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Integrating single Ni site and PtNi alloy on two-dimensional porous carbon nanosheet for efficient catalysis in fuel cell

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Nano Research 2024年第8期17卷 6916-6921页

作者： Fangyao Zhou Yaner ruan Feng li lin Tian Mengzhao Zhu Wenan Tie Xiaoyan Tian Bo Wang Peigen liu Jie Xu Xiaoping Gao Peng li Huang Zhou Yuen Wu Key Laboratory of Precision and Intelligent Chemistry University of Science and Technology of ChinaHefei 230026China Shanxi Yanchang Petroleum(Group)Co.Ltd. Xian 710065China College of Chemistry and Materials Engineering Wenzhou UniversityWenzhou 325035China

The performance of catalyst depends on the intrinsic activity of active sites and the structural characteristics of the ***,we simultaneously integrate single nickel(Ni)sites and platinum-nickel(PtNi)alloy nanoparticles(NPs)on a two-dimensional(2D)porous carbon nanosheet,demonstrating remarkable catalytic performance in the oxygen reduction reaction(ORR).The single Ni sites can activate the oxygen molecules into key oxygen-containing intermediate that is further efficiently transferred to the adjacent PtNi alloy NPs and rapidly reduced to H_(2)O,which establishes a relay catalysis between active *** porous structure on the carbon nanosheet support promotes the transfer of active intermediates between these active sites,which assists the relay catalysis by improving mass ***,the obtained catalyst demonstrates a half-wave potential of up to 0.942 V,a high mass activity of 0.54 A·mgPt^(−1),and negligible decay of activity after 30,000 cycles,which are all superior to the commercial Pt/C catalysts with comparable loading of *** theoretical calculation results reveal that the obtained catalyst with defect structure of carbon support presents enhanced relay catalytic effect of PtNi alloy NPs and single Ni sites,ultimately realizing improved catalytic *** work provides valuable inspiration for developing low platinum loading catalyst,integrating single atoms and alloy with outstanding performance in fuel cell.

关键词： two-dimensional porous carbon nanosheet Pt-based alloy single atom catalysts relay effect proton-exchange membrane fuel cells

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Interaction between ozone and paternal smoking on fetal congenital heart defects among pregnant women at high risk a multicenter maternal-fetal medicine study

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World Journal of Pediatrics 2024年第6期20卷 621-632页

作者： Huan Wang Yan-Ping ruan Sheng Ma Ya-Qi Wang Xiao-Yu Wan Yi-Hua He Jing li Zhi-Yong Zou Institute of Child and Adolescent Health School of Public HealthNational Health Commission Key Laboratory of Reproductive HealthPeking UniversityNo.38 Xueyuan RdHaidian DistrictBeijing 100191China Echocardiography Medical Center Beijing Anzhen Hospital.Capital Medical UniversityMaternal-Fetal Medicine center in Fetal Heart DiseaseBeijing Anzhen HospitalNo.2 Anzhen RdChaoyang DistrictBeijing 100029China

Background Evidence remains limited on the association between maternal ozone(O,)exposure and congenital heart defects(CHDs)in offspring,and few studies have investigated the interaction and modification of paternal smoking on this *** Using a sample including pregnant women at high risk of fetal CHD(with metabolic disease,first-trimester viral infection,family history of CHD,etc.)from a maternal-fetal medicine study covering 1313 referral hospitals in China during 2.13-2021,we examined the associations between maternal O_(3)exposure during 3-8 weeks of gestational age and fetal CHD in offspring and investigated the interaction and modification of paternal smoking on this *** was diagnosed by fetal echocardiograms,maximum daily 8-hour average O,exposure data at a 10 km×10 km spatial resolution came from the Tracking Air Pollution in China dataset,and paternal smoking was collected using *** regression models were used to estimate adjusted odds ratios(ORs)and 95%confidence intervals(CIs).Results Among 27,834 pregnant women at high risk of fetal CHD,17.4%of fetuses were diagnosed with *** 10μg/m^(3)increase in maternal O_(3)exposure was associated with a 17%increased risk of CHD in offspring(OR=1.17,95%CI=1.14-1.20).Compared with paternal nonsmoking and maternal low O_(3)exposure,the ORs(95%CI)of CHD for smoking and low O_(3)exposure,nonsmoking and high O_(3)exposure,and smoking and high O_(3)exposure were 1.25(1.08-1.45),1.81(1.56-2.08),and 2.23(1.84-2.71),*** smoking cessation seemingly mitigated the increased risk of *** Maternal O_(3)exposure and paternal smoking were interactively associated with an increased risk of fetal CHD in offspring,which calls for effective measures to decrease maternal exposure to O_(3)pollution and secondhand smoke for CHDprevention.

