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Science China Chemistry 2024年第9期67卷 2949-2957页

作者： Zhaojian Wang Wei Zhang Wenzhong Huang Ruohan Yu Changliang Chen Liqiang mai Liang Zhou State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan 430070China Sanya Science and Education Innovation Park Wuhan University of TechnologySanya 572000China Hubei Longzhong Laboratory Wuhan University of Technology(Xiangyang Demonstration Zone)Xiangyang 441000China

Most oxygen evolution reaction(OER)electrocatalysts show poor stability under industrial alkaline conditions(20–30 wt.%KOH).Therefore,it is essential to develop stable,efficient,and low-cost OER catalysts for industrial water ***,we present a straightforward approach for the complete electrochemical reconstruction of Ni-BDC,a Ni-based metal-organic framework,for *** method involves the continuous release of Fe^(3+)from Fe foam counter electrode in a high-concentration(6.0 M,25 wt.%)KOH *** continuously Fe^(3+)releasing not only realizes in situ Fe^(3+)doping,but also introduces abundant defects in the obtained catalyst during cyclic voltammetry activation,thereby accelerating the electrochemical *** reconstructed OER catalyst(Fe-doped nickel hydroxide/oxyhydroxide nanosheets supported on Ni foam,Fe-NiO_(x)(OH)y/NF)manifests a low overpotential of 217 mV at 10 mA cm^(-2)and 263 m V at 100 m A cm^(-2)in 1.0 M ***,the Fe-NiO_(x)(OH)_(y)/NF also demonstrates high stability in 30 wt.%*** strategy of regulating the electrochemical reconstruction process sheds light on the construction of stable and efficient OER catalysts for industrial water electrolysis.

关键词： oxygen evolution reaction industrial alkaline conditions metal-organic framework complete reconstruction

面向脉搏血氧监测系统的三元阳离子锡铅钙钛矿基高灵敏、快响应近红外光电探测器

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Science China Materials 2023年第12期66卷 4704-4710页

作者：吕一博岑国标李婉君赵传熙麦文杰 Siyuan Laboratory Guangdong Provincial Engineering Technology Research Center of Vacuum Coating Technologies and New Energy MaterialsDepartment of PhysicsJinan UniversityGuangzhou 510632China Guangdong Provincial Key Laboratory of Nanophotonic Manipulation Jinan UniversityGuangzhou 511443China

血氧饱和度已成为继心电图、呼吸和血压后的一项用于健康评价的重要生理参数.本研究中,我们制备出高质量窄带隙三元阳离子Sn-Pb钙钛矿薄膜,该光电薄膜呈现择优的生长晶向,且光吸收截止边拓宽至961 nm.通过双界面层修饰,构建的PPPB(PEDOT... 详细信息

血氧饱和度已成为继心电图、呼吸和血压后的一项用于健康评价的重要生理参数.本研究中,我们制备出高质量窄带隙三元阳离子Sn-Pb钙钛矿薄膜,该光电薄膜呈现择优的生长晶向,且光吸收截止边拓宽至961 nm.通过双界面层修饰,构建的PPPB(PEDOT:PSS/perovskite/PCBM/BCP)近红外光电探测器展现出增强的光电响应,极快的响应速度(373 ns),宽的线性动态范围(LDR=159 dB),高的比探测率(D*=1.56×10^(11)Jones),以及优异的光响应度(190 mA W^(−1)).基于器件出色的光电性能,我们探索并演示了该探测器在脉搏血氧仪系统中的应用,实现了对不同生理状态下心率和血氧饱和度的准确和非侵入性评估.本研究突显了三元阳离子锡铅钙钛矿光探测器在实时监测血氧饱和度和心率方面的应用潜力.

关键词： detector near-infrared Sn-Pb perovskite oxygen blood oxygen saturation

Identification,Characterization,and Probiotic Potentials of Lactobacillus pentosus SF-1

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Journal of Ocean University of China 2024年第2期23卷 509-517页

作者： JIAO Lin LIANG Shufei CHU Ruixia WANG Wentao mai Kangsen LIU Ming WAN Min Key Laboratory of Aquaculture Nutrition and Feed Ministry of Agriculture&Key Laboratory of MaricultureMinistry of EducationCollege of FisheriesOcean University of ChinaQingdao 266003China Engineering Research Center of Mariculture Ministry of EducationOcean University of ChinaQingdao 266003China

