检索结果-南通市图书馆

Enhanced photothermal dehydration of methanol over W_(18)O_(49)/Au/SAPO-34 catalysts with broadened light absorption

引用

Rare Metals 2024年第3期43卷 1139-1152页

作者： Ya-Qin Tang Meng-Xia Yan Chang-Qian Lu Shao-Yuan Li Kui-Xian Wei Tao Qu Wen-HuiMa Yong-Nian Dai Kong-Zhai Li Da-Jun Luo xue-liang zhang Yi-Ke Liu Faculty of Metallurgical and Energy Engineering Kunming University of Science and TechnologyKunming650093China School of Materials and Energy Engineering Guizhou Institute of TechnologyGuiyang550003China

Methanol-to-olefins(MTO)process is one of the most critical pathways to produce low carbon ***,the reaction is driven by thermal catalysis,which inevitably needs to consume large amounts of fossil *** a new technique to substitute for the fuel burning is urgent for MTO process to improve the industry prospects and ***,we report a novel W_(18)O_(49)/Au/SAPO-34(W/Au/S),a multifunctional photothermal catalyst for the MTO reaction.A high methanol conversion was achieved under xenonum(Xe)lamp irradiation,yielding methyl ether(ME)and ethylene as the main *** optimized W/Au/S catalysts showed ethylene yield as high as 250μmol in 60 min,which was 2.5 times higher than that of Au/*** physiochemical characterization revealed that the SAPO-34 molecular sieves were surrounded by Au and W_(18)O_(49)nanoparticles,which exhibited a strong localized surface plasmon resonance excitation around 540 nm and light absorption beyond 500 *** multifunctional catalysts showed a strong photothermal effect,arising from the broadened light absorption of Au and W_(18)O_(49)nanoparticles,leading to a temperature as high as 250℃on the surface of the *** study showed that the superior ethylene selectivity of W/Au/S catalysts was attributed to the moderating acidic sites of W_(18)O_(49)for methanol dehydration to *** research may provide new insight for designing heterostructures to improve photo-to-chemical conversion performance and is expected to accelerate progress toward the excellent multifunctional photothermal catalysts with broad light absorption for methanol activation and C-C bond formation.

关键词： Methanol conversion Ethylene Photothermal catalysis W_(18)O_(49) BrΦnsted-acid

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

Synchronization of three homodromy coupled exciters in a non-resonant vibrating system of plane motion

引用

Acta Mechanica Sinica 2012年第5期28卷 1424-1435页

作者： xue-liang zhang Bang-Chun Wen Chun-Yu Zhao School of Mechanical Engineering and Automation Northeastern University

In this paper, the synchronization problem of three homodromy coupled exciters in a non-resonant vibrating system of plane motion is studied. By introducing the average method of modified small parameters, we deduced dimensionless coupling equation of three exciters, which converted the problem of synchronization into that of the existence and stability of zero solutions for the average differential equations of the small parameters. Based on the dimensionless coupling torques and characteristics of the cor- responding limited functions, the synchronization criterion for three exciters was derived as the absolute value of dimensionless residual torque difference between arbitrary two motors being less than the maximum of their dimensionless coupling torques. The stability criterion of its synchronous state lies in the double-condition that the inertia coupling matrix is positive definite and all its elements are positive as well. The synchronization determinants are the coefficients of synchronization ability, also called as the general dynamical symmetry coefficients. The double-equilibrium state of the vibrating system is manifested by numeric method, and the numeric and simulation results derived thereof indicate the indispensable and crucial role the structural parameters of the vibrating system play in the stability criterion of synchronous operation. Besides, by adjusting its structural parameters, the elliptical motion of the vibrating system successfully met the requirements in engineering applications.

