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Progress in electrocatalytic nitrate reduction for green energy:Catalyst engineering,mechanisms,and techno-economic feasibility

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Journal of Energy Chemistry 2024年第8期95卷 380-406,I0009页

作者： Hafiz muhammad Adeel Sharif Hafiz muhammad Farooq Khan Sadeeq Ullah Yuwei Wang muhammad Ahmad Bo Yang Changping Li muhammad bilal asif Research Center for Eco-Environmental Engineering Dongguan University of TechnologyDongguan 523808GuangdongChina College of Chemistry and Engineering Shenzhen UniversityShenzhen 518060GuangdongChina FMH College of Medicine and Dentistry LahorePakistan School of Environment and Civil Engineering Research Center for Eco-Environment EngineeringDongguan University of TechnologyDongguan 523106GuangdongChina Advanced Membranes and Porous Materials Center(AMPMC) Physical Sciences and Engineering(PSE)King Abdullah University of Science and Technology(KAUST)Thuwal 23955Saudi Arabia

Ammonia(NH_(3))is an irreplaceable chemical that has been widely demanded to keep the sustainable development of modern ***,its industrial production consumes a huge amount of energy and releases extraordinary greenhouse gases(GHGs),leading to various environmental *** the green production of ammonia is a great challenge,which has been extensively pursued in the last *** this review,the most promising strategy,electrochemical nitrate reduction reaction(e-NO_(3)RR),is comprehensively investigated to give a complete understanding of its development and mechanism and provide guidance for future ***,owing to the complex reactions and limited selectivity,a comprehensive understanding of the mechanisms is crucial to further development and ***,NO_(3)^(-)RR is a promising strategy for simultaneous water treatment and NH_(3)production.A detailed overview of the recent progress in NO_(3)^(-)RR for NH_(3)production with nontransition and transition metal based electrocatalysts is *** addition,critical advanced techniques,future challenges,and prospects are discussed to guide future research on transition metal-based catalysts for commercial NH_(3)synthesis by NO_(3)^(-)reduction.

关键词： Nitrate reduction Electrolysis Pollution to solution Transition metal catalysts Ammonia synthesis Green energy

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Phonon Thermal Transport at Interfaces of a Graphene/Vertically Aligned Carbon Nanotubes/Hexagonal Boron Nitride Sandwiched Heterostructure

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Chinese Physics Letters 2024年第1期41卷 57-62页

作者：李檬璘 muhammad asif Shakoori 王瑞鹏李海鹏 School of Materials Science and Physics China University of Mining and TechnologyXuzhou 221116China

Molecular dynamics simulation is used to calculate the interfacial thermal resistance of a graphene/carbon nanotubes/hexagonal boron nitride(Gr/CNTs/hBN)sandwiched heterostructure,in which vertically aligned carbon nanotube(VACNT)arrays are covalently bonded to graphene and hexagonal boron nitride *** find that the interfacial thermal resistance(ITR)of the Gr/VACNT/hBN sandwiched heterostructure is one to two orders of magnitude smaller than the ITR of a Gr/hBN van der Waals heterostructure with the same plane *** is observed that covalent bonding effectively enhances the phonon coupling between Gr and hBN layers,resulting in an increase in the overlap factor of phonon density of states between Gr and hBN,thus reducing the ITR of Gr and *** addition,the chirality,size(diameter and length),and packing density of sandwich-layer VACNTs have an important influence on the ITR of the *** the same CNT diameter and length,the ITR of the sandwiched heterostructure with armchair-shaped VACNTs is higher than that of the sandwiched heterostructure with zigzag-shaped VACNTs due to the different chemical bonding of chiral CNTs with Gr and *** the armchair-shaped CNT diameter increases or the length decreases,the ITR of the sandwiched heterostructure tends to ***,the increase in the VACNT packing density also leads to a continuous decrease in the ITR of the sandwiched heterostructure,attributed to the extremely high intrinsic thermal conductivity of CNTs and the increase of out-of-plane heat transfer *** work may be helpful for understanding the mechanism for ITR in multilayer vertical heterostructures,and provides theoretical guidance for a new strategy to regulate the interlayer thermal resistance of heterostructures by optimizing the design of sandwich layer thermal interface materials.

