chemical adsorption.an. physical ***2+in.FCF-LDH/BVO provides the rich Lewis acid sites for the adsorption.of n.3-,an. the appropriate layer spacin. of FCF-LDH further promotes the physical en.ichmen. of n.3-in.its in.erior,thus realizin. the effective con.act between.n.3-an. active sites(Fe2+).FCF-LDH/BVO showed excellen. n.3production.performan.e(FEn.3=66.1%,rn.3=13.8 μg h-1cm-2) an. selectivity(FEn.2-=2.5%,rn.2-=4.9 μg h-1cm-2) in.0.5 mol *** addition.FCF-LDH/BVO main.ain. the desirable PEC stability for six cycle experimen.s,showin. great poten.ial for practical ***14n.3-an.15n.3-isotope test provides stron. eviden.e for further verification.of the origin.of n.in.the gen.rated *** LDH catalyst has a great poten.ial in.PEC removal of n.3-from groun.water.

关键词： LDH Lewis acid sites Physical en.ichmen. Photoelectrochemical n. 3 − Reduction Ammon.a

Effect of rice cultivar on.green.ouse-gas emission. from rice-fish co-culture

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The Crop Journ.l 2024年第3期12卷 888-896页

作者： Kexin.Xie Men.jie Wan. Xiaodan.Wan. Fen.bo Li Chun.hun.Xu Jin.ei Fen. Fupin. fang Chin. n.tion.l Rice Research In.titute Hangzhou 310006ZhejiangChina

In.aquaculture,co-culturin. rice with fish may mitigate green.ouse-gas *** this study,co-culture of four rice cultivars in.a laboratory-scale rice–fish system reduced CH_(4)an. n.(2)O emission. relative to fish *** in.CH_(4)an. n.(2)O emission. amon. rice cultivars primarily stem from the differen.ial effects of rice plan.s on.plan.-mediated CH_(4)tran.port,CH_(4)oxidation.an. n.trogen.absorption.

关键词： Green.ouse gas emission. Aquaculture Rice-fish system Rice cultivar

Effects of potassium lactate on.sen.ory attributes,bacterial commun.ty succession.an. biogen.c amin.s formation.in.Rugao ham

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Food Scien.e an. Human.Welln.ss 2024年第1期13卷 198-210页

作者： Ren.on. Liao Yin. Wan. Qian. Xia Chan.yu Zhou fang Gen. Daodon. Pan.Jin.uan.Cao State Key Laboratory for Man.gin. Biotic an. Chemical Threats to the Quality an. Safety of Agro-products Key Laboratory of Animal Protein Food Processing Technology of Zhejiang ProvinceNingbo UniversityNingbo 315211China Meat Processin. Key Laboratory of Sichuan.Provin.e School of Food and Biological EngineeringChengdu UniversityChengdu 610106China School of Food an. Health Beijing Technology and Business UniversityBeijing 100048China

To deepen.the un.erstan.in. in.the effect of potassium lactate on.the sen.ory quality an. safety of Rugao ham,sen.ory attributes,physicochemical parameters,total volatile basic n.trogen.TVBn.,microorgan.sm commun.ty an. biogen.c amin.s of Rugao ham man.factured with differen. potassium lactate levels(0%,0.5%,1%,2%)were in.estigated;the relation.hip between.microbial commun.ty an. the formation.of TVBn.an. biogen.c amin.s was further *** the in.rease of potassium lactate from 0%to 2%,the in.reased sen.ory scores an. the decreased total aerobic bacterial coun. an. TVBn.were observed;the abun.an.e of Staphylococcus in.reased,while the con.en. of Halomon.s *** effect size(LEf Se)an. correlation. an.lysis showed that Staphylococcus equorum an. Lactobacillus fermen.um could be the key species to improve sen.ory scores an. decrease biogen.c amin.s an. *** pathway an.lysis further showed that amin. acids metabolism an. n.trogen.metabolism were main.y in.olved in.decreasin. TVBn.an. biogen.c amin.s in.the treatmen. of 2%potassium lactate.

关键词： Rugao ham Potassium lactate Biogen.c amin.s Microbial commun.ty Metabolic pathways

Hydrocarbon.Chargin. an. Accumulation.Process of the Large Bozhon.19-6 Con.en.ate Gas Reservoirs in.the Southwestern.Bozhon. Sub-Basin.Bohai Bay Basin.Chin.

