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Dendritic nanoarchitecture imparts ZSM-5 zeolite with enhanced adsorption and catalytic performance in energy applications

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Journal of energy Chemistry 2023年第5期80卷 77-88,I0003页

作者： mar.a del mar.alonso-Doncel Cristina Ochoa-Hernández Gema Gómez-Pozuelo Adriana Oliveira JoséGonzález-Aguilar ángel Peral Raúl Sanz David P.Serrano Thermochemical Processes Unit IMDEA Energy InstituteAvda.Ramon de la Sagra3E28935MostolesMadridSpain Department of Heterogeneous Catalysis Max-Planck-Institut für KohlenforschungKaiser-Wilhem-Platz14540Muheim an der RuhGermay Department of Chemical and environmental Technology Rey Juan Carlos UniversityC/Tulipan s/nE28933MostolesMadridSpain High Temperature Processes Unit IMDEA Energy InstituteAvda.Ramon de la Sagra3E28935MostolesMadridSpain Department of Chemical Energy and Mechanical TechnologyRey Juan Carlos UniversityC/Tulipan s/n28933MostolesMadridSpain

The development of zeolites possessing dendritic features represents a great opportunity for the design of novel materials with applications in a large variety of fields and,in particular,in the energy sector to afford its transition towards a low carbon *** the current work,ZSM-5 zeolite showing a dendritic3D nanoarchitecture has been synthesized by the functionalization of protozeolitic nanounits with an amphiphilic organosilane,which provokes the branched aggregative growth of zeolite *** ZSM-5 exhibits outstanding accessibility arising from a highly interconnected network of radially-oriented mesopores(3-10 nm)and large cavities(20-80 nm),which add to the zeolitic micropores,thus showing a well-defined trimodal pore size *** singular features provide dendritic ZSM-5 with sharply enhanced performance in comparison with nano-and hierarchical reference materials when tested in a number of energy related applications,such as VOCs(toluene)adsorption(improved capacity),plastics(low-density polyethylene)catalytic cracking(boosted activity)and hydrogen production by methane catalytic decomposition(higher activity and deactivation resistance).

关键词： Dendritic ZSM-5 VOCs adsorption Plastics cracking Methane decomposition Hydrogen production

The impact of height-adjustable desks and classroom prompts on classroom sitting time,social,and motivational factors among adolescents

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Journal of Sport and Health Science 2023年第1期12卷 97-105页

作者： Bronwyn Sudholz Ana mar.a Contardo Ayala Anna Timperio David W.Dunstan David e.Conroy Gavin Abbott Bernie Holland Lauren Arundell Jo Salmon Pomegranate Community Mental Health St John of God Social OutreachBallaratVIC 3350Australia Institute for Physical Activity and Nutrition(IPAN) School of Exercise and Nutrition SciencesDeakin UniversityGeelongVIC 3128Australia Physical Activity Laboratory Baker Heart and Diabetes InstituteMelbourneVIC 3004Australia mary MacKillop Institute for Health Research Australian Catholic UniversityMelbourneVIC 3000Australia Department of Kinesiology Pennsylvania State UniversityUniversity ParkPA 16802USA Department of Preventive Medicine Northwestern UniversityChicagoIL 60611USA The Australian Council for Health and Physical education and Recreation AbbotsfordVIC 3067Australia

Purpose:This quasi-experimental study examined the impact of height-adjustable desks in combination with prompts to break up prolonged sitting time during class time and identified social and motivational factors associated with breaking up sitting time among ***’perceptions of strategies were also ***:Over 17 weeks,1 classroom in a government secondary school in Melbourne,Australia,was equipped with 27 height-adjustable desks and prompts(posters and desk stickers)to break up classroom sitting *** received professional development in the use of the desks and *** group of adolescents(n=55)had 2-5 lessons/week using the height-adjustable desks in an intervention classroom,and a comparison group matched by year level and subject(n=50)was taught in traditional“seated”*** wore an activPAL monitor at baseline(T0),4 weeks(T1),and 17 weeks(T2)and completed a survey at T0 and *** teachers participated in interviews at *** sizes were calculated(d).Results:Linear mixed models found that,compared to the traditional“seated”classrooms,the adolescents in the intervention classroom had significantly lower sitting time(T1:-9.7 min/lesson,d=-0.96;T2:-6.7 min/lesson,d=-0.70)and time spent in sitting bouts>15 min(T2:-11.2 min/lesson,d=-0.62),and had significantly higher standing time(T1:7.3 min/lesson,d=0.84;T2:5.8 min/lesson,d=0.91),number of breaks from sitting(T1:1.3 breaks/lesson,d=0.49;T2:1.8 breaks/lesson,d=0.67),and stepping time(T1:2.5 min/lesson,d=0.66).Intervention classroom adolescents reported greater habit strength(d=0.58),self-efficacy for breaking up sitting time(d=0.75),and indicated that having a teacher/classmate remind them to stand as helpful(d=0.50).Conclusion:This intervention shows promise for targeting sitting behaviors in the classroom and indicates that incorporating social and motivational strategies may further enhance outcomes.

