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metrology for sub-Rayleigh-length target positioning in~10^(22)W/cm^(2)laser-plasma experiments

high Power Laser science and Engineering 2024年第3期12卷 90-105页

作者： E.A.Vishnyakov A.sagisaka K.Ogura T.Zh.Esirkepov B.Gonzalez-Izquierdo C.d.Armstrong T.A.Pikuz s.A.Pikuz W.yan T.m.Jeong s.singh P.hadjisolomou O.Finke G.m.Grittani m.Nevrkla C.m.Lazzarini A.Velyhan T.hayakawa y.Fukuda J.K.Koga m.Ishino K.Kondo y.miyasaka A.Kon m.Nishikino y.V.Nosach d.Khikhlukha I.P.Tsygvintsev d.Kumar J.Nejdl d.margarone P.V.sasorov s.Weber m.Kando h.Kiriyama y.Kato G.Korn K.Kondo s.V.Bulanov T.Kawachi A.s.Pirozhkov ELI Beamlines Facility The Extreme Light Infrastructure ERICDolníBrežanyCzech Republic Kansai Institute for Photon science(KPsI) QSTKyotoJapan Central Laser Facility Rutherford Appleton LaboratorySTFCHarwell OxfordDidcotUK Institute for Open and Transdisciplinary Research Initiatives Osaka UniversityOsakaJapan hB11 Energy holdings FreshwaterAustralia Key Laboratory for Laser Plasmas(ministry of Education) School of Physics and AstronomyShanghai Jiao Tong UniversityShanghaiChina Collaborative Innovation Center of IFsA Shanghai Jiao Tong UniversityShanghaiChina Institute of Plasma Physics AsCR PragueCzech Republic FZU-Institute of Physics AsCR PragueCzech Republic Czech Technical University in Prague FNSPEPragueCzech Republic Institute of Laser Engineering Osaka UniversityOsakaJapan Institute of Physics National Academy of Sciences of UkraineKyivUkraine IsTEQ AR YerevanArmenia

Tight focusing with very small f-numbers is necessary to achieve the highest at-focus ***,tight focusing imposes strong demands on precise target positioning in-focus to achieve the highest on-target irradiance We describe several near-infrared,visible,ultraviolet and soft and hard X-ray diagnostics employed in a~10^(22)W/cm^(2)laser±plasma *** used nearly 10 J total energy femtosecond laser pulses focused into an approximately1.3-μm focal spot on 5±20μm thick stainless-steel *** discuss the applicability of these diagnostics to determine the best in-focus target position with approximately 5μm accuracy(i.e.,around half of the short Rayleigh length)and show that several diagnostics(in particular,3ωreflection and on-axis hard X-rays)can ensure this *** demonstrated target positioning within several micrometers from the focus,ensuring over 80%of the ideal peak laser intensity *** approach is relatively fast(it requires 10±20 laser shots)and does not rely on the coincidence of low-power and high-power focal planes.

关键词： laser-plasma interaction precise target positioning spectroscopy ultra-high intensity X-rays

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Tilted global solar irradiance in Bahrain:an experimental study

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Clean Energy 2024年第2期8卷 27-34页

作者： N.Vasilikos C.Georgantopoulou h.Alajaimi s.h.Almajed m.Ahmed d.mathioulakis school of mechanical Engineering Bahrain PolytechnicIsa TownPO Box 33349Kingdom of Bahrain school of mechanical Engineering National Technical University of AthensHeroon Polytechniou 7 StZografos 15773AthensGreece

