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Optimized the vanadium electrolyte with sulfate-phosphoric mixed acids to enhance the stable operation at high-temperature

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Frontiers of Chemical Science and Engineering 2024年第2期18卷 13-26页

作者： Ling Ge Tao liu {1. Zhang Hong liu School of Resource and Environmental Engineering Wuhan University of Science and TechnologyWuhan 430081China State Environmental Protection Key Laboratory of Mineral Metallurgical Resources Utilization and Pollution Control Wuhan University of Science and TechnologyWuhan 430081China Hubei Collaborative Innovation Center for High Efficient Utilization of Vanadium Resources Wuhan University of Science and TechnologyWuhan 430081China Hubei Provincial Engineering Technology Research Center of High Efficient Cleaning Utilization for Shale Vanadium Resource Wuhan University of Science and TechnologyWuhan 430081China School of Resource and Environmental Engineering Wuhan University of TechnologyWuhan 430070China

Herein, the influence of the concentration design and comprehensive performance of the sulfate-phosphoric mixed acid system electrolyte is investigated to realize an electrolyte that maintains high energy density and stable operation at high temperatures. Static stability tests have shown that VOPO4 precipitation occurs only with vanadium(V) electrolyte. The concentration of vanadium ion of 2.0–2.2.mol·L^(–1., phosphoric acid of 0.1.–0.1. mol·L^(–1., and sulfuric acid of 2.5–3.0 mol·L^(–1. are suitable for a vanadium redox flow battery in the temperature range from –2. to 50 ℃. The equations for predicting the viscosity and conductivity of electrolytes are obtained by the response surface method. The optimized electrolyte overcomes precipitation generation. It has 2.8 times higher energy density than the non-phosphate electrolyte, and a coulomb efficiency of 94.0% at 50 ℃. The sulfate-phosphoric mixed acid system electrolyte promotes the electrode reaction process, increases the current density, and reduces the resistance. This work systematically optimizes the concentrations of composition of positive and negative vanadium electrolytes with mixed sulfate-phosphoric acid. It provides a basis for the different valence states and comprehensive properties of sulfate-phosphoric mixed acid system vanadium electrolytes under extreme environments, guiding engineering applications.

关键词： all vanadium redox flow battery mixed-acid vanadium electrolyte concentration optimization response surface methodology high-temperature stability

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Logit prototype learning with active multimodal representation for robust open-set recognition

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Science china(Information Sciences) 2024年第6期67卷 297-312页

作者： yimin FU Zhunga {1. Zicheng WANG School of Automation Northwestern Polytechnical University

Robust open-set recognition(OSR) performance has become a prerequisite for pattern recognition systems in real-world applications. However, the existing OSR methods are primarily implemented on the basis of single-modal perception, and their performance is limited when single-modal data fail to provide sufficient descriptions of the objects. Although multimodal data can provide more comprehensive information than single-modal data, the learning of decision boundaries can be affected by the feature representation gap between different modalities. To effectively integrate multimodal data for robust OSR performance, we propose logit prototype learning(LPL) with active multimodal representation. In LPL, the input multimodal data are transformed into the logit space, enabling a direct exploration of intermodal correlations without the impact of scale inconsistency. Then, the fusion weights of each modality are determined using an entropybased uncertainty estimation method. This approach realizes adaptive adjustment of the fusion strategy to provide comprehensive descriptions in the presence of external disturbances. Moreover, the single-modal and multimodal representations are jointly optimized interactively to learn discriminative decision ***, a stepwise recognition rule is employed to reduce the misclassification risk and facilitate the distinction between known and unknown classes. Extensive experiments on three multimodal datasets have been done to demonstrate the effectiveness of the proposed method.

