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Extending homogeneous fluidization flow regime of Geldart-A particles by exerting axial uniform and steady magnetic field

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Chinese Journal of Chemical Engineering 2024年第1期65卷 169-177页

作者： qiang Zhang Wankun liu Hengjun Gai Quanhong Zhu College of Chemical Engineering Qingdao University of Science and TechnologyQingdao 266042China School of Chemical&Environmental Engineering China University of Mining&Technology-BeijingBeijing 100083China

The homogeneous/particulate fluidization flow regime is particularly suitable for handling the various gas–solid contact processes encountered in the chemical and energy *** work aimed to extend such a regime of Geldart-A particles by exerting the axial uniform and steady magnetic *** the action of the magnetic field,the overall homogeneous fluidization regime of Geldart-A magnetizable particles became composed of two parts:inherent homogeneous fluidization and newly-created magnetic *** the former remained almost unchanged whereas the latter became broader as the magnetic field intensity increased,the overall homogeneous fluidization regime could be extended *** for Geldart-A nonmagnetizable particles,certain amount of magnetizable particles had to be premixed to transmit the magnetic *** others,the mere addition of magnetizable particles could broaden the homogeneous fluidization *** added content of magnetizable particles had an optimal value with smaller/lighter ones working *** added magnetizable particles might raise the ratio between the interparticle force and the particle *** the magnetic field was exerted,the homogeneous fluidization regime was further expanded due to the formation of magnetic stabilization flow *** more the added magnetizable particles,the better the magnetic performance and the broader the overall homogeneous fluidization ***/lighter magnetizable particles were preferred to maximize the magnetic performance and extend the overall homogeneous fluidization *** phenomenon could be ascribed to that the added magnetizable particles themselves became more Geldart-A than-B type as their density or size decreased.

关键词： Fluidized-bed Fluidization Geldart-A particles Flow regimes Extend Magnetic stabilization

Cation-Dipole Interaction-Induced Coacervate Underwater Adhesives in Natural Seawater

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Chinese Journal of Polymer Science 2024年第7期42卷 984-991,I0009页

作者： Xu-Fei liu Chong-Rui Zhang Hua-Wen Peng qiang Zhao Key Laboratory of Material Chemistry for Energy Conversion and Storage Ministry of EducationSchool of Chemistry and Chemical EngineeringHuazhong University of Science and TechnologyWuhan430074China

Significant progress has been made in wet adhesives for low salinity water,but exploration of general ionic adhesives for natural seawater is less developed because the high salinity could weaken interfacial bonding and shields electrostatic interactions,resulting in adhesion ***,the design of adhesives for natural seawater represents challenges less ***,a cationic polyelectrolyte(PECHIA)containing imidazolacetonitrile unit was explored to prepare adhesives enabled by natural *** combining the ion shielding effect with the“cation-dipole”interactions between PECHIA chains,aqueous solution of the PECHIA underwent coacervation and self-crosslinking in natural seawater,allowing for underwater adhesion to various substrates in *** instantaneous lap-shear and tensile adhesion strengths are 47 and 119 kPa,respectively,while the cured adhesive shows~739 k Pa tensile adhesion in natural *** design of PECHIA enables wet adhesives viable for applications in the diversified scenarios of natural seawater.

关键词： Coacervate Underwater adhesives Seawater Cation-dipole interaction

Genome-Wide Characterization of the Hyaluronidase Gene Family and Their Potential Roles in Viviparous Black Rockfish(Sebastes schlegeli)

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Journal of Ocean University of China 2024年第2期23卷 487-498页

作者： liu Zhiying NIU Jingning ZHAO xi liu Huaxiang LI Zibin HE Yan QI Jie MOE Key Laboratory of Marine Genetics and Breeding College of Marine Life SciencesOcean University of ChinaQingdao 266003China Key Laboratory of Tropical Aquatic Germplasm of Hainan Province Sanya Oceanographic InstituteOcean University of ChinaSanya 572025China