In the present work,tilted global solar irradiance data are presented and analysed,measured for a period of 1 year on the campus of Bahrain Polytechnic,Kingdom of Bahrain,from both a fixed photovoltaic panel and a moving one via a two-axis solar *** fixed panel faces south with an angle of 26°with respect to the horizontal,coinciding with the local geographical *** second panel is moved by two motors,controlled by a global positioning system and suitable software so that the sun’s rays are perpendicular to the panel surface.A pyranometer is installed on each panel,recording the tilted global solar irradiance,stored by using a data *** analysis of the data obtained shows a 33%solar energy gain on an annual basis for the moving panel(2780 versus 2088 kWh/m^(2) on the fixed panel).more importantly,in June,when the energy demand in Bahrain is elevated due to the increased residential cooling loads,the solar energy received by the moving panel is 54.7%higher compared with that of the fixed *** a percentage basis,the increase in solar energy from the moving panel is profound in the early morning and late evening ***,the reduction in the solar energy received by the fixed panel from may to June does not appear in the moving panel because of the adjustable orientation of the *** the year,the mean daily solar power varies between 0.37 and 0.56 kW/m^(2) for the fixed panel,and 0.45 and 0.70 kW/m^(2) for the moving *** winter,solar energy fluctuations are elevated due to erratic weather conditions that present a peak standard deviation of 28%of the corresponding *** data presented are useful for potential solar investments in Gulf countries.

关键词： tilted solar irradiance renewable energy solar tracking photovoltaic Gulf Cooperation Council Countries

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sTCF conceptual design report (Volume 1): Physics & detector

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Frontiers of physics 2024年第1期19卷 1-154页

