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A hybrid nickel/iron-pyromellitic acid electrocatalyst for oxygen evolution reaction

Nano Research 2024年第4期17卷 2481-2491页

作者： Guoqi li lin li Wenlong li Fusheng li Chunze Yuan Nian Zhang Hui Zhang Tsu-Chien Weng School of Physical Science and Technology ShanghaiTech UniversityShanghai 201210China Center for Transformative Science ShanghaiTech UniversityShanghai 201210China State Key Lab of Fine Chemicals Institute of Artificial PhotosynthesisDUT-KTH Joint Education and Research Center on Molecular DevicesDalian University of Technology(DUT)Dalian 116024China State Key Laboratory of Functional Materials for Informatics Shanghai Institute of Microsystem and Information TechnologyChinese Academy of SciencesShanghai 200050China

The migration of protons during the oxygen evolution reaction(OER)is a key factor that affects the performance of OER *** enhance proton transportation,we designed a catalyst based on nickel/iron-pyromellitic acid(NiFe-PMA)prepared by the electrochemical deposition *** catalyst exhibited a low overpotential of 188 mV at a current density of 10 mA·cm^(-2),a Tafel slope of 28.2 mV·dec^(-1),and long-term stability for 30 days with a current of 50 mA·cm^(-2).We characterized the NiFe-PMA catalyst using various techniques,including Fourier transform infrared(FTIR)spectroscopy,Raman spectroscopy,X-ray photoelectron spectroscopy(XPS),X-ray absorption spectroscopy(XAS),transmission electron microscopy(TEM),scanning electron microscopy(SEM),and inductively coupled plasma-optical emission spectrometry(ICP-OES).Our results showed that NiFe-PMA contains nickel,iron atoms,and both coordinated and uncoordinated carboxylate ***,XPS data confirmed that carboxylate ligands could adjust the outer electronic structure of metal ions,resulting in the high valence state of Ni in *** result of XAS indicated that the nickel atoms present in the catalyst might be easier to maintain a higher chemical *** investigations using kinetic isotope effects(KIEs)and proton inventory revealed that the uncoordinated carboxylic protons played a crucial role in receiving protons during the OER,which promoted the proton transfer of the rate-determining step of the *** novel electrocatalysts provide a new strategy for designing more active and cost-effective catalysts for the OER.

关键词： nickel/iron-pyromellitic acid oxygen evolution reaction kinetic isotope effects

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Progress of gaseous arsenic removal from flue gas by adsorption:Experimental and theoretical calculations

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Journal of Environmental Sciences 2024年第2期136卷 470-485页

作者： Xuelei Yan Qingzhu li Xiaowei Huang Bensheng li Shengtu li Qingwei Wang School of Metallurgy and Environment Central South UniversityChangsha 410083China National Engineering Research Centre for Control and Treatment of Heavy Metal Pollution Central South UniversityChangsha 410083China National Engineering Research Center for Rare Earth Materials General Research Institute for Non-Ferrous MetalsBeijing 100088China

Because of its high mobility and difficult capture,gaseous arsenic pollution control has become the focus of arsenic pollution *** mainly exists in the form of highly toxic As_(2)O_(3)in the flue ***,removing gaseous As_(2)O_(3)from flue gas is of great practical significance for arsenic pollution *** gaseous As_(2)O_(3)on the surface of adsorbents by physical or chemical adsorption is an effective way to reduce the content of arsenic in the flue gas and alleviate arsenic *** the past few decades,various adsorbents have been developed to capture gaseous As_(2)O_(3)in the flue gas,and their adsorption mechanisms have been studied in ***,it is necessary to review the strategies of arsenic removal from flue gas by adsorption,which can inspire further *** on summarizing the morphological distribution of gaseous As_(2)O_(3)in the flue gas,this review further summarizes the removal of gaseous As_(2)O_(3)by several adsorbents and the effect of temperature and the main components of the flue gas on arsenic *** addition,the mechanism of arsenic removal based on adsorption in the flue gas is discussed in depth through theoretical calculations,which is the particular focus of this ***,prospects based on the present research state of arsenic removal by adsorption are proposed to provide ideas for developing effective and stable adsorbents for arsenic removal from flue gas.

