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Peracetic acid catalytic activation using Co3O4 nanocluster decorated graphitic carbon nitride for cefapirin degradation in water

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Science China Technological Sciences 2024年第10期67卷 3103-3115页

作者： yin shiMei GAO YiXuan CHEN Long LI Fan liu XiaoNa QI Fei liu Wen Beijing Key Lab for Source Control Technology of Water Pollution College of Environmental Science and EngineeringBeijing Forestry University Key Laboratory of Water and Sediment Sciences (Ministry of Education) College of Environmental Sciences and EngineeringPeking University School of Environmental Science and Engineering Taiyuan University of Technology State Environmental Protection Key Laboratory of All Material Fluxes in River Ecosystems Peking University Beijing National Laboratory for Molecular Sciences Peking University

This study innovated cobalt-based catalytic nanocomposites（CCNs） for the heterogeneous activation of peracetic acid（PAA）,a green and efficient advanced oxidation process for removing antibiotics from *** Co3O4catalysts exhibit limited activity due to stable electronic *** overcome this,CCNs were synthesized using a one-step condensation method,incorporating a size control strategy that anchors Co3O4nanoclusters within 4-5 nm onto six-fold cavity of g-C3N4,simultaneously modifying the coordination environment of *** alteration significantly enhances the adsorption energy of PAA and catalytic activity compared to commercial *** improved performance of CCN2,in particular,is attributed to a shift in the cobalt d band center towards the Fermi level,facilitating electron delocalization and transfer,enhancing Co-O bonding,and accelerating PAA ***2's superior activity,with a cefapirin（CFP） degradation kinetic rate constant(k1=0.760 min-1)～11 times that of PAA direct oxidation(k1=0.070 min-1) and～5 times that of commercial Co3O4/PAA system(k1=0.164 min-1),is due to its ability to generate dominant reactive species for antibiotic degradation,including alkoxy radicals(CH3C（=O）OO·),high valence metal(CoⅣ（=O）2+),and singlet oxygen（1O2）,with the latter two being crucial for the degradation *** degradation of CFP involved three mechanisms,including direct oxidation by PAA,decarboxylation,and open-ring reactions at nitrogen *** research provides insights into developing high-activity catalysts for efficient PAA activation and antibiotic removal,leveraging the strategy of shifting the transition metal d band center.

关键词： peracetic acid Co3O4 nanocluster high valence metal singlet oxygen cefapirin

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A Survey on Graph Neural Network Acceleration: A Hardware Perspective

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Chinese Journal of Electronics 2024年第3期33卷 601-622页

作者： shi CHEN Jingyu liu Li SHEN School of Computer National University of Defense Technology Key Laboratory of Advanced Microprocessor Chips and Systems

Graph neural networks(GNNs) have emerged as powerful approaches to learn knowledge about graphs and *** rapid employment of GNNs poses requirements for processing *** to incompatibility of general platforms,dedicated hardware devices and platforms are developed to efficiently accelerate training and inference of *** conduct a survey on hardware acceleration for *** first include and introduce recent advances of the domain,and then provide a methodology of categorization to classify existing works into three ***,we discuss optimization techniques adopted at different *** finally we propose suggestions on future directions to facilitate further works.

关键词： Graph neural networks Deep learning acceleration Domain-specific architecture Hardware accelerator

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冰碛湖溃决灾害研究进展

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冰川冻土 2007年第4期29卷 626-635页

作者：王欣刘时银湖南科技大学地球空间信息科学研究所湖南湘潭411201 中国科学院寒区旱区环境与工程研究所冰冻圈科学国家重点实验室甘肃兰州730000

近年来随着全球气候变暖和冰川退缩,冰碛湖溃决灾害受到了广泛的关注,对冰碛湖溃决洪水/泥石流灾害的研究也取得较大进展,经历了由野外观测到遥感手段与野外观测相结合、由定性半定量到定量、由经验估算到基于物理过程建模模拟的发展过... 详细信息

近年来随着全球气候变暖和冰川退缩,冰碛湖溃决灾害受到了广泛的关注,对冰碛湖溃决洪水/泥石流灾害的研究也取得较大进展,经历了由野外观测到遥感手段与野外观测相结合、由定性半定量到定量、由经验估算到基于物理过程建模模拟的发展过程.从冰碛湖的识别与变化监测入手,综述了冰碛湖的溃决诱因与溃决机制、溃决风险评价指标体系、溃决洪水/泥石流的模拟以及溃决风险减缓措施等方面的研究进展与现状,展望了当前的研究工作的发展趋势,为进一步研究冰碛湖溃决洪水/泥石流灾害奠定基础.