关键词： Synchronization Vibrating system Stability Coupling dynamic - Vibratory synchronization transmission

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

Temperature-dependent evolution of oxide inclusions during heat treatment of stainless steel with yttrium addition

引用

International Journal of Minerals,Metallurgy and Materials 2020年第6期27卷 754-763页

作者： xue-liang zhang Shu-feng Yang Jing-she Li Jin-qiang Wu School of Metallurgical and Ecological Engineering University of Science and Technology BeijingBeijing 100083China Department of Material Science and Engineering Missouri University of Science and TechnologyRollaMO 65409USA Center for Innovation through Visualization and Simulation Purdue University NorthwestHammondIN 46323USA

The evolution of oxide inclusions during isothermal heating of 18Cr–8Ni stainless steel with yttrium addition at temperatures of 1273 to 1573 K was investigated *** spherical Al–Y–Si(–Mn–Cr)oxide inclusions were observed in as-cast *** heating,most of the homogeneous inclusions were transformed into heterogeneous inclusions with Y-rich and Al-rich parts,even though some homogeneous oxide particles were still observed at 1273 and 1573 *** the increase in heating temperature,more large-sized inclusions were *** shape of the inclusions also changed from spherical to *** maximum transformation temperature of inclusions was determined to be 1373 *** evolution mechanism of inclusions during heating was proposed to be the combined effect of the(i)internal transformation of inclusions due to the crystallization of glassy oxide and(ii)interfacial reaction between inclusions and steel ***,the internal transformation of inclusions was considered to be the main factor at heating temperatures less than 1473 K.

关键词： stainless steel rare earth metals oxide inclusions heating temperature

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

Interfacial reaction between oxide inclusion and steel matrix deoxidized by Si and Mn at 1473 K

引用

Journal of Iron and Steel Research International 2018年第1期25卷 1-8页

作者： xue-liang zhang Shu-feng Yang Cheng-song Liu Jing-she Li Qing Liu Gang Liu School of Metallurgical and Ecological Engineering University of Science and Technology BeijingBeijing 100083 China Beijing Key Laboratory of Special Melting and Preparationof High-End Metals Beijing 100083 China The State Key Laboratory of Refractories and MetallurgyWuhan University of Science and Technology Wuhan 430081 Hubei China

An improved diffusion couple method was used to simulate the dynamic process of the solid-state reaction at the interface between oxide inclusions and a steel matrix deoxidized by Si and Mn during heat treatment at 1473 K. Experimental results indicated that good contact between the oxide and steel matrix was attained after pre-treatment at 1673 K. In addition, the reaction between the oxide and steel matrix at 1673 K was suppressed, and the effect of this reaction on the diffusion couple experiments at 1473 K was minimized. In the diffusion couple experiments, the diffusion of oxygen from the oxide to the steel matrix resulted in the precipitation of fine oxide particles and a decrease in the Mn content in the steel matrix near the interface after heat treatment at 1473 K. With increasing heat treatment time, the widths of the particle precipitation zone （PPZ） and Mn-depleted zone （MDZ） gradually increased. In addition, the solid-state reaction at the interface between the oxide and steel matrix was intense, and the widths of the PPZ and MDZ increased rapidly during the 0-20 h stage of heat treatment, especially during the 0-5 h stage. The interfacial reaction was retarded, and the rates of width expansion of PPZ and MDZ decreased with increasing heat treatment time.

关键词： Oxide inclusion Diffusion couple Heat treatment Solid-state reaction Interfacial reaction

来源：

维普期刊数据库评论

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

A stable implicit nodal integration-based particle finite element method(N-PFEM)for modelling saturated soil dynamics

引用

Journal of Rock Mechanics and Geotechnical Engineering 2024年第6期16卷 2172-2183页

作者： liang Wang xue zhang Jingjing Meng Qinghua Lei Department of Earth Sciences ETH ZürichZürich8092Switzerland Department of Civil Engineering and Industrial Design University of LiverpoolLiverpoolL693BXUK Department of Civil Environmental and Natural Resources EngineeringLuleåUniversity of TechnologyLuleå97187Sweden Department of Earth Sciences Uppsala UniversityUppsala75105Sweden

In this study,we present a novel nodal integration-based particle finite element method(N-PFEM)designed for the dynamic analysis of saturated *** approach incorporates the nodal integration technique into a generalised Hellinger-Reissner(HR)variational principle,creating an implicit PFEM *** mitigate the volumetric locking issue in low-order elements,we employ a node-based strain smoothing *** discretising field variables at the centre of smoothing cells,we achieve nodal integration over cells,eliminating the need for sophisticated mapping operations after re-meshing in the *** express the discretised governing equations as a min-max optimisation problem,which is further reformulated as a standard second-order cone programming(SOCP)***,pore water pressure,and displacements are simultaneously determined using the advanced primal-dual interior point ***,our numerical model offers improved accuracy for stresses and pore water pressure compared to the displacement-based PFEM *** experiments demonstrate that the N-PFEM efficiently captures both transient and long-term hydro-mechanical behaviour of saturated soils with high accuracy,obviating the need for stabilisation or regularisation techniques commonly employed in other nodal integration-based PFEM *** work holds significant implications for the development of robust and accurate numerical tools for studying saturated soil dynamics.

