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Investigation on UV-curing Reprocessable Thermosets Bearing Hindered Urea Bonds and Their Composites with Modified Zinc Oxide Nanoparticles

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Chinese Journal of Polymer Science 2024年第6期42卷 751-765页

作者： jun-Hao Zhou li-Ming Tang Key Laboratory of Advanced Materials of Ministry of Education of China Department of Chemical EngineeringTsinghua UniversityBeijing100084China

In this study,a series of hindered urea bond(HUB)containing polyurethane-urea methacrylate prepolymers and a none HUB containing polyurethane methacrylate prepolymer were prepared using isobornyl methacrylate as the reactive diluent via one-pot *** prepolymers were characterized fully by various ***,their thermosets were fabricated via UV curing in presence of a photo initiator,and their mechanical property and thermal behavior were investigated and *** from the none HUB containing thermoset,the HUB containing thermosets(defined as PUT)could be recycled and reprocessed by hot press under relatively mild conditions with high recovery ratio of mechanical ***,zinc oxide(ZnO)nanoparticles were modified with 3-(trimethoxysilyl)propyl methacrylate and the modified ZnO(defined as ZnO-TPM)was dispersed and polymerized into PUT matrix to prepare their *** influence of ZnO-TPM on the mechanical performance of the composites was evaluated,which indicated that the Young’s modulus and tensile strength increased gradually to the maximum values at ZnO-TPM content of 1 wt%and then *** composites also displayed good reprocessability with improved recovery ratio compared to the pure PUT *** addition,the composite materials exhibited strong UV absorption capacity,implying their potential application in the circumstance where UV-shielding was required.

关键词： Polyurethane-urea methacrylate Hindered urea bond ZnO nanoparticles Reprocessing UV curing

Multiple Matching Attenuation Based on Curvelet Domain Extended Filtering

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Journal of Ocean University of China 2024年第4期23卷 924-932页

作者： HUA Qingfeng CheN Zhang he Huili TAN jun CheN Haifeng li Guanbao SONG Peng ZHAO Bo JIANG Xiuping Key Laboratory of Marine Geology and Metallogeny First Institute of OceanographyMinistry of Natural ResourcesQingdao 266061China Laboratory for Marine Mineral Resources Qingdao Marine Science and Technology CenterQingdao 266237China College of Marine Geoscience Ocean University of ChinaQingdao 266100China BGP Inc. China National Petroleum CorporationZhuozhou 072750China Key Laboratory of Submarine Geosciences and Prospecting Techniques Ministry of EducationQingdao 266100China

The paper develops a multiple matching attenuation method based on extended filtering in the curvelet domain,which combines the traditional Wiener filtering method with the matching attenuation method in curvelet ***,the method uses the predicted multiple data to generate the Hilbert transform records,time derivative records and time derivative records of Hilbert ***,the above records are transformed into the curvelet domain and multiple matching attenuation based on least squares extended filtering is ***,the attenuation results are transformed back into the time-space *** on the model data and field data show that the method proposed in the paper effectively suppress the multiples while preserving the primaries ***,it has higher accuracy in eliminating multiple reflections,which is more suitable for the multiple attenuation tasks in the areas with complex structures compared to the time-space domain extended filtering method and the conventional curvelet transform method.

关键词： multiple matching attenuation curvelet domain extended filtering

Unraveling the hydrothermal history of the Xinshuijing Na-metasomatite uranium deposit in the Longshoushan metallogenic belt， Northwest China by coupled hydrothermal zircon U–Pb and albite Ar–Ar dating

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Journal of Earth Science 2024年

作者： jun ZHONG MARK MIHALASKY MICheL CUNEY SheNG he jun-JIE li National Key Laboratory of Uranium Resource Exploration-Mining and Nuclear Remote Sensing， Beijing Research Institute of Uranium Geology International Atomic Energy Agency (IAEA)， Nuclear Fuel Cycle and Materials Section， Division of Nuclear Fuel Cycle and Waste Technology， Vienna International Center Université de Lorraine， GéoRessources CNRS State Key Laboratory of lithospheric Evolution (SKLLE)， Institute of Geology and Geophysics， Chinese Academy of Sciences