关键词： sandwich shaped packing

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A Comprehensive Systematic Review: Advancements in Skin Cancer Classification and Segmentation Using the ISIC Dataset

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Computer Modeling in Engineering & Sciences 2024年第9期140卷 2131-2164页

作者： Madiha Hameed Aneela Zameer muhammad asif Zahoor Raja Department of Computer Sciences Pakistan Institute of Engineering and Applied SciencesNilore50700Islamabad Future Technology Research Center National Yunlin University of Science and TechnologyDouliou64002Taiwan Directorate of IT Services University of GujratGujrat50700Pakistan

The International Skin Imaging Collaboration(ISIC)datasets are pivotal resources for researchers in machine learning for medical image analysis,especially in skin cancer *** datasets contain tens of thousands of dermoscopic photographs,each accompanied by gold-standard lesion diagnosis *** challenges associated with ISIC datasets have spurred significant advancements,with research papers reporting metrics surpassing those of human *** cancers are categorized into melanoma and non-melanoma types,with melanoma posing a greater threat due to its rapid potential for metastasis if left *** paper aims to address challenges in skin cancer detection via visual inspection and manual examination of skin lesion images,processes historically known for their *** notable advancements in machine learning and deep learning models,persistent challenges remain,largely due to the intricate nature of skin lesion *** review research on convolutional neural networks(CNNs)in skin cancer classification and segmentation,identifying issues like data duplication and augmentation *** explore the efficacy of Vision Transformers(ViTs)in overcoming these challenges within ISIC dataset *** leverage their capabilities to capture both global and local relationships within images,reducing data duplication and enhancing model ***,ViTs alleviate augmentation issues by effectively leveraging original *** a thorough examination of ViT-based methodologies,we illustrate their pivotal role in enhancing ISIC image classification and *** study offers valuable insights for researchers and practitioners looking to utilize ViTs for improved analysis of dermatological ***,this paper emphasizes the crucial role of mathematical and computational modeling processes in advancing skin cancer detection methodologies,highlighting their significance in improving algorithmic

关键词： Medical image skin cancer classification skin cancer segmentation international skin imaging collaboration convolutional neural network deep learning

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Characterization and physicochemical aspects of novel cellulose-based layered double hydroxide nanocomposite for removal of antimony and fluoride from aqueous solution

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Journal of Environmental Sciences 2021年第4期33卷 301-315页

作者： Hanen Bessaies Sidra Iftekhar muhammad bilal asif Jamel Kheriji Chaker Necibi Mika Sillanpää Bechir Hamrouni Laboratory of Desalination and Water Treatment LR19ES01 Faculty of Sciences of TunisTunis El Manar UniversityEl Manar I 2092Tunisia Department of Environmental Engineering University of Engineering and Technology TaxilaTaxila 47050Pakistan Department of Applied Physics University of Eastern FinlandKuopio 70210Finland A lnstitute of Environmental Engineering and Nano-Technology Tsinghua Shezhen International Graduate SchoolTsinghua UniversityShenzhen 518055China International Water Research Institute Mohammed VI Polythechnic UniversityGreen City Ben Guerir 43150Morocco Institute of Research and Development Duy Tan UniversityDa Nang 550000Vietnam Faculty of Environment and Chemical Engineering Duy Tan UniversityDa Nang 550000Vietnam School of Civil Engineering and Surveying Faculty of HealthEngineering and SciencesUniversity of Southern QueenslandWest StreetToowoombaQLD 4350Australia Department of Chemical Engineering School of MiningMetallurgy and Chemical EngineeringUniversity of JohannesburgDoornfontein 2028South Africa

A series of novel adsorbents composed of cellulose(CL)with Ca/Al layered double hydroxide(CC_(x)A;where x represent the Ca/Al molar ratio)were prepared for the adsorption of antimony(Sb(V))and fluoride(F^(-))ions from aqueous *** CC_(x)A was characterized by Fourier-transform infrared spectroscopy(FTIR),Brunauer–Emmett–Teller(BET),elemental analysis(CHNS/O),thermogravimetric analysis(TGA-DTA),zeta potential,X-ray photoelectron spectroscopy(XPS)and scanning electron microscopy with energy dispersive Xray spectroscopy(SEM-EDX)*** effects of varying parameters such as dose,pH,contact time,temperature and initial concentration on the adsorption process were *** to the obtained results,the adsorption processes were described by a pseudo-second-order kinetic *** adsorption isotherm model provided the best fit for the experimental data and was used to describe isotherm *** maximum adsorption capacity was found to be 77.2 and 63.1 mg/g for Sb(V)and F^(-),respectively by CC_(3)A(experimental conditions:pH 5.5,time 60 min,dose 15 mg/10 mL,temperature 298 K).The CC_(3)A nanocomposite was able to reduce the Sb(V)and F^(-)ions concentration in synthetic solution to lower than 6μg/L and 1.5 mg/L,respectively,which are maximum contaminant levels of these elements in drinking water according to WHO guidelines.

