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Computational study of laser fragmentation in liquid:Phase explosion,inverse Leidenfrost effect at the nanoscale,and evaporation in a nanobubble

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Science China(Physics,Mechanics & Astronomy) 2022年第7期65卷 99-114页

作者： Hao Huang leonid v.zhigilei School of Mechanical Science and Engineering Huazhong University of Science and TechnologyWuhan 430074China Department of Materials Science and Engineering University of VirginiaCharlottesville 22904-4745USA

Laser fragmentation in liquid is an effective and environment-friendly processing technique capable of yielding colloidal nanoparticles and atomic clusters with a narrow size distribution. The advancement of this technique can be facilitated by an improved understanding of processes that control the sizes, shapes, and structures of the produced nanoparticles. In this work, the dependence of the fragmentation mechanisms on the energy density deposited by the laser pulse is investigated in atomistic simulations performed for 20 nm Au nanoparticles irradiated in water by 10 ps laser pulses. The simulations reveal that the decrease in the absorbed laser energy leads to sequential transitions from the regime of “strong” phase explosion, when all products of an explosive phase decomposition of the irradiated nanoparticle are promptly injected into the water surrounding a nanobubble formed around the nanoparticle, to two distinct regimes of nanoparticle fragmentation leading to the formation of a large central nanoparticle surrounded by smaller satellite fragments. First, in the regime of “mild” phase explosion, the central nanoparticle is produced by the reflection of some of the hot metal droplets generated by the explosive decomposition of the nanoparticle from the boundary of the nanobubble. This reflection is attributed to the inverse Leidenfrost effect acting at the nanoscale. The reflected droplets converge in the center of the nanobubble and coalesce into a single droplet that solidifies shortly after the collapse of the nanobubble. Further decrease in the absorbed laser energy brings the irradiation conditions below the threshold for the phase explosion and results in the formation of a core-satellite structure of the fragmentation products through an interplay of the intense evaporation from the surface of the irradiated nanoparticle, evolution of the nanobubble, and condensation of the metal vapor into clusters and small satellite nanoparticles. The computationa

关键词： laser fragmentation in liquid molecular dynamics simulations phase explosion inverse Leidenfrost effect nanobubble nanoparticles

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Ultrashort pulse laser ablation in liquids:probing the first nanoseconds of underwater phase explosion

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Light(Science & Applications) 2022年第6期11卷 1005-1007页

作者： Chaobo Chen leonid v.zhigilei Department of Materials Science and Engineering University of Virginia395 McCormick RoadCharlottesvilleVA 22904-4745USA

The ultrafast pump-probe microscopy has shed new light on the complex dynamics of laser-induced explosive phase transformations and highlighted the importance of close integration of experimental,computational,and the... 详细信息

关键词： laser pump pulse

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Nonlinear interference in crystal superlattices

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Light(Science & Applications) 2020年第1期9卷 1239-1245页

作者： Anna v.Paterova leonid A.Krivitsky Institute of Materials Research and Engineering(IMRE) Agency for Science Technology and Research(A*STAR)138634 SingaporeSingapore

Nonlinear interferometers with correlated photons hold promise to advance optical characterization and metrology techniques by improving their performance and *** interferometers offer subshot noise phase sensitivity and enable measurements in detection-challenging regions using inexpensive and efficient *** sensitivity of nonlinear interferometers,defined by the ability to measure small shifts of interference fringes,can be significantly enhanced by using multiple nonlinear elements,or crystal ***,to date,experiments with more than two nonlinear elements have not been realized,thus hindering the potential of nonlinear ***,we build a nonlinear interferometer with up to five nonlinear elements,referred to as superlattices,in a highly stable and versatile *** study the modification of the interference pattern for different configurations of the superlattices and perform a proof-of-concept gas sensing experiment with enhanced *** approach offers a viable path towards broader adoption of nonlinear interferometers with correlated photons for imaging,interferometry,and spectroscopy.

关键词： spectroscopy nonlinear Nonlinear

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Dynamo saturation in rapidly rotating solar-type stars

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Research in Astronomy and Astrophysics 2015年第11期15卷 1801-1812页

作者： leonid L.Kitchatinov Serge v.Olemskoy Institute for Solar-Terrestrial Physics Pulkovo Astronomical Observatory

The magnetic activity of solar-type stars generally increases with stellar rotation rate. The increase, however, saturates for fast rotation. The Babcock-Leighton mechanism of stellar dynamos saturates as well when the mean tilt angle of active regions approaches ninety degrees. Saturation of magnetic activity may be a consequence of this property of the Babcock-Leighton mechanism. Stellar dynamo models with a tilt angle proportional to the rotation rate are constructed to probe this *** versions of the model- treating the tilt angles globally and using Joy＇s law for its latitude dependence- are considered. Both models show a saturation of dynamogenerated magnetic flux at high rotation rates. The model with latitude-dependent tilt angles also shows a change in dynamo regime in the saturation region. The new regime combines a cyclic dynamo at low latitudes with an（almost） steady polar dynamo.

