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Recent advances of high-entropy electrocatalysts for water electrolysis by electrodeposition technology:a short review

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Rare Metals 2024年第6期43卷 2371-2390页

作者： Han-ming Zhang Shao-Fei Zhang Li-Hao zuo jia-Kang Li jun-Xia Guo Peng Wang jin-Feng Sun Lei Dai Hebei Key Laboratory of Flexible Functional Materials School of Materials Science and EngineeringHebei University of Science and TechnologyShijiazhuang 050018China Department of Chemistry National University of SingaporeSingapore117543Singapore

Hydrogen is considered as the promising energy carrier to substitute traditional fossil fuel,due to its cleanliness,renewability and high energy *** electrolysis is a simple and eonvenient technology for hydrogen *** efficiency of water electrolysis for hydrogen production is limited by the electrocatalytic performances on hydrogen evolution reaction(HER)and oxygen evolution reaction(OER).The exorbitant Pt-and Ir-/Ru-based electrocatalysts as optimal HER and OER electrocatalysts,respectively,restrict water electrolysis ***,non-precious metal-based high-entropy electrocatalysts have exhibited excellent electrocatalytic activities and long-term stabilities for water electrolysis,as promising precious cataly st ***,the construction of the high-entropy electroc atalysts is vital to water electrolysis *** technology is an efficient method for the preparation of high-entropy electrocatalysts due to its simple,fast,energy-saving and environmental-friendly ***-component co-precipitation facilely occurs during the electroredox in electrodeposition ***-entropy alloys,oxides,(oxy)hydroxides,phosphides and phosphorus sulfide oxides have been successfully prepared by galvanostatic,potentiostatic electrodeposition,cyclic voltammetry,pulse,nanodroplet-mediated and cathodic plasma electrodeposition ***,introduction of the development of high-entropy electrocatalysts synthesized by electrodeposition technology is significant to researchers and *** and outlooks are also concluded to boost the industrial application of electrodeposition in water electrolysis and other energy conversion areas.

关键词： High-entropy electrocatalysts Electrodeposition technology Water electrolysis Multi-component co-precipitation Excellent electrocatalytic performances

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Dissociation cross sections ofψ(3770),ψ(4040),ψ(4160),andψ(4415)mesons with nucleons

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Communications in Theoretical Physics 2024年第4期76卷 93-112页

作者： Ruo-Qing Ding Xiao-ming Xu H j Weber Department of Physics Shanghai UniversityBaoshanShanghai 200444China Department of Physics University of VirginiaCharlottesvilleVA 22904United States of America

We study the dissociation of ψ(3770), ψ(4040), ψ(4160), and ψ(4415) mesons in collision with nucleons, which takes place in high-energy proton-nucleus collisions. The quark interchange between a nucleon and a ■ meson leads to the dissociation of the ■ meson. We consider the reactions:■, and■, where R stands for ψ(3770), ψ(4040), ψ(4160), or ψ(4415). A reaction of a neutron and a ■ meson corresponds to a reaction of a proton and the ■ meson by replacing the up quark with the down quark and vice versa. Transition-amplitude formulas are derived from the S-matrix *** cross sections are calculated with the transition amplitudes for scattering in the prior form and in the post form. The cross sections relate to nodes in the radial wave functions of ψ(3770), ψ(4040), ψ(4160), and ψ(4415) mesons.

关键词： inelastic nucleon-charmonium scattering quark interchange relativistic constituent quark potential model

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Tributyltin causes generational neurodevelopmental toxicity and the protective effect of folic acid in zebrafish

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journal of Environmental Sciences 2024年第3期137卷 615-625页

作者： Haoxing Cai Naying Zheng Chen Tang Yuxuan Zhang Zhenghong zuo Chengyong He State Key Laboratory of Cellular Stress Biology School of Life SciencesFaculty of Medicine and Life SciencesXiang’an Hospital of Xiamen UniversityXiamen UniversityXiamen 361005China