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Journ.l of Earth Scien.e 2024年第2期35卷 613-630页

作者： Quan.un.Miao Chan.gui Xu fang Hao Min.un.hi Xie Qi Wan. Jie Yin.Huayao Zou Gen.ral Prospectin. In.titute of Chin. n.tion.l Admin.stration.of Coal Geology Beijing100039China State Key Laboratory of Petroleum Resource an. Prospectin. China University of PetroleumBeijing102249China Tian.in.Bran.h of Chin. n.tion.l Offshore Oil Compan. Ltd. Tianjin300452China School of Geoscien.es China University of PetroleumQingdao266580China School of Geoscien.es Yangtze UniversityWuhan430100China

The Bozhon.19-6(BZ19-6)con.en.ate gas reservoirs,located in.the southwestern.Bozhon. sub-basin.Bohai Bay Basin.Chin.,were paleo-oil reservoirs in.the geological past an. have un.ergon. at least three successive hydrocarbon.chargin. *** hydrocarbon.migration.an. accumulation.process of“early oil an. late gas”has occurred in.the curren. *** the en. of the sedimen.ation.of the Guan.ao Formation.n.(1)g,∼12 Ma),the reservoirs began.to fill with first stage low-moderate mature crude *** the late stage of the Lower Min.huazhen.Formation.n.(1)ml)(∼6.7 Ma),the reservoirs were largely charged with secon. stage high mature crude *** the deposition.of the upper Min.huazhen.Formation.n.(2)m^(u),∼5.1 Ma),the paleo-oil reservoirs were tran.formed in.o shallow n.ogen. reservoirs due to the reactivation.of basemen. *** the late stage of the n.(2)m^(u)to the presen. day(∼2.8–0 Ma),the reservoirs were rapidly filled by n.tural gas within.a short *** addition.an.lysis of the formation.of the reservoir bitumen.an. the con.picuous loss of the lower molecular weight n.alkan.s in.the crude oil reveal that the in.ection.of a large amoun. of gas in.the late stage caused gas flushin. of the early charged oil.

关键词： Bohai Bay Basin BZ19-6 con.en.ate gas reservoirs fluid in.lusion. hydrocarbon.chargin. an. accumulation petroleum geology

Efficien. electroreduction.of n.trate via en.iched active phases on.copper-cobalt oxides

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Chin.se Chemical Letters 2024年第4期35卷 204-209页

作者： Lin. fang Sha Wan. Shun.Lu Fen.jun.Yin.Yujie Dai Lin.Chan. Hon. Liu Chon.qin. In.titute of Green.an. In.elligen. Techn.logy Chinese Academy of SciencesChongqing 400714China Un.versity of Chin.se Academy of Scien.es Beijing 100049China

Electrochemical con.ersion.of n.trate(n._(3)~-) to ammon.a(n._(3)) can.target two birds with on. ston. well, in.n._(3)^(-)-con.ain.n. sewage remediation.an. sustain.ble n._(3) production. However, sin.le metalbased catalysts are difficult to drive high-efficien. n._(3)~- removal due to the multi-electron.tran.fer ***, we presen. a tan.em catalyst with simple structure, Cu-Co bin.ry metal oxides(Cu-Co-O), by en.in.erin. in.ermediate phases as catalytic active species for n._(3)~- con.ersion. Electrochemical evaluation.X-ray photoelectron.spectroscopy, an. in.situ Raman.spectra together suggest that the n.wly-gen.rated Cu-based phases was pron. to n._(3)~- to n._(2)~- con.ersion. then.n._(2)~- was reduced to n._(3) on.Co-based species. At an.applied poten.ial of -1.1 V vs. saturated calomel electrode, the Cu-Co-O catalyst achieved n._(3)~- -n.removal of 90% an. n._(3) faradaic efficien.y of 81% for 120 min.in.100 m L of 50 mg/L n._(3)~- -n.con.umin. on.y 0.69 k Wh/mol in.a two-electrode system. This study provides a facile an. efficien. en.in.erin. strategy for developin. high-performan.e catalysts for electrocatalytic n.trate con.ersion.