关键词：冰碛湖溃决灾害研究进展

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度日模型在冰川与积雪研究中的应用进展

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冰川冻土 2006年第1期28卷 101-107页

作者：张勇刘时银中国科学院寒区旱区环境与工程研究所冰冻圈与环境联合重点实验室甘肃兰州730000

度日模型是基于冰川与积雪消融和气温,尤其是冰雪表面的正积温之间的线性关系建立的.度日模型已广泛应用于北欧、阿尔卑斯山、格陵兰冰盖、青藏高原等地区的冰雪消融、冰川物质平衡及对气候敏感性响应、冰川动力模型以及冰雪融水径流模... 详细信息

度日模型是基于冰川与积雪消融和气温,尤其是冰雪表面的正积温之间的线性关系建立的.度日模型已广泛应用于北欧、阿尔卑斯山、格陵兰冰盖、青藏高原等地区的冰雪消融、冰川物质平衡及对气候敏感性响应、冰川动力模型以及冰雪融水径流模拟等的研究中.度日模型尽管是对冰雪表面消融能量平衡这一复杂过程的简化描述,但在流域尺度上,通常可以获取类似于能量平衡模型的输出结果.度日模型也有其不足之处,仍需进一步的改进与完善.

关键词：冰川与积雪消融正积温度日模型

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Substrate screening for superclean graphene growth using firstprinciples calculations

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Nano Research 2024年第4期17卷 2216-2222页

作者： Zhihao Li Xiucai Sun Xiaoli Sun Wan-Jian yin Zhongfan liu College of Energy Soochow Institute for Energy and Materials InnovationS(SIEMIS)and Jiangsu Provincial Key Laboratory for Advanced Carbon Materials and Wearable Energy TechnologiesSoochow UniversitySuzhou 215006China Graphene Basic Science Research Center Beijing Graphene Institute(BGI)Beijing 100095China Center for Nanochemistry Beijing Science and Engineering Center for NanocarbonsBeijing National Laboratory for Molecular ScienceCollege of Chemistry and Molecular EngineeringPeking UniversityBeijing 100871China

Suppressing the formation of amorphous surface carbon and contaminants during the preparation of graphene by chemical vapor deposition remains an ongoing ***,we analyzed how substrate characteristics affect graphene quality by simulating margin extension,the nucleation process,and defect pegging configurations on mono-crystalline oriented metal substrates with the aim of enhancing graphene *** formation energy and nucleation potential,which are indirect substrate–graphene interaction features,were found to appropriately evaluate graphene *** crystallographic orientation of the metal substrate was discovered to be critical for producing superclean graphene.A low graphene defect density and high nucleation rate on the Cu(100)facet guarantee growth of high-quality graphene,especially in terms of suppressing the formation of amorphous *** addition,rapid kink growth and self-healing on the Cu(100)facet facilitate rapid graphene synthesis,which is also promoted by rapid kink splicing and margin self-repair on this *** study provides theoretical insight useful for the synthesis of superclean graphene.

关键词： superclean graphene defects nucleation metal substrates density functional theory calculations

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Gravel hardness effect on compaction characteristics of gravelly soil

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Journal of Mountain Science 2024年第4期21卷 1432-1443页

作者： shi Yunfang LI Shengang JIANG Chen liu Jinning School of Resources and Civil Engineering Northeastern UniversityShenyang 110004China

The compaction characteristics of gravelly soil are affected by gravel *** investigate the evolution and influencing mechanism of different gravel hardness on the compaction characteristics of gravelly soil,heavy compaction tests and crushing tests were conducted on gravelly soils with gravels originated from hard,soft and extremely soft *** to orthogonal experiments and variance analysis,it was found that hardness has a significant impact on the maximum dry density of gravelly soil,followed by gravel content,and lastly,moisture *** gravel compositions with an average saturated uniaxial compressive strength less than 60 MPa,the order of compacted maximum dry density is soft gravels>hard gravels>extremely soft *** type of gravelly soil has a threshold for gravel content,with 60%for hard and soft gravels and 50%for extremely soft *** these thresholds,the compacted dry density decreases *** is a certain interaction between hardness,gravel content,and moisture *** hardness increases the influence of gravel content,whereas lower hardness increases the influence of moisture *** soils with the coarse aggregate(CA)between 0.7 and 0.8 typically achieve higher dry densities after *** addition,the prediction equations for the particle breakage rate and CA ratio in the Bailey method were proposed to estimate the compaction performance of gravelly soil *** results further revealed the compaction mechanism of different gravelly soils and can provide reference for subgrade filling construction.

