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Gradient‑Layered MXene/Hollow Lignin Nanospheres Architecture Design for Flexible and Stretchable Supercapacitors

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Nano-Micro Letters 2025年第2期17卷 447-462页

作者： Haonan Zhang cheng Hao Tongtong Fu Dian Yu Jane Howe Kaiwen Chen ning Yan Hao Ren Huamin Zhai Jiangsu Provincial Key Lab of Sustainable Pulp and Paper Technology and Biomass Materials NanJing Forestry UniversityNanjing 210037People’s Republic of China Department of Chemical Engineering and Applied Chemistry University of Toronto200 College StreetTorontoON M5S 3E5Canada Department of Materials Science and Engineering University of Toronto184 College StreetTorontoON M5S 3E4Canada College of Materials Science and Engineering Nanjing Forestry UniversityNanjing 210037People’s Republic of China

With the rapid development of flexible wearable electronics,the demand for stretchable energy storage devices has *** this work,a novel gradient-layered architecture was design based on single-pore hollow lignin nanospheres(HLNPs)-intercalated two-dimensional transition metal carbide(Ti_(3)C_(2)T_(x) MXene)for fabricating highly stretchable and durable *** depositing and inserting HLNPs in the MXene layers with a bottom-up decreasing gradient,a multilayered porous MXene structure with smooth ion channels was constructed by reducing the overstacking of MXene ***,the micro-chamber architecture of thin-walled lignin nanospheres effectively extended the contact area between lignin and MXene to improve ion and electron accessibility,thus better utilizing the pseudocapacitive property of *** these strategies effectively enhanced the capacitive performance of the *** addition,HLNPs,which acted as a protective phase for MXene layer,enhanced mechanical properties of the wrinkled stretchable electrodes by releasing stress through slip and deformation during the stretch-release cycling and greatly improved the structural integrity and capacitive stability of the *** electrodes and symmetric flexible all-solid-state supercapacitors capable of enduring 600%uniaxial tensile strain were developed with high specific capacitances of 1273 mF cm^(−2)(241 F g^(−1))and 514 mF cm^(−2)(95 F g^(−1)),***,their capacitances were well preserved after 1000 times of 600%stretch-release *** study showcased new possibilities of incorporating biobased lignin nanospheres in energy storage devices to fabricate stretchable devices leveraging synergies among various two-dimensional nanomaterials.

关键词： Hollow lignin nanospheres MXene Gradient-layered architecture Wrinkled electrodes Stretchable supercapacitors

An Unprecedented Efficiency with Approaching 21%Enabled by Additive‑Assisted Layer‑by‑Layer Processing in Organic Solar Cells

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Nano-Micro Letters 2025年第2期17卷 372-375页

作者： Shuai Xu Youdi Zhang Yanna Sun Pei cheng Zhaoyang Yao ning Li Long Ye Lijian Zuo Ke Gao Key Laboratory of Advanced Green Functional Materials College of ChemistryChangchun Normal UniversityChangchun 130032People’s Republic of China Shandong Provincial Key Laboratory for Science of Material Creation and Energy Conversion School of Chemistry and Chemical EngineeringShandong UniversityQingdao 266237People’s Republic of China College of Polymer Science and Engineering Sichuan UniversityChengdu 610065People’s Republic of China State Key Laboratory and Institute of Elemento‑Organic Chemistry Centre of Nanoscale Science and Technology and Key Laboratory of Functional Polymer MaterialsRenewable Energy Conversion and Storage Center(RECAST)College of ChemistryNankai UniversityTianjin 300071People’s Republic of China Institute of Polymer Optoelectronic Materials and Devices State Key Laboratory of Luminescent Materials and Devices South China University of TechnologyGuangzhou 510640People’s Republic of China Tianjin Key Laboratory of Molecular Optoelectronic Sciences School of Materials Science and EngineeringTianjin UniversityTianjin 300350People’s Republic of China State Key Laboratory of Silicon Materials MOE Key Laboratory of Macromolecular Synthesis and FunctionalizationDepartment of Polymer Science and EngineeringZhejiang UniversityHangzhou 310027People’s Republic of China

Recently published in Joule,Feng Liu and colleagues from Shanghai Jiaotong University reported a record-breaking 20.8%power conversion efficiency in organic solar cells(OSCs)with an interpenetrating fibril network active layer morphology,featuring a bulk p-in structure and proper vertical segregation achieved through additive-assisted layer-by-layer *** optimized hierarchical gradient fibrillar morphology and optical management synergistically facilitates exciton diffusion,reduces recombination losses,and enhances light capture *** approach not only offers a solution to achieving high-efficiency devices but also demonstrates the potential for commercial applications of OSCs.