关键词： Adolescent School Sedentary behavior Sitting Standing

Precipitation Kinetics on a Nb-V Microalloyed Steel

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Journal of Iron and Steel Research International 2011年第S1期18卷 148-153页

作者： Cartaya elio Armando Cabrera José mar.a Prado José Manuel Departamento de Ciencia de Materiales e Ingeniería Metalúrgica ETSEIBUniversidad Politécnica de Catalua Av.Diagonal 64708028 BarcelonaSpain Departamento de Manufactura y Materiales Facultad de Ingeniería MecánicaUniversidad de OrienteSantiago de CubaCuba Fundación CTM Centro Tecnológico Av.Bases de Manresa 108242 ManresaSpain

The precipitation kinetics in a low carbon high strength low alloy (HSLA) steel,microalloyed with V+Nb has been studied by using the stress relaxation *** technique was carried out in a dynamic dilatometer and allows to determine the onset and finishing precipitation times in hot deformed *** evolution of the precipitates was also observed using field emission scanning electron microscopy (FeSeM) on samples quenched at different times at given *** is completed with the predictions by the thermodynamic software FactSage to identify stable precipitate phases under equilibrium *** confirm the feasibility of the stress relaxation technique as an efficient method for investigating precipitation kinetics.

关键词： stress relaxation microalloyed steels precipitation FeSeM

Current Knowledge on Hepatitis e

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Journal of Clinical and Translational Hepatology 2015年第2期3卷 117-126页

作者： mar.a Teresa Pérez-Gracia mario García Beatriz Suay mar.a Luisa Mateos-Lindemann (A)rea de Microbiología Departamento de Farmacia Instituto de Ciencias Biomédicas Facultad de Ciencias de la Salud Universidad CEU Cardenal Herrera Valencia Spain Unidad de Virología Servicio de Microbiología Hospital Universitario Ramóny Cajal Madrid Spain

Although only a single serotype of hepatitis e virus (HeV),the causative agent of hepatitis e,has been identified,there is great genetic variation among the different HeV isolates *** are at least four major recognized genotypes of HeV:genotypes 1 and 2 are mainly restricted to humans and linked to epidemic outbreaks in nonindustrialized countries,whereas genotypes 3 and 4 are zoonotic in both developing and industrialized *** human strains,genotype 3 and 4 strains of HeV have been genetically characterized from swine,sika deer,mongooses,sheep,and ***,there are approximately 11,000 human and animal sequences of HeV available at the International Nucleotide Sequence Database *** is the major cause of waterborne outbreaks of hepatitis in areas of poor ***,it is responsible for sporadic cases of viral hepatitis in not only endemic but industrialized countries as *** of HeV occurs predominantly by the fecal-oral route,although parenteral and perinatal routes have been *** infection develops in most individuals as a self-limiting,acute,icteric hepatitis;with mortality rates around 1%.However,some affected individuals will develop fulminant hepatic failure,a serious condition that is frequently fatal without a liver *** complication is particularly common when the infection occurs in pregnant women,where mortality rates rise dramatically to up to 25%.Among the preventive measures available to avoid HeV infection,two separate subunit vaccines containing recombinant truncated capsid proteins of HeV have been shown to be highly effective in the prevention of *** of them,HeV 239,was approved in China,and its commercialization by Innovax began in November 2012 under the name Hecolin(R).

关键词： Hepatitis e virus Hepatitis e HeV Zoonosis

Spectrum of neuropsychiatric symptoms in chronic post-stroke aphasia

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World Journal of Psychiatry 2022年第3期12卷 450-469页

作者： Lisa edelkraut Diana López-Barroso mar.a JoséTorres-Prioris Sergio e Starkstein Ricardo e Jorge Jessica Aloisi marcelo L Berthier Guadalupe Dávila Department of Psychobiology and Methodology of Behavioral Science Faculty of Psychology and Speech TherapyUniversity of MalagaMalaga 29071Spain Cognitive Neurology and Aphasia Unit Centro de Investigaciones Médico-SanitariasUniversity of MalagaMalaga 29010Spain Instituto de Investigación Biomédica de Málaga University of MalagaMalaga 29010Spain School of Psychiatry and Neurosciences The University of Western AustraliaPerth 6009Australia Department of Psychiatry and Behavioral Sciences Baylor College of MedicineHoustonTX 77030United States