关键词： Gravelly soil Hardness Compaction characteristics Crushing characteristics Particle breakage rate Bailey method

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Comparative Transcriptome Analysis of Shell-Matrix-Protein Genes and Observation of the Shell Microstructure in the Deep-Sea Clam Calyptogena marissinica

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Journal of Ocean University of China 2024年第3期23卷 797-810页

作者： shi Yu liu Dongting YAO Gaoyou HE Maoxian CAS Key Laboratory of Tropical Marine Bio-Resources and Ecology Guangdong Provincial Key Laboratory of Applied Marine BiologySouth China Sea Institute of OceanologyChinese Academy of SciencesGuangzhou 510301China Southern Marine Science and Engineering Guangdong Laboratory(Guangzhou) Guangzhou 511458China University of Chinese Academy of Sciences Beijing 100049China

The deep-sea clam Calyptogena marissinica is widely distributed in the Haima cold seep ecosystem on the northwes-tern slope of the South China Sea with low pH values,low temperature and high *** information is available on the biomineralization of this *** this research,we generated a comprehensive transcript dataset of ***’s mantle tissue,and a total of 19821 unigenes were *** shell matrix proteins(SMP)-related genes were *** qPCR results showed that four out of six prismatic matrix genes(MSP2,MSP5,prisilkin-39,and shematrin),four out of the six nacreous matrix genes(perlucin,pif,pif97,and papilin),and two extrapallial fluid proteins(SPARC and calmodulin)were significantly expressed in the *** the nacreous and the prismatic layers are chrysanthemum-shaped,which are stacked on the top of each other to form a laminated nacreous *** alignment and phylogenetic analysis of MSP-5,Prisilkin-39,Perlucin,and Pif homologues showed that some amino acids of *** that differed from those detected in other molluscs may cause the different shape of the nacreous and prismatic layers,but do not lead to a change in the species’evolutionary *** results indicated the conservation of the functions of SMP-related genes in ***,and the specific shape of the prismatic and nacreous layers of this deep-sea mollusc,which will contribute to the research on the molecular regulation mechanisms of biomineralization in *** and provide a new perspective to investigate biomineralization in deep-sea clams in general.

关键词： transcriptome biomineralization mantle tissue shell Calyptogena marissinica

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Clinical Study on the Prevention and Treatment of Intestinal Fibrosis in Ulcerative Colitis by Moxibustion

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Journal of Acupuncture and Tuina Science 2003年第2期1卷 14-17页

作者： WU Huan-gan AN Guang-qing liu Hui-rong shi Zheng CHEN Han-ping liu shi-min shi yin XIAO Yuan-chun Shanghai Research Center of Acupuncture and Meridian 200030 China Shanghai Research Center of Acupuncture and Meridian 200030 China Shanghai Research Center of Acupuncture and Meridian 200030 China Shanghai Research Center of Acupuncture and Meridian 200030 China Shanghai Research Center of Acupuncture and Meridian 200030 China Shanghai Research Center of Acupuncture and Meridian 200030 China Shanghai Research Center of Acupuncture and Meridian 200030 China

Objective To observe the therapeutic effects and action mechanism of moxibustion in the treatment of intestinal fibrosis in ulcerative *** Tianshu (ST25) and Qihai (CV6) were the main acupoint; other points were used according to syndrome differentiation. Sixty-five patients were randomized into two groups: Group A in which 32 cases were treated by herbpartitioned moxibustion and group B in which 33 cases were treated by bran-partitioned moxibustion. The therapeutic effects and TGF-β1, I and III collagen expressions were measured before and after *** In group A, 17 cases were cured, 12 cases improved and 3 failed; in group B, 11 cases were cured, 16 cases improved and 6 cases failed. I, III collagen expressions were obviously inhibited in the two groups, in group A in *** In the prevention and treatment of intestinal fibrosis, moxibustion may reduce the expression of TGF-β1, and hence to block or inhibit the synthesis of I, III collagens, and improve the structure and function. Key Words Colonitis - Ulcerative - Collagen - Herbpartitioned Moxibustion - Bran-partitioned Moxibustion Foundation Item: This study supported by the National Natural Science Foundation of China, No.39970922, and Shanghai Science and Technology Committee and State Administration Bureau of Traditional Chinese MedicineTranslator: XIAO Yuan-chun

关键词： Colonitis Ulcerative Collagen Herbpartitioned Moxibustion Bran-partitioned Moxibustion

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Responses of the Southern Ocean mixed layer depth to the eastern and central Pacific El Niño events during austral winter