关键词： Organic solar cells Additive-assisted layer-by-layer processing Three-dimensional fibril morphology Bulk p-i-n structure Optical management

Controlled Radical Polymerization:from Oxygen Inhibition and Tolerance to Oxygen Initiation

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Chinese Journal of Polymer Science 2021年第9期39卷 1084-1092页

作者： ning Li Xiang-cheng Pan State Key Laboratory of Molecular Engineering of Polymers Department of Macromolecular ScienceFudan UniversityShanghai 200438China

Molecular oxygen is a radical scavenger in both conventional and controlled radical polymerization(CRP),resulting in many time-consuming methods for physically removing oxygen before the *** approaches have been developed to have oxygen toleranee by chemically consuming or converting molecular oxygen into non-initiating species to address this ***,we propose another approach called oxygen initiation that directly transforms molecular oxygen into the initiating carbon radical in *** feature article summarizes our rece nt developments in this *** n-initiated reversible additi on-fragmentation transfer(RAFT)polymerization has been successfully conducted using oxygen and trialkylborane as co-initiators under the ambient conditions and atmosphere without any prior degassed *** gas-triggered initiation provides the opportunity for spatiotemporal control of the polymerization by molecular oxygen or *** synthesized alkylborane compounds could derive the predesigned structure of the initiating alkyl radical to minimize the side reacti ons and free polymer chai ns,achievi ng the synthesis of ultra-high molecular weight *** challe nges and perspectives are also discussed in the end.

关键词： Oxygen Radical polymerization Controlled Alkylborane RAFT

Stereotypes About Enterotype: the Old and New Ideas

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Genomics, Proteomics & Bioinformatics 2019年第1期17卷 4-12页

作者： Mingyue cheng Kang ning Key Laboratory of Molecular Biophysics of the Ministry of Education Hubei Key Laboratory of Bioinformatics and Molecular-imaging Department of Bioinformatics and Systems Biology College of Life Science and TechnologyHuazhong University of Science and Technology

In 2011, the term ‘‘enterotype" first appeared to the general public in Nature, which refers to stratification of human gut microbiota. However, with more studies on enterotypes conducted nowadays, doubts about the existence and robustness of enterotypes have also emerged. Here we reviewed current opinions about enterotypes from both conceptual and analytical points of *** firstly illustrated the definition of the enterotype and various factors influencing enterotypes,such as diet, administration of antibiotics, and age. Then we summarized lines of evidence that pose the concept against the enterotype, and described the current methods for enterotype ***, we showed that the concept of enterotype has been extended to other ecological *** on current studies on enterotypes, it has been clear that more studies with larger sample sizes are needed to characterize the enterotypes. Improved computational methods are also required to build sophisticated models, reflecting the dynamics and resilience of enterotypes.

关键词： Enterotype Gut microbiome Biomarker Continuity Computational methods

Analysis of temperature,stress,and displacement distributions of staves for a blast furnace

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International Journal of Minerals,Metallurgy and Materials 2009年第5期16卷 512-516页

作者： Xiao-jun ning Shu-sen cheng ning-qiang Xie School of Metallurgical and Ecological Engineering University of Science and Technology Beijing Beijing 100083 China

The temperature of gas flow inside a blast furnace （BF） changes significantly when the blast furnace is under unstable operations, and the temperature and stress distributions of cooling staves （CS） for BF work the same pattern. The effect of gas temperature on the temperature, stress, and displacement distributions of the cooling stave were analyzed as the gas temperature inside the blast furnace rose from 1000 to 1600℃ in 900 s. The results show that both the temperature and temperature gradient of the hot side of CS increase when the gas flow temperature inside BF rises. The temperature gradient of the hot side of CS is greater than that of the other area of CS and it can reach 65℃/mm. In the vertical direction of the hot side of CS, closer to the central part of CS, the stress intensity is greater than that of the other area of the hot side of CS, which causes cracks on the hot side of CS in the vertical di- rection. As the gas temperature increases, the stress intensity rate near the fixed pin increases and finally reaches 45 MPa/s. Fatigues near the fixed pin and bolts are caused by great stress intensity rate and the area around the pin can be damaged easily. The edge of CS bends toward the cold side and the central part of CS shifts toward the hot surface.