Na-metasomatite uranium deposits are an important type of large-tonnage low-grade uranium deposit. They are characterized by an intimate association between uranium minerals and albite， and by the common development of syn-ore hydrothermal zircons. Similar to other types of uranium deposits， constraining an accurate age of mineralization remains a challenge for the Na-metasomatite type ones. In this study， we present for the first time， an approach that combines age dating results from the syn-ore albites (40Ar-39Ar) and hydrothermal zircons （U-Pb） for a typical Na-metasomatite uranium deposit， the Xinshuijing deposit in the Longshoushan metallogenic belt of northwest China. The hydrothermal zircon U-Pb and albite40Ar-39Ar ages are consistent with each other （378-366 Ma; within error）， but also identical to the previously reported uraninite chemical U-Pb ages （approximately 370 Ma）. The coupled application of hydrothermal zircon U-Pb and albite40Ar-39Ar age dating is thus regarded as a robust approach for constraining the age of mineralization for Na-metasomatite uranium deposits. An age gap of approximately 70 m.y. between uranium mineralization （～ 370 Ma） and host granitoid emplacement （about 440 Ma） suggests no direct genetic linkage between the two. Further exploration in the surrounding metamorphic units is therefore suggested， rather than only focusing on the host granitoids， especially where intensive wallrock alteration and structural features are pervasive. The varied hydrothermal zircon δ18O isotope compositions are attributed to the significant fluid-wallrock interaction during the uranium mineralization， which is consistent with our previous fluid inclusion and geochemical studies. Our study highlights the importance of selecting appropriate isotopic dating methods， which is informed by detailed paragenetic and geochemical analysis of dateable minerals formed before or coeval to the main-stage uranium mineralization. Moreover， it is underlined that the e

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Enriched electrophilic oxygen species facilitate acidic oxygen evolution on Ru-Mo binary oxide catalysts

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Nano Research 2024年第3期17卷 1165-1172页

作者： Yaya Wang Yunzhou Wen Yumeng Cheng Xinhong Chen Mengjiao Zhuansun Tongbao Wang jun li Debora Meira Huarui Sun jun Wei Jia Zhou Yuhang Wang Sisi he Shenzhen Key Laboratory of Flexible Printed Electronics Technology Harbin Institute of Technology(Shenzhen)University TownShenzhen 518055China School of Science Harbin Institute of Technology(Shenzhen)University TownShenzhen 518055China Institute of Functional Nano&Soft Materials(FUNSOM) Jiangsu Key Laboratory of Advanced Negative Carbon TechnologiesSoochow UniversitySuzhou 215123China Frontiers Science Center for Transformative Molecules Shanghai Jiao Tong UniversityShanghai 200240China Science Division Canadian Light SourceSaskatoonSKS7N 2V3Canada Photon Science Division Argonne National LaboratoryLemontIL60439USA School of Materials Science and Engineering Harbin Institute of Technology(Shenzhen)University TownShenzhen 518055China

The polymer electrolyte membrane(PEM)electrolyzers are burdened with costly iridium(Ir)-based catalysts and high operation overpotentials for the oxygen evolution reaction(OER).The development of earth-abundant,highly active,and durable electrocatalysts to replace Ir is a critical step in reducing the cost of green hydrogen *** we develop a Ru5Mo4Ox binary oxide catalyst that exhibits high activity and stability in acidic *** electron-withdrawing property of Mo enriches the electrophilic surface oxygen species,which promotes acidic OER to proceed via the adsorbate evolution *** a result,we achieve a 189 mV overpotential at 10 mA·cm^(-2) and a Tafel slope of 48.8 mV·dec^(-1).Our catalyst demonstrates a substantial 18-fold increase in intrinsic activity,as evaluated by turnover frequency,compared to commercially available RuO_(2) and IrO_(2) ***,we report a stable OER operation at 10 mA·cm^(-2) for 100 h with a low degradation rate of 2.05 mV·h^(-1).

