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Interfacial Zn2+-solvation regulator towards reversible and stable Zn anode

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journal of Energy Chemistry 2025年第1期100卷 684-692页

作者： miao Zhou Xiongbin Luo Hang Li Shan Guo Zhuang tong Xiaotao Zhou Xu Li Zhaohui Hou Shuquan Liang Guozhao Fang College of mechanical Engineering Key Laboratory of Hunan Province for Advanced Carbon-based Functional Materials Hunan Institute of Science and Technology School of materials Science and Engineering Key Laboratory of Electronic Packaging and Advanced Functional Materials of Hunan Province Central South University College of materials and metallurgy Guizhou University National Energy metal Resources and New materials Key Laboratory Central South University

Aqueous zinc-ion batteries （AZIBs） are fundamentally challenged by the instability of the electrode/electrolyte interface,predominantly due to irreversible zinc （Zn） deposition and hydrogen ***,the intricate mechanisms behind the electrochemical discrepancies induced by interfacial Zn2+-solvation and deposition behavior demand comprehensive *** molecules endowed with special functional groups （such as hydroxyl,carboxyl,etc.） have the potential to significantly optimize the solvation structure of Zn2+and regulate the interfacial electric double layer （EDL）.By increasing nucleation overpotential and decreasing interfacial free energy,these functional groups facilitate a lower critical nucleation radius,thereby forming an asymptotic nucleation model to promote uniform Zn ***,this study presents a pioneering approach by introducing trace amounts of n-butanol as solvation regulators to engineer the homogenized Zn （H-Zn） anode with a uniform and dense *** interfacial reaction and structure evolution are explored by in/ex-situ experimental techniques,indicating that the H-Zn anode exhibits dendrite-free growth,no by-products,and weak hydrogen evolution,in sharp contrast to the bare ***,the H-Zn anode achieves a remarkable Zn utilization rate of approximately 20% and simultaneously sustains a prolonged cycle life exceeding 500 ***,the H-Zn//NH4V4O10（NVO） full battery showcases exceptional cycle stability,retaining 95.04%capacity retention after 400 cycles at a large current density of 5 A *** study enlightens solvation-regulated additives to develop Zn anode with superior utilization efficiency and extended operational lifespan.

关键词： Aqueous zinc-ion batteries Interfacial reaction Asymptotic nucleation model Reversible and stable Zn anode

Exosomes originating from neural stem cells undergoing necroptosis participate in cellular communication by inducing TSC2 upregulation of recipient cells following spinal cord injury

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Neural Regeneration Research 2025年第11期20卷 3273-3286页

作者： Shiming Li jianfeng Li Guoliang Chen Tao Lin Penghui Zhang Kuileung tong Ningning Chen Shaoyu Liu Shenzhen Key Laboratory of Bone Tissue Repair and Translational Research Department of Orthopedic SurgeryThe Seventh Affiliated HospitalSun Yat-sen UniversityShenzhenGuangdong ProvinceChina Department of Orthopedic Surgery The First Affiliated Hospital of Jinan UniversityGuangzhouGuangdong ProvinceChina Department of Orthopedics and Traumatology Zhujiang HospitalSouthern Medical UniversityGuangzhouGuangdong ProvinceChina Department of Orthopedic Surgery The Third Affiliated Hospital of Sun Yat-sen UniversityGuangzhouGuangdong ProvinceChina Department of Orthopedic Surgery The First Affiliated Hospital of Sun Yat-sen UniversityGuangzhouGuangdong ProvinceChina

