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High-entropy sulfurization enables efficient non-noble metal-based NiCoFeCuS electrocatalyst for alkaline oxygen evolution reaction

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Particuology 2024年第10期93卷 180-185页

作者： Pan yang Mengxiang Sun Jingchuan wang Jinfeng Li Ruizhu yang Yawei Hao Li Qi Lijun yang Xue liu Institute of Materials China Academy of Engineering PhysicsJiangyou621908China State Key Laboratory of Metastable Materials Science and Technology Yanshan UniversityQinhuangdao066004China Science and Technology on Surface Physics and Chemistry Laboratory Jiangyou621907China

Highly active and cost-effective oxygen evolution reaction electrocatalysts have become essential to replace commercial electrocatalysts that rely on rare noble ***-entropy sulfide nanomaterials,characterized by abundant randomly distributed elements and inherent stability,possess significant potential for ***,challenges such as uneven composition,partial oxidation,or imprecise synthesis control still remain in the materials ***,a simple and effective two-step hydrothermal method was employed to synthesize NiCoFeCuS nanoparticles supported on foam nickel *** the catalytic active sites produced by electron density redistribution in high-entropy and sulfurization,NiCoFeCuS exhibits excellent alkaline OER performance,with an overpotential of 261 mV and a Tafel slope of 57.97 mV dec^(−1) at the current density of 10 mA cm^(−2),which is only 88%of commercial RuO_(2) without any noble metals.

关键词： High-entropy Sulfurization NiCoFeCuS electrocatalyst Oxygen evolution reaction Overpotentials

Plant life form determines spatiotemporal variability and climate response of plant seed rain in subtropical forests

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Forest Ecosystems 2024年第2期11卷 193-201页

作者： Yuyang Xie Zehao Shen Xuejing wang liu yang Jie Zhang MOE Laboratory for Earth Surface Processes Institute of EcologyCollege of Urban and Environmental SciencesPeking UniversityBeijing100871China

Spatiotemporal variation of seed rain reflects the response of plants in terms of their reproductive strategy to environmental *** this study,we collected seeds from four sites in the Dalaoling Nature Reserve,Hubei Province,China,between 2011 and 2014,measured seed output and seed mass as seed rain traits,and compared their interannual and elevational ***,we ran phylogenetic generalized mixed linear models(PGLMMs) to explore the effects of temperature and precipitation as well as interspecific differences on seed rain,and fitted the best regression models for seed rain *** of canopy and understory *** results showed no correlation between values of seed output and seed ***,the variation of the two traits showed significantly positive *** output of canopy species generally decreased with increasing elevation,and showed significant interannual difference;however,seed output of understory species and seed mass for both canopy and understory species did not show consistency tends along elevational or in interannual *** output was significantly affected by temperature and precipitation,while seed mass mainly varied due to interspecific *** explained more the variation of the seed output of canopy species than that of understory species,with R^(2) values of 43.0%and 29.9%,*** results suggested that canopy plants contributed more to the reproductive dynamics of the whole communities,and the canopy's buffer effect on the underground weakened the response of understory plants to weather variation in terms of their reproductive strategy.

关键词： Seed rain Seed output Seed mass Elevation Interannual variation Lifeform

Amide as an efficient ligand in the palladium-catalyzed Suzuki coupling reaction in water/ethanol under aerobic conditions

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Chinese Chemical Letters 2011年第6期22卷 738-740页

作者： Hai yang liu Kun wang Hai Yan Fu Mao Lin Yuan Hua Chen Rui Xiang Li Key Lab of Green Chemistry and Technology Ministry of Education the Institute of Homogeneous Catalysis College of Chemistry Sichuan University Chengdu 610064 China

Amide,which is derived from proline and is inexpensive and air-stable,has been synthesized and characterized by ~1H NMR,^（13）C NMR,and *** was found to be an efficient ligand in the palladium-catalyzed Suzuki cross-coupling *** the Pd/amide catalytic system,aryl bromides can be coupled with phenylboronic acid in ethanol/water（1：2;v/v） in excellent yields even with a low Pd loading of 0.01 mol%.Moreover,the scope of the reaction is broad,and a wide variety of functional groups are tolerant.

