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Tuning electronic structure of RuO_(2)by single atom Zn and oxygen vacancies to boost oxygen evolution reaction in acidic medium

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Journal of Energy Chemistry 2024年第1期88卷 94-102,I0003页

作者： Qing Qin Tiantian Wang Zijian Li Guolin Zhang Haeseong Jang liqiang Hou Yu Wang Min Gyu Kim Shangguo liu Xien liu College of Chemical Engineering Qingdao University of Science and TechnologyQingdao 266042ShandongChina Department of Chemistry City University of Hong KongHong Kong 999077China Department of Advanced Materials Engineering Chung-Ang UniversityAnseong-siGyeonggi-do 17546SeoulRepublic of Korea Beamline Research Division Pohang Accelerator Laboratory(PAL)Pohang 37673Gyeongsangbuk-doRepublic of Korea

The poor stability of RuO_(2)electrocatalysts has been the primary obstacles for their practical application in polymer electrolyte membrane *** dramatically enhance the durability of RuO_(2)to construct activity-stability trade-off model is full of significance but ***,a single atom Zn stabilized RuO_(2)with enriched oxygen vacancies(SA Zn-RuO_(2))is developed as a promising alternative to iridium oxide for acidic oxygen evolution reaction(OER).Compared with commercial RuO_(2),the enhanced Ru–O bond strength of SA Zn-RuO_(2)by forming Zn-O-Ru local structure motif is favorable to stabilize surface Ru,while the electrons transferred from Zn single atoms to adjacent Ru atoms protects the Ru active sites from ***,the optimized surrounding electronic structure of Ru sites in SA ZnRuO_(2)decreases the adsorption energies of OER intermediates to reduce the reaction *** a result,the representative SA Zn-RuO_(2)exhibits a low overpotential of 210 mV to achieve 10 mA cm^(-2)and a greatly enhanced durability than commercial RuO_(2).This work provides a promising dual-engineering strategy by coupling single atom doping and vacancy for the tradeoff of high activity and catalytic stability toward acidic OER.

关键词： Electrocatalyst Acidic oxygen evolution reaction Electronic structure engineering Durability Reaction barrier

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Preparation and Photostriction Properties of BiFeO_(3)-BaTiO_(3)Ceramics

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Journal of Wuhan University of Technology(Materials Science) 2024年第5期39卷 1079-1086页

作者： ZHENG Zewei ZHANG liqiang CHEN Chen CAO Minghe YI Zhiguo liu Hanxing School of Materials Science and Engineering Wuhan University of TechnologyWuhan 430070China State Key Laboratory of High Performance Ceramics and Superfine Microstructure Shanghai Institute of CeramicsChinese Academy of SciencesShanghai 200050China School of Microelectronics Shanghai UniversityShanghai 200444China International School of Materials Science and Engineering Wuhan University of TechnologyWuhan 430070China

Under illumination by 405,520 and 655 nm monochromatic visible light(light intensity of 30 kW/m^(2)),large photostriction(ΔL/L)of 0.19%,0.13%and 0.26%for 67BiFeO_(3)-33BaTiO_(3)(67BF-33BT)lead-free ferroelectric ceramics are obtained,*** studying the ferroelectric and photoelectric properties in conjunction with in situ Raman spectroscopy,it is found that the photostrictive effect of 67BF-33BT is not caused by the electrical strain induced by abnormal photovoltaic voltage,but related to the optical induced oxygen octahedral *** 67BF-33BT lead-free ferroelectric material with excellent photostrictive response in the visible light region is expected to play an important role in the field of optical drive electromechanical devices.

关键词： ferroelectric ceramics photostrictive effect visible light response

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First-Principle Studies on the Ga and As Doping of Germanane Monolayer

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Journal of Applied Mathematics and Physics 2019年第1期7卷 46-54页

作者： Lei liu Yanju Ji Yifan liu liqiang liu School of Science Shandong Jianzhu University Jinan China

The study of energetics, structural, the electronic and optical properties of Ga and As atoms substituted for doped germanane monolayers were studied by first-principles calculations based on density functional theory. Both of the two doping are thermodynamically stable. According to the band structure and partial density of the states, gallium is p-type doping. Impurity bands below the conduction band lead the absorption spectrum moves in the infrared direction. Arsenic doping has impurity level passing through the Fermi level and is n-type doping. The analysis of optical properties confirms the value of bandgap and doping properties.