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Acta Oceanologica Sinica 2024年第7期43卷 1-14页

作者： Yuxin shi Hailong liu Xidong Wang Quanan Zheng School of Oceanography Shanghai Jiao Tong UniversityShanghai 200240China Yunnan Key Laboratory of Meteorological Disasters and Climate Resources in the Greater Mekong Subregion Yunnan UniversityKunming 600650China College of Oceanography Hohai UniversityNanjing 210098China Department of Atmospheric and Oceanic Science University of Maryland at College ParkCollege Park 20742USA

Based on the Ocean Reanalysis System version 5(ORAS5)and the fifth-generation reanalysis datasets derived from European Centre for Medium-Range Weather Forecasts(ERA5),we investigate the different impacts of the central Pacific(CP)El Niño and the eastern Pacific(EP)El Niño on the Southern Ocean(SO)mixed layer depth(MLD)during austral *** MLD response to the EP El Niño shows a dipole pattern in the South Pacific,namely the MLD dipole,which is the leading El Niño-induced MLD variability in the *** tropical Pacific warm sea surface temperature anomaly(SSTA)signal associated with the EP El Niño excites a Rossby wave train propagating southeastward and then enhances the Amundsen Sea low(ASL).This results in an anomalous cyclone over the Amundsen *** a result,the anomalous southerly wind to the west of this anomalous cyclone advects colder and drier air into the southeast of New Zealand,leading to surface cooling through less total surface heat flux,especially surface sensible heat(SH)flux and latent heat(LH)flux,and thus contributing to the mix layer(ML)*** east of the anomalous cyclone brings warmer and wetter air to the southwest of Chile,but the total heat flux anomaly shows no significant *** warm air promotes the sea ice melting and maintains fresh water,which strengthens *** results in a shallower *** the CP El Niño,the response of MLD shows a separate negative MLD anomaly center in the central South *** Rossby wave train triggered by the warm SSTA in the central Pacific Ocean spreads to the Amundsen Sea,which weakens the ***,the anomalous anticyclone dominates the Amundsen ***,the anomalous northerly wind to the west of anomalous anticyclone advects warmer and wetter air into the central and southern Pacific,causing surface warming through increased SH,LH,and longwave radiation flux,and thus contributing to the ML ***,to the east of the anomalous anticyclone,there is n

关键词： Southern Ocean mixed layer depth Central Pacific El Niño Eastern Pacific El Niño Rossby wave train

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Assessment of climate damage in China based on integrated assessment framework

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Advances in Climate Change Research 2024年第1期15卷 124-133页

作者： Jie liu Xiang-Zhen shi Li YANG Chang-Yi liu Jin-Cheng WANG Rui-Min ZHU Xue-Li shi Qiu-Feng liu International Business School Shanxi Normal UniversityXi'an 710062China University of Chinese Academy of Social Sciences Bejing 102488China School of Economics and Management Xinjiang UniversityUrumqi 830046China Global Energy Interconnection Development and Cooperation Organization(GEIDCO) Bejing 100031China Hubei Enshi College Enshi 445099China CMA Earth System Modeling and Prediction Centre China Meteorological AdministrationBeijing 100081China National Climate Centre China Meteorological AdministrationBeijing 100081China

Developing a localized and consistent model framework for climate loss and damage assessment is crucial for the policy-making of climate change mitigation and *** study introduces a comprehensive,multidisciplinary Integrated Assessment Model(IAM)framework for evaluating climate damage in China,utilizing BCC-SESM climate model and FUND sectoral climate damage model under the SSP2-RCPs *** a bottom-up approach,the research estimates climate damage across eight major sectors,recalibrates sectoral climate damage functions and parameters for China,and elucidates distinctions among direct climate loss,market climate loss,and aggregate climate *** findings reveal that the total climate damage function for China follows a quadratic pattern in response to temperature *** 2050,the estimated climate damage is projected to be 5.4%,5.7%,and 8.2%of GDP under RCP2.6,RCP4.5,and RCP8.5,***,both direct and market climate losses are projected to remain below 2%of GDP by 2050,while the aggregate climate loss could reach as high as 8.2%,which is predominantly attributed to non-market *** a sectoral perspective,under the RCP8.5 scenario,human health damage constitutes the largest share(61.9%)of the total climate loss by 2050,followed by sea-level rise damage(18.6%).This study sheds lights on the adaptation policy that should attach importance to the non-market sectors,particularly focusing on human health and sea-level rise.

关键词： Climate loss and damage Integrated assessment model(IAM) FUND model Representative concentration pathways(RCPs)scenario BCC-SESM

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