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International Journal of Mining Science and Technology 2024年第5期34卷 699-712页

作者： Binwei Xia Yanmin zhou Xingguo Zhang lei zhou Zikun Ma State Key Laboratory of Coal Mine Disaster Dynamics and Control Chongqing UniversityChongqing 400044China School of Resources and Safety Engineering Chongqing UniversityChongqing 400044China

Ground hydraulic fracturing plays a crucial role in controlling the far-field hard roof,making it imperative to identify the most suitable target stratum for effective *** experiments are conducted based on engineering properties to simulate the gradual collapse of the roof during longwall top coal caving(LTCC).A numerical model is established using the material point method(MPM)and the strain-softening damage constitutive model according to the structure of the physical *** simulations are conducted to analyze the LTCC process under different hard roofs for ground hydraulic *** results show that ground hydraulic fracturing releases the energy and stress of the target stratum,resulting in a substantial lag in the fracturing of the overburden before collapse occurs in the hydraulic fracturing *** hydraulic fracturing of a low hard roof reduces the lag effect of hydraulic fractures,dissipates the energy consumed by the fracture of the hard roof,and reduces the abutment ***,it is advisable to prioritize the selection of the lower hard roof as the target stratum.

关键词： Target stratum selection Ground hydraulic fracturing Hard roof control Fracture network Material point method

Research progress in performance improvement strategies and sulfur conversion mechanisms of Li-S batteries based on Fe series nanomaterials

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Nano Research 2024年第9期17卷 8045-8067页

作者： Ziyang Huang Zhenghua Wang lei zhou Jun Pu Key Laboratory of Functional Molecular Solids(Ministry of Education) College of Chemistry and Materials ScienceAnhui Provincial Engineering Laboratory for New-Energy Vehicle Battery Energy-Storage MaterialsAnhui Normal UniversityWuhu 241000China School of Energy and Power Engineering Jiangsu UniversityZhenjiang 212013China Department of Electrical Engineering Eindhoven University of TechnologyEindhoven MB 5600The Netherlands

Lithium-sulfur(Li-S)batteries hold the potential to revolutionize energy storage due to the high theoretical capacity and energy ***,the commercialization process is seriously hindered by the rapid capacity decay and low utilization of sulfur,caused by the inevitable slow dynamics and the“shuttle effect”.The incorporation of metal-based electrocatalysts into sulfur cathodes shows promise in promoting the conversion of lithium polysulfides(LiPSs),reducing the“shuttle effect”,and enhancing cell kinetics and cycle *** these,Fe-based materials,characterized by environmental friendliness,low cost,abundant reserves,and high activity,are extensively used in sulfur cathode *** article reviews the advancements of Fe-based materials in enhancing Li-S batteries in recent *** from single/multi-component Fe-based metal compounds and single/bimetallic atoms,the influence of different Fe coordination environments on the conversion mechanism of LiPSs is *** is hoped that this review and the proposed prospects can further stimulate the development and application of the Fe element in Li-S batteries in the future.

关键词： Li-S batteries Fe-based nanomaterials shuttle effect reaction kinetics

Effect of internal structure of a batch-processing wet-etch reactor on fluid flow and heat transfer

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Chinese Journal of Chemical Engineering 2024年第8期72卷 177-186页

作者： Qinghang Deng Junqi Weng lei zhou Guanghua Ye Xinggui zhou State Key Laboratory of Chemical Engineering School of Chemical EngineeringEast China University of Science and TechnologyShanghai 200237China

Batch-processing wet-etch reactors are the key equipment widely used in chip fabrication,and their performance is largely affected by the internal *** work develops a three-dimensional computational fluid dynamics(CFD)model considering heat generation of wet-etching reactions to investigate the fluid flow and heat transfer in the wet-etch *** backflow is observed below and above the wafer region,as the flow resistance in this region is *** temperature on the upper part of a wafer is higher due to the accumulation of reaction heat,and the average temperature of the side wafer is highest as its convective heat transfer is *** the gap between wafer and reactor wall can force the etchant to flow in the wafer region and then facilitate the convective heat transfer,leading to better within-wafer and wafer-to-wafer etch *** inlet angle of 60°balances fluid by-pass and mechanical energy loss,and it yields the best temperature and etch *** batch with 25wafers has much wider flow channels and much lower flow resistance compared with that with 50wafers,and thus it shows better temperature and etch *** results and the CFD model should serve to guide the optimal design of batch-processing wet-etch reactors.

关键词： Wet-etch reactor Batch-processing Computational fluid dynamics Reaction heat Internal structure Etch uniformity

Accurate atomic scanning transmission electron microscopy analysis enabled by deep learning

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Nano Research 2024年第4期17卷 2971-2980页

作者： Tianshu Chu lei zhou Bowei Zhang Fu-Zhen Xuan Shanghai Key Laboratory of Intelligent Sensing and Detection Technology East China University of Science and TechnologyShanghai 200237China School of Mechanical and Power Engineering East China University of Science and TechnologyShanghai 200237China Key Laboratory of Pressure Systems and Safety of Ministry of Education East China University of Science and TechnologyShanghai 200237China

Currently,the machine learning(ML)-based scanning transmission electron microscopy(STEM)analysis is limited in the simulative stage,its application in experimental STEM is needed but ***,we built up a universal model to analyze the vacancy defects and single atoms accurately and rapidly in experimental STEM images using a full convolution *** our model,the unavoidable interference factors of noise,aberration,and carbon contamination were fully considered during the training,which were difficult to be considered in the *** toward the simultaneous identification of various vacancy types and low-contrast single atoms in the low-quality STEM images,our model showed rapid process speed(45 images per second)and high accuracy(>95%).This work represents an improvement in experimental STEM image analysis by ML.