关键词： Congenital heart defects Fetal heart development Ozone exposure Tobacco smoking

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Orthopedic revolution:The emerging role of nanotechnology

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World Journal of Orthopedics 2024年第10期15卷 932-938页

作者： Wen-Jie ruan Si-Si Xu Dong-Hui Xu Zhi-Peng li department of Sports Medicine Zhejiang Provincial People's Hospital(The Affiliated People's Hospital)Hangzhou 310000Zhejiang ProvinceChina School of Medicine Taizhou UniversityTaizhou 318000Zhejiang ProvinceChina The Second department of Orthopedics The Fifth Affiliated Hospital of Zhengzhou UniversityZhengzhou 450015Henan ProvinceChina

This review summarizes the latest progress in orthopedic nanotechnology,ex-plores innovative applications of nanofibers in tendon repair,and evaluates the potential of selenium and cerium oxide nanoparticles in osteoarthritis and osteo-blast *** review also describes the emerging applications of inje-ctable hydrogels in cartilage engineering,emphasizing the critical role of inter-disciplinary research and highlighting the challenges and future prospects of in-tegrating nanotechnology into orthopedic clinical *** comprehensive approach provides a holistic perspective on the transformative impact of nanote-chnology in orthopedics,offering valuable insights for future research and clinical applications.

关键词： Cerium oxide nanoparticles Injectable hydrogels Interdisciplinary research Orthopedic nanotechnology Selenium nanoparticles

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Double-layered skeleton of li alloy anchored on 3D metal foam enabling ultralong lifespan of li anode under high rate

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Chinese Chemical Letters 2024年第3期35卷 479-485页

作者： Chaohui Wei Zeyu Yao Jin ruan Zhicui Song Aijun Zhou Yingze Song Donghuang Wang Jicheng Jiang Xin Wang Jingze li Yangtze Delta Region Institute(Huzhou) University of Electronic Science and Technology of ChinaHuzhou 313000China School of Materials and Energy University of Electronic Science and Technology of ChinaChengdu 611731China State Key Laboratory of Environmental-Friendly Energy Materials Tianfu Institute of Research and InnovationSchool of Materials and ChemistrySouthwest University of Science and TechnologyMianyang 621010China

The high specific capacity and low negative electrochemical potential of lithium metal anodes(LMAs),may allow the energy density threshold of li metal batteries(LMBs)to be pushed ***,the existing detrimental issues,such as dendritic growth and volume expansion,have hindered the practical implementation of *** three-dimensional frameworks(e.g.,copper and nickel foam),have been regarded as one of the fundamental strategies to reduce the local current density,aiming to extend the Sand'***,the local environment far from the skeleton is almost the same as the typical plane li,due to macroporous space of metal ***,we built a double-layered 3D current collector of li alloy anchored on the metal foam,with micropores interconnected macropores,via a viable thermal infiltration and cooling *** to the excellent electronic and ionic conductivity coupled with favorable lithiophilicity,the li alloy can effectively reduce the nucleation barrier and enhance the li^(+)transportation rate,while the metal foam can role as the primary promotor to enlarge the surface area and buffer the dimensional ***,the li composite anode with hierarchical structure of primary and secondary scaffolds realized the even deposition behavior and minimum volume expansion,outputting preeminent prolonged cycling performances under high rate.

关键词： Double-layered skeleton li alloy 3D Metal foam Ultralong lifespan lithium metal batteries High rate

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An MPXV mRNA-LNP vaccine candidate elicits protective immune responses against monkeypox virus

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Chinese Chemical Letters 2024年第8期35卷 466-470页

作者： Yuxin Tian Mengjun li Yang Yang Chunhui li Yun Peng Haiyin Yang Mengyuan Zhao Pengfei Wu Shaobo ruan Yuanyu Huang Chenguang Shen Minghui Yang Advanced Research Institute of Multidisciplinary Science School of Life ScienceKey Laboratory of Molecular Medicine and BiotherapyBeijing Institute of TechnologyBeijing 100081China BSL-3 Laboratory(Guangdong) Guangdong Provincial Key Laboratory of Tropical Disease ResearchSchool of Public HealthDepartment of Laboratory MedicineZhujiang HospitalSouthern Medical UniversityGuangzhou 510280China National Clinical Research Center for infectious disease Shenzhen Third People’s HospitalSecond Hospital Affiliated to Southern University of Science and TechnologyShenzhen 518112China

The monkeypox virus(MPXV)outbreak,declared a Public Health Emergency of International Concern(PHEIC)by the World Health Organization(WHO)in 2022,continues to pose a significant threat due to the absence of vaccines or drugs for MPXV *** this study,we developed an mRNA vaccine that expressing the A29L antigen,a specific protein of the intracellular mature *** vaccine utilizes a thermostable ionizable lipid nanoparticle(iLNP)platform and has been administered to *** find-ings demonstrate that the MPXV A29L mRNA vaccine candidate induces robust cross-neutralizing immune responses against both vaccinia virus(VACV)and MPXV live ***,immunization with the vaccine candidate provided protection against the VACV challenge in *** findings underscore the potential of mRNA-LNP vaccines as safe and effective candidates against monkeypox *** the current absence of specific interventions for MPXV infection,our study represents a significant step forward in developing a viable solution to combat this ongoing public health threat.

