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Engineering single-atom Mn on nitrogen-doped carbon to regulate lithium-peroxide reaction kinetics for rechargeable lithium-oxygen batteries

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Journal of Energy Chemistry 2024年第7期94卷 199-207页

作者： Yaling Huang Yong liu Yang liu Chenyang Zhang Wenzhang li Jie li School of Chemistry and Chemical Engineering Central South UniversityChangsha 410083HunanChina School of Minerals Processing and Bioengineering Central South UniversityChangsha 4003HunanChina

Precision engineering of catalytic sites to guide more favorable pathways for li_(2)O_(2) nucleation and decom-position represents an enticing kinetic strategy for mitigating overpotential,enhancing discharge capac-ity,and improving recycling stability of li-O_(2) *** this work,we employ metal-organic frameworks(MOFs)derivation and ion substitution strategies to construct atomically dispersed Mn-N_(4) moieties on hierarchical porous nitrogen-doped carbon(Mn SAs-NC)with the aim of reducing the over-potential and improving the cycling stability of li-O_(2) *** porous structure provides more chan-nels for mass transfer and exposes more highly active sites for electrocatalytic reactions,thus promoting the formation and decomposition of li_(2)O_(2).The li-O_(2) batteries with Mn SAs-NC cathode achieve lower overpotential,higher specific capacity(14290 mA h g^(-1) at 100 mAg^(-1)),and superior cycle stability(>100 cycles at 200 mA g^(-1))compared with the Mn NPs-NC and *** functional theory(DFT)cal-culations reveal that the construction of Mn-N_(4) moiety tunes the charge distribution of the pyridinic N-rich vacancy and balances the affinity of the intermediates(liO_(2) and li_(2)O_(2)).The initial nucleation of li_(2)O_(2) on Mn SAs-NC favors the O_(2)-→liO_(2)→li_(2)O_(2) surface-adsorption pathway,which mitigates the overpoten-tials of the oxygen reduction(ORR)and oxygen evolution reaction(OER).As a result,Mn SAs-NC with Mn-N_(4) moiety effectively facilitates the li_(2)O_(2) nucleation and enables its reversible *** work establishes a methodology for constructing carbon-based electrocatalysts with high activity and selectivity for li-O_(2)batteries.

关键词： Single-atom Mn MOFs-oriented architecture Rechargeable li-O_(2)battery N-doped carbon Density functional theory calculation

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Success rate of current human-derived gastric cancer organoids establishment and influencing factors:A systematic review and meta-analysis

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World Journal of Gastrointestinal Oncology 2024年第4期16卷 1626-1646页

作者： Kai-lin Jiang Xiang-Xiang Wang Xue-Jiao liu li-Kun Guo Yong-Qi Chen Qing-ling Jia Ke-Ming Yang Jiang-Hong ling Department of Gastroenterology Shuguang HospitalShanghai 200021China Department of Pathology Shuguang HospitalShanghai 200021China

BACKGROUND Human-derived gastric cancer organoids(GCOs)are widely used in gastric cancer research;however,the culture success rate is generally *** To explore the potential influencing factors,and the literature on successful culture rates of GCOs was reviewed using *** PubMed,Web of Science,and EMBASE were searched for *** trained researchers selected the studies and extracted *** 17.0 software was used for meta-analysis of the incidence of each outcome *** adjusted Methodological Index for Non-Randomized Studies scale was used to assess the quality of the included *** plots and Egger’s test were used to detect publication *** analyses were conducted for sex,tissue source,histo-logical classification,and the pathological tumor-node-metastasis(pTNM)cancer staging *** Eight studies with a pooled success rate of 66.6%were *** derived from women and men had success rates of 67%and 46.7%,*** from surgery or biopsy/endoscopic submucosal dissection showed success rates of 70.9%and 53.7%,*** of poorly-differentiated,moderately-differentiated and signet-ring cell cancer showed success rates of 64.6%,31%,and 32.7%,*** with pTNM stages I-II and III-IV showed success rates of 38.3%and 65.2%,respectively.Y-27632 and non-Y-27632 use showed success rates of 58.2%and 70%,*** generated with collagenase were more successful than those constructed with liberase TH and TrypLE(72.1%vs 71%,respectively).EDTA digestion showed a 50%lower success rate than other methods(P=0.04).CONCLUSION GCO establishment rate is low and varies by sex,tissue source,histological type,and pTNM *** Y-27632,and using liberase TH,TrypLE,or collagenase yields greater success than EDTA.