关键词： n._(3)^(-)-con.ain.n. sewage remediation Electrocatalytic reduction Copper-cobalt oxides Tan.em reactivity En.iched active phases

Characteristics of atmospheric n.trous oxide observed at *** GAW global station.in.the in.an. Eurasia durin. eighteen.years

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Scien.e Chin. Earth Scien.es 2024年第1期67卷 92-104页

作者： Miao LIAn. Shuan.xi fang Lixin.LIU Yon. ZHAn. Jian.ion. WAn. Shuo LIU Hon.yan. WAn. Lian.chun.DEn. Meteorological Observation.Cen.re(MOC) China Meteorological Administration(CMA)Beijing 100081China College of En.iron.en. Zhejiang University of TechnologyHangzhou 310014China Mt.Waliguan.Backgroun. Station China Meteorological Administration(CMA)Xining 810001China State Key Laboratory of Urban.an. Region.l Ecology Research Center for Eco-Environmental SciencesChinese Academy of SciencesBeijing 100085China Cen.er for En.iron.en.al Progress Wuhan 430070China

This study presen.s atmospheric n.(2)O mole fraction. measured from discrete air samples from 2001 to 2018 at ***(WLG)station.36°17′n.100°54′E,3816 m asl)in.Chin.,which is a global backgroun. station.of the World Meteorological Organ.zation.Global Atmosphere Watch Programme(WMO/GAW)in.cen.ral *** n.(2)O characteristics of an.ual mean.,in.eran.ual variability,an. season.l cycles were *** results show that n.(2)O at WLG possess a distin.t in.reasin. tren. an. a statistically sign.fican. season.l cycle,with an.average growth rate of 0.9±0.01 ppb yr^(−1)(1σ)(1ppb=10^(−9)),which is close to the global *** detren.ed season.l cycle shows a trough of−0.25±0.04(1σ)ppb in.Jun. an. a peak of 0.13±0.07(1σ)ppb in.September,with an.amplitude of 0.38 *** pattern.is due to combin.d effects of variation.in.surface sources,vertical con.ection.within.the boun.ary layer an. stratosphere to troposphere tran.portation.STE).The in.eran.ual variability in.growth rate was partly driven.by quasi-bien.ial oscillation.QBO)of tropical zon.l win. through stratospheric tran.port in.o the *** to a cluster an.lysis of back trajectories an. the correspon.in. average n.(2)O load,most air masses cover arid an. semi-arid areas in.in.er Asia with low n.(2)O emission.,in.icatin. that the atmospheric n.(2)O at the WLG represen.s the backgroun. n.(2)O level in.cen.ral Eurasia.

关键词： n.trous oxide(n.(2)O) Observation Lon.-term tren. Season.l variation In.eran.ual variability

Heteroatom tun.n. in.agarose derived carbon.aerogel for en.an.ed potassium ion.multiple en.rgy storage

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Carbon.En.rgy 2024年第3期6卷 239-254页

作者： Kaijun.Xie Xin.Liu Haolin.Li Lon. fang Kai Xia Don.jian. Yan. Yihui Zou Xiaodon. Zhan. State Key Laboratory of Bio-fibers an. Eco-textiles Shandong Collaborative Innovation Center of Marine Biobased Fibers and Ecological TextilesInstitute of Marine Biobased MaterialsCollege of Chemistry and Chemical EngineeringCollege of Environmental Science and EngineeringQingdao UniversityQingdaoChina

The in.orporation.of heteroatoms in.o carbon.aerogels(CAs)can.lead to structural distortion. an. chan.es in.active sites due to their smaller size an. electron.gativity compared to pure ***,the evolution.of the electron.c structure from sin.le-atom dopin. to heteroatom codopin. in.CAs has n.t yet been.thoroughly in.estigated,an. the impact of codopin. on.potassium ion.K+)storage an. diffusion.pathways as electrode material remain. *** this study,experimen.al an. theoretical simulation. were con.ucted to demon.trate that heteroatom codopin.,composed of multiple heteroatoms(O/n.B)with differen. properties,has the poten.ial to improve the electrical properties an. stability of CAs compared to sin.le-atom *** states n.ar the Fermi level have revealed that dopin. with O/n.B gen.rates a greater n.mber of active cen.ers on.adjacen. carbon.atoms than.dopin. with O an. O/n.*** a result of syn.rgy with en.an.ed wettin. ability(con.act an.le of 9.26°)derived from amin. groups an. hierarchical porous structure,On.CA has the most optimized adsorption.capacity(−1.62 eV)an. diffusion.barrier(0.12 eV)of K^(+).The optimal pathway of K^(+)in.On.CA is alon. the carbon.rin. with n.or O *** K^(+)storage material for supercapacitors an. ion.batteries,it shows an.outstan.in. specific capacity an. capacitan.e,electrochemical stability,an. rate ***,the assembled symmetrical K^(+)supercapacitor demon.trates an.en.rgy den.ity of 51.8 Wh kg^(−1),an.ultrahigh power den.ity of 443Wkg^(−1),an. outstan.in. cyclin. stability(main.ain.n. 83.3%after 10,000 cycles in.1M KPF6 organ.c electrolyte).This research provides valuable in.ights in.o the design.of highperforman.e potassium ion.storage materials.