关键词： Particle finite element method Nodal integration Dynamic saturated media Second-order cone programming(SOCP)

来源：

维普期刊数据库评论

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Combining unscented Kalman filter and wavelet neural network for anti-slug

引用

Petroleum Science 2023年第6期20卷 3752-3765页

作者： Chuan Wang Long Chen Lei Li Yong-Hong Yan Juan Sun Chao Yu Xin Deng Chun-Ping liang xue-liang zhang Wei-Ming Peng School of Mechanical Engineering Southwest Petroleum UniversityChengdu610500SichuanChina Energy Equipment Institute Southwest Petroleum UniversityChengdu610500SichuanChina CNPC National Engineering Research Center for Oil and Gas Drilling Equipment Co.LTD Baoji721000ShaanxiChina Oil Production Service Co. CETS LTD.Tianjin300000China

The stability of the subsea oil and gas production system is heavily influenced by slug flow. One successful method of managing slug flow is to use top valve control based on subsea pipeline pressure. However, the complexity of production makes it difficult to measure the pressure of subsea pipelines, and measured values are not always accessible in real-time. The research introduces a technique for integrating Unscented Kalman Filter (UKF) and Wavelet Neural Network (WNN) to estimate the state of subsea pipeline pressure using historical data and a state model. The proposed method treats multiphase flow transport as a nonlinear model, with a dynamic WNN serving as the state observer. To achieve real-time state estimation, the WNN is included into the UKF algorithm to create a WNN-based UKF state equation. Integrate WNN and UKF in a novel way to predict system state accurately. The simulated results show that the approach can efficiently predict the inlet pressure and manage the slug flow in real-time using the riser's top pressure, outlet flow and valve opening. This method of estimate can significantly increase the control effect.

关键词： State estimation Stable control Method fusion Wavelet neural network Unscented Kalman filter

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

Fully sprayed MXene-based high-performance flexible piezoresistive sensor for image recognition

引用

Nano Materials Science 2024年第1期6卷 77-85页

作者： Zhi-Dong zhang xue-Feng Zhao Qing-Chao zhang Jie liang Hui-Nan zhang Tian-Sheng zhang Chen-Yang xue Key Laboratory of Instrumentation Science&Dynamic Measurement of Ministry of Education North University of ChinaTaiyuan030051People's Republic of China State Key Laboratory of ASIC and System Shanghai Institute of Intelligent Electronics&SystemsSchool of MicroelectronicsFudan UniversityShanghai200433People's Republic of China Shanxi Hosipital of Acupuncture and Moxibustion Taiyuan030006People's Republic of China

High-performance flexible pressure sensors provide comprehensive tactile perception and are applied in human activity monitoring,soft robotics,medical treatment,and human-computer ***,these flexible pressure sensors require extensive nano-architectural design and complicated manufacturing and are ***,a highly sensitive,flexible piezoresistive tactile sensor is designed and fabricated,consisting of three main parts:the randomly distributed microstructure on T-ZnOw/PDMS film as a top substrate,multilayer Ti_(3)C_(2)-MXene film as an intermediate conductive filler,and the few-layer Ti_(3)C_(2)-MXene nanosheetbased interdigital electrodes as the bottom *** MXene-based piezoresistive sensor with randomly distributed microstructure exhibits a high sensitivity over a broad pressure range(less than 10 kPa for 175 kPa^(-1))and possesses an out-standing permanence of up to 5000 ***,a 16-pixel sensor array is designed,and its potential applications in visualizing pressure distribution and an example of tactile feedback are *** fully sprayed MXene-based pressure sensor,with high sensitivity and excellent durability,can be widely used in,electronic skin,intelligent robots,and many other emerging technologies.

