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Highly polar CoP/Co_(2)P heterojunction composite as efficient cathode electrocatalyst for li-air battery

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Chinese Chemical Letters 2024年第9期35卷 486-490页

作者： Miaomiao li Mengwei Yuan Xingzi Zheng Kunyu Han Genban Sun Fujun li Huifeng li Beijing Key Laboratory of Energy Conversion and Storage Materials College of ChemistryBeijing Normal UniversityBeijing 100875China Key Laboratory of Advanced Energy Materials Chemistry(Ministry of Education) College of ChemistryNankai UniversityTianjin 300071China Center for Advanced Materials Research Beijing Normal UniversityZhuhai 519087China

In order to advance the commercialization of rechargeable li-air batteries,it is of importance to explore cathode catalyst with efficient catalytic *** metal oxides have poor electrical conductivity,while cobalt phosphide has excellent electrical conductivity and large specific surface ***,its application in organic li-air batteries has been much less studied,and the electrocatalytic activity desires to be further ***,CoP/Co_(2)P heterojunction composite with higher polarity was *** discharge product of high-polarity CoP/Co_(2)P had a new porous box-like morphology,which was easy to be decomposed and exposed more active *** highly polar CoP/Co_(2)P heterostructure composite had homogeneous pores,the synergistic effect existed between CoP and Co_(2)P,and the discharge product was porous box mixed with li_(2)O_(2)and liOH,which made CoP/Co_(2)P achieve high specific capacity of14632 m Ah/g and cycle stably 161 times when used as air electrode cathode *** work furnished a thought for the construction of cathode catalysts with efficient catalytic activity for li-air batteries.

关键词： li-air battery Cathode catalyst CoP/Co_(2)P Heterojunction structure High polarity

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编制森林经营密度控制表的研究

山西林业科技 2008年第1期37卷 22-24页

作者：李双全山西省林业调查规划院山西太原030012

编制森林经营密度控制表,是从6种数学模型中选出最佳模型编制了依林分平均胸径而编的断面积蓄积量标准表,再以此表为依据,利用林分疏密度编制而成的。该方法比常规依林分平均高编表的方法简捷,更便于生产单位应用。

关键词：标准表疏密度经营密度控制表

螺栓法兰连接设计方法对比分析及国内研究现状综述

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机电工程技术 2021年第8期50卷 16-20页

作者：李双权中石化广州工程有限公司广州510620

螺栓法兰连接接头是工业设备和管道中最常用的静密封连接方式,因为其结构简单和拆装检修方便的特点,在炼化、制药、食品等众多行业中得到了广泛的应用。简要介绍了螺栓法兰连接系统设计方法的发展历程,重点对比分析了3种主要螺栓法兰设... 详细信息

螺栓法兰连接接头是工业设备和管道中最常用的静密封连接方式,因为其结构简单和拆装检修方便的特点,在炼化、制药、食品等众多行业中得到了广泛的应用。简要介绍了螺栓法兰连接系统设计方法的发展历程,重点对比分析了3种主要螺栓法兰设计方法——Waters法、PVRC法以及EN13445-3附录G方法 (EN1591法)的异同。ASME规范Ⅷ-1篇附录2给出了法兰强度的校核方法,但不能保证法兰连接密封的泄漏率;EN13445-3附录G方法不仅给出了螺栓法兰强度计算方法,还考虑了螺栓法兰连接的紧密性。近年来我国的专家学者在垫片泄漏计算模型、垫片性能参数及测试方法研究、螺栓载荷计算等方面取得了众多成果,也是探讨的重点内容。最后对基于控制泄漏率的螺栓法兰连接设计方法研究工作的重点方向进行了展望。

关键词：螺栓法兰连接垫片泄漏率法兰设计方法紧密性

Synergy effect of regulated li-plating and functional solid electrolyte interphase on graphite anodes

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Nano Research 2024年第9期17卷 8077-8085页

作者： Panpan Wang Baojia Xia Jianling li State Key Laboratory of Advanced Metallurgy University of Science and Technology BeijingBeijing 100083China Shanghai Institute of Microsystem and Information Technology Chinese Academy of SciencesShanghai 201800China