关键词： Gaseous arsenic Flue gas Adsorption Theoretical calculation Mechanism

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Alignment efficient image-sentence retrieval considering transferable cross-modal representation learning

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Frontiers of Computer Science 2024年第1期18卷 77-91页

作者： Yang YANG Jinyi GUO Guangyu li Lanyu li Wenjie li Jian YANG School of Computer Science and Engineering Nanjing University of Science and TechnologyNanjing 210094China Department of Computing Hong Kong Polytechnic UniversityHong Kong 100872China State Key Lab.for Novel Software Technology Nanjing UniversityNanjing 210094China 14th Research Institute of China Electronics Technology Group Corporation Nanjing 210094China guangyu.li2017@***

Traditional image-sentence cross-modal retrieval methods usually aim to learn consistent representations of heterogeneous modalities,thereby to search similar instances in one modality according to the query from another modality in *** basic assumption behind these methods is that parallel multi-modal data(i.e.,different modalities of the same example are aligned)can be obtained in *** other words,the image-sentence cross-modal retrieval task is a supervised task with the alignments as ***,in many real-world applications,it is difficult to realign a large amount of parallel data for new scenarios due to the substantial labor costs,leading the non-parallel multi-modal data and existing methods cannot be used *** the other hand,there actually exists auxiliary parallel multi-modal data with similar semantics,which can assist the non-parallel data to learn the consistent ***,in this paper,we aim at“Alignment Efficient Image-Sentence Retrieval”(AEIR),which recurs to the auxiliary parallel image-sentence data as the source domain data,and takes the non-parallel data as the target domain *** single-modal transfer learning,AEIR learns consistent image-sentence cross-modal representations of target domain by transferring the alignments of existing parallel ***,AEIR learns the image-sentence consistent representations in source domain with parallel data,while transferring the alignment knowledge across domains by jointly optimizing a novel designed cross-domain cross-modal metric learning based constraint with intra-modal domain adversarial ***,we can effectively learn the consistent representations for target domain considering both the structure and semantic ***,extensive experiments on different transfer scenarios validate that AEIR can achieve better retrieval results comparing with the baselines.

关键词： image-sentence retrieval transfer learning semantic transfer structure transfer

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Rainbow Pancyclicity in a Collection of Graphs Under the Dirac-type Condition

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Acta Mathematicae Applicatae Sinica 2024年第2期40卷 269-274页

作者： Lu-yi li Ping li Xue-liang li Center for Combinatorics and LPMC Nankai UniversityTianjin 300071China School of Mathematics and Statistics Shaanxi Normal UniversityXi’an 710062China

Let G={Gi:i∈[n]} be a collection of not necessarily distinct n-vertex graphs with the same vertex set V,where G can be seen as an edge-colored(multi)graph and each Gi is the set of edges with color i.A graph F on V is called rainbow if any two edges of F come from different Gis’.We say that G is rainbow pancyclic if there is a rainbow cycle Cℓof lengthℓin G for each integerℓ2[3,n].In 2020,Joos and Kim proved a rainbow version of Dirac’s theorem:Ifδ(Gi)≥2/n for each i∈[n],then there is a rainbow Hamiltonian cycle in *** this paper,under the same condition,we show that G is rainbow pancyclic except that n is even and G consists of n copies of Kn/2,n/*** result supports the famous meta-conjecture posed by Bondy.

关键词： rainbow Hamiltonian cycle rainbow pancyclic meta-conjecture

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Prenatal cadmium exposure impairs neural tube closure via inducing excessive apoptosis in neuroepithelium

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Journal of Environmental Sciences 2024年第4期138卷 572-584页

作者： Shiyong Zhu Xuenan li Xueyan Dai Jinlong li College of Veterinary Medicine Northeast Agricultural UniversityHarbin 150030China Key Laboratory of the Provincial Education Department of Heilongjiang for Common Animal Disease Prevention and Treatment Northeast Agricultural UniversityHarbin 150030China Heilongjiang Key Laboratory for Laboratory Animals and Comparative Medicine Northeast Agricultural UniversityHarbin 150030China

Birth defects have become a public health *** hazardous environmental factors exposure to embryos could increase the risk of birth ***,a toxic environmental factor,can cross the placental barrier during *** woman may be subjected to cadmium before taking precautionary protective ***,the link between birth defects and cadmium remains *** exposure can induce excessive apoptosis in neuroepithelium during embryonic development *** exposure activated the p53 via enhancing the adenosine 5‘-monophosphate(AMP)-activated protein kinase(AMPK)and reactive oxygen species'(ROS)*** cadmium decreases the level of Paired box 3(Pax3)and murine double minute 2(Mdm2),disrupting the process of p53 *** p53 accumulation induced excessive apoptosis in neuroepithelium during embryonic development *** apoptosis led to the failure of neural tube *** study emphasizes that environmental materials may increase the health risk for *** caused the failure of neural tube closure during early embryotic *** women may be exposed by cadmium before taking precautionary protective actions,because of cadmium concentration-containing foods and environmental tobacco *** suggests that prenatal cadmium exposure is a threatening risk factor for birth defects.