Tributyltin(TBT),a common organotin environmental pollutant,may pose a threat to human development during critical early-life *** aimed to assess the neurodevelopmental intergenerational toxicity of early-life exposure to TBT and the protective effect of DNA methyl donor folic acid(FA).Specifically,after early-life exposure(1–21 days postfertilization,dpf)to TBT(0,1,10 and 100 ng/L),zebrafish(Danio rerio)were cultured in clean medium until sexual *** exposed females were mated with unexposed males to produce embryos(F1).The F1 generation were cultured(4–120 hours post-fertilization,hpf)with and without 1 mmol/L *** neurotoxic effects of early-life TBT exposure for zebrafish and their offspring(F1)were significantly enhanced anxiety and reduced aggression,decreased gene expression of DNA methyltransferase in the brain and increased serotonin levels in the ***,the intergenerational neurodevelopmental toxicity,as manifested in the F1 generation,was attenuated by FA *** summary,early-life TBT exposure led to intergenerational neurodevelopmental deficits in zebrafish,and DNA methyl donors had a protective effect on F1 neurodevelopment,which can inform the prevention and treatment of intergenerational neurotoxicity due to organotin pollutants.

关键词： Tributyltin Neurodevelopment Intergeneration DNA methylation Folic acid Zebrafish

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Local Regularity Criteria for the 3D Co-rotational Beris-Edwards System in Lorentz Spaces

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Acta Mathematicae Applicatae Sinica 2024年

作者： Zhong-bao zuo School of Mathematics and Statistics Central South University

In this paper, we present some new regularity criteria for suitable weak solutions to the 3D corotational Beris-Edwards system. First, we prove that suitable weak solutions are regular if the scaled Lp;q-norm of the velocity field or gradient of velocity is small with 2/p+3/q= 2, 1 j. Evol. Equ. 21:1627-1650, 2021) for Navier-Stokes equations.

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Biological scaffold as potential platforms for stem cells:Current development and applications in wound healing

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World journal of Stem Cells 2024年第4期16卷 334-352页

作者： jie-Yu Xiang Lin Kang Zi-ming Li Song-Lu Tseng Li-Quan Wang Tian-Hao Li Zhu-jun Li jiu-zuo Huang Nan-Ze Yu Xiao Long Department of Plastic and Reconstructive Surgery Peking Union Medical College HospitalChinese Academy of Medical Sciences and Peking Union Medical CollegeBeijing 100730China Biomedical Engineering Facility Institute of Clinical MedicinePeking Union Medical College HospitalChinese Academy of Medical SciencesBeijing 100021China

Wound repair is a complex challenge for both clinical practitioners and *** approaches for wound repair have several *** cell-based therapy has emerged as a novel strategy to address this issue,exhibiting significant potential for enhancing wound healing rates,improving wound quality,and promoting skin ***,the use of stem cells in skin regeneration presents several ***,stem cells and biomaterials have been identified as crucial components of the wound-healing *** therapy involving the development of biocompatible scaffolds,accompanying cells,multiple biological factors,and structures resembling the natural extracellular matrix(ECM)has gained considerable *** scaffolds encompass a range of biomaterials that serve as platforms for seeding stem cells,providing them with an environment conducive to growth,similar to that of the *** scaffolds facilitate the delivery and application of stem cells for tissue regeneration and wound *** article provides a comprehensive review of the current developments and applications of biological scaffolds for stem cells in wound healing,emphasizing their capacity to facilitate stem cell adhesion,proliferation,differentiation,and paracrine ***,we identify the pivotal characteristics of the scaffolds that contribute to enhanced cellular activity.

