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Acta Geologica Sinica(English Edition) 2024年第3期98卷 641-656页

作者： WANG Qiuyu CHEN Shouming ZHANG Hongrui li saisai SinoProbe Laboratory Institute of GeologyChinese Academy of Geological SciencesBeijing 100037China Guangxi Key Laboratory of Hidden Metallic Ore Deposit Exploration GuilinGuangxi 541004China

High-silica granitoids record the formation and evolution of the continental crust.A new intrusive complex has been recognized among silicic volcanic rocks of the Weixi arc,Southwest *** intrusions consist of granites,granitic porphyries,and *** U-Pb age data indicate that the Weixi granitoids formed at 248-240 Ma and were coeval with silicic volcanic rocks of the Weixi *** Weixi granitoids are enriched in Rb,Th,and U,depleted in Ba,Sr,Nb,Ta,and Ti,and have high light/heavy rare earth element ratios and slightly negative Eu *** Weixi granitoids have negative ε_(Nd)(t)values(-9.8 to-7.8)and negative zircon ε_(Hf)(t)values(-12.02 to-5.11).The geochemical and isotopic features suggest the Weixi granitoids were derived by partial melting of ancient crustal *** Weixi granitoids and silicic volcanic rocks were derived from the same magma by crystal accumulation and melt extraction,respectively,and they record the formation of a continental arc in the central Sanjiang orogenic belt.

关键词： granitoids geochemistry crystal accumulation continental crust Sanjiang orogen

用户需求驱动下的病区物流机器人服务系统设计

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机械设计 2024年第4期41卷 164-169页

作者：李赛赛孙博文谭佳怡安徽工程大学设计学院安徽芜湖241000 北京理工大学设计与艺术学院北京100081

为协助医护人员开展病区服务工作,提升患者临床康复体验,提出基于用户需求的产品服务系统设计方法。以病区场景下的物流机器人服务系统为研究对象,采用模糊Kano模型和熵权法确定用户需求类型及优先级;结合用户关键需求,进行产品外观与... 详细信息

为协助医护人员开展病区服务工作,提升患者临床康复体验,提出基于用户需求的产品服务系统设计方法。以病区场景下的物流机器人服务系统为研究对象,采用模糊Kano模型和熵权法确定用户需求类型及优先级;结合用户关键需求,进行产品外观与结构、人机交互模式及产品信息显示的设计改进,并采用逼近理想解排序法(Technique for Order Preference by Similarity to Ideal Solution,TOPSIS)评估设计方案的可行性。研究结果表明:采用定量和定性相结合的设计方法有利于提升服务系统设计的客观性和准确性,为同类产品的服务系统设计提供参考。

关键词：产品设计物流机器人模糊Kano模型熵权法逼近理想解排序法产品服务系统

地质温度计在桂东南那卜韧性剪切带花岗质糜棱岩中的适用性

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地球科学 2024年第6期49卷 1946-1965页

作者：辛良伟李赛赛冯佐海刘兴源吴江波王秋宇有色金属矿产勘查与资源高效利用省部共建协同创新中心桂林理工大学广西桂林541004 桂林理工大学地球科学学院广西桂林541004

糜棱岩的变质变形温度测定对其变形演化过程和热年代学同位素定年结果解释具有重要的意义.本文仅讨论各地质温度计在那卜韧性剪切带中的适用性.利用糜棱岩中的矿物组合、矿物动态重结晶特征以及EBSD(electron back-scattered diffracti... 详细信息

糜棱岩的变质变形温度测定对其变形演化过程和热年代学同位素定年结果解释具有重要的意义.本文仅讨论各地质温度计在那卜韧性剪切带中的适用性.利用糜棱岩中的矿物组合、矿物动态重结晶特征以及EBSD(electron back-scattered diffraction)石英轴组构等塑性变形特征,估算出那卜韧性剪切带的变质变形温度范围为400~550℃.在电子探针分析技术基础上,利用绿泥石成分地质温度计、白云母-绿泥石地质温度计以及白云母/黑云母Ti温度计对那卜韧性剪切带中的花岗质糜棱岩样品进行变质变形温度计算,获得相应的温度分别为305~325℃、390~500℃、395~492℃和473~565℃、431~574℃.通过对比分析发现,利用绿泥石成分地质温度计获得的结果明显低于利用塑性变形特征估算出的温度范围和其他温度计的计算结果,结合前人研究结果表明其仅适用于低温变质变形作用的温度计算;而另外3种温度计获得的结果在误差范围内均位于利用塑性变形特征估算出的温度范围内,表明其均适用于该剪切带的变质变形温度计算.其中白云母-绿泥石地质温度计适用于低温糜棱岩,白云母/黑云母Ti温度计适用于相对高温的糜棱岩.