作者： m.Achasov X.C.Ai L.P.An R.Aliberti Q.An X.Z.Bai y.Bai O.Bakina A.Barnyakov V.Blinov V.Bobrovnikov d.Bodrov A.Bogomyagkov A.Bondar I.Boyko Z.h.Bu F.m.Cai h.Cai J.J.Cao Q.h.Cao X.Cao Z.Cao Q.Chang K.T.Chao d.y.Chen h.Chen h.X.Chen J.F.Chen K.Chen L.L.Chen P.Chen s.L.Chen s.m.Chen s.Chen s.P.Chen W.Chen X.Chen X.F.Chen X.R.Chen y.Chen y.Q.Chen h.y.Cheng J.Cheng s.Cheng T.G.Cheng J.P.dai L.y.dai X.C.dai d.dedovich A.denig I.denisenko J.m.dias d.Z.ding L.y.dong W.h.dong V.druzhinin d.s.du y.J.du Z.G.du L.m.duan d.Epifanov y.L.Fan s.s.Fang Z.J.Fang G.Fedotovich C.Q.Feng X.Feng y.T.Feng J.L.Fu J.Gao y.N.Gao P.s.Ge C.Q.Geng L.s.Geng A.Gilman L.Gong T.Gong B.Gou W.Gradl J.L.Gu A.Guevara L.C.Gui A.Q.Guo F.K.Guo J.C.Guo J.Guo y.P.Guo Z.h.Guo A.Guskov K.L.han L.han m.han X.Q.hao J.B.he s.Q.he X.G.he y.L.he Z.B.he Z.X.heng B.L.hou T.J.hou y.R.hou C.y.hu h.m.hu K.hu R.J.hu W.h.hu X.h.hu y.C.hu J.hua G.s.huang J.s.huang m.huang Q.y.huang W.Q.huang X.T.huang X.J.huang y.B.huang y.s.huang N.hüsken V.Ivanov Q.P.Ji J.J.Jia s.Jia Z.K.Jia h.B.Jiang J.Jiang s.Z.Jiang J.B.Jiao Z.Jiao h.J.Jing X.L.Kang X.s.Kang B.C.Ke m.Kenzie A.Khoukaz I.Koop E.Kravchenko A.Kuzmin y.Lei E.Levichev C.h.Li C.Li d.y.Li F.Li G.Li G.Li h.B.Li h.Li h.N.Li h.J.Li h.L.Li J.m.Li J.Li L.Li L.Li L.y.Li N.Li P.R.Li R.h.Li s.Li T.Li W.J.Li X.Li X.h.Li X.Q.Li X.h.Li y.Li y.y.Li Z.J.Li h.Liang J.h.Liang y.T.Liang G.R.Liao L.Z.Liao y.Liao C.X.Lin d.X.Lin X.s.Lin B.J.Liu C.W.Liu d.Liu F.Liu G.m.Liu h.B.Liu J.Liu J.J.Liu J.B.Liu K.Liu K.y.Liu K.Liu L.Liu Q.Liu s.B.Liu T.Liu X.Liu y.W.Liu y.Liu y.L.Liu Z.Q.Liu Z.y.Liu Z.W.Liu I.Logashenko y.Long C.G.Lu J.X.Lu N.Lu Q.F.Lü y.Lu y.Lu Z.Lu P.Lukin F.J.Luo T.Luo X.F.Luo y.h.Luo h.J.Lyu X.R.Lyu J.P.ma P.ma y.ma y.m.ma F.maas s.malde d.matvienko Z.X.meng R.mitchell A.Nefediev y.Nefedov s.L.Olsen Q.Ouyang P.Pakhlov G.Pakhlova X.Pan y.Pan E.Passemar y.P.Pei h.P.Peng L.Peng X.y.Peng X.J.Peng K.Peters s.Pivovarov E.Pyata B.B.Qi y.Q.Qi W.B.Qian y.Qian C.F.Qiao J.J.Qin J.J.Qin L.Q.Qin X.s.Qin T.L.Qiu J.Rademacker C.F.Redmer h.y.sang Anhui University Hefei 230039China Beihang University Beijing 100191China Budker Institute of Nuclear Physics Novosibirsk 630090Russia CAs Key Laboratory of Theoretical Physics Institute of Theoretical PhysicsChinese Academy of SciencesBeijing 100190China Cavendish Laboratory University of CambridgeJJ Thomson AveCambridge CB30HEUnited Kingdom Central China Normal University Wuhan 430079China Central south University Changsha 410083China China University of Geosciences Wuhan 430074China China University of mining and Technology Xuzhou 221116China École Polytechnique Fédérale de Lausanne(EPFL) LausanneSwitzerland Fudan University Shanghai 200433China Goethe University Frankfurt D-60325 Frankfurt am MainGermany Guangxi Normal University Guilin 541004China Guangxi Uninversity Nanning 530004China hangzhou Institute for Advanced study UCASHangzhou 310024China hebei Normal University Shijiazhuang 050024China hebei University Baoding 071002China hefei University of Technology Hefei 230601China helmholtz Institute mainz Staudinger Weg 18D-55099 MainzGermany henan Normal University Xinxiang 453007China henan University Kaifeng 475004China high Energy Physics Center Chung-Ang UniversitySeoul 06974Korea higher school of Economy 11 Pokrovsky Bulvar Moscow 109028Russia huangshan University Huangshan 245000China hubei University of Automotive Technology Shiyan 442002China hunan Normal University Changsha 410081China hunan University of science and Technology Xiangtan 411201China hunan University Changsha 410082China Indiana University BloomingtonIndiana 47405USA Inner mongolia University Hohhot 010021China Institute of Advanced science Facilities Shenzhen 518107China Institute of high Energy Physics Chinese Academy of SciencesBeijing 100049China Institute of modern Physics Chinese Academy of SciencesLanzhou 730000China Institute of Physics Academia SinicaTaipeiTaiwan 11529China Institute of Theoretical Physics Chinese Academy of SciencesBeijing 100190China Jilin University Changch

The superτ-charm facility(sTCF)is an electron–positron collider proposed by the Chinese particle physics *** is designed to operate in a center-of-mass energy range from 2 to 7 GeV with a peak luminosity of 0.5×10^(35) cm^(–2)·s^(–1) or *** sTCF will produce a data sample about a factor of 100 larger than that of the presentτ-charm factory—the BEPCII,providing a unique platform for exploring the asymmetry of matter-antimatter(charge-parity violation),in-depth studies of the internal structure of hadrons and the nature of non-perturbative strong interactions,as well as searching for exotic hadrons and physics beyond the standard *** sTCF project in China is under development with an extensive R&d *** document presents the physics opportunities at the sTCF,describes conceptual designs of the sTCF detector system,and discusses future plans for detector R&d and physics case studies.

