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Landslide susceptibility mapping(LSM)based on different boosting and hyperparameter optimization algorithms:A case of Wanzhou District,China

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Journal of Rock Mechanics and Geotechnical Engineering 2024年第8期16卷 3221-3232页

作者： Deliang sun Jing Wang Haijia Wen YueKai Ding Changlin mi Key Laboratory of GIS Application Research Chongqing Normal UniversityChongqing 401331China Key Laboratory of New Technology for Construction of Cities in Mountain Area Ministry of EducationChongqing UniversityChongqing 400045China National Joint Engineering Research Center of Geohazards Prevention in the Reservoir Areas Chongqing UniversityChongqing 400045China School of Civil Engineering Chongqing UniversityChongqing 400045China Natural Resources Development Service Center of Linyi Linyi 276000China

Boosting algorithms have been widely utilized in the development of landslide susceptibility mapping(LSM)***,these algorithms possess distinct computational strategies and hyperparameters,making it challenging to propose an ideal LSM *** investigate the impact of different boosting algorithms and hyperparameter optimization algorithms on LSM,this study constructed a geospatial database comprising 12 conditioning factors,such as elevation,stratum,and annual average *** XGBoost(XGB),LightGBM(LGBM),and CatBoost(CB)algorithms were employed to construct the LSM ***,the Bayesian optimization(BO),particle swarm optimization(PSO),and Hyperband optimization(HO)algorithms were applied to optimizing the LSM *** boosting algorithms exhibited varying performances,with CB demonstrating the highest precision,followed by LGBM,and XGB showing poorer ***,the hyperparameter optimization algorithms displayed different performances,with HO outperforming PSO and BO showing poorer *** HO-CB model achieved the highest precision,boasting an accuracy of 0.764,an F1-score of 0.777,an area under the curve(AUC)value of 0.837 for the training set,and an AUC value of 0.863 for the test *** model was interpreted using SHapley Additive exPlanations(SHAP),revealing that slope,curvature,topographic wetness index(TWI),degree of relief,and elevation significantly influenced landslides in the study *** study offers a scientific reference for LSM and disaster prevention *** study examines the utilization of various boosting algorithms and hyperparameter optimization algorithms in Wanzhou *** proposes the HO-CB-SHAP framework as an effective approach to accurately forecast landslide disasters and interpret LSM ***,limitations exist concerning the generalizability of the model and the data processing,which require further exploration in subsequent studies.

关键词： Landslide susceptibility Hyperparameter optimization Boosting algorithms SHapley additive exPlanations(SHAP)

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Ultra-high specific surface area activated carbon from Taihu cyanobacteria via KOH activation for enhanced methylene blue adsorption

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Chinese Journal of Chemical Engineering 2024年第3期67卷 106-116页

作者： Yifang mi Wenqiang Wang Sen Zhang Yalong Guo Yufeng Zhao Guojin sun Zhihai Cao Key Laboratory of Advanced Textile Materials and Manufacturing Technology and Engineering Research Center for Eco-Dyeing&Finishing of Textiles Ministry of EducationZhejiang Provincial Engineering Research Center for Green and Low-carbon Dyeing&FinishingZhejiang Sci-Tech UniversityHangzhou 310018China Key Laboratory for Technology in Rural Water Management of Zhejiang Province Zhejiang University of Water Resources and Electric PowerHangzhou 310018China

Cyanobacteria-based activated carbon(CBAC)was successfully prepared by pyrolysis-activation of Taihu *** the impregnation ratio and activated temperature were 2 and 800-C,respectively,the optimal CBACs possessed an ultra-high specific surface(2178.90 m^(2)·g^(-1))and plenty of micro-and meso-pores,as well as a high pore volume(1.01 cm^(3)·g^(-1)).Ascribed to ultra-high surface area,π-π interaction,electrostatic interaction,as well as hydrogen-bonding interactions,the CBACs displayed huge superiority in efficient dye *** saturated methylene blue adsorption capacity by CBACs could be as high as 1143.4 mg·g^(-1),superior to that of other reported biomass-activated *** adsorption was endothermic and modeled well by the pseudo-second-order kinetic,intra-particle diffusion,and Langmuir *** work presented the effectiveness of Taihu cyanobacteria adsorbent ascribed to its super large specific surface area and high adsorption ability.