关键词： Suzuki cross-coupling Palladium catalyst Aryl bromides Amide Water

Genome-wide association study identifies 12 new genetic loci associated with growth traits in pigs

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Journal of Integrative Agriculture 2024年第1期23卷 217-227页

作者： Mu Zeng Binhu wang Lei liu Yalan yang Zhonglin Tang Guangdong Provincial Key Laboratory of Animal Molecular Design and Precise Breeding/Key Laboratory of Animal Molecular Design and Precise Breeding of Guangdong Higher Education Institutes School of Life Science and EngineeringFoshan UniversityFoshan 528231China Kunpeng Institute of Modern Agriculture at Foshan Agricultural Genomics Institute at ShenzhenChinese Academy of Agricultural SciencesFoshan 528200China Shenzhen Branch Guangdong Laboratory of Lingnan Modern Agriculture/Key Laboratory of Livestock and Poultry Multi-omics of Ministry of Agriculture and Rural AffairsAgricultural Genomics Institute at ShenzhenChinese Academy of Agricultural SciencesShenzhen 518124China

Growth traits are among the most important economic traits in pigs and are regulated by polygenes with complex regulatory *** the major indicators of growth performance,the backfat thickness(BFT),loin eye area(LEA),and days to 100 kg(D100)traits are commonly used to the genetics improvement in ***,the available genetic markers for these traits are *** uncover novel loci and candidate genes associated with growth performance,we collected the phenotypic information of BFT,LEA,and D100 in 1,186 pigs and genotyped all these individuals using the Neogen GGP porcine 80K *** performed a genome-wide association study(GWAS)using 4 statistical models,including mixed linear models(MLM),fixed and random model circulating probability unification(FarmCPU),settlement of MLM under progressively exclusive relationships(SUPER),Bayesian-information and linkage-disequilibrium Iteratively nested keyway(Blink),and identified 5,3,and 6 high-confidence single nucleotide polymorphisms(SNPs)associated with BFT,LEA,and D100,*** annotation and quantitative trait locus(QTL)mapping analysis suggested that6 genes(SKAP2,SATB1,PDE7B,PPP1R16B,WNT3,and WNT9B)were potentially associated with growth performance in *** analysis suggested that the expression of Src Kinase Associated Phosphoprotein 2(SKAP2)was higher in prenatal muscles than in postnatal muscles,and the expression of Phosphodiesterase 7B(PDE7B)continuously increased during the prenatal stages and gradually decreased after birth,implying their potential roles in prenatal skeletal muscle ***,this study provides new candidate loci and genes for the genetic improvement of pigs.

关键词： GWAS pig growth trait QTL mapping skeletal muscle

Flow characteristics of radial inflow in impeller rear cavity with baffle plate

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Chinese Journal of Aeronautics 2024年第2期37卷 270-282页

作者： yang BAI Xiang LUO Dongdong liu Zeyu WU Xiaoqiang ZHANG Sipeng wang Research Institute of Aero-Engine Beihang UniversityBeijing 100191China National Key Laboratory of Science and Technology on Aero-Engine Aero-Thermodynamics Beihang UniversityBeijing 100191China School of Energy and Power Engineering Beihang UniversityBeijing 100191China