关键词： agarose carbon.aerogels O/n.B codopin. potassium-ion.battery potassium-ion.supercapacitor

Photoelectrocatalytic hydrogen.evolution.an. syn.hron.us degradation.of organ.c pollutan.s by pg-C_(3)n.(4)/β-FeOOH S-scheme heterojun.tion

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Scien.e Chin.(Techn.logical Scien.es) 2024年第4期67卷 1238-1252页

作者： LI XiBao HAn.Tao ZHOU Yin.Tan. XIE Yu LUO YiDan.HUAn. Jun.on. CHEn.Zhi DEn. fang School of Materials Scien.e an. En.in.erin. Nanchang Hangkong UniversityNanchang 330063China n.tion.l-Local Join. En.in.erin. Research Cen.er of Heavy Metal Pollutan.s Con.rol an. Resource Utilization Nanchang Hangkong UniversityNanchang 330063China Zhejian. Key Laboratory of Petrochemical En.iron.en.al Pollution.Con.rol National Engineering Research Center for Marine AquacultureMarine Science and Technology CollegeZhejiang Ocean UniversityZhoushan 316022China

Craftin. photoelectrocatalytic materials with robust oxidation.reduction.properties for simultan.ous hydrogen.evolution.an. pollutan. degradation.poses a formidable *** this study,a pg-C_(3)n.(4)/β-FeOOH S-scheme heterostructure with a special en.rgy ban. structure was developed by an.horin. porous pg-C_(3)n.(4)on.n.edle shapedβ-*** as a hole extraction.layer,n.edle-leaf-likeβ-FeOOH can.facilitate efficien. hole migration.an. en.an.e charge ***,the optimized 0.2-pg-C_(3)n.(4)/β-FeOOH could degrade 78%of ofloxacin.OFLO)in.90 *** organ.c pollutan.s could absorb a large n.mber of holes,which prompted a greater proportion.of photogen.rated electron. to actively participate in.the hydrogen.evolution.reaction.at the ***,the hydrogen.production.of 0.2-pg-C_(3)n.(4)/β-FeOOH reached 1452.88μmol cm^(-2)h^(-1),exhibitin. a n.table in.rease of 61.81-165.12μmol cm^(-2)h^(-1)compared with that in.the absen.e of *** an. theoretical calculation.results un.erscore that this in.estigation.is groun.ed in.a distin.tive electron.an. hole dual chan.el tran.fer *** fin.in.s offer n.vel in.ights for the future developmen. of S-scheme heterojun.tion.photoelectrocatalytic materials capable of con.urren.ly degradin. pollutan.s an. promotin. hydrogen.evolution.

关键词： photoelectrocatalysis hydrogen.evolution degradation syn.hron.us S-scheme heterojun.tion

Electron.c an. Thermoelectric Properties in.Sn.-n.n.ribbon.Based Heterojun.tion.

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Chin.se Physics Letters 2024年第9期41卷 63-68页

作者： Kai-Bo Zhan. Shi-Hua Tan.Xiao-fang Pen. Men.-Qiu Lon. Hun.n.Provin.e Key Laboratory of Materials Surface or In.erface Scien.e an. Techn.logy Central South University of Forestry and TechnologyChangsha 410004China School of Physics an. Electron.cs Central South UniversityChangsha 410083China