关键词： Monkeypox virus mRNA vaccine lipid-nano particle A29L VACV

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Preparation of MXene-based hybrids and their application in neuromorphic devices

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International Journal of Extreme Manufacturing 2024年第2期6卷 164-188页

作者： Zhuohao Xiao Xiaodong Xiao ling Bing Kong Hongbo Dong Xiuying li Bin He Shuangchen ruan Jianpang Zhai Kun Zhou Qin Huang liang Chu School of Materials Science and Engineering Jingdezhen Ceramic UniversityJingdezhen 333403JiangxiPeople’s Republic of China School of Mechanical and Vehicle Engineering Linyi UniversityLinyi 276000ShandongPeople’s Republic of China College of New Materials and New Energies Shenzhen Technology UniversityShenzhen 518118GuangdongPeople’s Republic of China School of Mechanical&Aerospace Engineering Nanyang Technological University50 Nanyang AvenueSingapore 639798Singapore Ningbo Institute of Materials Engineering and Technology Chinese Academy of ScienceNingbo 315201ZhejiangPeople’s Republic of China Institute of Carbon Neutrality and New Energy&School of Electronics and Information Hangzhou Dianzi UniversityHangzhou 310018ZhejiangPeople’s Republic of China

The traditional von Neumann computing architecture has relatively-low information processing speed and high power consumption,making it difficult to meet the computing needs of artificial intelligence(AI).Neuromorphic computing systems,with massively parallel computing capability and low power consumption,have been considered as an ideal option for data storage and AI computing in the ***,as the fourth basic electronic component besides resistance,capacitance and inductance,is one of the most competitive candidates for neuromorphic computing systems benefiting from the simple structure,continuously adjustable conductivity state,ultra-low power consumption,high switching speed and compatibility with existing CMOS *** memristors with applying MXene-based hybrids have attracted significant attention in recent ***,we introduce the latest progress in the synthesis of MXene-based hybrids and summarize their potential applications in memristor devices and neuromorphological *** explore the development trend of memristors constructed by combining MXenes with other functional materials and emphatically discuss the potential mechanism of MXenes-based memristor ***,the future prospects and directions of MXene-based memristors are briefly described.

关键词： MXene etching fabrication memristor neuromorphic

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Study on damage characteristics of iron ore under variable line density charge structure blasting

Rock Mechanics Bulletin

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Rock Mechanics Bulletin 2024年第4期3卷 1-14页

作者： Xinmin Ma Yiyin Hu Xinshuo li Yongsheng ruan Yuan Jin Wenqing Yang School of Mechanics and Civil Engineering China University of Mining and Technology(Beijing)Beijing100083China

Blasting test research was conducted on iron ore specimens with variable line density charging *** tomography(CT),digital image processing,and three-dimensional model reconstruction techniques were used to analyze the damage characteristics of iron ore specimens after blasting based on the calculated number of box *** results show that increasing the variable line density section charge uncoupling coefficient reduces the overall damage to the specimen by up to 1.73%,indicating that the overall damage size negatively correlates with the size of the variable line density section charge uncoupling *** damage characteristics of iron ore specimens from different layers(uncoupled charging section,transition section,coupled charging section)have some variability;when the uncoupling coefficient of the uncoupled charging section was reduced,the uncoupled section of the center of the damaged layer increased and then *** contrast,the transition section shows a trend of increase,and the coupled section shows a minor difference,fully demonstrating the change in the variable line density section of the uncoupling coefficient of the specimen blasting damage *** study concludes that in the actual blasting project,choosing a reasonable variable line charge density structure can make the release of explosive blast energy more uniform to efficiently and thoroughly use explosive power to improve the iron ore crushing effect.

关键词： Iron ore Blasting Variable line density charges Damage characterization

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PFL-DSSE:A Personalized Federated Learning Approach for Distribution System State Estimation

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CSEE Journal of Power and Energy Systems 2024年第5期10卷 2265-2270页

作者： Huayi Wu Zhao Xu Jiaqi ruan Xianzhuo Sun department of Electrical and Electronic Engineering The Hong Kong Polytechnic UniversityHong Kong SARChina department of Electrical and Electronic Engineering Shenzhen Research InstituteResearch Institute of Smart EnergyThe Hong Kong Polytechnic UniversityHong Kong SARChina. department of Electrical and Electronic Engineering The Hong Kong Polytechnic UniversityHong Kong SARChina.