关键词： electrocatalysis oxygen evolution reaction(OER) ruthenium(Ru)-based oxide molybdenum electrophilic oxygen

Prediction models of burst strength degradation for casing with considerations of both wear and corrosion

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Petroleum Science 2024年第1期21卷 458-474页

作者： Jie-li Wang Wen-jun Huang De-li Gao MOE Key Laboratory of Petroleum Engineering China University of PetroleumBeijing102249China State Key Laboratory of Petroleum Resources and Prospecting China University of PetroleumBeijing102249China

Casing wear and casing corrosion are serious problems affecting casing integrity failure in deep and ultra-deep *** paper aims to predict the casing burst strength with considerations of both wear and ***,the crescent wear shape is simplified into three categories according to common mathematical ***,based on the mechano-electrochemical(M-E)interaction,the prediction model of corrosion depth is built with worn depth as the initial condition,and the prediction models of burst strength of the worn casing and corroded casing are ***,the accuracy of different prediction models is validated by numerical simulation,and the main influence factors on casing strength are *** last,the theoretical models are applied to an ultra-deep well in Northwest China,and the dangerous well sections caused by wear and corrosion are predicted,and the corrosion rate threshold to ensure the safety of casing is *** results show that the existence of wear defects results in a stress concentration and enhanced M-E interaction on corrosion depth *** accuracy of different mathematical models is different:the slot ring model is most accurate for predicting corrosion depth,and the eccentric model is most accurate for predicting the burst strength of corroded *** burst strength of the casing will be overestimated by more than one-third if the M-E interaction is neglected,so the coupling effect of wear and corrosion should be sufficiently considered in casing integrity evaluation.

关键词： Deep well Casing integrity Casing wear Casing corrosion Burst strength

Low-protein diet supplemented with 1% L-glutamine improves growth performance, serum biochemistry, redox status, plasma amino acids, and alters fecal microbiota in weaned piglets

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Animal Nutrition 2024年第2期17卷 144-154页

作者： jun li jun Bai Ying Yang Zhenlong Wu State Key Laboratory of Animal Nutrition and Feeding Department of Companion Animal Science China Agricultural University

Glutamine, one of the most abundant amino acids in the body, has been shown to exert various beneficial effects in pigs. However, knowledge regarding the role of dietary glutamine in low-protein diet-fed piglets remains scarce. The present study aimed to investigate the effects of different levels of L-glutamine on growth performance, serum biochemistry parameters, redox status, amino acids, and fecal microbiota in low-protein diet-fed piglets. A total of 128 healthy crossbred piglets(Landrace × Yorkshire)were randomly allocated into 4 groups of 4 replicate pens, with 8 piglets per pen. Piglets in the 4 groups were fed with corn and soybean meal-based low-protein diets(crude protein level, 17%) that contained0%, 1%, 2%, and 3% L-glutamine, respectively, for 28 d. Pigs administered 1% L-glutamine had greater body weight on d 28 and average daily gain(ADG, P hereas a lower feed to gain ratio(F:G) from d 1to 28(P he other three groups. Besides, lower body weight on d 14 and 28, ADG,average daily feed intake, and higher F:G from d 15 to 28 and d 1 to 28 were observed in response to 2%and 3% L-glutamine treatments than 0% and 1% L-glutamine treatments(P her investigation revealed that 1% L-glutamine upregulated the serum glutamine, lysine, methionine, tyrosine, and reduced plasma valine content(P he abundance of p＿75＿a5, Clostridium, Lactobacillus, Prevotellaceae＿Prevotella,and Gemmiger in the stool of piglets on d 14, with the Streptococcus lev

关键词： Glutamine Low protein diet Pig Redox status Amino acid Microbiota

Computed tomography-based radiomics combined with machine learning allows differentiation between primary intestinal lymphoma and Crohn's disease

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World Journal of Gastroenterology 2024年第25期30卷 3155-3165页

作者： Meng-jun Xiao Yu-Teng Pan Jia-he Tan Hai-Ou li Hai-Yan Wang Department of Radiology Shandong Provincial Hospital Affiliated to Shandong First Medical UniversityJinan 250021Shandong ProvinceChina Medical Science and Technology Innovation Center Shandong First Medical University&Shandong Academy of Medical SciencesJinan 250000Shandong ProvinceChina University of California DavisCA 95616United States Qilu Hospital Cheeloo College of MedicineShandong UniversityJinan 250012Shandong ProvinceChina