关键词： Activated carbon Biomass Dye adsorption Taihu cyanobacteria

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A stable radiochromic semiconductive viologen-based metal-organic framework for dual-mode direct X-ray detection

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Chinese Chemical Letters 2024年第9期35卷 437-441页

作者： Xuying Yu Jiarong mi Yulan Han Cai sun mingsheng Wang Guocong Guo State Key Laboratory of Structural Chemistry Fujian Institute of Research on the Structure of MatterChinese Academy of SciencesFuzhou 350608China College of Chemistry Fuzhou UniversityFuzhou 350108China University of Chinese Academy of Sciences Beijing 100049China School of Chemistry and Chemical Engineering Queen’s University BelfastBelfast BT95AGUnited Kingdom

Direct X-ray detectors,which directly convert X-rays into electrical signals through semiconductors,have higher space solution than scintillator-mediated indirect X-ray ones and are high desirable for early cancer detection and other applications,but the mainstream commercialα-Se detector is still largely limited by high production costs,large leakage current and low *** article reports an easily prepared,stable radiochromic semiconductive metal–organic framework(MOF),(MV)[Cd_(3)(tdc)_(4)]·2H_(2)O(RCS-1,H_(2)tdc=2,5-thiophenedicarboxylic acid;MV^(2+)=methyl viologen cation)with direct X-ray detecting *** a large bulk resistivity of 8.40×10^(9)Ωcm,this material ensures minimal dark current and low noise for X-ray ***,it exhibits higher sensitivity to W KαX-rays(98.58μC Gy^(-1)cm^(-2))thanα-Se(~20μC Gy^(-1)cm^(-2)).Meanwhile,unlike most reported direct X-ray detecting semiconductors,compound RCS-1 shows remarkable color change upon X-ray irradiation owing to the presence of photochromism-active viologen *** feature offers an appealing visual detecting ability to direct X-ray detectors that provide only the electrical signals.

关键词： Metal-organic framework Viologen Photochromism Conductance X-ray detection

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Upconversion-based chiral nanoprobe for highly selective dual-mode sensing and bioimaging of hydrogen sulfide in vitro and in vivo

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Light(Science & Applications) 2024年第9期13卷 1878-1887页

作者： Yang Lu Xu Zhao Dongmei Yan Yingqian mi Peng sun Xu Yan Xiaomin Liu Geyu Lu State Key Laboratory of Integrated Optoelectronics College of Electronic Science and EngineeringJilin University130012 ChangchunChina Department of Immunology College of Basic Medical SciencesJilin University130021 ChangchunChina

Chiral assemblies have become one of the most active research areas due to their versatility,playing an increasingly important role in bio-detection,imaging and *** this work,chiral UCNPs/CuxOS@ZIF nanoprobes are prepared by encapsulating upconversion nanoparticles(UCNPs)and CuxOS nanoparticles(NPs)into zeolitic imidazolate framework-8(ZIF-8).The novel excited-state energy distribution-modulated upconversion nanostructure(NaYbF4@-NaYF4:Yb,Er)is selected as the fluorescence source and energy donor for highly efficient fluorescence resonance energy transfer(FRET).CuxOS NP is employed as chiral source and energy acceptor to quench upconversion luminescence(UCL)and provide circular dichroism(CD)*** the natural adsorption and sorting advantages of ZIF-8,the designed nanoprobe can isolate the influence of other common disruptors,thus achieve ultra-sensitive and highly selective UCL/CD dual-mode quantification of H2S in aqueous solution and in living ***,the nanoprobe is also capable of in vivo intra-tumoral H2S *** work highlights the multifunctional properties of chiral nanocomposites in sensing and opens a new vision and idea for the preparation and application of chiral nanomaterials in biomedical and biological analysis.