关键词： Germanane Doping Electronic Properties Optical Properties First-Principle

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低温氢气透平膨胀机实验系统设计

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真空与低温 2024年第4期30卷 368-374页

作者：刘弘民熊联友彭楠李空荣柯长磊张晓华刘立强董留涛杨坤中国科学院理化技术研究所低温科学与技术重点实验室北京100190 中国科学院大学北京100049 北京中科富海低温科技有限公司北京100198

氢气透平膨胀机是大型氢液化器中核心部件之一,为探究其性能,设计了一套专门针对常温至液氢温区工作的低温氢气透平膨胀机实验系统。系统设计的核心目标是实现氢液化设备中的膨胀制冷流程,并对氢气透平膨胀机的热力性能和机械性能进行... 详细信息

氢气透平膨胀机是大型氢液化器中核心部件之一,为探究其性能,设计了一套专门针对常温至液氢温区工作的低温氢气透平膨胀机实验系统。系统设计的核心目标是实现氢液化设备中的膨胀制冷流程,并对氢气透平膨胀机的热力性能和机械性能进行测试与分析。热力性能测试内容包括绝热效率、实际制冷量和膨胀比,用来评估氢透平膨胀机的性能。机械性能测试内容包括连续免维护运行时间和启停次数,用来评估氢透平膨胀机的可靠性以及使用寿命。此外,对测试过程中可能出现的误差进行了分析。本实验系统为低温氢气透平膨胀机的性能评估提供测试平台,从而掌握低温氢气透平膨胀机的关键技术参数,并在此基础上优化设计,进一步提高氢气透平膨胀机组以及氢液化流程的性能。

关键词：氢液化氢透平膨胀机实验系统性能测试

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Enhanced wear resistance,antibacterial performance,and biocompatibility using nanotubes containing nano-Ag and bioceramics in vitro

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Bio-Design and Manufacturing 2024年第5期7卷 670-686页

作者： Qingge Wang Jia liu Hong Wu Jingbo liu Yaojia Ren Luxin Liang Xinxin Yan Ian Baker Shifeng liu V.V.Uglov Chengliang Yang liqiang Wang State Key Laboratory of Powder Metallurgy Central South UniversityChangsha 410083China Affiliated Hospital of Youjiang Medical University for Nationalities Guangxi Key Laboratory for Preclinical and Translational Research on Bone and Joint Degenerative DiseasesGuangxi Zhuang Autonomous Region Engineering Research Center for Biomaterials in Bone and Joint Degenerative DiseasesGuangxi Key Laboratory for Biomedical Material ResearchBaise 533000China Department of Orthopedics The Second Xiangya HospitalCentral South UniversityChangsha 410011China Department of Orthopedics Renmin HospitalWuhan UniversityWuhan 430060China Thayer School of Engineering Dartmouth CollegeHanoverNH 03755-8000USA School of Metallurgical Engineering Xi’an University of Architecture and TechnologyXi’an 710055China Belarusian State University 220030 MinskBelarus State Key Laboratory of Metal Matrix Composites School of Material Science and EngineeringShanghai Jiao Tong UniversityShanghai 200240China

A good Ti-based joint implant should prevent stress shielding and achieve good bioactivity and anti-infection *** meet these requirements,the low-elastic-modulus alloy—Ti–35Nb–2Ta–3Zr—was used as the substrate,and functional coatings that contained bioceramics and Ag ions were prepared for coating on TiO_(2)nanotubes(diameter:(80±20)nm and(150±40)nm)using anodization,deposition,and spin-coating *** effects of the bioceramics(nano-β-tricalcium phosphate,microhydroxyapatite(micro-HA),and meso-CaSiO_(3))and Ag nanoparticles(size:(50±20)nm)on the antibacterial activity and the tribocorrosion,corrosion,and early in vitro osteogenic behaviors of the nanotubes were *** tribocorrosion and corrosion results showed that the wear rate and corrosive rate were highly dependent on the features of the nanotube ***-HA showed great wear resistance with a wear rate of(1.26±0.06)×10^(−3)mm^(3)/(N·m)due to adhesive and ***-CaSiO_(3)showed enhanced cell adhesion,proliferation,and alkaline phosphatase *** coatings that contained nano-Ag exhibited good antibacterial activity with an antibacterial rate of≥89.5%against Escherichia *** findings indicate that hybrid coatings may have the potential to accelerate osteogenesis.