关键词： Layered double hydroxide Adsorption Antimony removal Fluoride removal Kinetics

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Modelling of debris-flow susceptibility and propagation: a case study from Northwest Himalaya

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Journal of Mountain Science 2024年第1期21卷 200-217页

作者： Hamza DAUD Javed Iqbal TANOLI Sardar muhammad asif muhammad QASIM muhammad ALI Junaid KHAN Zahid Imran BHATTI Ishtiaq Ahmad Khan JADOON Badong National Observation and Research Station of Geohazards China University of GeosciencesWuhan 430074China Department of Earth Sciences COMSATS University IslamabadAbbottabad Campus 22010Pakistan Department of Earth Sciences Sultan Qaboos UniversityAl-KhoudMascat 123Oman Faculty of Engineering China University of Geosciences(Wuhan)Wuhan 430074China Department of Earth Sciences Abbottabad University of Science and TechnologyHavelian 22500Pakistan

The geological and geographical position of the Northwest Himalayas makes it a vulnerable area for mass movements particularly landslides and debris flows. Mass movements have had a substantial impact on the study area which is extending along Karakorum Highway(KKH) from Besham to Chilas. Intense seismicity, deep gorges, steep terrain and extreme climatic events trigger multiple mountain hazards along the KKH, among which debris flow is recognized as the most destructive geohazard. This study aims to prepare a field-based debris flow inventory map at a regional scale along a 200 km stretch from Besham to Chilas. A total of 117 debris flows were identified in the field, and subsequently, a point-based debris-flow inventory and catchment delineation were performed through Arc GIS analysis. Regional scale debris flow susceptibility and propagation maps were prepared using Weighted Overlay Method(WOM) and Flow-R technique sequentially. Predisposing factors include slope, slope aspect, elevation, Topographic Roughness Index(TRI), Topographic Wetness Index(TWI), stream buffer, distance to faults, lithology rainfall, curvature, and collapsed material layer. The dataset was randomly divided into training data(75%) and validation data(25%). Results were validated through the Receiver Operator Characteristics(ROC) curve. Results show that Area Under the Curve(AUC) using WOM model is 79.2%. Flow-R propagation of debris flow shows that the 13.15%, 22.94%, and 63.91% areas are very high, high, and low susceptible to debris flow respectively. The propagation predicated by Flow-R validates the naturally occurring debris flow propagation as observed in the field surveys. The output of this research will provide valuable input to the decision makers for the site selection, designing of the prevention system, and for the protection of current infrastructure.

关键词： North Pakistan Debris flow Flow-R Propagation Susceptibility mapping Debris-flow inventory Weighted Overlay Method

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USpider-乌尔都语文本到SQL的数据集

USpider-乌尔都语文本到SQL的数据集

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作者： muhammad Waleed asif 中山大学

学位级别：硕士

在自然语言处理(NLP)领域中,文本到SQL转换上取得的显著进步,使得用自然语言与数据库交互成为可能。然而,它在低资源语言如乌尔都语上的表现不足。本研究提出USpider,一个乌尔都语文本到SQL转换数据集,旨在解决文本到SQL任务在乌尔都语... 详细信息