关键词： Cadmium Neural tube closure Excessive apoptosis p53 Embryogenesis

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Gut microbiota intervention attenuates thermogenesis in broilers exposed to high temperature through modulation of the hypothalamic 5‑HT pathway

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Journal of Animal Science and Biotechnology 2024年第2期15卷 679-698页

作者： Sheng li Xiaoqing li Kai Wang Yansen li Kentaro Nagaoka Chunmei li Research Centre for livestock Environmental Control and Smart Production College of Animal Science and TechnologyNanjing Agricultural UniversityNanjing 210095China Laboratory of Veterinary Physiology Department of Veterinary MedicineFaculty of AgricultureTokyo University of Agriculture and TechnologyTokyo 183‑8509Japan

Background Broilers have a robust metabolism and high body temperature,which make them less tolerant to hightemperature(HT)environments and more susceptible to challenges from elevated *** microbes,functioning as symbionts within the host,possess the capacity to significantly regulate the physiological functions and environmental adaptability of the *** study aims to investigate the effects of gut microbial intervention on the body temperature and thermogenesis of broilers at different ambient temperatures,as well as the underlying mechanism involving the"gut-brain"*** Broilers were subjected to gut microbiota interference with or without antibiotics(control or ABX)starting at 1 day of *** 21 day of age,they were divided into 4 groups and exposed to different environments for 7 d:The control and ABX groups at room temperature(RT,24±1℃,60%relative humidity(RH),24 h/d)and the control-HT and ABX-HT groups at high temperature(HT,32±1℃,60%RH,24 h/d).Results The results demonstrated that the antibiotic-induced gut microbiota intervention increased body weight and improved feed conversion in broiler chickens(Pliver(Plistipes was enriched in control *** contrast,antibioticinduced gut microbiota intervention resulted in a decrease in the relative abundance of Alistipes(P<0.05).Moreover,this difference was accompanied by increased hypothalamic 5-hydroxytryptamine(5-HT)content and TPH2 expression(P<0.05).Conclus

关键词： 5-HT Broiler chickens Gut microbiota Thermogenesis Thermoregulation

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Style-conditioned music generation with Transformer-GANs

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Frontiers of Information Technology & Electronic Engineering 2024年第1期25卷 106-120页

作者： Weining WANG Jiahui li Yifan li Xiaofen XING School of Electronic and Information Engineering South China University of TechnologyGuangzhou 510600China

Recently,various algorithms have been developed for generating appealing ***,the style control in the generation process has been somewhat *** style refers to the representative and unique appearance presented by a musical work,and it is one of the most salient qualities of *** this paper,we propose an innovative music generation algorithm capable of creating a complete musical composition from scratch based on a specified target style.A style-conditioned linear Transformer and a style-conditioned patch discriminator are introduced in the *** style-conditioned linear Transformer models musical instrument digital interface(MIDI)event sequences and emphasizes the role of style ***,the style-conditioned patch discriminator applies an adversarial learning mechanism with two innovative loss functions to enhance the modeling of music ***,we establish a discriminative metric for the first time,enabling the evaluation of the generated music’s consistency concerning music *** objective and subjective evaluations of our experimental results indicate that our method’s performance with regard to music production is better than the performances encountered in the case of music production with the use of state-of-the-art methods in available public datasets.