关键词： βTi alloy Surface modification Wear resistance Corrosion resistance Osteogenic behavior Antibacterial activity

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HUNK inhibits cargo uptake and lysosomal traffic in the caveolar pathway via the AGAP3/ARF6

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Science Bulletin 2024年第2期69卷 173-178页

作者： Siyuan Jiang Xiaoqi Han Tihui liu Ying He Zidong Zhao Tongfeng liu Shuwen Cheng Jihang Zhang liqiang Duan Yajuan liu Tianyou Cheng Yong liu Qinong Ye Shan Gao Zhongda Hospital Medical SchoolAdvanced Institute for Life and HealthSoutheast UniversityNanjing 20096China Medical School of Guizhou University Guiyang 550025China Shanxi Academy of Advanced Research and Innovation Taiyuan 030032China Zhongda Hospital School of Life Sciences and TechnologyAdvanced Institute for Life and HealthSoutheast UniversityNanjing 210096China Nanjing University Medical School Nanjing 210046China Hubei Key Laboratory of Cell Homeostasis College of Life SciencesTaiKang Center for Life and Medical SciencesWuhan UniversityWuhan 430072China Department of Medical Molecular Biology Beijing Institute of BiotechnologyCollaborative Innovation Center for Cancer MedicineBeijing 100850China

Endocytosis is a crucial cellular process that takes up cargos by enclosing them in membrane-bound vesicles,and transports cargos to different parts of the cell,such as the lysosomes[1].Endocytosis is classified into several mechanistically and morphologically pathways,including clathrin-mediated endocytosis(CME)and caveolae-mediated endocytosis(CavME)[1,2].

关键词： endocytosis cargo uptake

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Insights into effects of thermotolerant nitrifying and sulfur-oxidizing inoculants on nitrogen-sulfur co-metabolism in sewage sludge composting

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Journal of Environmental Sciences 2024年第10期144卷 76-86页

作者： Tingting Hou Yujie Zhou Rongchun Du Jiali liu Weiguang Li Shumei Zhang Muzi Li Junhong Chu liqiang Meng Institute of Microbiology Heilongjiang Academy of SciencesHarbin 150010China Hebei University of Environmental Engineering Hebei Key Laboratory of Agroecological SafetyQinhuangdao 066102China School of Environment Harbin Institute of TechnologyHarbin 150090China

In this study,high temperature thermotolerant nitrifying bacteria(TNB)and high temperature thermotolerant sulfide oxidizing bacteria(TSOB)were obtained from compost samples and inoculated into sewage sludge(SS)*** effects of inoculation on physical and chemical parameters,ammonia and hydrogen sulfide release,nitrogen form and sulfur compound content change and physical-chemical properties during nitrogen and sulfur conversion were *** results showed that inoculation of TNB and TSOB increased the temperature,pH,OM degradation,C/N ratio and germination index(GI)of *** with the control treatment(CK),the addition of inoculants reduced the release of NH3 and H2S,and transformed them into nitrogen and sulfur compounds,the hydrolysis of polymeric ferrous sulfate was promoted,resulting in relatively high content of sulfite and *** the same time,the physical and chemical properties of SS have a strong correlation with nitrogen and sulfur compounds.

关键词： Sewage sludge Composting Inoculation Thermotolerant nitrifying bacteria Thermotolerant sulfurized oxidizing bacteria

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Extraction of the key infrared radiation temperature features concerning stress and crack evolution of loaded rocks

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International Journal of Mining Science and Technology 2024年第8期34卷 1059-1081页

作者： Wei liu liqiang Ma Michel Jaboyedoff Marc-Henri Derron Qiangqiang Gao Fengchang Bu Hai Sun Key Laboratory of Xinjiang Coal Resources Green Mining(Xinjiang Institute of Engineering) Ministry of EducationUrumqi 830023China Xinjiang Key Laboratory of Coal-bearing Resources Exploration and Exploitation Xinjiang Institute of EngineeringUrumqi 830023China Xinjiang Engineering Research Center of Green Intelligent Coal Mining Xinjiang Institute of EngineeringUrumqi 830023China School of Mines China University of Mining&TechnologyXuzhou 221116China Institute of Earth Sciences University of LausanneLausanne 1015Switzerland School of Civil Engineering Liaoning Petrochemical UniversityFushun 113001China