关键词： electron–positron collider tau-charm region high luminosity sTCF detector conceptual design

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Radioisotope production using lasers:From basic science to applications

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matter and Radiation at Extremes 2024年第3期9卷 31-44页

作者： m.R.d.Rodrigues A.Bonasera m.scisciò J.A.Pérez-hernández m.Ehret F.Filippi P.L.Andreoli m.huault h.Larreur d.singappuli d.molloy d.Raffestin m.Alonzo G.G.Rapisarda d.Lattuada G.L.Guardo C.Verona Fe.Consoli G.Petringa A.mcNamee m.La Cognata s.Palmerini T.Carriere m.Cipriani G.di Giorgio G.Cristofari R.de Angelis G.A.P.Cirrone d.margarone L.Giuffrida d.Batani P.Nicolai K.Batani R.Lera L.Volpe d.Giulietti s.Agarwal m.Krupka s.singh Fa.Consoli Cyclotron Institute Texas A&M UniversityCollege StationTexas 77840USA Laboratori Nazionali del sud Istituto Nazionale di Fisica Nucleare(LNS-INFN)CataniaItaly ENEA Fusion and Technologies for Nuclear Safety and Security Department-CFrascatiItaly Centro de Láseres Pulsados(clpu) VillamayorSpain Universidad de salamanca SalamancaSpain Centre Lasers Intenses et Applications(CELIA) Universitéde BordeauxCNRSCEATalenceFrance hB11 Energy holdings Pty FreshwaterNew South WalesAustralia school of mathematics and Physics Queen’s University BelfastBelfastUnited Kingdom dipartimento di Fisica e Astronomia“E.majorana ”Università di CataniaCataniaItaly Facoltàdi Ingegneria e Architettura Universitàdegli Studi di Enna“Kore”EnnaItaly dipartimento di Ingegneria Industriale Universitàdi Roma“Tor Vergata”RomaItaly dipartimento di Fisica e Geologia Universitàdegli Studi di PerugiaPerugiaItaly Istituto Nazionale di Fisica Nucleare Sezione di PerugiaPerugiaItaly ELI Beamlines Facility the Extreme Light Infrastructure ERICDolni BrezanyCzech Republic ETsIA Universidad Politécnica de MadridMadridSpain dipartimento Fisica “E.Fermi”Universitàdi Pisa and INFNPisaItaly FZU–Institute of Physics of Czech Academy of sciences PragueCzech Republic Institute of Plasma Physics of Czech Academy of sciences PragueCzech Republic

The discovery of chirped pulse amplification has led to great improvements in laser technology,enabling energetic laser beams to be compressed to pulse durations of tens of femtoseconds and focused to a few *** with energies of tens of meV can be accelerated using,for instance,target normal sheath acceleration and focused on secondary *** such conditions,nuclear reactions can occur,with the production of radioisotopes suitable for medical *** use of high-repetition lasers to produce such isotopes is competitive with conventional methods mostly based on *** this paper,we study the production of^(67)Cu,^(63)Zn,^(18)F,and^(11)C,which are currently used in positron emission tomography and other *** the same time,we study the reactions^(10)B(p,α)^(7)Be and^(70)Zn(p,4n)^(67)Ga to put further constraints on the proton distributions at different angles,as well as the reaction^(11)B(p,α)^(8)Be relevant for energy *** experiment was performed at the 1 PW laser facility at VegaⅢin salamanca,*** distributions of radioisotopes in the forward(with respect to the laser direction)and backward directions were measured using a high purity germanium *** results are in reasonable agreement with numerical estimates obtained following the approach of Kimura and Bonasera[*** ***.,sect.A 637,164–170(2011)].