在自然语言处理(NLP)领域中,文本到SQL转换上取得的显著进步,使得用自然语言与数据库交互成为可能。然而,它在低资源语言如乌尔都语上的表现不足。本研究提出USpider,一个乌尔都语文本到SQL转换数据集,旨在解决文本到SQL任务在乌尔都语上的资源稀缺问题,为构建该领域在乌尔都语上的发展奠定基础。USpider包含9,693个乌尔都语自然语言问题及其对应的SQL查询,涉及133个不同领域的166个不同的数据库。数据集的创建采用严谨方法,结合机器翻译、人工改进和迭代审查,确保语言的准确性、连贯性和文化相关性。由此产生的高质量数据集展现了乌尔都语在数据库查询中的丰富性和复杂性。为了验证USpider的科研和使用价值,实验部分我们使用了大型语言模型(LLM),具体是GPT-3.5,应用DINSQL方法进行少样本学习。实验通过执行准确性和匹配准确性等指标进行评估,展示了模型在简单和中等难度查询上表现出色。对于简单查询,模型在不同测试批次中达到69%至72%的执行准确性和54%至58%的精确匹配准确性。对于中等难度查询,执行准确性和精确匹配准确性分别在59%至63%和42%至48%之间。这些发现证实了USpider在提高准确SQL查询方面的作用。然而,实验亦揭示了处理复杂查询和语言变化时的挑战。随着查询难度的增加,困难级别查询的执行准确性下降到40%-59%,非常困难级别的查询下降到38%-42%。精确匹配准确性在这些类别中分别在10%-34%和0%-23%之间。USpider数据集对乌尔都语社区将会具有重大意义,将能开启医疗保健、教育、金融和电子政务等领域数据库的自然语言接口。通过让乌尔都语使用者使用母语与技术互动,研究有助于缩小数字鸿沟,推动NLP的包容性。此外,本研究的发现将对更广泛的NLP领域,尤其是对低资源语言有重要启示。DINSQL方法成功应用于乌尔都语,,强调了为低资源语言专门构建数据集的重要性。USpider的创建方法将为其他语言中的类似挑战提供参考。未来的研究方向包括改进USpider以适应较弱的LLM,探索LLM的局限性,并适应Spider数据集的演变。随着Spider 2.0的预期发布,我将开发USpider 2.0,与它的查询复杂性和多样性的提高保持同步,同时利用LLM架构和训练技术的最新进展。总的来说,USpider为乌尔都语上的NLP研究作出了贡献,提供全面翻译的数据集,并证明了它在乌尔都语文本到SQL转换中的效用。实验结果展示了准确生成SQL查询的潜力,同时指出了需要改进的方面。这项研究为开发兼容性强和可用性高的数据库自然语言接口奠定了基础,赋能乌尔都语社区,推动低资源语言NLP领域的发展。

关键词：文本到SQL 语义解析少样本学习大型语言模型 USpider

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Design of an Efficient and Provable Secure Key Exchange Protocol for HTTP Cookies

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Computers, Materials & Continua 2024年第7期80卷 263-280页

作者： Waseem Akram Khalid Mahmood Hafiz Burhan ul Haq muhammad asif Shehzad Ashraf Chaudhry Taeshik Shon Graduate School of Engineering Science and Technology National Yunlin University of Science and TechnologyYunlin64002Taiwan Future Technology Research Center National Yunlin University of Science and TechnologyYunlin64002Taiwan Department of Computer Science Lahore Garrison UniversityLahore54920Pakistan Department of Computer Science and Information Technology College of EngineeringAbu Dhabi UniversityAbu Dhabi69911United Arab Emirates Department of Software Engineering Faculty of Engineering and ArchitectureNisantasi UniversityIstanbul34398Turkey Department of Cybersecurity Ajou UniversitySuwon16499Republic of Korea

Cookies are considered a fundamental means of web application services for authenticating various Hypertext Transfer Protocol(HTTP)requests andmaintains the states of clients’information over the *** cookies are exploited to carry client patterns observed by a *** client patterns facilitate the particular client’s future visit to the corresponding ***,security and privacy are the primary concerns owing to the value of information over public channels and the storage of client information on the *** protocols have been introduced that maintain HTTP cookies,but many of those fail to achieve the required security,or require a lot of resource *** this article,we have introduced a lightweight Elliptic Curve Cryptographic(ECC)based protocol for authenticating client and server transactions to maintain the privacy and security of HTTP *** proposed protocol uses a secret key embedded within a *** proposed protocol ismore efficient and lightweight than related protocols because of its reduced computation,storage,and communication ***,the analysis presented in this paper confirms that proposed protocol resists various known attacks.

关键词： Cookies authentication protocol impersonation attack ECC

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Quintessence anisotropic stellar models in quadratic and Born-Infeld modified teleparallel Rastall gravity

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Chinese Physics B 2024年第3期33卷 179-189页

作者： Allah Ditta 夏铁成 Irfan Mahmood asif Mahmood Department of Mathematics Shanghai University and Newtouch Center for Mathematics of Shanghai UniversityShanghai 200444China Centre for High Energy Physics University of the PunjabLahorePakistan College of Engineering Chemical Engineering DepartmentKing Saud University RiyadhSaudi Arabia

This study aims to discuss anisotropic solutions that are spherically symmetric in the quintessence field,which describe compact stellar objects in the modified Rastall teleparallel theory of *** achieve this goal,the Krori and Barua arrangement for spherically symmetric components of the line element is *** explore the field equations by selecting appropriate off-diagonal tetrad ***-Infeld function of torsion f(T)=β√λT+1-1 and power law form h(T)=δTn are *** Born-Infeld gravity was the first modified teleparallel gravity to discuss *** use the linear equation of state pr=ξρto separate the quintessence *** obtaining the field equations,we investigate different physical parameters that demonstrate the stability and physical acceptability of the stellar *** use observational data,such as the mass and radius of the compact star candidates PSRJ 1416-2230,Cen X-3,&4U 1820-30,to ensure the physical plausibility of our findings.