关键词：糜棱岩韧性剪切带地质温度计变质变形温度那卜镇构造地质

Employ ionic liquid to stabilize black-phase formamidinium perovskites

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Science China Chemistry 2021年第8期64卷 1263-1264页

作者： saisai li Mingjian Yuan Key Laboratory of Advanced Energy Materials Chemistry(Ministry of Education) Renewable Energy Conversion and Storage Center(RECAST)College of ChemistryNankai UniversityTianjin300071China

The certified power conversion efficiency(PCE)of per-ovskite solar cells which have emerged as the most promising candidates for next-generation thin-film photovoltaics has exceeded 25%.Among all available compositions,formamidinium lead iodide perovskite(FAPbI_(3))has a theoretically higher efficiency than the other perovskite analogues due to its narrower bandgap[1,2]and hence has attracted widespread attention.

关键词： perovskite hence narrow

玻璃纤维基隔热多孔陶瓷的制备及其对中子的屏蔽性能

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材料研究学报 2024年第6期38卷 471-480页

作者：吴倩芳何群常兵全宇鑫胡敬文李赛赛曹迎楠安徽工业大学材料科学与工程学院马鞍山243002 中钢洛阳耐火材料研究院洛阳471309

以玻璃纤维和玻璃颗粒为主要原料、以Isobam-104为分散剂、羧甲基纤维素钠为稳泡剂、十二烷基硫酸钠为发泡剂、氧化钆为中子屏蔽填料,用泡沫凝胶注模法制备玻璃纤维基隔热多孔陶瓷复合材料,研究了热处理温度对其物相组成、微观结构、机... 详细信息

以玻璃纤维和玻璃颗粒为主要原料、以Isobam-104为分散剂、羧甲基纤维素钠为稳泡剂、十二烷基硫酸钠为发泡剂、氧化钆为中子屏蔽填料,用泡沫凝胶注模法制备玻璃纤维基隔热多孔陶瓷复合材料,研究了热处理温度对其物相组成、微观结构、机械性能和热导率的影响以及氧化钆的含量对其理化性能和中子屏蔽性能的影响。结果表明,热处理温度从700℃提高到800℃,使多孔陶瓷的强度、体积密度和热导率显著提高、气孔率降低,其抗压强度和抗折强度分别从0.75和0.3 MPa提高到10.7和5.1 MPa,热导率从0.075 W/(m·K)提高到0.28 W/(m·K)。热处理温度为750℃的材料其抗折强度、抗压强度、开口气孔率和热导率分别为1.4 MPa、2.1 MPa、79.8%和0.11 W/(m·K)。氧化钆的添加量(质量分数,下同)从0提高到6%,多孔陶瓷复合材料的强度逐渐降低、对中子的屏蔽效率逐渐提高。氧化钆添加量为6.0%的多孔陶瓷其抗折强度仅为0.63 MPa,抗压强度为0.86 MPa,中子屏蔽率为50.8%,热中子屏蔽率高达82.9%,但是不影响多孔陶瓷的热导率。

关键词：无机非金属材料多孔陶瓷玻璃纤维氧化钆屏蔽性能

Methylammonium-and bromide-free perovskites enable efficient and stable photovoltaics

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Journal of Energy Chemistry 2021年第12期30卷 12-24,I0002页

作者： saisai li Tingwei He Yuanzhi Jiang Mingjian Yuan Key Laboratory of Advanced Energy Materials Chemistry(Ministry of Education) Renewable Energy Conversion and Storage Center(RECAST)College of ChemistryNankai UniversityTianjin 300071China