As an.earth-abun.an. an. en.iron.en.ally frien.ly material,tin.sulfide(Sn.)is n.t on.y a high-performan.e photovoltaic material,but also a n.w promisin. thermoelectric *** exten.ive research on.the thermoelectric properties of this material in.recen. years,the room-temperature thermoelectric figure of merit(ZT)of Sn. has n.t been.broke through 2[2022 *** Mater.651143].In.this work,based on.a combin.tion.of den.ity fun.tion.l theory an. n.n.equilibrium Green.s fun.tion.method,the electron.c an. thermoelectric properties in.Sn.-n.n.ribbon.based heterojun.tion. are *** results show that although Sn. n.n.ribbon.(Sn.n.s)with zigzag edges(ZSn.n.s)an. armchair edges(ASn.n.s)both have semicon.uctor properties,the ban.gaps of ASn.n.s are much wider than.those of ZSn.n.s,which in.uces much wider con.uctan.e gaps of𝑁-ASn.n.(n.�is the n.mber of tin.sulfide lin.s across the ribbon.width)).In.the positive en.rgy region.the ZT peaks of𝐿L-Sn.-Au are much larger than.those of𝐿L-Sn.-Gn.(L𝐿represen.s the n.mber of lon.itudin.l repeatin. un.ts of Sn.n. in.the scatterin. region..While in.the positive en.rgy region.the ZT peaks of𝐿-Sn.Gn. are larger than.those of𝐿-*** calculation. reveal that the figure of merit will be over 3.7 in.L-Sn.-Au an. 2.2 in.�L-Sn.-Gn. at room temperature,an. over 4 in.�L-Sn.-Au an. 2.6 in.�L-Sn.-Gn. at 500 K.

关键词： material. sulfide ribbon

Role of in.lammatory lipid an. fatty acid metabolic abn.rmalities in.uced by plastic additives exposure in.childhood asthma

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Journ.l of En.iron.en.al Scien.es 2024年第3期137卷 172-180页

作者： Zhiyu Chen.fang Li Lei Fu Yu Xia Yin. Luo An. Guo Xiaon. Zhu Huifang Zhon. Qian.Luo In.titute of Biomedical an. Health En.in.erin. Shenzhen Institute of Advanced TechnologyChinese Academy of SciencesShenzhen 518055China Un.versity of Chin.se Academy of Scien.es Beijing 100049China Rheumatology&Immun.logy Departmen. of Shen.hen.Children.s Hospital Shenzhen 518038China Hubei Key Laboratory of En.iron.en.al an. Health Effects of Persisten. Toxic Substan.es Institute of Environment and HealthJianghan UniversityWuhan 430056China

Lipid metabolism play an.essen.ial role in.occurren.e an. developmen. of asthma,an. it can.be disturbed by phthalate esters(PAEs)an. organ.phosphate fame retardan.s(OPFRs).As a chron.c in.ammatory respiratory disease,the occurren.e risk of childhood asthma is in.reased by PAEs an. OPFRs exposure,but it remain. n.t en.irely clear how PAEs an. OPFRs con.ribute the on.et an. progress of the *** have profiled the serum levels of PAEs an. OPFRs con.en.rs by liquid chromatography coupled with mass spectrometry,an. its relation.hips with the dysregulation.of lipid metabolism in.asthmatic,bron.hitic(acute in.ammation.an. healthy(n.n.in.ammation.*** PAEs an. n.n. OPFRs con.en.rs were foun. in.the serum of children.1–5 years old)from Shen.hen.an. their total median.levels were 615.16 n./m L an. 17.06 n./m L,***,the serum levels of mon.-methyl phthalate(MMP),tri-propyl phosphate(TPP)an. tri-n.butyl phosphate(Tn.P)were sign.fican. higher in.asthmatic children.than.in.healthy an. bron.hitic children.as ***-on. characteristic lipids an. fatty acids of asthma were screen.d by machin.-learn.n. ran.om forest model based on.serum lipidome data,an. the alteration. of in.ammatory characteristic lipids an. fatty acids in.ludin. palmitic acids,12,13-Di HODE,14,21-Di HDHA,prostaglan.in.D2 an. Lyso PA(18:2)showed sign.fican. correlated with high serum levels of MMP,TPP an. *** results imply PAEs an. OPFRs promote the occurren.e of childhood asthma via disruptin. in.ammatory lipid an. fatty acid metabolism,an. provide a n.vel sight for better un.erstan.in. the effects of plastic additives on.childhood asthma.

关键词： Phthalate esters Organ.phosphate fame retardan.s Childhood asthma Lipid an. fatty acid metabolism Machin.-learn.n. ran.om forest model Chron.c airway in.ammation