关键词： chiral sulfide donor

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Lateral root elongation in maize is related to auxin synthesis and transportation mediated by N metabolism under a mixed NO_(3)^(–) and NH_(4)^(+) supply

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Journal of Integrative Agriculture 2024年第3期23卷 1048-1060页

作者： Peng Wang Lan Yang Xichao sun Wenjun Shi Rui Dong Yuanhua Wu Guohua mi Key Laboratory of Tobacco Biology and Processing of ministry of Agriculture and Rural Affairs Tobacco Research InstituteChineseAcademy of Agricultural SciencesQingdao 266101China Department of Plant Nutrition College of Resources and Environmental SciencesChina Agricultural UniversityBeijing 100193China College of Resources Hunan Agricultural UniversityChangsha 410128China Agro-Environmental Protection Institute Ministry of Agriculture and Rural AffairsTianjin 300191China

A mixed nitrate (NO_(3)^(–)) and ammonium (NH_(4)^(+)) supply can promote root growth in maize (Zea mays),however,the changes in root morphology and the related physiological mechanism under different N forms are still ***,maize seedlings were grown hydroponically with three N supplied in three different forms (NO_(3)^(–)only,75/25 NO_(3)^(–)/NH_(4)^(+)and NH_(4)^(+)only).Compared with sole NO_(3)^(–)or NH_(4)^(+),the mixed N supply increased the total root length of maize but did not affect the number of axial *** main reason was the increased total lateral root length,while the average lateral root (LR) length in each axle was only slightly *** addition,the average LR density of 2nd whorl crown root under mixed N was also *** with sole nitrate,mixed N could improve the N metabolism of roots (such as the N influx rate,nitrate reductase (NR) and glutamine synthase (GS)enzyme activities and total amino content of the roots).Experiments with exogenously added NR and GS inhibitors suggested that the increase in the average LR length under mixed N was related to the process of N assimilation,and whether the NR mediated NO synthesis participates in this process needs further ***,an investigation of the changes in root-shoot ratio and carbon (C) concentration showed that C transportation from shoots to roots may not be the key factor in mediating lateral root elongation,and the changes in the sugar concentration in roots further proved this ***,the synthesis and transportation of auxin in axial roots may play a key role in lateral root elongation,in which the expression of ZmPIN1B and ZmPIN9 may be involved in this *** study preliminarily clarified the changes in root morphology and explored the possible physiological mechanism under a mixed N supply in maize,which may provide some theoretical basis for the cultivation of crop varieties with high N efficiency.

关键词： maize NO_(3)^(–)/NH_(4)^(+)ratio lateral root elongation N assimilation indole-3-acetic acid

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A novel Tb^(3+) and Eu^(3+) co-doped dual-emitting phosphate K_(3)SrBi(P_(2)O_(7))_(2) phosphor for application in FIR thermometers

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Journal of Rare Earths 2024年第3期42卷 455-463,I0001页

作者： Baochen Wang Shifeng sun Zeqi Li Zongwang Li Weiwei Lin Chao Zeng Yan-gai Liu Ruiyu mi School of Chemical and Environmental Engineering Anhui Polytechnic UniversityWuhu241000China State-Province Joint Engineering Laboratory of Zeolite Membrane Materials Key Lab of Fluorine and Silicon for Energy Materials and Chemistry of Ministry of EducationInstitute of Advanced MaterialsCollege of Chemistry and Chemical EngineeringJiangxi Normal UniversityNanchang330022China Beijing Key Laboratory of Materials Utilization of Nonmetallic minerals and Solid Wastes National Laboratory of Mineral MaterialsSchool of Materials Science and TechnologyChina University of GeosciencesBeijing100083China

Rare earth co-doped phosphor for fluorescence intensity ratio(FIR) thermometer has gained increasing attention in recent years. Herein, the novel Tb^(3+)and Eu^(3+)co-doped K_(3)SrBi(P_(2)O_(7))_(2)(KSBP) phosphate phosphors were reported. The crystal structure of the title phosphor was determined using Rietveld refinement and proved to have a three-dimensional structure. The time-resolved spectroscopy reveals that there is almost no energy transfer between Tb^(3+)and Eu^(3+). More importantly, Tb^(3+)and Eu^(3+)emissions show different thermal quenching behaviors, which claims the potential of this material for application in optical thermometer. The FIR of the typical KSBP:0.02Tb^(3+),0.04Eu^(3+)sample demonstrates a polynomial relationship as a function of temperature and the absolute and relative sensitivity are0.025 K^(-1) and 0.59%/K, respectively. In general, our study reports a novel and potential KSBP:Tb^(3+),Eu^(3+)phosphate phosphor that is promising for use in high-sensitive FIR thermometers.