We previously demonstrated that inhibiting neural stem cells necroptosis enhances functional recovery after spinal cord *** exosomes are recognized as playing a pivotal role in neural stem cells exocrine function,their precise function in spinal cord injury remains *** investigate the role of exosomes generated following neural stem cells necroptosis after spinal cord injury,we conducted singlecell RNA sequencing and validated that neural stem cells originate from ependymal cells and undergo necroptosis in response to spinal cord ***,we established an in vitro necroptosis model using neural stem cells isolated from embryonic mice aged 16-17 days and extracted *** results showed that necroptosis did not significantly impact the fundamental characteristics or number of *** sequencing of exosomes in necroptosis group identified 108 differentially expressed messenger RNAs,104 long non-coding RNAs,720 circular RNAs,and 14 microRNAs compared with the control *** of a competing endogenous RNA network identified the following hub genes:tuberous sclerosis 2(Tsc2),solute carrier family 16 member 3(Slc16a3),and forkhead box protein P1(Foxp1).Notably,a significant elevation in TSC2 expression was observed in spinal cord tissues following spinal cord ***2-positive cells were localized around SRY-box transcription factor 2-positive cells within the injury ***,in vitro analysis revealed increased TSC2 expression in exosomal receptor cells compared with other *** assessment of cellular communication following spinal cord injury showed that Tsc2 was involved in ependymal cellular communication at 1 and 3 days post-injury through the epidermal growth factor and midkine signaling *** addition,Slc16a3 participated in cellular communication in ependymal cells at 7 days post-injury via the vascular endothelial growth factor and macrophage migration inhibitory factor signaling

关键词： cellular communication competing endogenous RNA exosomes Foxp1 necroptosis neural stem cells Slc16a3 spinal cord injury transcriptome sequencing Tsc2

Study on the hydrogen absorption properties of a YGdTbDyHo rare-earth high-entropy alloy

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International journal of minerals,metallurgy and materials 2025年第1期32卷 127-135页

作者： tongyue Li Ziliang Xie Wenjiao Zhou Huan tong Dawen Yang Anjia Zhang Yuan Wu Xiping Song State Key Laboratory for Advanced metals and materials University of Science and Technology BeijingBeijing 100083China Whole Win(Beijing)materials Sci.&Tech.Co. Ltd.Beijing 100083China

This study investigated the microstructure and hydrogen absorption properties of a rare-earth high-entropy alloy(HEA),*** indicated that the YGdTbDyHo alloy had a microstructure of equiaxed grains,with the alloy elements distributed *** hydrogen absorption,the phase structure of the HEA changed from a solid solution with an hexagonal-close-packed(HCP)structure to a high-entropy hydride with an faced-centered-cubic(FCC)structure without any secondary phase *** alloy demonstrated a maximum hydrogen storage capacity of 2.33 H/m(hydrogen atom/metal atom)at 723 K,with an enthalpy change(ΔH)of-141.09 kj·mol^(-1)and an entropy change(ΔS)of-119.14 j·mol^(-1)·K^(-1).The kinetic mechanism of hydrogen absorption was hydride nucleation and growth,with an apparent activation energy(E_(a))of 20.90 kj·mol^(-1).Without any activation,the YGdTbDyHo alloy could absorb hydrogen quickly(180 s at 923 K)with nearly no incubation period *** reason for the obtained value of 2.33 H/m was that the hydrogen atoms occupied both tetrahedral and octahedral *** results demonstrate the potential application of HEAs as a high-capacity hydrogen storage material with a large H/m ratio,which can be used in the deuterium storage field.

关键词： rare-earth high-entropy alloy hydrogen absorption capacity pressure–composition–temperature curves kinetics

基于UFAC应力吸收层的抗反射裂缝性能评价

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河南理工大学学报（自然科学版） 2025年第1期44卷 185-192页

作者：李智童竞华南理工大学土木与交通学院广东广州510641

目的为了解决“白加黑”技术中的反射裂缝问题,针对目前常用的悬浮密实型高弹改性沥青混合料(super flexible asphalt concrete,SFAC)应力吸收层变形量较大、容易造成上部沥青加铺层不利于受力的缺陷,方法提出基于CAVF法和富沥青理念优... 详细信息