In recent years probiotics have been considered as a potential substitution of antibiotics to control pathogens and treat infectious diseases in *** the present study a strain of Lactobacillus pentosus,named as *** SF-1,was isolated from waters in *** species identification of this strain was conducted by 16S rRNA sequence,and the physiological and biochemical characteristics of this strain were ***,the virulence,antibiotic sensitivity,cell surface characteristics and acid/base-resistance of *** SF-1 were determined to evaluate the probiotic potentials of this ***,*** SF-1 is sensitive to most common antibiotics,and no hemolysin was generated from it,indicating the safety of this strain to *** addition,*** SF-1 was able to tolerate the artificial gastric juice at pH 3 for 4 h and the artificial intestinal fluid at pH 6.8 or 8.0 for 6 ***,the analysis of self-aggregation and the adhesion of *** SF-1 to organic solvents suggested a high potential of *** SF-1 to inhabit the hosts,which was confirmed by testing the colonization of *** SF-1 in germ-free ***,*** SF-1 displayed a high bactericidal activity against several bacterial ***,the incubation of *** SF-1 significantly promoted the expression of antimicrobial components in zebrafish,contributing to the protection of the fish from *** infection in *** together,the probiotic strain *** SF-1 could be applied as anti-infection reagent in aquaculture.

关键词： Lactobacillus pentosus probiotics antibiotics hemolysis cell surface characteristics bactericidal activity infection

Expanding the liver donor pool worldwide with hepatitis C infected livers, is it the time?

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World Journal of Transplantation 2024年第2期14卷 13-27页

作者： mai Hashem Mohammed A Medhat Doaa Abdeltawab Nahed A Makhlouf Fellow of Tropical Medicine and Gastroenterology Assiut University HospitalAssiut 71515Egypt Department of Tropical Medicine and Gastroenterology Faculty of MedicineAssiut UniversityAssiut 71515Egypt Department of Tropical Medicine and Gastroenterology Al-Rajhi Liver HospitalAssiut UniversityAssiut 71515Egypt

Liver transplantation(LT)provides a life-saving option for cirrhotic patients with complications and hepatocellular *** the increasing number of liver transplants performed each year,the number of LT candidates on the waitlist remains unchanged due to an imbalance between donor organ supply and the demand which increases the waitlist time and *** donor liver transplant had a great role in increasing the donor pool and shortened waitlist time for LT ***,further strategies can be implemented to increase the pool of potential donors in deceased donor LT,such as reducing the rate of organ *** hepatitis C virus(HCV)seropositive liver grafts is one of the expanded donor organ criteria.A yearly increase of hundreds of transplants is anticipated as a result of maximizing the utilization of HCV-positive organs for HCV-negative ***-acting antiviral therapy's efficacy has revolutionized the treatment of HCV infection and the use of HCV-seropositive donors in *** American Society of Transplantation advises against performing transplants from HCV-infected liver donors(D+)into HCV-negative recipient(R-)unless under Institutional Review Board-approved study rules and with full informed consent of the knowledge gaps associated with such *** selection of patients to be transplanted with HCV-infected grafts and confirming their access to direct-acting antivirals if needed is *** and international consensuses are needed to regulate this process to ensure the maximum benefit and the least adverse events.

关键词： Donor pool Hepatitis C-viremic organs Non-viremic organs Direct acting antivirals Hepatitis C virus treated Liver transplantation

On equidistribution theorem for multi-sequences of holomorphic line bundles

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Science China Mathematics 2024年

作者： Manli Liu Weixiong mai Guokuan Shao Department of Mathematics South China Agricultural University Macao Center for Mathematical Sciences Macau University of Science and Technology School of Mathematics (Zhuhai) Sun Yat-sen University

Given several sequences of Hermitian holomorphic line bundles {(Lkp, hkp)}p∞=1, we establish the distribution of common zeros of random holomorphic sections of Lkpwith respect to singular measures. We also study the ...

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Ultrafast Laser-Induced Excellent Thermoelectric Performance of PEDOT:PSS Films

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Energy & Environmental Materials 2024年第3期7卷 425-431页

作者： Xuewen Wang Yuzhe Feng Kaili Sun Nianyao Chai Bo mai Sheng Li Xiangyu Chen Wenyu Zhao Qingjie Zhang State Key Laboratory of Advanced Technology for Materials Synthesis and Processing International School of Materials Science and EngineeringWuhan University of TechnologyNo.122Luoshi Rd.Wuhan 430070China Foshan Xianhu Laboratory of the Advanced Energy Science and Technology Guangdong Laboratory No.1Yangming Rd.Foshan 528200China