关键词： Gastric cancer organoids Human-derived organoids Gastric cancer Cell lines In vitro research models

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Experimental Investigation on Vertical Hydraulic Transport of Ores in Deepsea Mining

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China Ocean Engineering 2024年第1期38卷 42-53页

作者： liu Lei liu Jian-cheng li Xin XU li-xin ZHANG Xiu-zhan State Key Laboratory of Ocean Engineering Shanghai Jiao Tong UniversityShanghai 200240China School of Naval Architecture Ocean and Civil EngineeringShanghai Jiao Tong UniversityShanghai 200240China Sanya Yazhou Bay Institution of Deep-sea Sci-Tech Shanghai Jiao Tong UniversitySanya 572000China China Merchants Marine And Offshore Research Institute Co. Ltd.Shenzhen 518067China China Merchants Deepsea Research Institute(Sanya)Co. Ltd.Sanya 572000China School of Naval Architecture and Ocean Engineering Jiangsu University of Science and TechnologyZhenjiang 212100China

Deepsea mining has been proposed since the 1960s to alleviate the lack of resources on *** hydraulic transport of collected ores from the seabed to the sea surface is considered the most promising method for industrial *** the present study,an indoor model test of the vertical hydraulic transport of particles was conducted.A noncontact optical method has been proposed to measure the local characteristics of the particles inside a vertical pipe,including the local concentration and particle *** hydraulic gradient of ore transport was evaluated with various particle size distributions,particle densities,feeding concentrations and mixture flow *** transport,the local concentration is larger than the feeding concentration,whereas the particle velocity is less than the mixture *** qualitative effects of the local concentration and local fluid velocity on the particle velocity and slip velocity were *** local fluid velocity contributes significantly to particle velocity and slip velocity,whereas the effect of the local concentration is marginal.A higher feeding concentration and mixture flow velocity result in an increased hydraulic *** effect of the particle size gradation is slight,whereas the particle density plays a crucial role in the transport.

关键词： deepsea mining vertical hydraulic transport experiment flow characteristics

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Sigmatropic rearrangements of B(MIDA)-propargylic alcohols towards the diverse synthesis of α-functionalized organoborons

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Science China Chemistry 2024年第2期67卷 568-575页

作者： Jiasheng Qian li-Cai liu Zhi-Hao Chen Yuan liu Yin li Qingjiang li Honggen Wang Guangdong Key Laboratory of Chiral Molecule and Drug Discovery School of Pharmaceutical SciencesSun Yat-Sen UniversityGuangzhou510006China

α-Functionalized organoborons are useful building blocks and key structural elements in functional *** previous synthesis relied on the famous Matteson reaction or the late-stage borylative modification of alkynes or ***,the synthetic transformation of borylated building blocks offers another useful strategy and is currently actively *** report herein that B(MIDA)-propargylic alcohols(BPAs) are a useful type of borylated building *** two complementary functional group handles(alkyne and hydroxyl) in close proximity,the redox-neutral [3,3] and [2,3] sigmatropic rearrangements of BPAs allow the efficient synthesis of several types of α-functionalized boronates,including α,β-unsaturated acylborons,α-S/P-substituted allenylborons,boryl-substituted thiazoles and a borylated α,β-unsaturated hydrazine,some of which are otherwise challenging targets using other synthetic methods.

关键词： organoboron diverse synthesis sigmatropic rearrangement heteroarene amide

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Cyclosporine treatment in idiopathic membranous nephropathy nephrotic syndrome in adults： a retrospective study spanning 15 years

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Chinese Medical Journal 2011年第21期124卷 3490-3494页

作者： TAO Jian-ling liu li-li WEN Yu-bing GAO Rui-tong li Hang li Ming-xi li Xue-mei li Xue-wang Division of Nephrology Peking Union Medical College Hospital Peking Union Medical College Chinese Academy of Medical Science Beijing 100730 China