目的为了解决“白加黑”技术中的反射裂缝问题,针对目前常用的悬浮密实型高弹改性沥青混合料(super flexible asphalt concrete,SFAC)应力吸收层变形量较大、容易造成上部沥青加铺层不利于受力的缺陷,方法提出基于CAVF法和富沥青理念优化设计的骨架密实型UFAC应力吸收层。采用有限元ABAQUS数值模拟方法对“白加黑”路面结构进行受力分析,并通过加速加载试验、冲击韧性试验和劈裂试验对材料与结构的抗反射裂缝性能进行评价。结果重载条件下,UFAC应力吸收层和高弹改性沥青应力吸收层的竖向位移相差5.93×10^(-2)mm,沥青加铺层底部所受竖向压应力σy、最大主应力σ_(max)、最大剪应力τ_(12)分别降低24%,32.3%,27.7%。当路面存在严重脱空或常规脱空情况时,基于UFAC应力吸收层的路面结构比GAC加铺路面结构的抗疲劳开裂性能分别提升48%,36%。与传统的悬浮型砂粒式AC-5应力吸收层相比,UFAC-5应力吸收层的冲击韧性增加60.8%,劈裂抗拉强度提高16.8%。结论基于UFAC应力吸收层的沥青加铺技术,通过增大常规改性沥青膜厚保证必要的疲劳抗拉能力,并采用骨架密实型级配显著提高集料间的嵌挤能力和内摩阻力,减小层间结构变形,可有效减缓沥青加铺层反射裂缝的产生与发展。

关键词：应力吸收层薄层富沥青混合料骨架密实型有限元数值模型抗压变形

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基于剩余碰撞时间的线控制动分层控制策略

江苏大学学报（自然科学版） 2025年第1期46卷 28-35,63页

作者：童叙王宇宁关艺博田韶鹏吴桐武汉理工大学现代汽车零部件技术湖北省重点实验室湖北武汉430070 武汉理工大学汽车零部件技术湖北省协同创新中心湖北武汉430070 武汉理工大学湖北省新能源与智能网联车工程技术研究中心湖北武汉430070 武汉理工大学佛山仙湖实验室广东佛山528200

针对不同制动工况需求的制动策略存在差异的情况,提出一种线控制动分层控制策略.在该分层策略的上层,利用二阶TTC安全碰撞时间模型计算出车辆与前车的剩余碰撞时间,以此作为依据进行制动策略的选取,并建立了汽车二自由度模型、车身法向... 详细信息

针对不同制动工况需求的制动策略存在差异的情况,提出一种线控制动分层控制策略.在该分层策略的上层,利用二阶TTC安全碰撞时间模型计算出车辆与前车的剩余碰撞时间,以此作为依据进行制动策略的选取,并建立了汽车二自由度模型、车身法向受力模型和Burckhardt轮胎模型;在该分层策略的下层,进行了制动力在轮间的分配,使用序列二次规划(SQP)方法,分别在一般制动、紧急制动、失稳制动3种工况下,以轮胎滑移率为对象建立优化函数,对车辆制动力进行了优化分配.使用mATLAB/Simulink和Carsim进行了联合仿真,对所提出3种工况下的制动分配策略进行了有效性验证.结果表明:在一般制动工况下,采用该策略时相比对照工况制动距离减少18.08%,制动时间减少25.12%;在紧急制动工况下,采用该策略时相比对照工况制动距离减少19.17%,制动时间减少12.79%;在失稳制动工况下,该策略可通过轮胎差扭来提升车辆的横向稳定性.采用文中制动策略显著提升了车辆的制动效能.

关键词：线控制动制动力优化分配分层控制序列二次规划方法 ECE法规制动仿真滑模控制碰撞时间

FIBONACCI SEQUENCE AND CANTOR'S TERNARY SET

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Chinese Annals of mathematics,Series B 1998年第1期19卷 129-132页

作者： tong jINGCHENG SAmONS ,j. Univ N Florida Dept Math & Stat Jacksonville FL 32224 USA

Let N be the set of positive integers and C be Cantor's ternary set. A function xi : N --> [0, 1] is established by the help of the Fibonacci sequence such that , the closure of the set xi(N), is homeomorphic to the s... 详细信息

