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Simultaneous enhancements of strength and toughness by multiscale lamellar structure in Ti_(2)AlNb based intermetallic

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Journal of materials Science & Technology 2024年第7期174卷 249-261页

作者： Fan Zhang Weidong Zeng Penghui Zhang Haoyuan ma Jianwei Xu State Key Laboratory of Solidification Processing School of Materials Science and EngineeringNorthwestern Polytechnical UniversityXi’an 710072China Defense Technologies Innovation Center of precision forging and ring rolling School of Materials Science and EngineeringNorthwestern Polytechnical UniversityXi’an 710072China

Multi-scale lamellar structure significantly improves toughness of Ti_(2)AlNb based alloys,which are inher-ently brittle intermetallics,without compromising their *** structure was achieved through-B2-transus-forging(TBTF)combined with O+B2 two-phase region heat *** types of multi-scale lamellar structures were obtained by controlling the cooling rate after *** variations were mainly attributed to differences in the distribution,content,and size of the thick lamellar O phase and the size and crystallographic orientation of B2 *** analyzing the microstructural characteristics and crystallographic orientation near the crack propagation path,it was found that the crack propaga-tion resistance of thick lamellae,sub grain and grain boundaries(GBs)O phase increased sequentially,accompanied by more tortuous crack propagation ***,B2 grains with high misorientation significantly deflected the crack propagation by cleavage ridges between adjoining cleavage ***-tionally,the development of numerous secondary cleavage ridges,resulting from the transition through varying secondary cleavage planes in distinct sub B2 grains,further hindered the quick propagation of *** was clarified that the cleavage planes were dominantly belonging to{110}.These findings pro-vided valuable guidance for the design of damage tolerance strategies for Ti_(2)AlNb-based intermetallics.

关键词： Multiscale lamellae structure Fracture toughness Crack propagation Ti_(2)AlNb-based intermetallic Through-B2-transus-forging

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Design of new chemicals for advanced electrolytes

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Science China Chemistry 2024年第5期67卷 1378-1380页

作者： Haoran Cheng Zheng ma Qian Li Jun Ming State Key Laboratory of Rare Earth Resource Utilization Changchun Institute of Applied ChemistryChinese Academy of SciencesChangchun130022China University of Science and Technology of China Hefei 230026China

This highlight is inspired by a recent article in Nature Energy in which Liu and co-workers [1] from Tsinghua University designed a new asymmetric lithium salt (i.e., lithium 1,1,1-trifluoro-N-[2-[2-(2-methoxy ethoxy)ethoxy]ethyl] methanesulfonamide (Li FEA)) and applied it as a new lithium-salt additive in the conventional carbonate-based electrolyte,overcoming the incompatibility issue of carbonate electrolytes with lithium metal in lithium metal batteries (LMBs),even achieving a fast-charging feature.

关键词： lithium carbonate electrolyte

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A review of CFD simulation in pressure driven membrane with fouling model and anti-fouling strategy

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Frontiers of Environmental Science & Engineering 2024年第8期18卷 1-29页

作者： Shiyong Miao Jiaying ma Xuefei Zhou Yalei Zhang Huaqiang Chu State Key Laboratory of Pollution Control and Resource Reuse Tongji UniversityShanghai 200092China Shanghai Institute of Pollution Control and Ecological Security Tongji UniversityShanghai 200092China

Pressure-driven membrane filtration systems are widely utilized in wastewater treatment,desalination,and water reclamation and have received extensive attention from *** fluid dynamics(CFD)offers a convenient approach for conducting mechanistic studies of flow and mass transfer characteristics in pressure-driven *** a signature phenomenon in membrane systems,the concentration polarization that accompanies the permeation process is a key factor in membrane performance degradation and membrane fouling *** fouling models(scaling,biofouling and colloidal particle fouling)based on CFD theory have been constructed,and considerable research has been *** representative antifouling strategies with special simulation methods,including patterned membranes,vibration membranes,rotation membranes,and pulsatile flows,have also been *** studies should focus on refining fouling models while considering local hydrodynamic characteristics;experimental observation tools focusing on the internal structure of inhomogeneous fouling layers;techno-economic model of antifouling strategies such as vibrational,rotational and pulsatile flows;and unfavorable hydraulic phenomena induced by rapidly changing flows in simulations.