Because poly(3,4-ethylenedioxythiophene)-poly(styrenesulfonate)(PEDOT:PSS)is water processable,thermally stable,and highly conductive,PEDOT:PSS and its composites have been considered to be one of the most promising flexible thermoelectric ***,the PEDOT:PSS film prepared from its commercial aqueous dispersion usually has very low conductivity,thus cannot be directly utilized for TE ***,a simple environmental friendly strategy via femtosecond laser irradiation without any chemical dopants and treatments was *** optimal conditions,the electrical conductivity of the treated film is increased to 803.1 S cm^(-1)from 1.2 S cm^(-1)around three order of magnitude higher,and the power factor is improved to 19.0μW m^(-1)K^(-2),which is enhanced more than 200 *** mechanism for such remarkable enhancement was attributed to the transition of the PEDOT chains from a coil to a linear or expanded coil conformation,reduction of the interplanar stacking distance,and the removal of insulating PSS with increasing the oxidation level of PEDOT,facilitating the charge *** work presents an effective route for fabricating high-performance flexible conductive polymer films and wearable thermoelectric devices.

关键词： electrical conductivity PEDOT:PSS thermoelectric film ultrafast laser irradiation

Speed and surface steepness affect internal tibial loading during running

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Journal of Sport and Health Science 2024年第1期13卷 118-124页

作者： Hannah Rice Markus Kurz Patrick mai Leon Robertz Kevin Bill Timothy R.Derrick Steffen Willwacher Department of Physical Performance Norwegian School of Sport SciencesOslo 0806Norway Sports Tech Research Centre Mid Sweden UniversityÖstersund SE-83125Sweden Department of Mechanical and Process Engineering Offenburg University of Applied SciencesOffenburg 77652Germany Institute of Biomechanics and Orthopaedics German Sport University CologneCologne 50933Germany Department of Kinesiology Iowa State UniversityAmesIA 50011USA

Background:Internal tibial loading is influenced by modifiable factors with implications for the risk of stress *** encounter varied surface steepness(gradients)when running outdoors and may adapt their speed according to the *** study aimed to quantify tibial bending moments and stress at the anterior and posterior peripheries when running at different speeds on surfaces of different ***:Twenty recreational runners ran on a treadmill at 3 different speeds(2.5 m/s,3.0 m/s,and 3.5 m/s)and gradients(level:0%;uphill:+5%,+10%,and+15%;downhill:-5%,-10%,and-15%).Force and marker data were collected synchronously *** moments were estimated at the distal third centroid of the tibia about the medial-lateral axis by ensuring static equilibrium at each 1%of *** was derived from bending moments at the anterior and posterior peripheries by modeling the tibia as a hollow ***-way repeated-measures analysis of variance were conducted using both functional and discrete statistical ***:There were significant main effects for running speed and gradient on peak bending moments and peak anterior and posterior *** running speeds resulted in greater tibial *** uphill at+10%and+15%resulted in greater tibial loading than level *** downhill at-10%and-15%resulted in reduced tibial loading compared to level *** was no difference between+5%or-5%and level ***:Running at faster speeds and uphill on gradients≥+10%increased internal tibial loading,whereas slower running and downhill running on gradients≥-10%reduced internal *** running speed according to the gradient could be a protective mechanism,providing runners with a strategy to minimize the risk of tibial stress injuries.

关键词： Bending moments Gradient Musculoskeletal modeling Overuse injury Tibial stress Training factors

Explainable AI-Based DDoS Attacks Classification Using Deep Transfer Learning

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Computers, Materials & Continua 2024年第9期80卷 3785-3802页

作者： Ahmad Alzu’bi Amjad Albashayreh Abdelrahman Abuarqoub mai A.M.Alfawair Department of Computer Science Jordan University of Science and TechnologyIrbid22110Jordan Department of Computer Science The University of JordanAmman11942Jordan Cardiff School of Technologies Cardiff Metropolitan UniversityCardiffCF52YBUK Prince Abdullah bin Ghazi Faculty of Information and Communication Technology Al-Balqa Applied UniversitySalt19117Jordan

In the era of the Internet of Things(IoT),the proliferation of connected devices has raised security concerns,increasing the risk of intrusions into diverse *** the convenience and efficiency offered by IoT technology,the growing number of IoT devices escalates the likelihood of attacks,emphasizing the need for robust security tools to automatically detect and explain *** paper introduces a deep learning methodology for detecting and classifying distributed denial of service(DDoS)attacks,addressing a significant security concern within IoT *** effective procedure of deep transfer learning is applied to utilize deep learning backbones,which is then evaluated on two benchmarking datasets of DDoS attacks in terms of accuracy and time *** leveraging several deep architectures,the study conducts thorough binary and multiclass experiments,each varying in the complexity of classifying attack types and demonstrating real-world ***,this study employs an explainable artificial intelligence(XAI)AI technique to elucidate the contribution of extracted features in the process of attack *** experimental results demonstrate the effectiveness of the proposed method,achieving a recall of 99.39%by the XAI bidirectional long short-term memory(XAI-BiLSTM)model.