关键词： purity estimates backward

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Assessment of bisphenols in children's toy and baby products in the middle East

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Emerging Contaminants 2024年第3期10卷 336-342页

作者： K.martínez-Guijarro B.Gevao m.Porcelli s.Al-salem saif Uddin m.Bahloul h.Taqi m.hajeyah d.Krishnan s.Rajagopalan A.Boota Environment Pollution and Climate Program Kuwait Institute for Scientific ResearchP.O.Box 23884SafatKuwait EPA Sierra Leone

A major concern from the scientific community has been raised since evidence of Bisphenol A(BP-A)can leach out from the products where they are incorporated as well as its endocrine disrupting effects observed in animals and ***-A and several related chemicals such as Bisphenol AP(BP-AP),Bisphenol B(BPeB),Bisphenol s(BPes),Bisphenol AF(BP-AF),Bisphenol(BPeP),Bisphenol Z(BP-Z)were analyzed in this ***-A and BP-s were the only bisphenols detected in the samples analyzed in this *** median(range;mean)concentrations of BP-A found in this study was 321 ng/g(11-200932;4893 ng/g).The analysis was carried out by sonicating 0.1 g of a cryo-milled sample aliquot in methanol followed by UPLC-ms/ms *** concentrations of BP-A were found in several products labeled as BP-A free such as nursing bottles which are particularly problematic from the children's exposure point of *** study presents the first reliable bisphenols in children's toys and baby products commercialized in the middle *** is,however,a need to continue monitoring these compounds,especially in low-cost toys,and the so-called BP-A-free products,which appear to have high levels of target contaminants and can pose an exposure risk for infants and children in the region.

关键词： Bisphenols Bisphenol A(BP-A) Bisphenol s(BPes) Children Toys

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The soft X-ray Imager(sXI)on the smILE mission

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Earth and Planetary Physics 2024年第1期8卷 5-14页

作者： s.sembay A.L.Alme d.Agnolon T.Arnold A.Beardmore A.Belén Balado margeli C.Bicknell C.Bouldin G.Branduardi-Raymont T.Crawford J.P.Breuer T.Buggey G.Butcher R.Canchal J.A.Carter A.Cheney y.Collado-Vega h.Connor T.Crawford N.Eaton C.Feldman C.Forsyth T.Frantzen G.Galgóczi J.Garcia G.y.Genov C.Gordillo h-P.Gröbelbauer m.Guedel y.Guo m.hailey d.hall R.hampson J.hasiba O.hetherington A.holland s-y.hsieh m.W.J.hubbard h.Jeszenszky m.Jones T.Kennedy K.Koch-mehrin s.Kögl s.Krucker K.d.Kuntz C.Lakin G.Laky O.Lylund A.martindale J.miguel mas hesse R.Nakamura K.Oksavik N.Østgaard h.Ottacher R.Ottensamer C.Pagani s.Parsons P.Patel J.Pearson G.Peikert F.s.Porter T.Pouliantis B.h.Qureshi W.Raab G.Randal A.m.Read N.m.m.Roque m.E.Rostad C.Runciman s.sachdev A.samsonov m.soman d.sibeck s.smit J.søndergaard R.speight s.stavland m.steller TianRan sun J.Thornhill W.Thomas K.Ullaland B.Walsh d.Walton C.Wang s.yang school of Physics and Astronomy University of LeicesterLeicesterLE17RHUK space Park Leicester University of LeicesterLeicesterLE17RHUK mullard space science Laboratory University College LondonDorkingRH56NTUK Centre for Electronic Imaging Open UniversityMilton KeynesMK76 AAUK Birkeland Centre for space science Department of Physics and TechnologyUniv.of BergenN-5007 BergenNorway University of Vienna A-1010 ViennaAustria space Research Institute Austrian Academy of SciencesA-8042 GrazAustria National Institute of Aerospace Technology MadridSpain EsTEC European Space Agency2201 AZ NoordwijkNetherlands state Key Laboratory of space Weather National Space Science CentreBeijing 100190China University of Applied sciences and Arts Northwestern switzerland CH-5210 WindischSwitzerland Koegl space Gmbh CH-8157 DielsdorfSwitzerland space Acoustics Gmbh CH-8157 DielsdorfSwitzerland Zurich University of Applied sciences 8400 WinterhurSwitzerland Genov solutions N-5172 LoddefjordNorway sTm Engineering N-5165 LaksevagNorway John hopkins University Applied Physics Laboratory MD 20723USA NAsA/Goddard space Flight Centre MD 20771USA Center for space Physics Boston UniversityBostonMA 02215USA department of Theoretical Physics and Astrophysics Masaryk University60177 BrnoCzech Republic Institute of Physics E¨otvo¨s Lor´and University1053 BudapestHungary Aerospace Information Research Institute Chinese Academy of SciencesBeijing 100045China Centro de Astrobiologia(CAB) CSIC-INTAMadridSpain