BACKGROUND Neuropsychiatric symptoms(NPS)have been insufficiently examined in persons with aphasia(PWA)because most previous studies exclude participants with language and communication *** To report a two-part study consisting of a literature review and an observational study on NPS in post-stroke *** Study 1 reviewed articles obtained from PubMed,PsycINFO,Google Scholar and Cochrane databases after cross-referencing key words of post-stroke aphasia to NPS and *** 2 examined language deficits and activities of daily living in 20 PWA(median age:58,range:28-65 years;13 men)with the Western Aphasia Battery-Revised and the Barthel Index,*** of these 20 PWA were proxy-evaluated with the Neuropsychiatric Inventory and domain-specific scales,including the Stroke Aphasia Depression Questionnaire-10 item version and the Starkstein Apathy *** addition,an adapted version of the Hospital Anxiety and Depression Scale was directly administered to the PWA *** observational study is based on the baseline assessment of an intervention clinical trial(eudraCT:2017-002858-36;*** identifier:NCT04134416).ReSULTS The literature review revealed a broad spectrum of NPS in PWA,including depression,anxiety,apathy,agitation/aggression,eating and sleep disorders,psychosis,and hypomania/*** findings alert to the need for improving assessment and treatment approaches of NPS taking into consideration their frequent occurrence in *** 2 showed that the 20 participants had mild-to-moderate aphasia severity and were functionally independent.A wide range of comorbid NPS was found in the post-stroke aphasic population(median number of NPS:5,range:1-8).The majority of PWA(75%)had depressive symptoms,followed by agitation/aggression(70%),irritability(70%),anxiety(65%)and appetite/eating symptoms(65%).Half of them also presented symptoms of apathy,whereas euphoria and psychotic symptoms were rare(5%).Domain

关键词： Aphasia Stroke Neuropsychiatric symptoms Anxiety Apathy Depression

Loss of mismatch repair signaling impairs the WNT–bone morphogenetic protein crosstalk and the colonic homeostasis

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Journal of Molecular Cell Biology 2020年第6期12卷 410-423页

作者： Katrine Nørgaard Carolin Müller Nadja Christensen mar.a L.Chiloeches Cesilie L.Madsen Sabine S.Nielsen Tine e.Thingholm Antoaneta Belcheva Department of Biochemistry and Molecular Biology University of Southern DenmarkCampusvej 555230 Odense MDenmark Department of Molecular Medicine University of Southern DenmarkJ.B.Winsløws Vej 255230 Odense MDenmark

The fine balance between proliferation,differentiation,and apoptosis in the colonic epithelium is tightly controlled by the interplay between WNT,Notch,and bone morphogenetic protein(BMP)*** these complex networks coordinate the colonic homeostasis,especially if cancer predisposing mutations such as mutations in the DNA mismatch repair(MMR)are present,is *** of the MMR system has long been linked to colorectal cancer;however,little is known about its role in the regulation of the colonic *** has been shown that loss of MMR promotes the proliferation of colon epithelial cells that renders them highly susceptible to *** mechanism through which MMR mediates this effect,yet,remains to be *** an MMR-deficient mouse model,we show that increased methylation of Dickkopf1 impacts its expression,and consequently,the ability to negatively regulate WNT *** a result,excessive levels of activeβ-catenin promote strong crypt progenitor-like phenotype and abnormal *** these settings,the development and function of the goblet cells are ***-deficient mice have fewer goblet cells with enlarged mucin-loaded *** further show that MMR inactivation impacts the WNT–BMP signaling crosstalk.

关键词： MMR colonic epithelium WNT BMP crypt homeostasis

Robot-assisted lobectomy in a patient with poor lung function:Another advantage of robot-assisted thoracoscopic surgery

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Laparoscopic, endoscopic and Robotic Surgery 2021年第2期4卷 57-60页

作者： Miguel R.Buitrago marco e.Guerrero Kristin L.eckland Ana mar.a Ramírez eric e.Vinck Department of Thoracic and Robotic Thoracic Surgery National Cancer InstituteMarly ClinicBogotaColombia Department of Medicine and Surgery Marly ClinicBogotaColombia Department of Cardiothoracic Surgery University of CaliforniaSan FranciscoUSA Department of Thoracic Surgery El Bosque UniversityBogotaColombia Department of Cardiovascular Surgery Cardio VID ClinicMedellínColombia

Patients with poor lung function have a high-risk for pulmonary complications following *** development of minimally invasive thoracic surgical techniques allows sicker patients to safely undergo lung *** lobectomy could benefit these higher risk *** we present a case of a 58-year-old female patient with poor lung function presented with a 3-cm mass in her lower left pulmonary lobe,who successfully underwent lobectomy via robot-assisted thoracoscopic *** forced expiratory volume in one second was slightly improved compared to the preoperative *** forced vital capacity continued to improve in the follow-up *** was no recorded recurrence during the three years follow-up period.