Hybrid perovskite solar cell(PSC)has attracted extensive research interest due to its rapid increase in efficiency,regarding as one of the most promising candidates for the next-generation photovoltaic *** certified power conversion efficiency of the devices based on formamidinium lead iodide(FAPbI_(3))perovskite has reached 25.5%,approaching the record of monocrystalline silicon solar ***,the blackα-phase FAPbI_(3)materials can spontaneously transform to non-optically activeδ-phase at room temperature,which greatly hinder their photovoltaic *** order to overcome this problem,various strategies,especially introducing methylammonium(MA^(+)),caesium(Cs^(+))and bromide(Br^(-))ions into the materials,have been widely ***,MA^(+)can largely reduce the thermal stability of the ***,the introduction of Br^(-)can enlarge the materials'bandgap,resulting in a reduced theoretical *** these in mind,developing the strategies which without using MA^(+)and Br^(-)is the inevitable ***,we focus on the recent progresses of stabilizingαFAPbI_(3)without employing MA^(+)and Br^(-),and discuss the advantages of inorganic ions doping and dimensionality engineering to stabilizedαFAPbI_(3).Meanwhile,in order to deeply understand the relationship between the semiconducting properties and device performance of the corresponding materials,we then summarize several significant strategies to suppress the non-radiation recombination,such as interface modification and trap ***,we propose to develop more effective'A-site'alternatives to stabilizeαFAPbI_(3),which is expected to achieve high-efficient PSCs with long-term stability,facilitating its commercialization process.

关键词： Perovskites Solar cells Stability α-FAPbI_(3) Dimensionality engineering

公共数据合作开发的动力机制与风险规避——基于政府与大数据平台企业合作的视角

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学术交流 2024年第1期 31-43页

作者：王张华李赛赛湘潭大学公共管理学院湖南湘潭411105

公共数据的开发利用已经成为数字化时代不可回避的重要议题,寻求与大数据平台企业等主体展开合作是公共数据开发的重要趋势。政府与大数据平台企业合作开发公共数据受到资源互补、利益共享和风险共担三重因素共同驱动,而公共数据开发可... 详细信息

公共数据的开发利用已经成为数字化时代不可回避的重要议题,寻求与大数据平台企业等主体展开合作是公共数据开发的重要趋势。政府与大数据平台企业合作开发公共数据受到资源互补、利益共享和风险共担三重因素共同驱动,而公共数据开发可能存在权力解构效应和权利诱导倾向,衍生出以“管制俘获、市场支配和公共意志裹挟”为代表的权力型风险和以“算法合谋、算法歧视、算法操纵和租值耗散”为代表的权利型风险。为此,可以通过明晰公共数据权属边界、落实公共数据权属责任、协调政企合作伙伴关系与激发政企合作主体动能等路径规避公共数据合作开发的潜在风险,真正走向公共数据价值共创。

关键词：公共数据政企合作价值共创权力风险权利风险

Three-dimensional graphitic carbon sphere foams as sorbents for cleaning oil spills

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International Journal of Minerals,Metallurgy and Materials 2022年第3期29卷 513-520页

作者： saisai li Haijun Zhang Longhao Dong Haipeng liu Quanli Jia Key Laboratory of Green Fabrication and Surface Technology of Advanced Metal Materials Anhui University of TechnologyMa’anshan 243002China The State Key Laboratory of Refractories and Metallurgy Wuhan University of Science and TechnologyWuhan 430081China High Temperature Ceramic Institute Zhengzhou UniversityZhengzhou 450052China

Frequent offshore oil spill accidents, industrial oily sewage, and the indiscriminate disposal of urban oily sewage have caused seri- ous impacts on the human living environment and health. The traditional oil-water separation methods not only cause easily environmental secondary pollution but also a waste of limited resources. Therefore, in this work, three-dimensional (3D) graphitic carbon sphere (GCS) foams (collectively referred hereafter as 3D foams) with a 3D porous structure, pore size distribution of 25-200 μm, and high porosity of 62vol% were prepared for oil adsorption via gel casting using GCS as the starting materials. The results indicate that the water contact angle (WCA) of the as-prepared 3D foams is 130°. The contents of GCS greatly influenced the hydrophobicity, WCA, and microstructure of the as-prepared samples. The adsorption capacities of the as-prepared 3D foams for paraffin oil, vegetable oil, and vacuum pump oil were approximately 12-15 g/g, which were 10 times that of GCS powder. The as-prepared foams are desirable characteristics of a good sorbent and could be widely used in oil spill accidents.