关键词： blast furnace cool stave gas temperature numerical simulation

Government environmental control measures on CO_(2) emission during the 2014 Youth Olympic Games in Nanjing:Perspectives from a top-down approach

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Journal of Environmental Sciences 2022年第3期34卷 165-178页

作者： cheng Hu cheng Liu ning Hu Jun Hong Xinyue Ai College of Biology and the Environment Joint Center for sustainable Forestry in Southern ChinaNanjing Forestry UniversityNanjing 210037China Yale-NUIST Center on Atmospheric Environment International Joint Laboratory on Climate and Environment Change(ILCEC)Nanjing University of InformationScience&TechnologyNanjing 210044China Jiangxi Province Key Laboratory of the Causes and Control of Atmospheric Pollution/School of Water Resources and Environmental Engineering East China University of TechnologyNanchang 330013China National Key Laboratory on Electromagnetic Environmental Effects and Electro-Optical Engineering Army Engineering UniversityNanjing 210022China

Strict air pollution control measures were conducted during the Youth Olympic Games(YOG)period at Nanjing city and surrounding areas in August *** event provides a unique chance to evaluate the effect of government control measures on regional atmospheric pollution and greenhouse gas *** previous studies have observed significant reductions of atmospheric pollution species and improvement in air quality,while no study has quantified its synergism on anthropogenic CO_(2)emissions,which can be coreduced with air *** better understand to what extent these pollution control measures have reduced anthropogenic CO_(2)emissions,we conducted atmospheric CO_(2)measurements at the suburban site in Nanjing city from 1^(st) July to 30^(th) September 2014 and 1^(st) August to 31^(st) August 2015,obvious decrease in atmospheric CO_(2)was observed between YOG and the rest *** coupling the a prioriemission inventory with atmospheric transport model,we applied the scale factor Bayesian inversion approach to derive the posteriori CO_(2)emissions in YOG period and regular *** indicate CO_(2)emissions from power industry decreased by 45%,and other categories also decreased by 16%for manufacturing combusting,and 37%for non-metallic mineral *** total anthropogenic CO_(2)emissions were 9.8(±3.6)×10^(9) kg/month CO_(2) for regular period and decreased to 6.2(±1.9)×10^(9) kg/month during the YOG period in Nanjing city,with a 36.7%*** scaling up to whole Jiangsu Province,anthropogenic CO_(2)emissions were 7.1(±2.4)×10^(10) kg/month CO_(2)for regular period and decreased to 4.4(±1.2)×10^(10)kg/month CO_(2) during the YOG period,yielding a 38.0%reduction.

关键词： Carbon dioxide Reduction measures Anthropogenic emissions Bayesian inversion

Risk Assessment of Tsunamis Along the Chinese Coast Due to Earthquakes

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International Journal of Disaster Risk Science 2022年第2期13卷 275-290页

作者： Chun Hui Lixin ning Changxiu cheng Key Laboratory of Environmental Change and Natural Disaster Beijing Normal UniversityBeijing 100875China State Key Laboratory of Earth Surface Processes and Resource Ecology Beijing Normal UniversityBeijing 100875China Faculty of Geographical Science Beijing Normal UniversityBeijing 100875China National Tibetan Plateau Data Center Beijing 100101China