关键词： Piezoresistive sensor Ti_(3)C_(2)-MXene T-ZnOw/PDMS film Randomly distributed microstructure

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

LAGRANGE REPRESENTATION OF MULTIVARIATE INTERPOLATION

引用

Science China Mathematics 1989年第4期32卷 385-396页

作者：梁学章 Institute of Mathematics Jilin University Changchun.

This paper gives a set of linearly independent interpolating functionals and a correspon-ding set of fundamental Lagrange polynomials for the multivariate extension (the liftedmultivariate map) of univariate generaliz... 详细信息

关键词： multivariate extension interpolation properly posed set of nodes Lagrange representation.

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

Engineering of geometrical configurations in dual-atom catalysts for electrocatalytic applications

引用

Journal of Energy Chemistry 2024年第7期94卷 273-287页

作者： Tao zhang Yifan Liu liang xue Jingwen Sun Pan Xiong Junwu Zhu Key Laboratory for Soft Chemistry and Functional Materials of Ministry Education School of Chemistry and Chemical EngineeringNanjing University of Science and TechnologyNanjing210094JiangsuChina

Geometrical configurations play a crucial role in dual-atom catalysts(DACs)for electrocatalytic *** progress has been made to design DACs electrocatalysts with various geometri-cal configurations,but in-depth understanding the relationship between geometrical configurations and metal-metal interaction mechanisms for designing targeted DACs is still *** this review,the recent progress in engineering of geometrical configurations of DACs is systematically *** on the polarity of geometrical configuration,DACs can be classified into two different types that are homonuclear and heteronuclear ***,with regard to the geometrical configurations of the active sites,homonuclear DACs are identified into adjacent and bridged configurations,and heteronuclear DACs can be classified into adjacent,bridged,and separated ***,metal-metal interactions in DACs with different geometrical configurations are ***,the applications of DACs in different electrocatalytic reactions are discussed,including the oxygen reduction reaction(ORR),oxygen evolution reaction(OER),hydrogen evolution reaction(HER),and other ***,the future challenges and perspectives for advancements in DACs are *** review aims to provide inspiration for the design of highly effcient DACs towards energy relatedapplications.

关键词： Dual-atom catalysts Geometrical configurations Homonuclear Heteronuclear Electrocatalysis

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

Surface Reconstruction of 3D Scattered Data with Radial Basis Functions

引用

Communications in Mathematical Research 2010年第2期26卷 183-192页

作者： Du XIN-WEI YANG XIAO-YING liang xue-zhang School of Mathematics Jilin University Changchun 130012 College of Mathematics Changchun University of Technology Changchun 130021

We use Radial Basis Functions （RBFs） to reconstruct smooth surfaces from 3D scattered data. An object＇s surface is defined implicitly as the zero set of an RBF fitted to the given surface data. We propose improvements on the methods of surface reconstruction with radial basis functions. A sparse approximation set of scattered data is constructed by reducing the number of interpolating points on the surface. We present an adaptive method for finding the off-surface normal points. The order of the equation decreases greatly as the number of the off-surface constraints reduces gradually. Experimental results are provided to illustrate that the proposed method is robust and may draw beautiful graphics.

关键词： radial basis function scattered data implicit surface surface reconstruction

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

欢迎您,

建议与咨询留下您的常用邮箱和电话号码，以便我们向您反馈解决方案和替代方法

时间限定

文献类型

馆藏选择

核心期刊

语言

文献类型

帮助

文字说明：

检索规则说明：

检索范例：

分类表

所选分类

限定检索结果

文献类型

馆藏范围

日期分布

学科分类号

主题

机构

作者

语言

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

请选择保存的检索档案：

请选择收藏分类：

通借通还

欢迎您,

建议与咨询 留下您的常用邮箱和电话号码，以便我们向您反馈解决方案和替代方法

时间限定

文献类型

馆藏选择

核心期刊

语言

文献类型

帮助

文字说明：

检索规则说明：

检索范例：

分类表

所选分类

限定检索结果

文献类型

馆藏范围

日期分布

学科分类号

主题

机构

作者

语言

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

请选择保存的检索档案： 新增检索档案 确定 取消

请选择收藏分类： 新增自定义分类 确定 取消

通借通还

建议与咨询留下您的常用邮箱和电话号码，以便我们向您反馈解决方案和替代方法

请选择保存的检索档案：

请选择收藏分类：