Black rockfish(Sebastes schlegelii)has evolved viviparous reproduction *** from the oviparous fishes,the spermatozoa of black rockfish are stored on the surface of ovarian follicle for over four months until the egg mature in ovary,while the adaptive evolution of fertilization-related genes remains to be *** the present study,based on the genome and transcriptome information of black rockfish,a total of 10 hyaluronidase genes were identified by phylogenetic and sequence analyses,including hyal1,hyal2,hyal3,hyal4,hyal6 and spam1a,spam1b,spam1c and *** spam1 subfamilies,including spam1a,spam1b,spam1c and spam1d,were significantly expanded compared to other *** adaptive evolution of hyaluronidase was further investigated by selection pressure analysis of branch model and branch site *** results showed that only spam1 subfamily was positively selected with a large number of positive selection sites,and the evolution rate was significantly higher thanthose of other *** positively selected sites,LYS-171 and GLY-164,were located in the neutral hyaluronidase activity domain,which was pivotal for SPAM1 to participate in enzymatic hydrolysis of the extracellular hyaluronic acid matrix and mediate acrosome reaction in ***,spam1 was mainly expressed in spermatocytes,secondary spermatocytes,and spermatids of testis,whereas it was not found in metamorphic sperm and mature sperm based on the spatiotemporal expression *** results indicated that spam1 might originate from the testis and might be an adaptation of viviparous trait in black rockfish.

关键词： adaptation of viviparous black rockfish(Sebastes schlegelii) hyaluronidase selective pressure analysis

Physics-data coupling-driven method to predict the penetration depth into concrete targets

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Theoretical & Applied Mechanics Letters 2024年第3期14卷 184-192页

作者： Shuai Qin Hao liu Jianhui Wang qiang Zhao Lei Zhang Institute of Defense Engineering AMSLuoyang 471000China Harbin Engineering University Harbin 150001China

The projectile penetration process into concrete target is a nonlinear complex *** the increase ofexperiment data,the data-driven paradigm has exhibited a new feasible method to solve such complex ***,due to poor quality of experimental data,the traditional machine learning(ML)methods,whichare driven only by experimental data,have poor generalization capabilities and limited prediction ***,this study intends to exhibit a ML method fusing the prior knowledge with experiment *** newML method can constrain the fitting to experimental data,improve the generalization ability and the predic-tion *** results show that integrating domain prior knowledge can effectively improve theperformance of the prediction model for penetration depth into concrete targets.

关键词： Penetration into concrete Artificial neural networks Prior knowledge fusion Prediction model

Distribution, bioaccumulation, trophic transfer and risk assessment of trace elements in fish from a typical shallow outflow lake basin, China

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Frontiers of Environmental Science & Engineering 2024年第7期18卷 141-156页

作者： Miao He Guijian liu xiaodan Shi Lei Wu qiang Chen CAS Key Laboratory of Crust-Mantle Materials and Environment School of Earth and Space SciencesUniversity of Science and Technology of ChinaHefei 230026China Anhui Academy of Environmental Sciences Hefei 230022China School of Resources and Environmental Engineering Hefei University of TechnologyHefei 230009China

Fish are important food sources for humans,and the availability of appropriate amount of trace elements(TEs)plays a crucial role in fish ***,due to large volumes of sewage discharge,high levels of certain elements are present in aquatic environments,and these elements accumulate in fish and potentially affect human *** this study,the distribution and bioaccumulation capacity of trace elements in six dominant fish species from Chaohu Lake(China)were *** results showed that the bioaccumulation capacity of fish for Zn was greater than other *** the source of the TEs in the fish were explored along with the concentration of the TEs in the aquatic environment,which indicated that TEs in fish were mainly obtained through ingestion and indirectly affected by the industrial activities in the ***,stable carbon and nitrogen isotopes were used to classify the trophic levels and explore the biological magnification of TEs of the *** was found that Sb and Sr showed biomagnification with the increase of trophic level of *** on the above analyses,the environmental biogeochemical cycle model of TEs in the lake was distinguished and established,which can offer valuable insights for sustainable fishery management in the downstream Yangtze River Delta ecosystem.