The growth of li dendrites poses potential safety hazard to lithium-ion batteries(liBs),and eliminating li dendrites thoroughly stills face tough difficulties ***,regulating li-plating is a critical optimization-direction to address the ***,a“graphite-li hybrid”anode with high reversibility is realized under the constant-capacity lithiation(CCL).Within CCL,the uniform distribution of li-plating on the graphite surface is successfully *** evolution in different states of solid electrolyte interphase(SEI)is investigated in detail to study the interaction between the potentials and impedance during the process of liintercalation and *** the potential below 0 V and the state of charge(SOC)of 110%relative to the theoretical capacity,the F-rich SEI with high stability is constructed to hinder the emergency of li dendrites and maintain the intact structure of graphite anode under long *** cell presents more than 100%Coulombic efficiency(CE)with the 900 cycles,demonstrating the reversible li-plating and the utilization of *** the CCL half-cell provides a good cycling performance and specific capacity of 900 cycles at 0.5 C,it is attributed to the synergy effect of stable inorganic-rich SEI and regulated active li-plating.

关键词： "graphite-li hybrid"anode li-plating reversibility solid electrolyte interphase(SEI)

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中承式钢拱桥稳定性影响参数分析

山西建筑 2016年第13期42卷 170-171页

作者：李双全厦门大学建筑与土木工程学院福建厦门361005

以某中承式钢拱桥为研究对象,基于有限元稳定分析理论,采用大型有限元软件ANSYS,对该拱桥的稳定安全系数进行了计算,并从荷载布置方式、拱肋抗弯刚度、主梁抗弯刚度、吊杆刚度等方面,分析了影响该拱桥稳定性的因素,得到了一些有价值的... 详细信息

以某中承式钢拱桥为研究对象,基于有限元稳定分析理论,采用大型有限元软件ANSYS,对该拱桥的稳定安全系数进行了计算,并从荷载布置方式、拱肋抗弯刚度、主梁抗弯刚度、吊杆刚度等方面,分析了影响该拱桥稳定性的因素,得到了一些有价值的结论。

关键词：钢拱桥稳定性有限元安全系数

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面向台区智能终端的即插即用和拓扑识别方法

电力系统自动化 2021年第10期45卷 166-173页

作者：钟加勇熊小伏何迎春单荣荣姜洪浪李双全输配电装备及系统安全与新技术国家重点实验室(重庆大学) 重庆市400030 国网重庆市电力公司重庆市400015 南瑞集团有限公司(国网电力科学研究院有限公司) 江苏省南京市211106 中国电力科学研究院有限公司北京市100192 杭州海兴电力科技股份有限公司浙江省杭州市310011

配电物联网背景下,海量台区智能终端与端设备采用人工接入的工作量十分庞大,且存在边-端拓扑维护与信息交互困难等问题。因此,提出了一种面向台区智能终端的即插即用与拓扑识别方法。首先,依据配电物联网"云-管-边-端"分层体系构建了台... 详细信息

配电物联网背景下,海量台区智能终端与端设备采用人工接入的工作量十分庞大,且存在边-端拓扑维护与信息交互困难等问题。因此,提出了一种面向台区智能终端的即插即用与拓扑识别方法。首先,依据配电物联网"云-管-边-端"分层体系构建了台区智能终端与智能电表等端设备架构场景,并在此基础上提出了相应的即插即用机制。其次,提出了台区智能终端与端设备的拓扑自动识别方法。最后,通过搭建实验系统,从终端接入验证、终端软件升级以及终端故障下线退出3个部分对所提即插即用与拓扑识别进行了验证分析。实验结果表明,所提方法具有良好的可扩展性与故障容错能力,能够实现海量台区智能终端与端设备的即插即用与拓扑关联自动运维。

关键词：配电物联网台区智能终端端设备即插即用拓扑识别

Robust chemo-mechanical stability of additives-free SiO_(2)anode realized by honeycomb nanolattice for high performance li-ion batteries

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Chinese Chemical Letters 2024年第10期35卷 442-446页

作者： Xinpin Pan Yongjian Cui Zhe Wang Bowen li Hailong Wang Jian Hao Feng li Jing li Advanced Energy Storage Materials Lab School of Materials and New EnergyNingxia UniversityYinchuan 750021China School of Chemistry and Chemical Engineering Ningxia UniversityYinchuan 750021China