The infrared radiation temperature(IRT)variation concerning stress and crack evolution of rocks is a critical focus in rock mechanics domain and engineering disaster *** this paper,a methodology to extract the key IRT features related to stress and crack evolution of loaded rocks is ***,the wavelet denoising and reconstruction in thermal image sequence(WDRTIS)method is employed to eliminate temporal noise in thermal image ***,the adaptive partition temperature drift correction(APTDC)method is introduced to alleviate temperature *** this basis,the spatial noise correction method based on threshold segmentation and adaptive median filtering(OTSU-AMF)is proposed to extract the key IRT features associated with microcracks of loaded *** temperature drift correction,IRT provides an estimation of the thermoelastic factor in rocks,typically around 5.29×10^(-5) MPa^(-1) for *** reveal that the high-temperature concentrated region in cumulative thermal images of crack evolution(TICE)can elucidate the spatiotemporal evolution of localized ***,heat dissipation of crack evolution(HDCE)acquired from TICE quantifies the progressive failure process of *** proposed methodology enhances the reliability of IRT monitoring results and provides an innovative approach for conducting research in rock mechanics and monitoring engineering disasters.

关键词： Infrared radiation(IR) Temperature drift Spatial background noise Rock fracture Average infrared radiation temperature(AIRT) Heat dissipation of crack evolution(HDCE)

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Electron-deficient ZnO induced by heterointerface engineering as the dominant active component to boost CO_(2)-to-formate conversion

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Carbon Energy 2024年第5期6卷 127-136页

作者： Qing Qin Zijian Li Yingzheng Zhang Haeseong Jang Li Zhai liqiang Hou Xiaoqian Wei Zhe Wang Min Gyu Kim Shangguo liu Xien liu College of Chemical Engineering Qingdao University of Science and TechnologyQingdaoChina Department of Chemistry City University of Hong KongHong Kong SARChina Department of Advanced Materials Engineering Chung-Ang UniversityAnseong-siGyeonggi-doRepublic of Korea Beamline Research Division Pohang Accelerator Laboratory(PAL)PohangRepublic of Korea

Electrocatalytic CO_(2)-to-formate conversion is considered an economically viable *** general,Zn-based nanomaterials are well-known to be highly efficient electrocatalysts for the conversion of CO_(2) to CO,but seldom do they exhibit excellent selectivity toward *** this article,we demonstrate that a heterointerface catalyst ZnO/ZnSnO3 with nanosheet morphology shows enhanced selectivity with a maximum Faradaic efficiency(FE)of 86%at−0.9 V versus reversible hydrogen electrode and larger current density for the conversion of CO_(2) to formate than pristine ZnO and *** particular,the FEs of the C1 products(CO+HCOO−)exceed 98%over the potential *** experimental measurements combined with theoretical calculations revealed that the ZnO in ZnO/ZnSnO3 heterojunction delivers the valence electron depletion and accordingly optimizes Zn d-band center,which results in moderate Zn-O hybridization of HCOO*and weakened Zn-C hybridization of competing COOH*,thus greatly boosting the HCOOH *** study highlights the importance of charge redistribution in catalysts on the selectivity of electrochemical CO_(2) reduction.

关键词： charge redistribution CO_(2)reduction reaction electrocatalyst heterointerfaces selectivity

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Integration of antibody-antigen and receptor-ligand reactions to establish a gold strip biosensor for detection of 33 β-lactam antibiotics

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Science China Materials 2021年第8期64卷 2056-2066页

作者： Yue Li liqiang liu Chuanlai Xu Hua Kuang Li Sun State Key Laboratory of Food Science and Technology Jiangnan UniversityWuxi 214122China International Joint Research Laboratory for Biointerface and Biodetection School of Food Science and TechnologyJiangnan UniversityWuxi 214122China Chinese Academy of Inspection and Quarantine Beijing 100176China

A novel lateral flow immunoassay biosensor,combining the receptor-ligand reaction and antigen-antibody reaction was developed for the detection of β-lactam antibiotics in milk. The receptor protein, the carboxy-terminal domain of β-lactam sensor-transducer mutant from ***, served as the recognition element. Colloidal gold(CG)-labelled receptor antibody-receptor ternary complex was applied as a signal transducer probe. The presence ofβ-lactams was identified through a color change in the test zone, where the reaction between the complex of CG/antireceptor antibody/receptor and β-lactam antigen on the test line could be inhibited by β-lactam residues in the sample,thus leading to a reduction in color signal. Based on the indirect labeling of the receptor with an antibody as a linker, the ability to detect 33 β-lactams was below or near the corresponding maximum residue limit. The proposed lateral flow immunoassay biosensor appears to be an excellent field-based screening tool for the qualitative screening of β-lactams in milk.

关键词： lactams antibiotics receptor monoclonal antibody lateral flow immunoassay colloidal gold

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