关键词： Trophic level Bioaccumulation Risk assessment Trace elements

Predicting carbon storage of mixed broadleaf forests based on the finite mixture model incorporating stand factors,site quality,and aridity index

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Forest Ecosystems 2024年第3期11卷 276-286页

作者： Yanlin Wang Dongzhi Wang Dongyan Zhang qiang liu Yongning Li College of Forestry Hebei Agricultural UniversityBaoding071001China College of Economics and Management Hebei Agricultural UniversityBaoding071001China

The diameter distribution function(DDF)is a crucial tool for accurately predicting stand carbon storage(CS).The current key issue,however,is how to construct a high-precision DDF based on stand factors,site quality,and aridity index to predict stand CS in multi-species mixed forests with complex *** study used data from70 survey plots for mixed broadleaf Populus davidiana and Betula platyphylla forests in the Mulan Rangeland State Forest,Hebei Province,China,to construct the DDF based on maximum likelihood estimation and finite mixture model(FMM).Ordinary least squares(OLS),linear seemingly unrelated regression(LSUR),and back propagation neural network(BPNN)were used to investigate the influences of stand factors,site quality,and aridity index on the shape and scale parameters of DDF and predicted stand CS of mixed broadleaf *** results showed that FMM accurately described the stand-level diameter distribution of the mixed *** and *** forests;whereas the Weibull function constructed by MLE was more accurate in describing species-level diameter *** combined variable of quadratic mean diameter(Dq),stand basal area(BA),and site quality improved the accuracy of the shape parameter models of FMM;the combined variable of Dq,BA,and De Martonne aridity index improved the accuracy of the scale parameter *** to OLS and LSUR,the BPNN had higher accuracy in the re-parameterization process of ***,LSUR,and BPNN overestimated the CS of *** but underestimated the CS of *** in the large diameter classes(DBH≥18 cm).BPNN accurately estimated stand-and species-level CS,but it was more suitable for estimating stand-level CS compared to species-level CS,thereby providing a scientific basis for the optimization of stand structure and assessment of carbon sequestration capacity in mixed broadleaf forests.

关键词： Weibull function Finite mixture model Linear seemingly unrelated regression Back propagation neural network Carbon storage

Heteroatom anchors Fe-Mn dual-atom catalysts with bi-functional oxygen catalytic activity for low-temperature rechargeable flexible Zn-air batteries

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Journal of Energy Chemistry 2024年第3期90卷 610-620,I0014页

作者： Yuting He Hongtao Li Yi Wang Yufei Jia Yongning liu qiang Tan State Key Laboratory for Mechanical Behaviour of Materials School of Materials Science&EngineeringXi’an Jiaotong UniversityXi’an 710049ShaanxiChina

M-N-C(M=Fe,Co,Ni,etc.) catalyst owns high catalytic activity in the oxygen catalytic reaction which is the most likely to replace the Pt-based *** it is still a challenge to further increase the active site *** article constructs the high-efficiency FeMn-N/S-C-1000 catalyst to realize ORR/OER bifunctional catalysis by hetero-atom,bimetal(Fe,Mn) doped simultaneously *** evaluated it as bi-functional electro-catalysts,FeMn-N/S-C-1000 exhibits excellent catalytic activity(E_(1/2)=0.924 V,E_(j=10)=1.617 V) in alkaline media,outperforms conventional Pt/C,RuO_(2) and most non-precious-metal catalysts reported recently,Such outstanding performance is owing to N,S co-coordinated with metal to form multi-types of single atom,dual atom active sites to carry out ***,nitrite poison test provides the proof that the active sites of FeMn-N/S-C are more than that of single-atom catalysts to promote catalytic reactions *** better understand the local structure of Fe and Mn active sites,XAS and DFT were employed to reveal that FeMn-N_5/S-C site plays the key role during ***,the FeMn-N/S-C-1000 based low-temperature rechargeable flexible Zn-air also exhibits superior discharge performance and extraordinary durability at-40℃.This work will provide a new idea to design diatomic catalysts applied in low-temperature rechargeable batteries.