Silicon-based anodes including Si,Si Oxand SiO_(2)could deliver ultra-large capacities,but degrade fast owing to huge volume change and low ***,large amounts of elastic binder and conductive additives were composited with nanosized silicon-based materials to yield reasonable cycling stability,which nevertheless not only decrease specific capacity but also induce inhomogeneous lithiation/delithiation as well as uneven stress *** nanolattice has exhibited superior mechanical properties which could be ideal structure for silicon-based anodes,but yet faces challenges in integration of chemical reactivity,conductivity and mechanical ***,we fabricate artificial SiO_(2)honeycomb nanolattice consisting of numerous nanoscale SiO_(2)cells interconnected by through-holes,and conformal coating of highly graphitic carbon on the nanolattice is achieved through in situ catalytic ***,the nanolattice is firmly bonded on Cu substrate through atomic interdiffusion irrespective of surface *** unique structure allows fast charge transportation and homogeneous lithiation/delithiation throughout the micron-meter nanolattice,which results in excellent stability and large reversible capacity over 500 cycles at 1 A/*** results highlight design and constructing artificial nanolattice can be an effective way to prevent chemo-mechanical degradation of silicon-based anode materials.

关键词： li-ion batteries Nanolattice SiO_(2)anode Stability Conductivity

Application and Development of Ornamental Vines in Urban Gardens

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Journal of Landscape Research 2012年第9期4卷 37-39页

作者： TANG Dengming li shuangquan Yancheng Biological Engineering Higher Vocational Technology School

Cultivated species and characters of the mostly-applied ornamental vines were introduced,such garden landscaping methods as pergola type,affiliated-to-wall type and hanging type as well as their respective landscape effects explored,current cultivation and problems *** trend of ornamental vines in garden landscaping was defined,modeling arts of ornamental vines were stressed,ecological adaptability of these species studied,selection and cultivation of improved varieties enhanced,maintenance and management valued to promote vertical greening and increase urban green quantity.

关键词： Ornamental vines Application Development Research

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沥青温拌技术分类及温拌效果的试验评价方法

材料导报 2024年第4期38卷 80-87页

作者：延西利郑涛蒋双全李卫成长安大学公路学院西安710064 四川高速公路建设开发集团有限公司成都610041 四川公路桥梁建设集团有限公司成都610041 安康市交通建设投资集团有限公司陕西安康725000

沥青温拌技术日益广泛应用于路面工程,为了定量评价温拌沥青混合料在拌和生产过程中的温拌效果,提供试验评价方法,本研究自主开发了一种沥青混合料变速拌和试验装置,采用70^(#)基质和SBS改性两种沥青、自主研发的一种表面活性剂型沥青... 详细信息

沥青温拌技术日益广泛应用于路面工程,为了定量评价温拌沥青混合料在拌和生产过程中的温拌效果,提供试验评价方法,本研究自主开发了一种沥青混合料变速拌和试验装置,采用70^(#)基质和SBS改性两种沥青、自主研发的一种表面活性剂型沥青温拌剂(取名为Alube)和一种有机降黏型沥青温拌剂(取名为ACMP),以市场成熟产品Evotherm为参照,分别制备了温拌沥青及其AC-13C型混合料,测试了不同沥青和温拌沥青的三大指标、布氏黏度和动态剪切流变指标,分析了沥青的黏温曲线特性,通过混合料的变温击实试验和变速拌和试验,研究了沥青混合料的压实特性和拌和流动特性,提出了沥青混合料的拌和流动模型。研究结果表明,有机降黏型温拌剂减小了沥青的黏度,增大了沥青的流动性,改变了沥青的技术性能,如针入度、延度、相位角等增大,软化点、布氏黏度等减小,而表面活性剂型温拌剂不改变沥青的基本技术性能;黏温曲线法仅可表征有机降黏型温拌沥青的温度变化,等黏温度降低约9℃,变温击实法和变速拌和法则可以同时表征两大类温拌剂的温拌效果;沥青混合料的拌和流动性服从宾汉黏塑性模型,从流变理论上解答了混合料的拌和流动性及和易性,推荐采用变速拌和试验来评价温拌沥青混合料的温拌效果;综合考察现有沥青温拌技术可知,在常用温拌剂掺量下,温拌沥青的生产拌和温度可比热拌沥青混合料低20~30℃,符合常规认识。

关键词：道路工程沥青混合料沥青温拌技术试验评价变速拌和试验宾汉模型