The research purpose of this paper is to explore the influence of the baffle plate on the airflow in the rear cavity of the centrifugal impeller and optimize the performance of the secondary air system’s air bleed *** this paper,a comprehensive experimental study was carried out on the flow characteristics in the impeller rear cavity with baffle *** windage torque,flow structure and pressure drop between inlet and outlet were measured *** experiment was carried out with the condition that the range of rotational Reynolds number was from 8.33×10^(5)to 22.2×10^(5)and the range of mass flow rate coefficient was from 0.92×10^(4)to 2.92×10^(4).The results show that the static cavity and the narrow stator-rotor cavity formed by the baffle plate effectively suppress the overall swirl coefficient in the ***,the static pressure and total pressure drop in the rotor-stator cavity were *** influence of the baffle plate on the windage torque of the rotary disk is related to the turbulence *** large turbulence parameters,the windage torque would be reduced with baffle plate,while under small turbulence parameters,the baffle plate would increase with baffle *** general,the baffle plate can improve the flow capacity and optimize the bleed air performance with proper structure and operation conditions.

关键词： Impeller rear cavity Baffle plate Flow structure Windage torque Pressure drop

Effects of dynamical spanwise retraction and stretch on flapping-wing forward flights

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Chinese Journal of Aeronautics 2024年第4期37卷 181-202页

作者： Kang liu Bifeng SONG Ang CHEN Zhihe wang Dong XUE Wenqing yang School of Aeronautics Northwestern Polytechnical UniversityXi’an 710072China Intelligent Aircraft Research Center Chengdu Technological UniversityChengdu 610031China Research&Development Institute of Northwestern Polytechnical University in Shenzhen Shenzhen 518057China Harbin Institute of Technology Shenzhen 518055China

Birds and bats retract and stretch their wings dynamically during each flap in level flights, implying intriguing mechanisms for the aerodynamic performance improvement of flapping wings. A numerical investigation into the aerodynamic effects of such bio-inspired concept in forward flights has been performed based on a three-dimensional wing in plunging motion and a twosection wing in flapping motion. The currently considered Reynolds number and Strouhal number are Re=1.5×10^(5) and St=0.3, respectively. During the research, the mean angle of attack is varied in relatively wide ranges to achieve lift-thrust interconversion for the wings. The conclusive results show that dynamical spanwise retraction and stretch has induced three absolutely desirable scenarios for the oscillating wings in forward flights, namely producing more lift and consuming less power for a given thrust generation, producing more thrust and consuming less power for a given lift generation, and producing more lift and more thrust while consuming less power. Furthermore,the morphing wings have alleviated periodical aerodynamic load fluctuations compared with the non-morphing baseline. The mechanism of the aerodynamic effects of the bionic morphing mode is analyzed with the aid of field visualization. The current article is the first to reveal the absolute advantages of the bionic spanwise morphing. Hopefully, it may help comprehend the behaviors of natural fliers and provide inspirations for performance enhancement of micro artificial flappingwing vehicles.

关键词： Flapping wing Morphing wing Bionic Aerodynamics Vortex Flight

Multisensory Conflict Impairs Cortico-Muscular Network Connectivity and Postural Stability: Insights from Partial Directed Coherence Analysis

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Neuroscience Bulletin 2024年第1期40卷 79-89页

作者： Guozheng wang Yi yang Kangli Dong Anke Hua Jian wang Jun liu Key Laboratory for Biomedical Engineering of Ministry of Education College of Biomedical Engineering&Instrument ScienceZhejiang UniversityHangzhou 310058China Taizhou Key Laboratory of Medical Devices and Advanced Materials Research Institute of Zhejiang University-TaizhouTaizhou 318000China Department of Sports Science College of EducationZhejiang UniversityHangzhou 310058China Center for Psychological Science Zhejiang UniversityHangzhou 310058China

Sensory conflict impacts postural control,yet its effect on cortico-muscular interaction remains *** aimed to investigate sensory conflict's influence on the cortico-muscular network and postural *** used a rotating platform and virtual reality to present subjects with congruent and incongruent sensory input,recorded EEG(electroencephalogram)and EMG(electromyogram)data,and constructed a directed connectivity *** results suggest that,compared to sensory congruence,during sensory conflict:(1)connectivity among the sensorimotor,visual,and posterior parietal cortex generally decreases,(2)cortical control over the muscles is weakened,(3)feedback from muscles to the cortex is strengthened,and(4)the range of body sway increases and its complexity *** results underline the intricate effects of sensory conflict on cortico-muscular *** the sensory conflict,the brain adaptively decreases the integration of conflicting *** this integrated information,cortical control over muscles may be lessened,whereas the muscle feedback may be enhanced in compensation.