China’s coastal areas are densely populated,economically developed, and located in close proximity to several potential tsunami sources;therefore, tsunami risk cannot be ignored. This study assessed tsunami risk in coastal areas of China by developing a framework for tsunami risk assessment from the perspectives of hazards,vulnerability, and exposure. First, a probabilistic tsunami hazard assessment(PTHA) model was applied to estimate the potential tsunami sources in both local crustal faults and circum-Pacific subduction zones based on numerical simulations. The output of the PTHA includes tsunami wave height distributions along the coast. Then, an indicator system reflecting exposure and vulnerability to tsunamis in the coastal areas of China was established by using the entropy method and analytic hierarchy *** PTHA findings show that the tsunami wave height is close to 3 m on the southern coast of the Bohai Sea, the Pearl River Estuary, and the Yangtze River Delta and exceeds 2 m near the Taiwan Strait for the 2000-year return period. The results of the tsunami risk assessment show that the cities at the highest risk level(level I) include Tangshan, Yantai, and Hong Kong, while cities at the high risk level(level II) include Fuzhou, Xiamen, and Quanzhou near the Taiwan Strait and many cities on the Yangtze River Delta, the Pearl River Estuary, and the southern coast of the Bohai Sea. Our findings can provide an understanding of differences in tsunami risk between Chinese coastal cities that may be affected by tsunamis in the future.

关键词： China coast Earthquakes Probabilistic tsunami hazard assessment Tsunami exposure Tsunami risk Vulnerability

Experimental investigation of penetration performance of shaped charge into concrete targets

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Acta Mechanica Sinica 2008年第3期24卷 345-349页

作者： cheng Wang Tianbao Ma Jianguo ning State Key Laboratory of Explosion Science and Technology Beijing Institute of Technology Beijing 100081 China

In order to develop a tandem warhead that can effectively destroy concrete targets, this paper explores the penetration performance of shaped charges with different cone angles and liner materials into concrete targets by means of experiments. The penetration process and the destruction mechanism of concrete targets by shaped charges and kinetic energy projectiles are analyzed and compared. Experimental results suggest that both kinetic energetic projectile and shaped charge are capable of destroying concrete targets, but the magnitudes of damage are different. Compared with a kinetic energy projectile, a shaped charge has more significant effect of penetration into the target, and causes very large spalling area. Hence, a shaped charge is quite suitable for first-stage charge of tandem warhead. It is also found that, with the increase of shaped charge liner cone angle, the depth of penetration decreases gradually while the hole diameter becomes larger. Penetration depth with copper liner is larger than of aluminum liner but hole diameter is relatively smaller, and the shaped charge with steel liner is between the above two cases. The shaped charge with a cone angle of 100° can form a jet projectile charge （JPC）. With JPC, a hole with optimum depth and diameter on concrete targets can be formed, which guarantees that the second-stage warhead smoothly penetrates into the hole and explodes at the optimum depth to achieve the desired level of destruction in concrete targets.

关键词： Shaped charge JPC Kinetic energy projectile Concrete Penetration

Highly sensitive piezoresistive pressure sensors based on laser-induced graphene with molybdenum disulfide nanoparticles

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Science China(Technological Sciences) 2021年第11期64卷 2408-2414页

作者： HAO DaPeng YANG RuoXi YI ning cheng HuanYu School of Science Xi'an Aeronautical UniversityXi'an 710077China Department of Engineering Science and Mechanics The Pennsylvania Stale UniversityUniversity ParkState College PA 16802USA School of Mechanical Engineering Hebei University of Technology'Tianjin 300401China Department of Materials Science and Engineering The Pennsylvania State UniversityUniversity ParkState College PA 16802USA

Wearable pressure sensors have drawn significant attention because of their extensive applications in motion detection, tactile sensing, and health monitoring. However, the complex manufacturing process and high cost of active materials make low-cost,large-scale production elusive. In this work, we report a flexible piezoresistive pressure sensor assembled with two 3D laserinduced graphene(LIG) foam electrodes on a polyimide thin film from a simple laser scribing process in the ambient environment. The design of the air gap between the two foam electrodes allows the sensor to showcase a low limit of detection of 0.274 Pa, which provides favorable sensing performance in motion detection and wrist pulse monitoring. The addition of spherical MoS2 nanoparticles between the two foam electrodes further enhances the sensitivity to 88 k Pa-1 and increases the sensing range to significantly outperform the previous literature reports. The demonstrated LIG pressure sensors also exhibit fast response/recovery rates and excellent durability/repeatability.

关键词： piezoresistive pressure sensor laser-induced graphene foam molybdenum disulfide nanoparticles health monitoring