关键词： Phosphor Thermometer Fluorescence intensity ratio Thermal stability Rare earths

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Serum N-glycan markers for diagnosing liver fibrosis induced by hepatitis B virus

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World Journal of Gastroenterology 2020年第10期26卷 1067-1079页

作者： Xi Cao Qing-Hua Shang Xiao-Ling Chi Wei Zhang Huan-ming Xiao mi-mi sun Gang Chen Yong An Chun-Lei Lv Lin Wang Yue-min Nan Cui-Ying Chen Zong-Nan Tan Xue-En Liu Hui Zhuang Department of microbiology and Center of Infectious Diseases School of Basic Medical SciencesPeking University Health Science CenterBeijing 100191China Department of Liver Disease No.88 Hospital of Chinese People’s Liberation ArmyTai'an 271000Shandong ProvinceChina Department of Hepatology Guangdong Provincial Hospital of Chinese MedicineGuangzhou 510120Guangdong ProvinceChina Department of Traditional and Western Medical Hepatology Third Hospital of Hebei Medical UniversityShijiazhuang 050051Hebei ProvinceChina Department of Molecular Biomedical Research Xian si-da Biotechnology Company LimitedNanjing 210000Jiangsu ProvinceChina

BACKGROUND Hepatitis B virus (HBV) infection is the primary cause of hepatitis with chronic HBV infection,which may develop into liver fibrosis,cirrhosis and hepatocellular *** of early-stage fibrosis related to HBV infection is of great clinical significance to block the progression of liver *** liver biopsy is regarded as the gold standard to detect and assess fibrosis;however,this method is invasive and prone to clinical sampling *** order to address these issues,we attempted to find more convenient and effective serum markers for detecting HBV-induced early-stage liver *** To investigate serum N-glycan profiling related to HBV-induced liver fibrosis and verify multiparameter diagnostic models related to serum N-glycan *** N-glycan profiles from the sera of 432 HBV-infected patients with liver fibrosis were *** changed N-glycan levels (peaks)(P minotransferase to platelet ratio index (APRI),fibrosis index based on the four factors (FIB-4),glutamyltranspeptidase platelet albumin index (S index),GlycoCirrho-test,and ***,we combined multiparameter diagnostic models with alanine aminotransferase (ALT) and platelet (PLT) tests and compared their diagnostic *** addition,the diagnostic accuracy of N-glycan models was also verified in the validation group of *** Multiparameter diagnostic models constructed based on N-glycan peak 1,3,4and 8 could distinguish between different stages of liver *** area under ROC curves (AUROCs) of Model A and Model B were 0.890 and 0.752,respectively differentiat

关键词： Chronic hepatitis B Liver fibrosis N-glycan Multiparameter diagnostic models Receiver operating characteristic curve analysis Diagnostic power

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The carbon border adjustment mechanism is inefficient in addressing carbon leakage and results in unfair welfare losses

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Fundamental Research 2024年第3期4卷 660-670页

作者： Xinlu sun Zhifu mi Lu Cheng D'Maris Coffman Yu Liu The Bartlett School of Sustainable Construction University College LondonLondon WC1E 7HBUnited Kingdom College of Urban and Environmental Sciences Peking UniversityBeijing 100871China

The European Commission has proposed a Carbon Border Adjustment Mechanism(CBAM)to reduce carbon leakage and create a level playing field for its domestic products and imported ***,the effectiveness of the proposal remains unclear,especially when it triggers threats of retaliation from trading partners of the European *** apply a Computable General Equilibrium model-Global Trade Analysis Project-to assess the economic and environmental impacts of different CBAM *** we show that the effectiveness of the CBAM to address carbon leakage risks is rather limited,and the CBAM raises concerns over global welfare costs,Correct to Gross Domestic Product(GDP)losses,and violation of equality *** retaliation leads to multiplied welfare losses,which would mostly be borne by poor *** results question the carbon leakage reduction effect of a unilateral trade policy and suggest that climate change mitigation still needs to be performed within the framework of international cooperation.