Background Cyclosporine is effective in treating nephrotic syndrome （NS） with idiopathic membranous nephropathy （IMN） in adults. But high relapse rate remains a major concern. The way to manipulate cyclosporine is inconclusive. The aim of this study was to introduce the way how to titrate the cyclosporine to maintain complete remission without relapse. Methods Patients with biopsy-proven IMN with NS treated with cyclosporine for at least 1 month from 1996 to 2011 at Peking Union Medical College Hospital were reviewed. Results Mean age of the 51 eligible patients was 52 years, with 39 men. Mean proteinuria was （7.47±3.14） g/d, serum albumin （24.50±6.29） g/L, and serum creatinine （82.62±21.18） μmol/L. Cyclosporine was commenced at a mean dose of （3.46±0.63） mg·kg^-1·d^-1. Oral prednisone （0.40±0.29） mg·kg^-1·d^-1 was given concomitantly in 38 patients. Cyclosporine was administered for a median of 16 months （range 1-93 months） and stopped in non-responders by month six. By month 3 （n=47）, the number in complete remission （CR） and partial remission （PR） was 3 and 24, which shifted to 12 and 17 by month 6 （n=41）. Male gender, heavy proteinuria, low serum albumin level, and high serum creatinine level were significant determinants in poor response by month six （P 〈0.05 in all variables compared with responders）. There was a significant reversible serum creatinine increase within 25% during month 3 to 12 （P 〈0.05 in all variables compared with baseline value）. Eleven patients maintained cyclosporine for more than 24 months with a cyclosporine dose of （1.04±1.06） mg·kg^-1·d^-1. Nine patients were in CR. Renal function, systolic and diastolic blood pressure remained stable. Renal impairment （〉30% rise of serum creatinine）, secondary infection, hypertension, gingival hyperplasia and liver impairment occurred in 6, 4, 10, 4, and 1 patients, respectively. Conclusions The observation time for cyclosporine to effectively induce CR of NS in IMN adults should be at least six month

关键词： cyclosporine idiopathic membranous nephropathy nephrotic syndrome treatment

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Input-to-State Stability of Impulsive Switched Systems Involving Uncertain Impulse-Switching Moments

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IEEE/CAA Journal of Automatica Sinica 2024年第6期11卷 1515-1517页

作者： Chang liu Wenlu liu Tengda Wei Xiaodi li School of Mathematical and Statistics Shandong Normal UniversityJinan 250014China

Dear Editor,This letter studies the input-to-state stability(ISS)for a class of impulsive switched systems,where uncertain impulse-switching moments are *** robustness of ISS with respect to the perturbations of the occurrence time of impulse-switching moments is revealed by several less conservative dwell-time conditions for the uncertain impulse-switching moments combined with Lyapunov ***,the Lyapunov conditions have multiple coefficients at discrete time so as to handle the hybrid effect of impulse-switching moments,and the case that time derivative of Lyapunov function is indefinite is also taken into ***,a numerical example is proposed to illustrate the effectiveness of the theoretical results.

关键词： letter conservative derivative

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Classification of anatomical morphology of cystic duct and its association with gallstone

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World Journal of Gastrointestinal Surgery 2024年第2期16卷 307-317页

作者： Jia-Hai Zhu Song-ling Zhao Qiang Kang Ya Zhu li-Xin liu Hao Zou Department of Hepatobiliary Pancreatic Surgery The Second Affiliated Hospital of Kunming Medical UniversityKunming 650106Yunnan ProvinceChina Department of Hepatobiliary Surgery The Second Affiliated HospitalKunming Medical UniversityKunming 650106Yunnan ProvinceChina

BACKGROUND Gallstones are common lesions that often require surgical ***-scopic cholecystectomy is the treatment of choice for symptomatic ***,the anatomical morphology of the cystic duct(CD),needs to be accurately recognized,especially when anatomical variations occur in the CD,which is otherwise prone to bile duct ***,at present,there is no optimal classification system for CD morphology applicable in clinical practice,and the relationship between anatomical variations in CDs and gallstones remains to be *** To create a more comprehensive clinically applicable classification of the morphology of CD and to explore the correlations between anatomic variants of CD and *** A total of 300 patients were retrospectively enrolled from October 2021 to January *** patients were divided into two groups:The gallstone group and the nongallstone *** clinical data and anatomical data of the CD based on magnetic resonance cholangiopancreatography(MRCP)were collected and analyzed to propose a morphological classification system of the CD and to explore its relationship with *** analysis was performed using logistic regression analyses to identify the independent risk factors using variables that were significant in the univariate *** Of the 300 patients enrolled in this study,200(66.7%)had *** mean age was 48.10±13.30 years,142(47.3%)were male,and 158(52.7%)were female.A total of 55.7%of the patients had a body mass index(BMI)≥24 kg/*** on the MRCP,the CD anatomical typology is divided into four types:Type I:linear,type II:n-shaped,type III:S-shaped,and type IV:*** analysis revealed differences between the gallstone and nongallstone groups in relation to sex,BMI,cholesterol,triglycerides,morphology of CD,site of CD insertion into the extrahepatic bile duct,length of CD,and angle between the common hepatic duct and *** to

关键词： Cystic duct Gallstone Classification Anatomy Magnetic resonance cholangiopancreatography Risk factor

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Constructing the Impossible Differential of Type-II GFN with Boolean Function and Its Application to WARP

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Chinese Journal of Electronics 2024年第1期33卷 80-89页