关键词： Stem-cell-based therapy Biological scaffolds Wound healing Extracellular matrix mimicry Cellular activities enhancement Scaffold characteristics

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Leflunomide: A versatile additive for defect reduction, enhanced optoelectronic properties and environmental stability of perovskite films

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Nano Research 2024年第4期17卷 2628-2637页

作者： Dingyue Sun ming Peng Taijin Wang Longju Yi Shizuo Zhang Feng Liu Gary j.Cheng The Institute of Technological Sciences Wuhan UniversityWuhan 430072China School of Power and Mechanical Engineering Wuhan UniversityWuhan 430072China School of Industrial Engineering Purdue UniversityWest LafayetteIN 47906USA

The development of perovskite photoelectric devices with excellent performance is largely dependent on the defects in the perovskite *** address this issue,a specific drug,leflunomide(LF,C_(12)H_(9)F_(3)N_(2)O_(2)),was incorporated into the perovskite to reduce defects and improve its photoelectric *** is believed that the C=O bond on LF molecule can interact with the uncoordinated Pb2+of the perovskite,thereby reducing non-radiative *** novel approach of incorporating LF into perovskite films has the potential to revolutionize the development of high-performance perovskite photoelectric *** trifluoromethyl functional(–CF_(3))group on LF can form a protective layer on the surface of the perovskite film,shielding it from water ***,LF can be utilized to alter the nucleation position of perovskite,thus minimizing the number of defects and optimizing the film ***,the LF-doped perovskite film displays low trap density and high photoelectric *** LF-doped perovskite film showed a trap density of 8.28×10^(11),which is notably lower than the 2.04×10^(12) of the perovskite film without *** responsivity and detectivity of the LF-doped perovskite photodetector were 0.771 A/W and 2.81×10^(11) jones,respectively,which are much higher than the 0.23 A/W and 1.06×10^(10) jones of the LF-undoped perovskite ***,the LF-doped photodetector maintained an initial photocurrent of 86%after 30 days of storage in air,indicating drastically increased environmental *** strongly suggests that LF is an effective additive for perovskites utilized in optoelectronic devices with high performance.

关键词： leflunomide additive engineering defect passivation perovskite

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High-rate CH_(4)-to-C_(2)H_(6) photoconversion enabled by Au/ZnO porous nanosheets under oxygen-free system

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Science China Chemistry 2024年第3期67卷 869-875页

作者： Kai Zheng Xiaojing Zhang jun Hu Chengbin Xu juncheng Zhu jing Li mingyu Wu Shan Zhu Li Li Shumin Wang Yumei Lv Xin He ming zuo Chengyuan Liu Yang Pan junfa Zhu Yongfu Sun Yi Xie Hefei National Laboratory for Physical Sciences at Microscale National Synchrotron Radiation LaboratoryUniversity of Science and Technology of ChinaHefei 230026China Key Laboratory of Photochemical Conversion and Optoelectronic Materials Technical Institute of Physics and ChemistryChinese Academy of SciencesBeijing 100190China State Grid Anhui Electric Power Research Institute Hefei 230601China

Photocatalytic CH_(4) coupling into high-valued C_(2)H_(6) is highly attractive,whereas the photosynthetic rate,especially under oxygen-free system,is still ***,we designed the negatively charged metal supported on metal oxide nanosheets to activate the inert C-H bond in CH_(4)and hence accelerate CH_(4) coupling *** an example,the synthetic Au/ZnO porous nanosheets exhibit the C_(2)H_(6) photosynthetic rate of 1,121.6μmol g^(-1)_(cat)h^(-1)and the CH_(4) conversion rate of 2,374.6μmol g^(-1)_(cat)h^(-1) under oxygen-free system,2 orders of magnitude higher than those of previously reported *** virtue of several in situ spectroscopic techniques,it is established that the generated Au^(δ-)and O^-species together polarized the C-H bond,while the Au^(δ-)and O^-species jointly stabilized the CH_(3) intermediates,which favored the coupling of CH_(3) intermediate to photosynthesize C_(2)H_(6) instead of overoxidation into CO_(x).Thus,the design of dual active species is beneficial for achieving high-efficient CH_(4)-to-C_(2)H_(6) photoconversion.