The soft X-ray Imager(sXI)is part of the scientific payload of the solar wind magnetosphere Ionosphere Link Explorer(smILE)*** is a joint science mission between the European space Agency(EsA)and the Chinese Academy of sciences(CAs)and is due for launch in *** is a compact X-ray telescope with a wide field-of-view(FOV)capable of encompassing large portions of Earth’s magnetosphere from the vantage point of the smILE *** is sensitive to the soft X-rays produced by the solar Wind Charge eXchange(sWCX)process produced when heavy ions of solar wind origin interact with neutral particles in Earth’s *** provides a mechanism for boundary detection within the magnetosphere,such as the position of Earth’s magnetopause,because the solar wind heavy ions have a very low density in regions of closed magnetic field *** sensitivity of the sXI is such that it can potentially track movements of the magnetopause on timescales of a few minutes and the orbit of smILE will enable such movements to be tracked for segments lasting many *** is led by the University of Leicester in the United Kingdom(UK)with collaborating organisations on hardware,software and science support within the UK,Europe,China and the United states.

关键词： soft X-ray Imaging micropore optics large area CCd

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model dependent analysis of ■→■ decays in beyond standard model

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Chinese Physics C 2024年第9期48卷 86-99页

作者： s.mahata m.mandal h.mahapatra s.Biswas s.sahoo department of Physics National Institute of Technology Durgapur

motivated by the recent experimental results of branching fractions for ■→■ decays,which deviate from their sm predictions,we hve investigated these decays in W' model and scalar leptoquark model to determine potential signatures of new physics(NP) in semileptonic charm decays induced by c→■ *** recent experimental results of branching fractions for semileptonic d meson decays,new coupling parameters are predicted for the aforementioned NP *** fraction,forward-backward asymmetry,and lepton polarization asymmetry are examined by considering the predicted NP coupling *** results of branching fractions in scalar leptoquark model are found very close to the experimental results and exist around the range of 1σ *** presented a comparative study of the NP models to check their sensitivity on these *** anticipate that further research on these decays will significantly support our findings.

关键词： $ W' $ boson charm decay flavour changing charged current new physics scalar leptoquark

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model dependent analysis of d^(+)_(s)→η^(′)l+v_(l) decays in beyond standard model

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Chinese Physics C 2024年第9期48卷 82-95页

作者： s.mahata m.mandal h.mahapatra s.Biswas s.sahoo department of Physics National Institute of Technology Durgapur Durgapur 713209West BengalIndia

motivated by the recent experimental results of branching fractions for d^(+)_(s)→η^(′)l+v_(l) decays,which deviate from their sm predictions,we hve investigated these decays in W' model and scalar leptoquark model to determine potential signatures of new physics(NP) in semileptonic charm decays induced by c→(s,d)l+v_(l) *** recent experimental results of branching fractions for semileptonic d meson decays,new coupling parameters are predicted for the aforementioned NP *** fraction,forward-backward asymmetry,and lepton polarization asymmetry are examined by considering the predicted NP coupling *** results of branching fractions in scalar leptoquark model are found very close to the experimental results and exist around the range of 1σ *** presented a comparative study of the NP models to check their sensitivity on these *** anticipate that further research on these decays will significantly support our findings.