关键词： logit prototype learning multimodal perception open-set recognition uncertainty estimation

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Effect of an impurity on 3-electron quantum dots in magnetic fields

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Science china(Physics,Mechanics & Astronomy) 2004年第5期47卷 521-530页

作者： liu yimin1,2. HUANG Gangming1.& BAO Chengguang1.1. Department of Physics, Zhongshan {1., guangzhou 5102.5, china 2. Department of Physics, Shaoguan {1., Shaoguan 51.005, china Department of Physics Zhongshan University Guangzhou China Department of Physics Shaoguan University Shaoguan China

The ground-state property of a 2.dimensional 3-electron quantum dot (QD) subjected to an external magnetic fieldB and affected by an impurity is studied. The impurity is located at thez-axis by a distanced from the plane of the dot. The evolution of the angular momentumL o and the spinS o of the ground state in accordance withB andd has been calculated, and the results are summarized and plotted in a (L o,S o) diagram. The spatial distribution of the electrons (the size and the geometric features) and the optical absorption have also been investigated. The (L o S o) diagram indicates thatL o andS o may jump whend and/orB vary. It was found that, due to the constraints arising from symmetry, each symmetric geometry is accessible only to a specific group of states having specificL o andS o.

关键词： quantum dot, ground state, charged impurity, magnetic field.

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Circulation Background and Genesis Mechanism of a Cold Vortex over the Tibetan Plateau during Late April 2.1.

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Advances in Atmospheric Sciences 2024年第6期41卷 1201-1216页

作者： Duming GAO Jiangyu MAO Guoxiong WU yimin {1. State Key Laboratory of Numerical Modeling for Atmospheric Sciences and Geophysical Fluid Dynamics(LASG) Institute of Atmospheric PhysicsChinese Academy of SciencesBeijing 100029China university of Chinese Academy of Sciences Beijing 100049China Heavy Rain and Drought-Flood Disasters in Plateau and Basin Key Laboratory of Sichuan Province Institute of Plateau MeteorologyChina Meteorological AdministrationChengdu 610072China Chinese Academy of Sciences Center for Excellence in Tibetan Plateau Earth Sciences Beijing 100101China

A cold vortex occurred over the northeastern Tibetan Plateau(TP)on 2. April 2.1. and subsequently brought excessive rainfall to the spring farming area in southern china when moving *** study investigates the genesis mechanism of the cold TP vortex(TPV)by diagnosing reanalysis data and conducting numerical *** demonstrate that the cold TPV was generated in a highly baroclinic environment with significant contributions of positive potential vorticity(PV)forcing from the tropopause and diurnal thermodynamic impact from the *** a positive PV anomaly in the lower stratosphere moved towards the TP,the PV forcing at the tropopause pushed the tropospheric isentropic surfaces upward,forming isentropic-isplacement ascent and reducing static stability over the *** descent of the tropopause over the TP also produced a tropopause folding over the northeastern TP associated with a narrow high-PV column intruding downwards over the TPV genesis site,resulting in ascending air in the free ***,in conjunction with the descending air in the valley area during the night,produced air stretching just at the TPV genesis *** the surface cooling at night increased the surface static stability,the aforementioned vertical air-stretching thus converted the produced static stability to vertical ***,the cold TPV was generated over the valley at night.

关键词： tropopause PV forcing air column stretching static stability vertical vorticity

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Multi-locomotion transition of tensegrity mobile robot under different terrains

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Science china(Technological Sciences) 2024年第2期67卷 536-557页

作者： YANG Qi liu XinYu WANG PanFeng SONG {1. SUN Tao Key Laboratory of Mechanism Theory and Equipment Design(Tianjin university) Ministry of EducationTianjin UniversityTianjin 300350China

Knowing how to make a multi-locomotion robot achieve locomotion transition under different terrains is a challenging problem,especially for tensegrity robots with multi-locomotion *** this study,a motion planning method for the transition of a multi-locomotion tensegrity robot(hereafter TJUBot)under different terrains is *** robot can achieve four locomotion modes:earthworm-like,inchworm-like,tumbling,and sliding locomotion with only two *** models of the four locomotion modes under five typical terrains,including flat ground,confined space,obstacle,gap,and descending slope,are established using the energy ***,the kinematic characteristics(driving law and initial position)of the robot under these terrains are *** this basis,motion planning for the locomotion transition of TJUBot is conducted,which includes a perception strategy based on three laser sensors and a transition strategy under different *** driving laws of the two motors that can ensure the effective locomotion transition of TJUBot under different terrains are naturally ***,experiments are *** demonstrate that the robot can achieve effective locomotion transition when the motion planning method is used.