A centralized framework-based data-driven framework for active distribution system state estimation(DSSE)has been widely ***,it is challenged by potential data privacy breaches due to the aggregation of raw measurement data in a data center.A personalized federated learningbased DSSE method(PFL-DSSE)is proposed in a decentralized training framework for *** validation confirms that PFL-DSSE can effectively and efficiently maintain data confidentiality and enhance estimation accuracy.

关键词： Terms-Distribution system state estimation personalized federated learning privacy protection

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Process and Mechanism of Controlling Outburst Floods of Landslide Dams through Artificial Structures: Physical Experiments

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Journal of Earth Science 2024年

作者： Hechun ruan Huayong Chen Xiaoqing Chen Wanyu Zhao Xiao li Key Laboratory of Mountain Hazards and Surface Processes， Institute of Mountain Hazards and Environment， Chinese Academy of Sciences University of Chinese Academy of Sciences

The scale of the outburst flood resulting from a landslide dam failure significantly influences the extent of the disaster and losses downstream. This study proposes a method for controlling the discharge of landslide dam failure using the artificial structure (AS). The primary approach involves strategically arranging the designed AS on both sides of the excavated spillway. As the breach is eroded， ASs gradually falls into the breach， serving to control the discharge. Fourteen sets of flume experiments were conducted to investigate the impact of various factors， including AS types， distances from the breach boundary， arrangements， columns， numbers， on the discharge control effectiveness. The mechanism how AS controls outburst discharge was revealed. Results indicate a pronounced control effect of AS on landslide dam-break discharge， with the maximum reducing rate of the peak discharge in the experiment reaching 47.4%. In controlling outburst discharge， four-sided framed structures demonstrate superior performance compared to four-sided solid structures， and serial structures outperform discrete structures. When arranging ASs， it is essential to ensure that the structure initiates its descent into the breach at the onset of the rapid increase in outburst discharge and continues until the peak discharge occurs. Building upon this foundation， augmenting the number of ASs and columns significantly enhances the efficacy of discharge control. The fundamental rationale for this discharge control lies in the AS’s capacity to reduce the headward scarp height， constrain sediment transport， and diminish the erosion capacity of the outburst flood， ultimately lowering the breach erosion rate. Lastly， a calculation method for the size design of the AS is established based on mechanical analysis. The research findings offer a new technological option for the emergency disposal of landslide dams.

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Covalent Organic Framework with 3D Ordered Channel and Multi-Functional Groups Endows Zn Anode with Superior Stability

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Nano-Micro Letters 2024年第4期16卷 350-363页

作者： Bin li Pengchao ruan Xieyu Xu Zhangxing He Xinyan Zhu liang Pan Ziyu Peng Yangyang liu Peng Zhou Bingan Lu Lei Dai Jiang Zhou School of Chemical Engineering North China University of Science and TechnologyTangshan 063009People’s Republic of China School of Materials Science and Engineering Central South UniversityChangsha 410083People’s Republic of China State Key Laboratory for Mechanical Behavior of Materials Xi’an Jiaotong UniversityXi’an 710049People’s Republic of China Hunan Provincial Key Defense Laboratory of High Temperature Wear‑Resisting Materials and Preparation Technology Hunan University of Science and TechnologyXiangtan 411201People’s Republic of China School of Physics and Electronics Hunan UniversityChangsha 410082People’s Republic of China

Achieving a highly robust zinc(Zn)metal anode is extremely important for improving the performance of aqueous Zn-ion batteries(AZIBs)for advancing“carbon neutrality”society,which is hampered by the uncontrollable growth of Zn dendrite and severe side reactions including hydrogen evolution reaction,corrosion,and passivation,***,an interlayer containing fluorinated zincophilic covalent organic framework with sulfonic acid groups(COF-S-F)is developed on Zn metal(Zn@COF-S-F)as the artificial solid electrolyte interface(SEI).Sulfonic acid group(-SO_(3)H)in COF-S-F can effectively ameliorate the desolvation process of hydrated Zn ions,and the three-dimensional channel with fluoride group(-F)can provide interconnected channels for the favorable transport of Zn ions with ion-confinement effects,endowing Zn@COF-S-F with dendrite-free morphology and suppressed side ***,Zn@COF-S-F symmetric cell can stably cycle for 1,000 h with low average hysteresis voltage(50.5 m V)at the current density of 1.5 m A cm^(-2).Zn@COF-S-F|Mn O_(2)cell delivers the discharge specific capacity of 206.8 m Ah g^(-1)at the current density of 1.2 A g^(-1)after 800 cycles with high-capacity retention(87.9%).Enlightening,building artificial SEI on metallic Zn surface with targeted design has been proved as the effective strategy to foster the practical application of high-performance AZIBs.

关键词： Aqueous Zn ion batteries Covalent organic framework Interfacial modification Zn ion flux regulation Desolvation effect

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