关键词： Music generation Style-conditioned Transformer Music emotion

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A novel evasion guidance for hypersonic morphing vehicle via intelligent maneuver strategy

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Chinese Journal of Aeronautics 2024年第5期37卷 441-461页

作者： Xun li Xiaogang WANG Hongyu ZHOU Yu li Department of Aerodynamics Harbin Institute of TechnologyHarbin 150001China Beijing Aerospace Technology Institute Beijing 100074China

This paper presents a novel evasion guidance law for hypersonic morphing vehicles,focusing on determining the optimized wing's unfolded angle to promote maneuverability based on an intelligent ***,the pursuit-evasion problem is modeled as a Markov decision *** the agent's action consists of maneuver overload and the unfolded angle of wings,which is different from the conventional evasion guidance designed for fixed-shape *** reward function is formulated to ensure that the miss distances satisfy the prescribed bounds while minimizing energy ***,to maximize the expected cumulative reward,a residual learning method is proposed based on proximal policy optimization,which integrates the optimal evasion for linear cases as the baseline and trains to optimize the performance for nonlinear engagement with multiple ***,offline training guarantees improvement of the constructed evasion guidance law over conventional ***,the guidance law for online implementation includes only analytical *** maps from the confrontation state to the expected angle of attack and the unfolded angle while retaining high computational *** show that the proposed evasion guidance law can utilize the change of unfolded angle to extend the maximum overload *** it surpasses conventional maneuver strategies by ensuring better evasion efficacy and higher energy efficiency.

关键词： Hypersonic vehicles Variable-sweep wings Evasion guidance Reinforcement learning Pursuit-evasion problem

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Predicting Turbidite Channel in Deep-Water Canyon Based on Grey Relational Analysis-Support VectorMachineModel:A Case Study of the lingshui Depression in Qiongdongnan Basin,South China Sea

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Energy Engineering 2024年第9期121卷 2435-2447页

作者： Haichen li Jianghai li li li Zhandong li School of Earth and Space Sciences Peking UniversityBeijing100871China Key Laboratory of Orogenic Belts and Crustal Evolution Peking UniversityBeijing100871China Geotechnical Physical and Mechanical Properties Laboratory Langfang Normal UniversityLangfang065000China Heilongjiang Northeast Petroleum University Science Park Development Co. Ltd.Daqing163318China College of Petroleum Engineering Northeast Petroleum UniversityDaqing163318China

The turbidite channel of South China Sea has been highly *** by the complex fault and the rapid phase change of lithofacies,predicting the channel through conventional seismic attributes is not accurate *** response to this disadvantage,this study used a method combining grey relational analysis(GRA)and support vectormachine(SVM)and established a set of prediction technical procedures suitable for reservoirs with complex geological *** the case study of the Huangliu Formation in Qiongdongnan Basin,South China Sea,this study first dimensionalized the conventional seismic attributes of Gas Layer Group I and then used the GRA method to obtain the main relational factors.A higher relational degree indicates a higher probability of responding to the attributes of the turbidite *** study then accumulated the optimized attributes with the highest relational factors to obtain a first-order accumulated sequence,which was used as the input training sample of the SVM model,thus successfully constructing the SVM turbidite channel *** results prove that the GRA-SVMmethod has a high drilling coincidence *** the core and logging data and taking full use of the advantages of seismic inversion in predicting the sand boundary of water channels,this study divides the sedimentary microfacies of the Huangliu Formation in the lingshui 17-2 Gas *** comprehensive study has shown that the GRA-SVM method has high accuracy for predicting turbidite channels and can be used as a superior turbidite channel prediction method under complex geological conditions.

关键词： Support vector machine channel Huangliu Formation Qiongdongnan Basin

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Optimization of Band Gap of 1D Elastic Metamaterial Under Impact Load by Regulating Stiffness

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Acta Mechanica Solida Sinica 2024年第1期37卷 148-154页

作者： Tong li Xianlong Jin Yongqiang li Peizhong Yang School of Mechanical Engineering Shanghai Jiao Tong UniversityShanghai 200240China State Key Laboratory of Mechanical System and Vibration Shanghai Jiaotong UniversityShanghai 200240China College of Science Northeastern UniversityShenyang 110819China

Designing materials that mitigate impacts effectively are crucial for protecting people and ***,a single-resonator metamaterial with negative mass characteristics is proposed for impact mitigation,and numerical analysis of wave propagation shows explicitly how the spring stiffness and number of unit cells influence that *** results show clearly that a metamaterial with differing microstructural stiffness is better at mitigating the effect of a shock wave than one with a unique ***,there is a critical number of unit cells beyond which the shock wave is not attenuated further,but the fabrication complexity *** the 40 groups of microstructural regions in this example,the attenuation effect no longer increases when there are more than 35 *** work offers guidance for microstructure designs in metamaterials and provides new ideas for using metamaterials to mitigate shock waves.

关键词： Elastic metamaterials Wave attenuation Stiffness Number of unit cells

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