关键词： Fibonacci sequence Cantor′s ternary set Homeomorphic

Ferroelectric Properties and Applications of Hybrid Organic-Inorganic Perovskites

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journal of Electronic Science and Technology 2017年第4期15卷 326-332页

作者： Xin tong Zhiming m. Wang Institute of Fundamental and Frontier Sciences University of Electronic Science and Technology of China Chengdu 610054 Institut National de la Recherche Scientifique Université du Québec Quebec G1K9H7 Canada Institute of Fundamental and Frontier Sciences University of Electronic Science and Technology of China Chengdu 610054

Hybrid organic-inorganic perovskites （e.g. CH;NH;PbI;） have attracted tremendous attention due to their promise for achieving next-generation cost-effective and high performance optoelectronic *** hybrid organic-inorganic perovskites possess excellent optical and electronic properties, including strong light absorption, high carrier abilities, optimized charge diffusion lengths, and reduced charge recombination etc., leading to their widespread applications in advanced solar energy technologies （*** efficiency perovskite solar cells）. However, there is still a lack of investigations regarding fundamental properties such as ferroelectricity in these *** conventional ferroelectric ceramics are prepared at high temperature and have no mechanically flexibility,low-temperature proceed and flexible perovskite ferroelectrics have become promising candidates and should be exploited for future flexible ferroelectric applications. Here, ferroelectric properties in hybrid organic-inorganic perovskites and several state-of-the-art perovskite ferroelectrics are reviewed. Novel ferroelectric applications of hybrid organic-inorganic perovskites are discussed as well, providing guideline for realizing future high performance and flexible ferroelectric devices.

关键词： Ferroelectricity ferroelectric materials flexible devices organic-inorganic perovskites

Unintended nutrient imbalance induced by wastewater effluent inputs to receiving water and its ecological consequences

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Frontiers of Environmental Science & Engineering 2022年第11期16卷 273-275页

作者： Yindong tong Xuejun Wang james j.Elser School of Environmental Science and Engineering Tianjin UniversityTianjin 300072China College of Urban and Environmental Sciences Peking UniversityBeijing 100871China Flathead Lake Biological Station University of MontanaPolsonMT 59860USA

Eutrophication is the most widespread water quality issue *** date,most efforts to control eutrophication have focused on reductions of external nutrient inputs,yet importance of nutrient stoichiometry and subsequent shift in plankton composition in aquatic ecosystem has been largely *** address eutrophication,improved sanitation is one of the United Nations Sustainable Development Goals,spurring the constructions of wastewater treatment facilities that have improved water quality in many lakes and ***,control measures are often targeted at and effective in removing a single nutrient from sewage and thus are less effective in removing the others,resulting in the changes of nutrient *** general,more effective phosphorus removal relative to nitrogen has occurred in wastewater treatment leading to substantial increases in N/P ratios in effluent relative to the ***,high N/P ratios in receiving waters can impose negative influences on ***,longterm strategies for domestic wastewater management should not merely focus on the total reduction of nutrient discharge but also consider their stoichiometric balances in receiving waters.

关键词： Nutrient stoichiometry Wastewater treatment Ecosystem functioning Water quality management

Size and temperature effects on dielectric breakdown of ferroelectric films

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journal of Advanced Ceramics 2021年第1期10卷 181-186页

作者： Sheng tong DePaul University 1 E.Jackson Blvd.ChicagoIL 60604USA

The paper introduces a model of dielectric breakdown *** model integrated thermal breakdown and defect models,representing the relationship between the electric field of ferroelectric films and dimensional parameters and operating *** model is verified with experimental results of the lead lanthanum zirconate titanate(PLZT)films of various film thickness(j=0.8-3μm),electrode area(A=0.0020-25 mm^(2))tested under a range of operating temperature(T=300-400 K)with satisfying fitting *** learned is a relationship that the recoverable electric energy density is directly proportional to the square of breakdown electric *** relationship is found viable in predicting the electric energy density in terms of variables of d,A,and T for the PLZT films.

关键词： film thickness electrode size ceramics energy storage