关键词： graphitic carbon spheres three dimensional foams gel casting oil adsorption

Advances and challenges in two-dimensional materials for oxygen evolution

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Nano Research 2022年第10期15卷 8714-8750页

作者： Tianmi Tang saisai li Jianrui Sun Zhenlu Wang Jingqi Guan Institute of Physical Chemistry College of ChemistryJilin UniversityChangchun 130021China School of Chemistry and life Science Changchun University of TechnologyChangchun 130012China

Oxygen evolution reaction(OER)plays an important role in many energy conversions and storage technologies,such as water splitting,rechargeable metal air batteries,renewable fuel cells,and electrocatalytic carbon dioxide reduction and nitrogen reduction,but its slow kinetics and high overpotential seriously affect the energy *** of high-performance and well-stocked OER catalysts is the key to the large-scale implementation of these energy-related ***-dimensional(2D)materials get a lot of attention as OER catalysts due to their large specific surface area,abundant active sites,and adjustable structures and ***,an overview is presented for the latest achievements in design and synthesis of 2D materials(including layered double hydroxides,metal-organic frameworks and their derivatives,covalent-organic frameworks,graphene,and black phosphorus)for the OER,emphasizing novel strategies(including metal/nonmetal doping,defect engineering,interface engineering,lattice strain,and fabrication of heterojunction)for achieving high electrocatalytic ***,the structure–function relationship is analyzed in detail to gain deeper insight into the reaction mechanism,which is crucial to rational design of more high-performance 2D materials for the ***,the remaining challenges to improve the OER performance of 2D electrocatalysts are put forward to indicate possible future development of 2D materials.

关键词： two-dimensional material oxygen evolution reaction layered double hydroxide metal-organic framework covalentorganic framework

杭州湾及其邻近海域夏季营养盐污染与富营养化评价

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海洋地质前沿 2024年第6期40卷 39-52页

作者：李赛赛裴绍峰赵俐红朱志强廖名稳段云莹山东科技大学地球科学与工程学院青岛266590 青岛海洋地质研究所生态地质与气候变化实验室青岛266237 中国地质调查局滨海湿地生物地质重点实验室青岛266237 青岛海洋科技中心海洋地质过程与环境功能实验室青岛266061

基于2022年夏季对杭州湾及其邻近海域的生态环境调查数据,采用单因子污染指数法、营养盐结构和限制性分析与富营养化状态指数法分别对该区表层营养盐和有机污染特征进行系统研究,对其富营养化状况进行系统评价,并通过Pearson相关性统计... 详细信息

基于2022年夏季对杭州湾及其邻近海域的生态环境调查数据,采用单因子污染指数法、营养盐结构和限制性分析与富营养化状态指数法分别对该区表层营养盐和有机污染特征进行系统研究,对其富营养化状况进行系统评价,并通过Pearson相关性统计分析初步探讨了营养盐污染对浮游植物生长的影响以及水域富营养化的控制因素。结果表明,该区氮(N)、磷(P)污染较为严重,溶解无机氮(DIN)和溶解无机磷(DIP)含量超过国家第Ⅲ类海水水质标准的站位数量占比分别为55%和80%;海水表层N/P和Si/P比值失衡,分别有20%和5%的站位水体浮游植物生长存在P和Si潜在限制。调查区叶绿素a(Chla)含量主要受水体透明度的影响,呈现东部高于西部、湾外高于湾内的空间分布特征;其中,湾外东部水域Chla含量较高,表明藻类细胞密度较大,存在暴发赤潮的风险。化学耗氧量(COD)的调查结果表明,该区总体有机污染并不显著,95%的站位符合国家第Ⅲ类水质标准。富营养化评价结果表明,该区90%的站位处于富营养化状态,其中40%的站位为重度富营养化;富营养化因子对E值的贡献排序为COD>DIN>DIP。初步研究表明,杭州湾及其邻近海域存在N、P营养盐污染,水体的富营养化问题值得关注并有待开展后续研究。

关键词：杭州湾营养盐富营养化浮游植物影响因素