关键词： dual surface-active sites selective methane coupling ethane room temperature

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Phase-Field Simulation of Sintering Process:A Review

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Computer Modeling in Engineering & Sciences 2024年第8期140卷 1165-1204页

作者： ming Xue Min Yi State Key Laboratory ofMechanics and Control forAerospace Structures&Institute for Frontier Science&Key Laboratory for Intelligent Nano Materials and Devices of Ministry of Education&College of Aerospace Engineering Nanjing University of Aeronautics and Astronautics(NUAA)Nanjing210016China

Sintering,a well-established technique in powder metallurgy,plays a critical role in the processing of high melting point materials.A comprehensive understanding of structural changes during the sintering process is essential for effective product *** phase-field method stands out for its unique ability to simulate these structural *** its widespread application,there is a notable absence of literature reviews focused on its usage in sintering ***,this paper addresses this gap by reviewing the latest advancements in phase-field sintering models,covering approaches based on energy,grand potential,and entropy *** characteristics of various models are extensively discussed,with a specific emphasis on energy-based models incorporating considerations such as interface energy anisotropy,tensor-form diffusion mechanisms,and various forms of rigid particle motion during ***,the paper offers a concise summary of phase-field sintering models that integrate with other physical fields,including stress/strain fields,viscous flow,temperature field,and external electric *** conclusion,the paper provides a succinct overview of the entire content and delineates potential avenues for future research.

关键词： Phase-field model review sintering additive manufacturing

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Adipose-derived stem cells in diabetic foot care:Bridging clinical trials and practical application

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World journal of Diabetes 2024年第6期15卷 1162-1177页

作者： Song-Lu Tseng Lin Kang Zhu-jun Li Li-Quan Wang Zi-ming Li Tian-Hao Li jie-Yu Xiang jiu-zuo Huang Nan-Ze Yu Xiao Long Department of Plastic and Reconstructive Surgery Chinese Academy of Medical Sciences and Peking Union Medical CollegeBeijing 100730China Department of Plastic and Reconstructive Surgery Peking Union Medical College HospitalChinese Academy of Medical Sciences and Peking Union Medical CollegeBeijing 100730China Biomedical Engineering Facility Institute of Clinical MedicinePeking Union Medical College HospitalChinese Academy of Medical Sciences BeijingBeijing 100021China

Diabetic foot ulcers(DFUs)pose a critical medical challenge,significantly impairing the quality of life of ***-derived stem cells(ADSCs)have been identified as a promising therapeutic approach for improving wound healing in *** extensive exploration of the mechanical aspects of ADSC therapy against DFU,its clinical applications remain *** this review,we aimed to bridge this gap by evaluating the use and advancements of ADSCs in the clinical management of *** review begins with a discussion of the classification and clinical management of diabetic foot *** then discusses the current landscape of clinical trials,focusing on their geographic distribution,reported efficacy,safety profiles,treatment timing,administration techniques,and dosing ***,the review discusses the preclinical strategies to enhance ADSC *** review shows that many trials exhibit biases in study design,unclear inclusion criteria,and intervention *** conclusion,this review underscores the potential of ADSCs in DFU treatment and emphasizes the critical need for further research and refinement of therapeutic approaches,with a focus on improving the quality of future clinical trials to enhance treatment outcomes and advance the field of diabetic wound care.

关键词： Adipose-derived stem cells Diabetic foot ulcers Wound healing Clinical

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德国足球青训体系发展经验及启示

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体育文化导刊 2024年第7期 82-88页

作者：房作铭广东第二师范学院体育学院广州510800

运用文献资料、专家访谈等方法,探究德国足球青训体系、发展经验,并提出对我国的启示。发展经验:开辟层次清晰的人才输送路径,打造精细化的人才培养模式,搭建科学、合理的青训赛事体系,培养高素质、专业化的教练员队伍,建立家、校、社... 详细信息

运用文献资料、专家访谈等方法,探究德国足球青训体系、发展经验,并提出对我国的启示。发展经验:开辟层次清晰的人才输送路径,打造精细化的人才培养模式,搭建科学、合理的青训赛事体系,培养高素质、专业化的教练员队伍,建立家、校、社多方联动的合作机制。启示:构建多维度的人才选拔机制,设立常态化的精英训练中心,构建高质量的训练和赛事体系,注重系统化的教练员培训过程,建立多元融合的精英保障体系。

关键词：竞技体育足球青训体系德国青少年

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