关键词： Carbon border adjustment mechanism Carbon leakage Climate change mitigation Floorcarbon price Trade retaliation

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Residual fluoride self-activated effect enabling upgraded utilization of recycled graphite anode

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Journal of Energy Chemistry 2024年第6期93卷 24-31,I0002页

作者： Shuzhe Yang Qingqing Gao Yukun Li Hongwei Cai Xiaodan Li Gaoxing sun Shuxin Zhuang Yujin Tong Hao Luo mi Lu School of Materials Science and Engineering Xiamen University of TechnologyXiamen 361024FujianChina Faculty of Physics University of Duisburg-EssenDuisburg D-47057Germany

Recycling graphite anode from spent lithium-ion batteries(SLIBs)is regarded as a crucial approach to promoting sustainable energy storage ***,the recycled graphite(RG)generally presents degraded structure and ***,the residual fluoride self-activated effect is proposed for the upgraded utilization of *** and low-energy water immersion treatment not only widens the interlayer spacing,but also retains appropriate fluoride on the surface of *** analysis and experiments demonstrate that the residual fluoride can optimize Li~+migration and deposition kinetics,resulting in better Li~+intercalation/deintercalation in the interlayer and more stable Li metal plating/stripping on the surface of RG,As a result,the designed LFP||RG full cells achieve ultrahigh reversibility(~100%Coulombic efficiency),high capacity retention(67%after 200 cycles,0.85 N/P ratio),and commendable adaptability(stable cycling without short-circuiting,0.15 N/P ratio).The energy density is improved from 334 Wh kg^(-1)of 1.1 N/P ratio to 367 Wh kg^(-1)of 0.85 N/P ratio(total mass based on cathode and anode).The exploration of RG by residual fluoride self-activated effect achieves upgraded utilization beyond fresh commercial graphite and highlights a new strategy for efficient reuse of SLIBs.

关键词： Spent lithium-ion batteries Recycled graphite anode Fluoride Self-activated effect Upgraded utilization

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Surface Temperature Field of Ti-66Al and Ti-Al and Ti-4848Al AlloysAl Alloys Under Continuous Laser AblationUnder Continuous Laser Ablation

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稀有金属材料与工程 2024年第9期53卷 2405-2412页

作者： sun Ruochen mi Guangbao Aviation Key Laboratory of Science and Technology on Advanced Titanium Alloys AECC Beijing Institute of Aeronautical MaterialsBeijing 100095China

The high temperature fire retardancy of titanium alloy is an important factor restricting its application in aero-engine,and the laser ignition method can accurately reflect the fire retardancy of titanium alloy under local *** to the limitations of laser ignition experiments on the microscopic boundary and the transient propagation mechanism of the temperature field,molecular dynamics(MD)simulations and JMatPro calculation were applied to study the temperature field of Ti-6Al and Ti-48Al *** results show that a molten pool is formed on the surface of Ti-Al alloys under continuous laser irradiation,and the temperature field of the molten pool is normally distributed from the center to the *** the center temperature reaches the critical point of ignition,the extended combustion occurs,and the extended combustion path advances along the direction of the air *** with Ti-6Al alloy,Ti-48Al alloy has higher fire retardancy under laser *** is due to the better heat transfer performance of Ti-48Al,which leads to the weakening of the heat concentration effect near the boundary of the spot temperature *** it is necessary to increase the partial pressure of oxygen,and thus to reduce the ignition point of the alloy in order to achieve the ignition boundary condition of Ti-48Al alloy under the same laser heat *** the aspect of extended combustion path,the boundary heat collection effect of specimens shown by MD models reveals another mechanism affecting combustion expansion path besides the direction of air *** is,the heat generated by the laser spot is interrupted when it is transmitted to the boundary of the specimen along the short side direction,resulting in a concentration of heat near the *** the combustion path also tends to expand along this direction.

关键词： Ti-Al alloys laser ignition molecular dynamics temperature field

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