关键词： saturation stellar latitude rotation rotating stars polar regime meridional consequence

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Basic formation mechanisms of Lake Doroninskoye soda water, East Siberia, Russia

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Acta Geochimica 2018年第4期37卷 546-558页

作者： Svetlana v. Borzenko leonid v. Zamana Larisa I. Usmanova Institute of Natural Resources Ecology and Cryology of Siberian Branch of Russian Academy of Sciences ChitaRussia 672049 Tomsk Department of the Trofimuk Institute of Petroleum-Gas Geology and Geophysics of Siberian Branch of the Russian Academy of Sciences Tomsk Russia 634050

The primary scientific goal of studying salt lakes is to better understand the formation of small continental- type hydrogeochemical systems. Many scientists have attributed the metamorphism of the chemical composition of salt lakes to the evaporative concentration of water. How- ever, the formation of soda water is inconsistent with this hypothesis. Thus, analyzing intrabasinal biochemical pro- cesses and water--rocks interactions during the evaporative concentration of water allows us to understand the major mechanisms of the formation and evolution of water com- positions. Therefore, the aim of this paper is to identify the key processes involved in the formation of the chemical composition of the water in Lake Doroninskoye. An analysis of the distribution of major components shows that Na＋, HCO3-, CO32-, and C1- are dominant in this water. High concentrations of these elements are the result of evaporative water concentration. Calcium, magnesium, and potassium are not accumulated because the water is saturated in min- erals containing these elements. The main barrier to the growth of the sulfate content of water is sulfate reduction. This process also contributes to the additional reproduction of carbon dioxide, which reacts with the products of the hydrolysis of aluminosilicates OH- to form HCO3- and CO32-, thus further contributing to the natural processes of soda formation.

关键词： Saline lake Sulfate reduction Thermodynamic equilibrium

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Argo floats revealing bimodality of large-scale mid-depth circulation in the North Atlantic

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Acta Oceanologica Sinica 2008年第2期27卷 1-10页

作者： CHU Peter C IvANOv leonid M MELNICHENKO Oleg v LI Rongfeng Department of Oceanography Naval Postgraduate School Monterey California USA International Pacific Research Center University of Hawaii at Manoa Hawaii USA Institute of Atmospheric Physics Chinese Academy of Sciences Beijing 100029 China

Analysis of Argo float trajectories at 1 000 m and temperature at 950 m in the North Atlantic between November 2003 and January 2005 demonstrates the existence of two different circulation modes with fast transition between them. Each mode has a pair of cyclonic - anticyclonic gyres. The difference is the location of the cyclonic gyre. The cyclonic gyre stretches from southeast to northwest in the first mode and from the southwest to the northeast in the second mode. The observed modes strongly affect the heat and salt transport in the North Atlantic. In particular, the second mode slows down the westward transport of the warm and saline water from the Mediterranean Sea.

关键词： Argo trajectory data Atlantic Ocean biomodality mid-depth circulation optimal spectral decomposition

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NIR emitting terephthalates(SmxDyyGd1-x-y)2(tph)3(H2O)4 for luminescence thermometry in the physiological range

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Journal of Rare Earths 2020年第5期38卷 492-497页

作者： Anastasia v.Orlova vladislava Yu.Kozhevnikova leonid S.Lepnev Alexander S.Goloveshkin Irina M.Le-Deigen valentina v.Utochnikova M.v.Lomonosov Moscow State University 1/3 Leninskye GoryMoscow119991Russian Federation P.N.Lebedev Physical Institute Leninsky prosp.531J9991MoscowRussian Federation A.N.Nesmeyanov Institute of Organoelement Compounds Russian Academy of SciencesVavilova St.28119991MoscowRussian Federation EvOLED Ltd. 1A-24 Puskina ielaRiga LV-1050Latvia

The first luminescence thermometer based on coordination compound of samarium and dysprosium is repo *** luminescence intensity and high signal resolution are reached thanks to the concentration quenching reduction due to the use of the trimetallic complexes of *** best thermometric properties in a wide temperature range among the studied systems are demonstrated by(Sm0.2Dy0.15Gd0.65)2(tph)3(H2O)*** sensitivity reaches 0.5%/K in visible range and 1.2%/K in NIR range at low temperatures and 0.5%/K and 0.8%/K in physiological range.