关键词： DDoS attack classification deep learning explainable AI cybersecurity

Recent progress of Pt-based oxygen reduction reaction catalysts for proton exchange membrane fuel cells

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Rare Metals 2024年第6期43卷 2444-2468页

作者： Feng Zhan Kun-Song Hu Jin-Hua mai Li-Sheng Zhang Zhen-Guo Zhang Huan He Xin-Hua Liu School of Resources Environment and MaterialsGuangxi UniversityNanning530004China School of Transportation Science and Engineering Beihang UniversityBeijing 102206China IDTECH(Suzhou)Co.Ltd Suzhou 215217China Dyson School of Design Engineering Imperial College LondonLondon SW72AZUK

With the increasing consumption of fossil fuels,proton exchange membrane fuel cells(PEMFCs)have attracted considerable attention as green and sustainable energy conversion *** slow kinetics of the cathodic oxygen reduction reaction(ORR)has a major impact on the performance of PEMFCs,and although platinum(Pt)can accelerate the reaction rate of the ORR,the scarcity and high cost of Pt resources still limit the development of ***,the development of low-cost high-performance ORR catalysts is essential for the commercial application and development of *** paper reviews the research progress of researchers on Pt-based ORR catalysts in recent years,including Pt/C catalysts,Pt-based alloy catalysts,Pt-based intermetallic compounds,and Pt-based single-atom catalysts(SACs),with a focus on Pt-based alloy catalysts with different *** described in detail the difficulties and solutions in the research process of various ORR catalysts and explained the principle of their activity enhancement with density functional theory(DFT).In addition,an outlook on the development of Pt-based catalysts is given,and reducing the amount of Pt used and improving the performance of catalysts are the directions to work on in the coming period.

关键词： Pt-based catalysts PEMFCs Pt-based intermetallic compounds Single-atom catalysts

Insight into the mechanism of 5-hydroxymethylfurfural electroreduction to 2,5-bis(hydroxymethyl)furan over Cu anchored N-doped carbon nanosheets

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Nano Research 2024年第9期17卷 7991-7999页

作者： Haoran Wu Xinwei Chen Haishan Xu Runlu Yang Xin Wang Junying Chen Zhenbing Xie Liang Wu Yiyong mai School of Chemical Engineering Zhengzhou UniversityZhengzhou 450001China School of Chemistry and Chemical Engineering Frontiers Science Center for Transformative MoleculesShanghai Key Laboratory of Electrical Insulation and Thermal AgeingShanghai Jiao Tong UniversityShanghai 200240China Department of Chemistry Tangshan Normal UniversityTangshan 063000China

Design of non-noble metal electrocatalysts for biomass conversion to high-value chemicals and understanding the related catalytic mechanisms are of profound significance but have remained a major ***,we developed a novel biomass-derived electrocatalyst(denoted as Cu/NC),featuring with electron-deficient copper nanoparticles anchored on N-doped carbon nanosheets,for the electrochemical reduction of 5-hydroxymethylfurfural(HMF)to 2,5-bis(hydroxymethyl)furan(BHMF,a vital precursor of functional polymers).The optimized Cu/NC electrocatalyst exhibited an excellent performance with high Faradaic efficiency(89.5%)and selectivity(90.8%)of BHMF at a low concentration of HMF(18.1 mM).Even at a very high HMF concentration(108.6 mM),the Faraday efficiency and selectivity of BHMF could still reach 74.8%and 81.1%,*** performance approached those of the reported noble metal-based *** study revealed that the N doping in the Cu/NC catalyst could regulate the electronic structure of Cu,strengthening the adsorption of the HMF carbonyl group,and thus boosting the selectivity of ***,strong electronic metal-support interactions of Cu and the N-doped carbon support optimized the charge transfer rate,thus promoting the dissociation of water to the active hydrogen(H^(*))species and boosting the reaction kinetic rate of H^(*)and HMF.

关键词： biomass 5-hydroxymethylfurfural electrochemical reduction N-doped carbon materials 2,5-bis(hydroxymethyl)furan