关键词： multi-locomotion robot tensegrity kinematic modeling locomotion transition

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The evolution of robotics:research and application progress of dental implant robotic systems

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International Journal of Oral Science 2024年第2期16卷 173-185页

作者： Chen liu Yuchen liu Rui Xie Zhiwen Li Shizhu Bai {2. Zhao State Key Laboratory of Oral&Maxillofacial Reconstruction and Regeneration Xi’anChina National Clinical Research Center for Oral Diseases Xi’anChina Shaanxi Key Laboratory of Stomatology Xi’anChina Digital Center School of StomatologyThe Fourth Military Medical UniversityXi’anChina

The use of robots to augment human capabilities and assist in work has long been an *** has been developing since the 1.60s when the first industrial robot was *** technology has advanced,robotic-assisted surgery has shown numerous advantages,including more precision,efficiency,minimal invasiveness,and safety than is possible with conventional techniques,which are research hotspots and cutting-edge *** article reviewed the history of medical robot development and seminal research papers about current research *** the autonomous dental implant robotic system as an example,the advantages and prospects of medical robotic systems would be discussed which would provide a reference for future research.

关键词： robot robotic application

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Shallow Convection Dataset Simulated by Three Different Large Eddy Models

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Advances in Atmospheric Sciences 2024年第4期41卷 754-766页

作者： Yaxin ZHAO Xiaocong WANG yimin {1. Guoxiong WU Yanjie {1. College of Earth and Planetary Sciences University of Chinese Academy of Sciences(UCAS)Beijing 100029China State Key Laboratory of Numerical Modeling for Atmospheric Sciences and Geophysical Fluid Dynamics(LASG) Institute of Atmospheric Physics(IAP)Chinese Academy of Sciences(CAS)Beijing 100029China

Shallow convection plays an important role in transporting heat and moisture from the near-surface to higher altitudes,yet its parameterization in numerical models remains a great challenge,partly due to the lack of high-resolution *** study describes a large eddy simulation(LES)dataset for four shallow convection cases that differ primarily in inversion strength,which can be used as a surrogate for real *** reduce the uncertainty in LES modeling,three different large eddy models were used,including SAM(System for Atmospheric Modeling),WRF(Weather Research and Forecasting model),and *** show that the different models generally exhibit similar behavior for each shallow convection case,despite some differences in the details of the convective *** addition to grid-averaged fields,conditionally sampled variables,such as in-cloud moisture and vertical velocity,are also provided,which are indispensable for calculation of the entrainment/detrainment *** the essentiality of the entraining/detraining process in the parameterization of cumulus convection,the dataset presented in this study is potentially useful for validation and improvement of the parameterization of shallow convection.

关键词： large eddy simulation SAM WRF UCLA-LES shallow convection entraining process

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Fully automatic AI segmentation of oral surgery-related tissues based on cone beam computed tomography images

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International Journal of Oral Science 2024年第3期16卷 413-424页

作者： Yu liu Rui Xie Lifeng Wang Hongpeng liu Chen liu yimin Zhao Shizhu Bai Wenyong liu Beijing Yakebot Technology Co. Ltd.BeijingChina School of Mechanical Engineering and Automation Beihang UniversityBeijingChina State Key Laboratory of Oral&Maxillofacial Reconstruction and Regeneration National Clinical Research Center for Oral DiseasesShaanxi Key Laboratory of StomatologyDigital CenterSchool of StomatologyThe Fourth Military Medical UniversityXi’anChina Key Laboratory of Biomechanics and Mechanobiology of the Ministry of Education Beijing Advanced Innovation Center for Biomedical EngineeringSchool of Biological Science and Medical EngineeringBeihang UniversityBeijingChina