关键词： anisotropic spheres quintessence field modified Rastall teleparallel gravity equation of state(EoS) f(T)gravity

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Synthesis and Thermal Characterization of Solar Salt-Based Phase Change Composites with Graphene Nanoplatelets

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Journal of Thermal Science 2024年第2期33卷 491-500页

作者： Pethurajan VIGNESHWARAN Saboor SHAIK Sivan SURESH Müslüm ARICI asif AFZAL Department of Thermal and Energy Engineering School of Mechanical Engineering(SMEC)Vellore Institute of TechnologyVelloreTamil NaduIndia Nanotechnology Research Laboratory Department of Mechanical EngineeringNational Institute of TechnologyTiruchirappalliTamil NaduIndia Mechanical Engineering Department Engineering FacultyKocaeli UniversityUmuttepe CampusKocaeli41001Turkey Department of Mechanical Engineering P.A.College of Engineering(affiliated to Visvesvaraya Technological UniversityBelagavi)Mangaluru574153India

Thermal energy storage(TES) systems use solar energy despite its irregular availability and day-night temperature *** work reports the thermal characterizations of solar salt-based phase change composites in the presence of graphene nanoplatelets(GNP).Solar salt(60:40 of NaNO_(3):KNO_(3)) possessing phase transition temperature and melting enthalpy of 221.01℃ and 134.58 kJ/kg is proposed as a phase change material(PCM) for high-temperature solar-based energy storage *** conductivity must be improved to make them suitable for widespread applications and to close the gap between the system needs where they are *** is added at weight concentrations of 0.1%,0.3%,and 0.5% with solar salt using the ball milling method to boost its thermal *** studies indicated the formation of a uniform surface of GNP on solar *** spectrum peaks identified the physical interaction between salt and *** characterization of the composites,such as thermal conductivity,DSC and TGA was carried out for the samples earlier and later 300 thermal cycles.0.5% of GNP has improved the thermal conductivity of salt by 129.67% and after thermal cycling,the enhancement reduced to 125.21% indicating that thermal cycling has a minor impact on thermal *** change temperature decreased by around 2.32% in the presence of0.5% GNP and the latent heat reduced by 4.34% after thermal *** thermograms depicted the composites initiated the weight loss at around 550℃ after which it was *** thermal cycling,the weight loss initiated at ~40℃ lower compared to pure salt,which was found to be a minor *** characterization of solar salt and GNP-based solar salt composites revealed that the composites can be used for enhanced heat transfer in high-temperature solar-based heat transfer and energy storage applications.

关键词： thermal energy storage high temperature solar salt graphene nanoplatelets thermal characterization

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Caching Strategies in NDN Based Wireless Ad Hoc Network:A Survey

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Computers, Materials & Continua 2024年第7期80卷 61-103页

作者： Ahmed Khalid Rana asif Rehman Byung-Seo Kim Department of Computer Science FAST School of ComputingNational University of Computer and Emerging SciencesLahore54000Pakistan Department of Software and Communications Engineering Hongik UniversitySejong City30016Republic of Korea

Wireless Ad Hoc Networks consist of devices that are wirelessly *** Ad Hoc Networks(MANETs),Internet of Things(IoT),and Vehicular Ad Hoc Networks(VANETs)are the main domains of wireless ad hoc *** is used in wireless ad hoc *** is based on Transmission Control Protocol(TCP)/Internet Protocol(IP)network where clients and servers interact with each other with the help of IP in a pre-defined *** fetches data from a fixed *** redundancy,mobility,and location dependency are the main issues of the IP network *** these factors result in poor performance of wireless ad hoc *** main disadvantage of IP is that,it does not provide in-network ***,there is a need to move towards a new network that overcomes these *** Data Network(NDN)is a network that overcomes these *** is a project of Information-centric Network(ICN).NDN provides in-network caching which helps in fast response to user *** NDN in wireless ad hoc network provides many benefits such as caching,mobility,scalability,security,and *** considering the certainty,in this survey paper,we present a comprehensive survey on Caching Strategies in NDN-based Wireless *** cachingmechanism-based results are also *** the last,we also shed light on the challenges and future directions of this promising field to provide a clear understanding of what caching-related problems exist in NDN-based wireless ad hoc networks.

关键词： Content centric network Internet of Things mobile ad hoc network named data network vehicular ad hoc network

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