关键词： Computational fluid dynamics Membrane Fouling model Concentration polarization

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Effects of electrothermal ageing on dielectric performance of metallised biaxial orientation polypropylene film capacitors in strong magnetic fields

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High Voltage 2024年第4期9卷 911-919页

作者： Haoliang Liu Boxue Du Meng Xiao Ke Chen Yanwei ma School of Electrical and Information Engineering Tianjin UniversityTianjinChina Institute of Electrical Engineering Chinese Academy of SciencesBeijingChina

The dielectric performance of the pristine and the electrothermal-aged metallised polypropylene capacitors are investigated under different magnetic *** energy storage capacity decreases under the magnetic *** 12 T,the capacitance value of the pristine capacitors decreases by 8.4%-17%and that of the aged capacitors declines by 15%-20%.The dielectric loss is reduced by 2.6%-6.3%,but the equivalent series resistance shows an 8.3%-23.1%*** leakage conductivity increases to 202%-354%,which leads to a weakened voltage holding *** addition to the effects of the magnetic fields,the impacts of ageing have also been *** effects of the magnetic field and ageing on the electrical parameters of the capacitors are discussed *** molecular chains of the dielectric are oxidised and decomposed during the ageing process,which reduces the insulating properties of the *** magnetic field inhibits polarisation by changing the polarisation behaviour through Lorentz force and excites the electrons to enhance charge transmission.

关键词： magnetic performance fields

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Lightweight Si_(3)N_(4)@SiO_(2) ceramic foam for thermal insulation and electromagnetic wave transparency

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Nano Research 2024年第5期17卷 4298-4306页

作者： Zongwei Tong Xiangjie Yan Yuexiang Wang Kexun Li Weihai ma China-Blarus Belt and Road Joint Laboratory on Electromagnetic Environment Effect the 33rd Research Institute of ChinaElectronics Technology Group CorporationTaiyuan 030032China Key Laboratory for Advanced Ceramics and machining Technology of Ministry of Education School of Material Science and EngineeringTianjin UniversityTianjin 300072China Department of materials Science and Engineering Jinzhong UniversityJinzhong 030619China

Increasing porosity is one of the most direct ways to improve the thermal insulation and dielectric properties of *** now,many wet methods for preparing Si_(3)N_(4) ceramic foams usually face the problems of complex rheology,long period,and expensive cost,and the reported pore sizes of Si_(3)N_(4) ceramic foams are typically micron-grade,resulting in a lack of competitiveness in thermal insulation and wave-transparent *** this paper,the Si_(3)N_(4)@SiO_(2) ceramic foams were prepared using an efficient dry-method,which combined three processes of low temperature chemical vapor deposition(LTCVD),template,and isostatic *** method has the advantages of simple operation and short preparation period,and can realize near-net size molding and mass *** addition,the evolution mechanisms of honeycomb microstructure and composition of Si_(3)N_(4)@SiO_(2) ceramic foam during sintering were studied by chemical reaction *** as-prepared Si_(3)N_(4)@SiO_(2) ceramic foam possesses low density(0.377 g·cm^(-3)),high compressive strength(7.5 MPa),low thermal conductivity(0.0808 W·m^(-1)·K^(-1)),and excellent dielectric properties(εmaximum working temperature in air can reach up to 1100℃.It will be recommended to be applied in the interlayer of Si_(3)N_(4) ceramic radome to improve its thermal insulation and electromagnetic wave transparency performances.