关键词： Poor lung function Lung cancer Robot-assisted thoracoscopic surgery Lobectomy

Mitochondrial protection by low doses of insulin-like growth factor-Ⅰin experimental cirrhosis

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World Journal of Gastroenterology 2008年第17期14卷 2731-2739页

作者： Raquel Pérez mar.a García-Fernández Matías Díaz-Sánchez Juan e Puche Gloria Delgado mar.an Conchillo Jordi Muntané Inma Castilla-Cortázar Departments of Human Physiology and Internal Medicine University of Navarra Department of Medical Physiology School of Medicine University of Málaga Department of Internal Medicine Liver Unit University of Córdoba

AIM： To characterize the mitochondrial dysfunction in experimental cirrhosis and to study whether insulin-like growth factor-Ⅰ （IGF-Ⅰ ） therapy （4 wk） is able to induce beneficial effects on damaged mitochondria leading to cellular protection. MeTHODS： Wistar rats were divided into three groups： Control group, untreated cirrhotic rats and cirrhotic rats treated with IGF-Ⅰ treatment （2 μg/1O0 g bw/d）. Mitochondrial function was analyzed by flow cytometry in isolated hepatic mitochondria, caspase 3 activation was assessed by Western blot and apoptosis by TUNeL in the three expedmental groups. ReSULTS： Untreated cirrhotic rats showed a mitochondrial dysfunction characterized by a significant reduction of mitochondrial membrane potential （in status 4 and 3）; an increase of intramitochondrial reactive oxigen species （ROS） generation and a significant reduction of ATPase activity. IGF-Ⅰ therapy normalized mitochondrial function by increasing the membrane potential and ATPase activity and reducing the intramitochondrial free radical production. Activity of the electron transport complexes Ⅰ and Ⅲ was increased in both cirrhotic groups. In addition, untreated cirrhotic rats showed an increase of caspase 3 activation and apoptosis. IGF- Ⅰ therapy reduced the expression of the active peptide of caspase 3 and resulted in reduced apoptosis. CONCLUSION： These results show that IGF- Ⅰ exerts a mitochondrial protection in experimental cirrhosis leading to reduced apoptosis and increased ATP production.

关键词： Insulin-like growth factor- Ⅰ Cirrhosis Mitochondrial protection Caspases Apoptosis Oxidativedamage

Magma chamber growth models in the upper crust: A review of the hydraulic and inertial constraints

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Geoscience Frontiers 2019年第3期10卷 1211-1218页

作者： eugenio Aragón Fernando J.D'eramo Lucio P.Pinotti Manuel Demartis José mar.a Tubía Roberto F.Weinberg Jorge e.Coniglio Centro de Investigaciones Geologicas (CONICeT-Universidad Nacional de La Plata).Diagonal 113 N° 275 Universidad Nacional de Río Cuarto CONICET Departamento de Geología (Ruta Nac.N° 36 Km 601) Departamento de Geodinámica Universidad del País Vasco (UPV/EHU) School of earth Atmosphere and Environment Monash University

Finite volumes of magma moving in confinement, store hydraulic potential energy for the generation,control and transmission of power. The Pascal's principle in a hydraulic jack arrangement is used to model the vertical and lateral growth of sills. The small input piston of the hydraulic jack is equivalent to the feeder dike, the upper large expansible piston equivalent to the magmatic chamber and the inertial force of the magma in the dike is the input force. This arrangement is particularly relevant to the case of sills expanding with blunt tips, for which rapid fracture propagation is inhibited. Hydraulic models concur with experimental data that show that lateral expansion of magma into a sill is promoted when the vertical ascent of magma through a feeder dike reaches the bottom contact with an overlying, flat rigid-layer. At this point, the magma is forced to decelerate, triggering a pressure wave through the conduit caused by the continued ascent of magma further down(fluid-hammer effect). This pressure wave can provide overpressure enough to trigger the initial hydraulic lateral expansion of magma into an incipient sill, and still have enough input inertial force left to continue feeding the hydraulic system. The lateral expansion underneath the strong impeding layer, causes an area increase and thus, further hydraulic amplification of the input inertial force on the sides and roof of the incipient sill, triggering further expansion in a self-reinforcing process. Initially, the lateral pressure increase is larger than that in the roof allowing the sill to expand. However, expansion eventually increases the total integrated force on the roof allowing its uplift into either a laccolith, if the roof preserves continuity, or into a piston bounded by a circular set of fractures. Hydraulic models for shallow magmatic chambers, also suggest that laccolith-like intrusions require the existence of a self-supported chamber roof. In contrast, if the roof of magmatic cham

关键词： Pascal’s principle Geologic hydraulic jack emplacement Sills growth Fluid hammer