关键词： charm decay new physics W′boson scalar leptoquark flavour changing charged current

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Exact solutions for magnetohydrodynamic nanofluids flow and heat transfer over a permeable axisymmetric radially stretching/shrinking sheet

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Chinese Physics B 2024年第2期33卷 108-114页

作者： U.s.mahabaleshwar G.P.Vanitha L.m.Pérez Emad h.Aly I.Pop department of studies in mathematics Davangere UniversityShivagangothriDavangereIndia departamento de F´ısica FACIUniversidad de Tarapac´aCasilla 7DAricaChile department of mathematics Faculty of EducationAin Shams UniversityRoxyCairoEgypt department of mathematics Babes-Bolyai University400084 Cluj-NapocaRomania

We report on the magnetohydrodynamic impact on the axisymmetric flow of Al_(2)O_(3)/Cu nanoparticles suspended in h_(2)O past a stretched/shrinked *** the use of partial differential equations and the corresponding thermophysical characteristics of nanoparticles,the physical flow process is *** resultant nonlinear system of partial differential equations is converted into a system of ordinary differential equations using the suitable similarity *** transformed differential equations are solved *** of the magnetic parameter,solid volume fraction and stretching/shrinking parameter on momentum and temperature distribution have been analyzed and interpreted *** skin friction and Nusselt number were also *** addition,existence of dual solution was deduced for the shrinking sheet and unique solution for the stretching ***,Al_(2)O_(3)/h_(2)O nanofluid flow has better thermal conductivity on comparing with Cu/h_(2)O ***,it was found that the first solutions of the stream are stable and physically realizable,whereas those of the second ones are unstable.

关键词： magnetohydrodynamic nanofluid stretching/shrinking sheet axisymmetric flow analytical solution suction/injection

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Ferroelectricity Induced by Oxygen Vacancies in Rhombohedral ZrO_(2) Thin Films

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Energy & Environmental materials 2024年第1期7卷 229-237页

作者： Veniero Lenzi José P.B.silva Břetislav Šmíd Vladimir matoín Cosmin m.Istrate Corneliu Ghica Judith L.macmanus-driscoll Luís marques Physics Center of minho and Porto Universities(CF-Um-UP) University of MinhoCampus de Gualtar 4710-057Braga Portugal Laboratory of Physics for materials and Emergent Technologies LapMETUniversity of Minho4710-057Braga Portugal department of surface and Plasma science Faculty of Mathematics and PhysicsCharles UniversityV Holešovičkách 218000Prague 8 Czech Republic National Institute of materials Physics 105 bis Atomistilor 077125Magurele Romania department of materials science and metallurgy 27 Charles Babbage Rd.Cambridge CB3 OFSUK

Rhombohedral phase hf_(x)Zr_(1.x)O_(2)(hZO,x from 0 to 1)films are promising for achieving robust ferroelectric polarization without the need for an initial wake-up pre-cycling,as is normally the case for the more commonly studied orthorhombic ***,a large spontaneous polarization observed in rhombohedral films is not fully understood,and there are also large discrepancies between experimental and theoretical *** this work,in rhombohedral ZrO_(2)thin films,we show that oxygen vacancies are not only a key factor for stabilizing the phase,but they are also a source of ferroelectric polarization in the *** is shown experimentally through the investigation of the structural properties,chemical composition and the ferroelectric properties of the films before and after an annealing at moderate temperature(400℃)in an oxygen environment to reduce the V_(o)concentration *** experimental work is supported by density functional theory(dFT)calculations which show that the rhombohedral phase is the most stable one in highly oxygen defective ZrO_(2)*** dFT calculations also show that V_(o)contribute to the ferroelectric *** findings reveal the importance of V_(o)for stabilizing rhombohedral ZrO_(2)thin films with superior ferroelectric properties.

关键词： charged defects ferroelectric polarization rhombohedral phase stability zirconia

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