关键词： silicon nitride ceramic foam honeycomb microstructure dielectric properties thermal insulation

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Control of aluminum distribution in ZSM-5 zeolite for enhancement of its catalytic performance for propane aromatization

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Frontiers of Chemical Science and Engineering 2024年第8期18卷 15-24页

作者： Zhao ma Dezhi Shi Sen Wang Mei Dong Weibin Fan State Key Laboratory of Coal Conversion Institute of Coal ChemistryChinese Academy of SciencesTaiyuan 030001China University of Chinese Academy of Sciences Beijing 100049China

Regulation of aluminum distribution in zeolite framework is an effective method for improving its catalytic performance for propane ***,we found that recrystallization and post-realuminization of ZSM-5 cannot only create hollow structures to enhance the diffusion ability,but also adjust the content and position of paired aluminum species in its *** characterizations results confirmed that increase of paired aluminum content and inducement of more aluminum atoms sited in the intersection cavity are beneficial to the formation of aromatic products in propane *** a result,the hollow-structured ZSM-5 zeolite with more paired aluminum(H-200-hollow)showed higher propane conversion and aromatics selectivity than other samples at the same *** catalytic performance of H-200-hollow can be further improved by ion-exchanging with a small amount of Ga(III)*** propane conversion and aromatics selectivity of Ga-200-hollow reached as high as 95%and 70%,respectively,at 540°C and 1 atm.

关键词： propane aromatization zeolite aluminum distribution recrystallization and post-realuminization

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真空热处理制备微米级多孔铜

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热加工工艺 2022年第24期51卷 134-137,141页

作者：武夏鹏马玉豪冷利黄庆利任伊宾沈阳理工大学材料科学与工程学院辽宁沈阳110159

对Cu_(75)Zn_(25)、Cu_(50)Zn_(50)和Cu_(25)Zn_(75)合金在450、500和550℃进行真空热处理,制备微米级多孔铜。采用XRD、SEM和EDS对制备的多孔铜进行分析,研究温度和成分对真空热处理后孔形貌的影响。结果表明,真空热处理制备的多孔铜... 详细信息

对Cu_(75)Zn_(25)、Cu_(50)Zn_(50)和Cu_(25)Zn_(75)合金在450、500和550℃进行真空热处理,制备微米级多孔铜。采用XRD、SEM和EDS对制备的多孔铜进行分析,研究温度和成分对真空热处理后孔形貌的影响。结果表明,真空热处理制备的多孔铜孔径为0.5~8.0μm。温度升高使得孔径逐渐增大;铜锌合金中Zn元素含量增多,越容易形成多孔结构和较大的孔径。

关键词：真空热处理多孔铜饱和蒸汽压 Kirkendall效应

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Fluorophosphates and fluorosulfates cathode materials: Progress towards high energy density sodium-ion battery

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Nano Research 2024年第3期17卷 1427-1440页

作者： Mohammed Hadouchi Jingrong Hou Toshinari Koketsu Abdelilah Lahmar Jiwei ma Laboratoire de Chimie Appliquée des matériaux Centre des Sciences des MatériauxFaculty of ScienceMohammed V University in RabatAvenue Ibn BattoutaBP 1014RabatMorocco Shanghai Key Laboratory for R&D and Application of Metallic Functional materials Institute of New Energy for VehiclesSchool of Materials Science and EngineeringTongji UniversityShanghai 201804China Battery materials Development Section Business Creation Sector R&D CenterMitsui Mining&Smelting Co.Ltd.362-0021 SaitamaJapan Laboratoiry of Condensed matter Physics University of Picardie Jules Verne33 Rue Saint-Leu 80039AmiensFrance

The rapid diffusion of renewable energy boosts the wide deployment of large-scale energy storage *** the low cost and high crustal abundance,sodium-ion battery(SIB)technology is expected to become a dominant technology in that area in the *** the practical application,novel cathode materials are urged to develop that show high energy density without sacrificing their cost and benignity to the *** the years of many studies,this still remains a huge challenge to battery *** this review,we discuss recent breakthroughs in SIB cathode materials with high energy density,namely fluorphosphates and *** design of materials,the crystal structure,the electrochemical performance,and the underlaying intercalation mechanism are systematically *** strategies and research directions are also provided to advance future high-energy,low-cost,and ecofriendly cathode materials for next generation SIB.