Accurate segmentation of oral surgery-related tissues from cone beam computed tomography(CBCT)images can significantly accelerate treatment planning and improve surgical *** this paper,we propose a fully automated tissue segmentation system for dental implant ***,we propose an image preprocessing method based on data distribution histograms,which can adaptively process CBCT images with different *** on this,we use the bone segmentation network to obtain the segmentation results of alveolar bone,teeth,and maxillary *** use the tooth and mandibular regions as the ROI regions of tooth segmentation and mandibular nerve tube segmentation to achieve the corresponding *** tooth segmentation results can obtain the order information of the *** corresponding experimental results show that our method can achieve higher segmentation accuracy and efficiency compared to existing *** average Dice scores on the tooth,alveolar bone,maxillary sinus,and mandibular canal segmentation tasks were 96.5%,95.4%,93.6%,and 94.8%,*** results demonstrate that it can accelerate the development of digital dentistry.

关键词： surgery CBCT beam

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A multichannel thermal bubble-actuated impedance flow cytometer with on-chip TIA based on CMOS-MEMS

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Journal of Semiconductors 2024年第5期45卷 41-49页

作者： Shengxun Cai Jianqing Nie Kun Wang yimin Guan Demeng {1. School of Microelectronics Shanghai UniversityShanghai 201800China Shanghai AURE Technology Limited Company Shanghai 201800China

Electrochemical impedance spectroscopy(EIS)flow cytometry offers the advantages of speed,affordability,and portability in cell analysis and cytometry ***,the integration challenges of microfluidic and EIS read-out circuits hinder the downsizing of cytometry *** address this,we developed a thermal-bubble-driven impedance flow cytometric application-specific integrated circuit(ASIC).The thermal-bubble micropump avoids external piping and equipment,enabling high-throughput *** a total of 36 cell counting channels,each measuring 884×2.0μm^(2.,the chip significantly enhances the throughput of flow *** cell counting channel incorporates a differential trans-impedance amplifier(TIA)to amplify weak biosensing *** eliminating the parasitic parameters created at the complementary metal-oxidesemiconductor transistor(CMOS)-micro-electromechanical systems(MEMS)interface,the counting accuracy can be *** on-chip TIA can adjust feedback resistance from 5 to 60 kΩto accommodate solutions with different *** chip effectively classifies particles of varying sizes,demonstrated by the average peak voltages of 0.052. and 0.451. mV for 7 and 1.μm polystyrene beads,***,the counting accuracies of the chip for polystyrene beads and MSTO-2.0}H cells are both greater than 97.6%.The chip exhibits potential for impedance flow cytometer at low cost,high-throughput,and miniaturization for the application of point-of-care diagnostics.

关键词： EIS flow cytometry CMOS-MEMS thermal bubble lab-on-chip

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Research on the method for retrieving soil moisture using thermal inertia model

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Science china Earth Sciences 2006年第5期49卷 539-545页

作者： liu Zhenhua1.& ZHAO Yingshi2.1. Information College, South{1. Agricultural {1., guangzhou 51.642.{1. 2. Graduate {1. of Chinese Academy of Sciences, Beijing 1.0049,{1. Information College South China Agricultural University Guangzhou China Graduate university of Chinese Academy of Sciences Beijing China

In order to improve accuracy of soil moisture inversion using remote sensing, a new thermal inertia model is proposed in this paper. The improved model needs only surface maximum temperature as the temperature parameter input instead of input of the surface temperature difference, as well as the surface sensible and latent fluxes are introduced into boundary conditions of thermal conductivity equation. Furthermore, surface soil conductive heat transfer equation of two-layer model is used to solve the soil thermal inertia so that the remote sensing thermal inertia method can be ap- plied to regions with better-covered vegetation, but usually only for the bare areas or worse vegetation covered areas. The model has been tested at several locations in the area of west Inner Mongolia. Comparing the simulation of the new model with the measurements obtained by apparent thermal inertia and by field test, the result shows that the inertia thermal model can be used to estimate soil moisture in more reasonable accuracy.

关键词： thermal model, thermal conductivity equation, soil initial, sensible flux, latent flux, two-layer model.

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