关键词： Cortico-muscular interaction Postural control Virtual reality Electroencephalogram Electromyography Sensory integration

CRBFT:A Byzantine Fault-Tolerant Consensus Protocol Based on Collaborative Filtering Recommendation for Blockchains

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Computers, Materials & Continua 2024年第7期80卷 1491-1519页

作者： Xiangyu Wu Xuehui Du Qiantao yang Aodi liu Na wang Wenjuan wang He’nan Province Key Laboratory of Information Security Information Engineering UniversityZhengzhou450000China School of Cyber Science Engineering Zhengzhou UniversityZhengzhou450000China

Blockchain has been widely used in finance,the Internet of Things(IoT),supply chains,and other scenarios as a revolutionary *** protocol plays a vital role in blockchain,which helps all participants to maintain the storage state ***,with the improvement of network environment complexity and system scale,blockchain development is limited by the performance,security,and scalability of the consensus *** address this problem,this paper introduces the collaborative filtering mechanism commonly used in the recommendation system into the Practical Byzantine Fault Tolerance(PBFT)and proposes a Byzantine fault-tolerant(BFT)consensus protocol based on collaborative filtering recommendation(CRBFT).Specifically,an improved collaborative filtering recommendation method is designed to use the similarity between a node’s recommendation opinions and those of the recommender as a basis for determining whether to adopt the recommendation *** can amplify the recommendation voice of good nodes,weaken the impact of cunningmalicious nodes on the trust value calculation,andmake the calculated resultsmore *** addition,the nodes are given voting power according to their trust value,and a weight randomelection algorithm is designed and implemented to reduce the risk of *** experimental results show that CRBFT can effectively eliminate various malicious nodes and improve the performance of blockchain systems in complex network environments,and the feasibility of CRBFT is also proven by theoretical analysis.

关键词： Blockchain consensus byzantine fault-tolerant collaborative filtering trust

Seismic effectiveness evaluation and optimized design of tie up method for securing museum collections

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Earthquake Engineering and Engineering Vibration 2024年第3期23卷 741-763页

作者： wang Meng Yan Yi yang Weiguo liu Pei Ge Jiaqi Ma Botao School of Civil Engineering Beijing Jiaotong UniversityBeijing 100044China Beijing’s Key Laboratory of Structural Wind Engineering and Urban Wind Environment Beijing 100044China Beijing General Municipal Engineering Design&Research Institute Co. LtdBeijing 100082China China Aviation Planning and Design Institute(Group)Co.Ltd. Beijing 100120China

To quantify the seismic effectiveness of the most commonly used fishing line tie up method for securing museum collections and optimize fixed strategies for exhibitions,shaking table tests of the seismic systems used for typical museum collection replicas have been carried *** influence of body shape and fixed measure parameters on the seismic responses of replicas and the interaction behavior between replicas and fixed measures have been *** on the results,seismic effectiveness evaluation indexes of the tie up method are *** suggestions for fixed strategies are given,which provide a basis for the exhibition of delicate museum collections considering the principle of minimizing seismic responses and *** analysis results show that a larger ratio of height of mass center to bottom diameter led to more intense rocking *** the initial pretension of fishing lines was conducive to reducing the seismic responses and stress variation of the *** comprehensive consideration of the interaction forces and effective securement,it is recommended to apply 20%of breaking stress as the initial *** specific museum collections that cannot be effectively protected by the independent tie up method,an optimized strategy of a combination of fishing lines and fasteners is recommended.

关键词： tie up method museum collections shaking table test seismic effectiveness optimized design