关键词： fluorophosphates fluorosulfates crystal structure intercalation mechanism high energy density sodium-ion battery

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Conductive edge-warping graphite mesas for robust structural superlubricity

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Science China(Technological Sciences) 2024年第7期67卷 2040-2049页

作者： FENG WeiJia LIU Ying ma Ming PENG DeLi NIE JinHui State Key Laboratory of Tribology in Advanced Equipment&Department of Mechanical Engineering Tsinghua UniversityBeijing 100084China Center for Nano and Micro Mechanics Tsinghua UniversityBeijing 100084China Institute of Superlubricity Technology Research Institute of Tsinghua University in ShenzhenShenzhen 518057China

Structural superlubricity(SSL) refers to a state of ultralow friction and zero wear when two solid surfaces slide against each other. Recent investigations have identified amorphous carbon at the edge of the graphite mesa as the primary source of friction in such SSL systems. Here, the tensile stress of metal thin film is exploited to engineer vertically conductive edge-warping graphite mesas(EWGM). Through this approach, robust SSL performance is realized, demonstrated by sliding an 8 μm side length square EWGM on an atomically smooth Au substrate for 10000 cycles at a constant voltage of 1 m V. In this SSL system,differential friction coefficients lower than 1.5 × 10^(-4) are achieved, with static contact resistance between EWGM and Au substrate as low as 28Ω and sliding contact resistance as low as 32Ω. Moreover, the EWGM exhibits SSL behavior on polished Si wafer substrates. Furthermore, because of the no-edge contact with the substrate during sliding, friction is independent of the sliding speed of the EWGM. This study presents the first successful fabrication of conductive EWGM. Remarkably, in both EWGM-Au and EWGM-Si SSL systems, the measured frictions are more than one order of magnitude lower than those of ordinary self-retracting graphite mesas with no-edge warping, and no wear is observed during extended current-carrying ***, these findings establish a solid groundwork for the future realization of macroscale conductive SSL systems.

关键词： structural superlubricity graphite mesa contact resistance tensile stress edge warping

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Heptagonal intramolecular-lock strategy enables high-performance thermally activated delayed fluorescence emitters

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Science China Chemistry 2024年第4期67卷 1181-1186页

作者： Zhenmei Huang Dezhi Yang Dongge ma Zhengyang Bin Jingsong You Key Laboratory of Green Chemistry and Technology of Ministry of Education College of ChemistrySichuan UniversityChengdu 610064China Institute of Polymer Optoelectronic materials and Devices State Key Laboratory of Luminescent Materials and DevicesSouth China University of TechnologyGuangzhou 510640China

The development of highly efficient thermally activated delayed fluorescence(TADF)emitters is persistently pursued for the application of organic light-emitting diodes(OLED)in full-colour display and solid-state ***,we present a heptagonal intramolecular-lock strategy to design high-performance TADF *** a proof-of-concept,a new type of tribenzotropone(TBP)acceptor has been designed and synthesized by a cascade decarboxylative cyclization of aryl oxoacetic acid derivative with biphenyl boronic *** with the unlocked benzophenone(BP)acceptor,the TBP acceptor has a highly twisted heptagonal geometry with moderate rigidity and flexibility,which enables a high-performance TADF emitter with a small single-triplet energy gap(ΔE_(ST))of 0.04 e V,a high photoluminescence quantum yield(Φ_(PL))of 99% and a large horizontal orientation factor(Θ_(//))of 84.0%.Consequently,highly efficient OLEDs with an external quantum efficiency as high as 33.8% are assembled,which is significantly higher than those of DPAC-BP with a highly rotatable BP acceptor(23.8%)as well as DPACFO with a rigid fluorenone(FO)acceptor(6.9%).

关键词： organic light-emitting diodes medium-ring intramolecular-lock thermally activated delayed fluorescence molecular orientation

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