BACKGROUND Due to similar clinical manifestations and imaging signs,differential diagnosis of primary intestinal lymphoma(PIL)and Crohn's disease(CD)is a challenge in clinical *** To investigate the ability of radiomics combined with machine learning methods to differentiate PIL from *** We collected contrast-enhanced computed tomography(CECT)and clinical data from 120 patients form center 1.A total of 944 features were extracted singlephase images of CECT *** the last absolute shrinkage and selection operator model,the best predictive radiographic features and clinical indications were *** from 54 patients were collected at center 2 as an external validation set to verify the robustness of the *** area under the receiver operating characteristic curve,accuracy,sensitivity and specificity were used for *** A total of five machine learning models were built to distinguish PIL from *** on the results from the test group,most models performed well with a large area under the curve(AUC)(>0.850)and high accuracy(>0.900).The combined clinical and radiomics model(AUC=1.000,accuracy=1.000)was the best model among all *** Based on machine learning,a model combining clinical data with radiologic features was constructed that can effectively differentiate PIL from CD.

关键词： Primary intestinal lymphoma Crohn's disease Radiomics Machine learning Diagnosis

Safflower Yellow Inhibits Progression of hepatocellular Carcinoma by Modulating Immunological Tolerance via FAK Pathway

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Chinese Journal of Integrative Medicine 2024年第4期30卷 339-347页

作者： JI Hua-feng YANG Zi-qiang HAN jun-jun li he-fang JIN Zhao-qing CheN Wei-qing CheN Fei-hua GONG Mou-chun Department of General Surgery First People's Hospital of Hangzhou Lin'an DistrictHangzhou(311300)China

Objective To explore the anti-tumor effect of safflower yellow(SY)against hepatocellular carcinoma(HCC)and the underlying potential *** An in vitro model was established by mixing Luc-hepa1-6 cells and CD3^(+)CD8^(+)T cells,followed by adding programmed cell death protein 1(PD-1)antibody(Anti-mPD-1)with or without *** apoptosis was detected by flow cytometry and the level of inflammatory cytokines was determined by enzyme-linked immunosorbent *** protein levels of programmed cell death 1 ligand 1(PD-L1),chemokine ligand(CCL5),C-X-C motif chemokine ligand 10(CXCL10)were measured by Western *** in situ animal model was established in mice followed by treatment with anti-mPD-1 with or without *** imaging was monitored with an AniView 100 imaging *** establish the FAK-overexpressed Luc-hepa1-6 cells,cells were transfected with adenovirus containing pcDNA3.1-FAK for 48 *** The fluorescence intensity,apoptotic rate,release of inflammatory cytokines,and CCL5/CXCL10 secretion were dramatically facilitated by anti-mPD-1(Pher enhanced by SY(Plitated release of inflammatory cytokines,inactivated PD-1/PD-L1 axis,and increased CCL5/CXCL10 secretion were observed in Anti-mPD-1 treated mice(Phermore,the enhanced effects of SY on inhibiting tumor cell growth,facilitating apoptosis and inflammatory cytokine releasing,suppressing the PD-1/PD-L1 axis,and inducing the CCL5/CXCL10 secretion in Anti-mPD-1 treated mixture of Luc-hepa1-6 cells and CD3+CD8+T cells were abolished by FAK overexpression(Phe progression of HCC by mediating immunological tolerance through inhibiting FAK.

关键词： hepatocellular carcinoma safflower yellow Chinese medicine tumor microenvironment programmed cell death protein 1 focal adhesion kinase

An innovative approach to effective breeding blanket design for future fusion reactors

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Plasma Science and Technology 2024年第10期26卷 133-138页

作者： Changle liU Lei li Yanzi he Peng ZHANG Yu ZHOU jun SONG Songtao WU West Anhui University Lu’an 237012People’s Republic of China Institute of Plasma Physices Chinese Academy of SciencesHefei 230031People’s Republic of China Huazhong University of Science and Technology Wuhan 430074People’s Republic of China

An effective breeding blanket is critical to support tritium self-sufficiency for future fusion *** difficulty is to achieve tritium breeding ratio(TBR)target of 1.05 or *** paper presents a new design approach to the blanket design *** indicates that fusion blanket design is affected by universal functions based on *** aspects are worth more attention from fusion engineers in the *** first factor is that the iterations on the material fractions affect not only structure scheme but also TBR *** second factor is the cooling condition affecting final TBR due to the change of the structure material *** third factor is temperature field related to the tritium *** particular,it is suggested that the statistical calculation of effective TBR must be under reasonable control of the blanket temperature *** approach is novel for blanket engineering in development of a fusion reactor.

关键词： TBR tritium release temperature field blanket design fusion reactor