关键词： Fe Mn-N/S-C-1000 ORR OER Rechargeable flexible Zn-air batteries

Liquid metal droplet dynamics

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Droplet 2024年第1期3卷 61-94页

作者： xi Zhao Mengwen Qiao Yingxin Zhou Jing liu Key Laboratory of Cryogenics Technical Institute of Physics and ChemistryChinese Academy of SciencesBeijingChina School of Future Technology University of Chinese Academy of SciencesBeijingChina Department of Biomedical Engineering School of MedicineTsinghua UniversityBeijingChina

The unique properties to combine the dual merits of both liquids and metals together make the gallium‐based liquid metal(LM)droplets a class of unconventional substitute which possess great potential for a group of newly emerging areas,such as stretchable electronics,soft devices,micro sensors and *** addition,LM droplets are undoubtedly an intriguing target worth of pursuing in fundamental hydrodynamic investigations due to their extremely high surface tension nature compared to classical nonmetallic *** the discovery of the diverse transformation phenomena and self‐fueled droplet mollusks of LM that can move automatically in solution via single electricity or even without any external energy supply,tremendous attentions were attracted to this special fluidic object of LM *** the past decade,there has been a proliferation of explorations on LM droplet dynamics,while the involved contents are heterogeneous due to the interfacial physical/chemical activity of the LM and the diversity of the kinetic *** better understand and manipulate the droplet behavior and to promote further development of the LMs,this review is dedicated to summarize the latest progress and presents an overview on basic findings related to LM macrodroplet ***,the extended definition of LM droplets and the corresponding fabrication methods are ***,typical works on LM droplet dynamics are systematically interpreted based on their different behavior ***,the perspectives,main obstacles and challenges restricting the development of LM droplet dynamics are pointed out.

关键词： dynamics behavior doubt

A comparative study on mechanical and vibroacoustic performance of sandwich cylindrical shells with positive,negative,and zero Poisson’s ratio cellular cores

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Journal of Ocean Engineering and Science 2024年第4期9卷 379-390页

作者： Qing Li Peichang Li Yongjin Guo xi’an liu State Key Laboratory of Ocean Engineering Shanghai Jiao Tong UniversityShanghai200240China China Ship Development and Design Center Wuhan430064China MOE Key Laboratory of Marine Intelligent Equipment and System Shanghai Jiao Tong UniversityShanghai200240China

Deep-sea submersibles are significant mobile platforms requiring multi-functional capabilities that are strongly determined by the constituent *** cylindrical protective cover can be advanced by designing their sandwiched cellular materials whose physical properties can be readily parameterized and flexibly *** honeycomb materials are capable of possessing tuned positive,negative,or zero Poisson’s ratios(PPR,NPR,and ZPR),which is expected to produce distinct physical performance when utilized as a cellular core of cylindrical shells for the deep-sea submersibles.A novel cylindrical meta-structure sandwiched with the semi-re-entrant ZPR metamaterial has been designed as well as its similarly-shaped sandwich cylindrical shell structures with PPR and NPR *** mechanical and vibroacoustic performance of sandwich cylindrical shells with cellular materials featuring a full characteristic range of Poisson’s ratios are then compared systematically to explore their potential for engineering applications on submerged pressure-resistant *** respective unit cells are designed to feature an equivalent load-bearing *** properties of pressure resistance,buckling,and sound insulation are simulated,respectively,and the orders of each property are then generalized by systematic *** results indicate that the PPR honeycomb core takes advantage of higher structural strength and stability while the ZPR one yields better energy absorption and sound insulation *** NPR one yields moderate properties and has the potential for lower circumferential *** work explores the application of cellular materials with varied Poisson’s ratios and provides guidance for the multi-functional design of sandwich cylindrical meta-structures.

关键词： Sandwich cylindrical shells Poisson’s ratio Pressure-resistant Buckling Vibroacoustic