关键词： Luminescence Lanthanides Carboxylates Thermometry NIR range Rare earths

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Isotopic Composition of Dissolved Carbonates Meromictic Soda Lake Doroninskoe(Eastern Transbaikalia,Russia)

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Acta Geologica Sinica(English Edition) 2014年第S1期88卷 395-397页

作者： leonid v.ZAMANA Svetlana v.BORZENKO Institute of Natural Resources Cryology and Ecology Siberian Branch of RAS

1 Introduction Meromictic soda Lake Doroninskoe localized in the intermountain area,filled with continental sediments of the Mesozoic,in the upper basin of the river *** of its location are N51°14’42"E112°14’40",

关键词： Soda lake dissolved carbonates sulfate reduction hydrogen sulfide isotopic composition carbon oxygen

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Autoimmunity in acute ischemic stroke and the role of bloodbrain barrier: the dark side or the light one?

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Frontiers of Medicine 2019年第4期13卷 420-426页

作者： Nikolay v. Tsygan Alexandr P. Trashkov Igor v. Litvinenko viktoriya A. Yakovleva Alexandr v. Ryabtsev Andrey G. vasiliev leonid P. Churilov Department of Molecular and Radiation Biophysics B.P. Konstantinov Petersburg Nuclear Physics Institute Gatchina Leningrad Region 188300 Russian Federation Department of Nervous Diseases S.M. Kirov Military Medical Academy Saint Petersburg 194044 Russian Federation Department of Experimental Pharmacology I.M. Sechenov Institute of Evolutionary Physiology and Biochemistry Saint Petersburg 194223 Russian Federation Department of Pathological Physiology with the Course of Immunopathology Saint Petersburg State Pediatric Medical University Saint Petersburg Russian Federation Department of Pathology Laboratory of the Mosaic of Autoimmunity Saint Petersburg State University Saint Petersburg 199034 Russian Federation

This article presents a synopsis of the current data on the mechanisms of blood-brain barrier (BBB) alteration and autoimmune response in acute ischemic stroke. Most researchers confirm the relationship between the severity of immunobiochemical changes and clinical outcome of acute ischemic stroke. Ischemic stroke is accompanied by aseptic inflammation, which alters the brain tissue and exposes the co-stimulatory molecules of the immune system and the neuronal antigens. To date, BBB is not considered the border between the immune system and central nervous system, and the local immune subsystems are found within and behind the BBB. BBB disruption contributes to the leakage of brain autoantigens and induction of secondary autoimmune response to neuronal antigens and long-term inflammation. Glymphatic system function is altered and jeopardized both in hemorrhagic and ischemic stroke types. The receptors of innate immunity (toll-like receptor-2 and toll-like receptor-4) are also involved in acute ischemia-reperfusion injury. Immune response is related to the key processes of blood clotting and fibrinolysis. At the same time, the stroke-induced immune activation may promote reparation phenomena in the brain. Subsequent research on the reduction of the acute ischemic brain injury through the target regulation of the immune response is promising.

关键词： stroke blood-brain barrier autoimmunity innate immunity inflammation cell death

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Subcritical dynamo and hysteresis in a Babcock-Leighton type kinematic dynamo model

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Research in Astronomy and Astrophysics 2021年第10期21卷 250-256页

作者： vindya vashishth Bidya Binay Karak leonid Kitchatinov Department of Physics Indian Institute of Technology(BHU)Varanasi 221005India Institute of Solar-Terrestrial Physics SB RAS Lermontov Str.126A664033IrkutskRussia Pulkovo Astronomical Observatory Pulkovskoe Sh.65St.Petersberg196140Russia

In the Sun and Sun-like stars,it is believed that cycles of the large-scale magnetic field are produced due to the existence of differential rotation and helicity in the plasma flows in their convection zones(CZs).Hence,it is expected that for each star,there is a critical dynamo number for the operation of a large-scale *** a star slows down,it is expected that the large-scale dynamo ceases to operate above a critical rotation *** our study,we explore the possibility of the operation of the dynamo in the subcritical region using the Babcock–Leighton type kinematic dynamo *** some parameter regimes,we find that the dynamo shows hysteresis behavior,i.e.,two dynamo solutions are possible depending on the initial parameters—decaying solution if starting with weak field and strong oscillatory solution(subcritical dynamo)when starting with a strong ***,under large fluctuations in the dynamo parameter,the subcritical dynamo mode is unstable in some parameter ***,our study supports the possible existence of subcritical dynamo in some stars which was previously demonstrated in a mean-field dynamo model with distributedαand MHD turbulent dynamo simulations.

关键词： magnetic field Sun:activity Sun:magnetic fields stars:rotation stars:dynamo stars

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