作者： Jiali SHI Guoqiang liu Chao li College of liberal Arts and Sciences National University of Defense Technology Hunan Engineering Research Center of Commercial Cryptography Theory and Technology Innovation State Key Laboratory of Information Security Institute of Information Engineering

Type-Ⅱ generalized Feist el network(GFN) has attracted a lot of attention for its simplicity and high *** differential attack is one of the powerful cryptanalytic approaches for word-oriented block ciphers such as Feistel-like *** deduce the impossible differential of Type-Ⅱ GFN by analyzing the Boolean function in the middle *** main idea is to investigate the expression with the variable representing the plaintext(ciphertext) difference words for the internal state *** adopting the miss-in-the-middle approach,we can construct the impossible differential of Type-Ⅱ *** an illustration,we apply this approach to WARP,a lightweight 128-bit block cipher with a 128-bit key which was presented by Banik et *** SAC *** structure of WARP is a 32-branch Type-Ⅱ ***,we find two 21-round truncated impossible differentials and implement a 32-round key recovery attack on *** the 32-round key recovery attack on WARP,some observations are used to mount an effective *** the advantage of the early abort technique,the data,time,and memory complexities are 2125.69chosen plaintexts,2126.6832-round encryptions,and 2100-bit,*** the best of our knowledge,this is the best attack on WARP in the single-key scenario.

关键词： Ciphers Boolean functions Parallel processing Complexity theory

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Bandgap adjustment of a sandwich-like acoustic metamaterial plate with a frequency-displacement feedback control method

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Applied Mathematics and Mechanics(English Edition) 2024年第10期45卷 1807-1820页

作者： Jianing liu Jinqiang li Ying WU School of Aerospace Engineering Xi’an Jiaotong UniversityXi’an 710049China College of Aerospace and Civil Engineering Harbin Engineering UniversityHarbin 150001China

Several types of acoustic metamaterials composed of resonant units have been developed to achieve low-frequency *** most of these structures,bandgaps are determined by their geometric configurations and material *** paper presents a frequency-displacement feedback control method for vibration suppression in a sandwich-like acoustic metamaterial *** band structure is theoretically derived using the Hamilton principle and validated by comparing the theoretical calculation results with the finite element simulation *** this method,the feedback voltage is related to the displacement of a resonator and the excitation *** applying a feedback voltage on the piezoelectric fiber-reinforced composite(PFRC)layers attached to a cantilever-mass resonator,the natural frequency of the resonator can be *** ensures that the bandgap moves in a frequency-dependent manner to keep the excitation frequency within the *** on this frequency-displacement feedback control strategy,the bandgap of the metamaterial plate can be effectively adjusted,and the vibration of the metamaterial plate can be significantly suppressed.

关键词： acoustic metamaterial Hamilton principle electromechanical coupling vibration control local resonance

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Tribological study of two ammonium chloride-decanoic acid deep eutectic solvents(DESs)as high-performance lubricants

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Friction 2024年第11期12卷 2441-2457页

作者： Zhuocheng li Enhui ZHANG Weimin li Haichao liu State Key Laboratory of Solid Lubrication Lanzhou Institute of Chemical PhysicsChinese Academy of SciencesLanzhou 730000China Center of Materials Science and Optoelectronics Engineering University of Chinese Academy of SciencesBeijing 100049China Zibo Innovation Center of High-End Synthetic Lubricating Materials Zibo 255000China

Deep eutectic solvents(DESs)are acknowledged as a novel class of functional *** share similar physical properties with ionic liquids(ILs)and have the potential to be a novel class of *** this study,two DESs,namely tetrabutylammonium chloride-decanoic acid DES(C4-DES)and methyl tricaprylmethylammonium chloride-decanoic acid DES(C8-DES),were synthesized,and their physico-chemical properties and tribological performances were ***-analysis of the rubbing surfaces used multiple techniques to gain insights into the lubrication *** show that the coefficient of friction(COF)and wear were reduced by approximately 29%and 91%for the C4-DES,and 36%and 94%for the C8-DES,compared to an ester base *** friction reduction behavior of the DESs is attributed to the monolayer adsorption of the polar group in the decanoic acid(DEAC),whose effectiveness is affected by the component of the ammonium salts in the DESs and the operating *** addition to the adsorbed film,worn surface analysis revealed that an ultra-thin tribochemical film with a thickness of 3–7 nm was formed on the surfaces lubricated with the *** composition of the film was studied,and the lubrication mechanisms of the two DESs were discussed.

关键词： deep eutectic solvent(DES) lubricants tribological performance boundary lubrication

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