关键词： deep learning low-dimensional materials atomic defects single atoms

Data-driven rational design of single-atom materials for hydrogen evolution and sensing

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Nano Research 2024年第4期17卷 3352-3358页

作者： lei zhou Pengfei Tian Bowei Zhang Fu-Zhen Xuan Shanghai Key Laboratory of Intelligent Sensing and Detection Technology East China University of Science and TechnologyShanghai 200237China School of Mechanical and Power Engineering East China University of Science and TechnologyShanghai 200237China Key Laboratory of Pressure Systems and Safety of Ministry of Education East China University of Science and TechnologyShanghai 200237China

Herein we proposed a data-driven high-throughput principle to screen high-performance single-atom materials for hydrogen evolution reaction(HER)and hydrogen sensing by combing the theoretical computations and a topology-based multi-scale convolution kernel machine learning *** the rational training by 25 groups of data and prediction of all 168 groups of single-atom materials for HER and sensing,respectively,a high prediction accuracy(>0.931 R^(2) score)was achieved by our *** show that the promising HER catalysts include Pt atoms in C_(4) and Sc atoms in C_(1)N_(3) coordination ***,Y atoms in C_(4) coordination environment and Cd atoms in C_(2)N_(2)-ortho coordination environment were predicted with great potential as hydrogen sensing *** method provides a way to accelerate the discovery of innovative materials by avoiding the time-consuming empirical principles in experiments.

关键词： machine learning single-atom materials sensing hydrogen evolution

Polymer ionogels and their application in flexible ionic devices

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SmartMat 2024年第2期5卷 4-42页

作者： Jinqiao Wen lei zhou Tengling Ye Department of Applied Chemistry School of Chemistry and Chemical EngineeringHarbin Institute of TechnologyHarbinChina State Key Laboratory of Luminescent Materials and Devices South China University of TechnologyGuangzhouChina

Polymer ionogel(PIG)is a new type of flexible,stretchable,and ion-conductive material,which generally consists of two components(polymer matrix materials and ionic liquids/deep eutectic solvents).More and more attention has been received owing to its excellent properties,such as nonvolatility,good ionic conductivity,excellent thermal stability,high electrochemical stability,and *** this review,the latest research and developments of PIGs are comprehensively reviewed according to different polymer ***,the development of novel structural designs,preparation methods,basic properties,and their advantages are respectively ***,the typical applications of PIGs in flexible ionic skin,flexible electrochromic devices,flexible actuators,and flexible power supplies are *** novel working mechanism,device structure design strategies,and the unique functions of the PIG-based flexible ionic devices are briefly ***,the perspectives on the current challenges and future directions of PIGs and their application are discussed.

关键词： electrochromism device flexible ionic devices flexible ionic skin ionic liquid ionogel

Current progress in glass-based nanochannels

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International Journal of Smart and Nano Materials 2024年第1期15卷 222-237页

作者： Yixin Ling Xuelian Yang lei zhou Zhenkang lei Yaqi Hou Xu Hou state Key Laboratory of Physical Chemistry of Solid Surfaces and Department of ChemistryCollege of Chemistry and Chemical EngineeringXiamen UniversityXiamenChina Institute of Flexible Electronics(IFE Future Technologies)Xiamen UniversityXiamenChina Institute of Artificial Intelligence Xiamen UniversityXiamenChina Department of Physics Research Institute for Biomimetics and Soft MatterFujian Provincial Key Laboratory for Soft Materials ResearchJiujiang Research InstituteCollege of Physical Science and TechnologyXiamen UniversityXiamenChina

Glass-based nanochannels have become powerful tools for chemi-cal and biological sensing due to their advantages of easy prepara-tion,flexible modification,and high ***,research on ion transport behaviors in glass-based nanochannels and their applications in nanofluidic iontronics has gradually become a focus,including various ion transport behaviors such as resistive-pulse,ion rectification,ionic current memory,*** this review,we summarize the progress of manufacturing methods for glass-based nanochannels and discuss several typical ion transport behaviors of glass-based nanochannels,as well as the main application scenarios of glass-based nanochannels in terms of biosensing,detection,and neuromorphic *** enormous assistance of artificial intel-ligence in the standardized manufacturing process of glass-based nanochannels was anticipated,and the potential development of glass-based nanochannels in achieving neuromorphic functions was expected.

关键词： Glass-based nanochannels biosensing ionic rectification ionic memristive effect nanofluidic neuromorphic functions

The growth ofβphase in Mg-Gd-Y-Ni alloy by experimental and first-principles study

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Journal of Magnesium and Alloys 2024年第2期12卷 506-515页

作者： Yiqiang Hao lei zhou Zhiqing Chen Zhixian Zhao Bin Chen School of Materials Science and Engineering Shanghai Jiao Tong University800 Dongchuan RoadShanghai200240China

The paper reports on the atomic investigation aboutβphase in Mg_(96)Gd_(2)Y_(1)Ni_(1) alloy by using the first-principles study and the high-angle annular dark-field scanning transmission electron microscope(HAADF-STEM)corrected by atomic *** using HAADF-STEM,the rectangularβphases were observed in the underage and peak aging stages in Mg_(96)Gd_(2)Y_(1)Ni_(1) ***βphase could be precipitated from the previously precipitatedβphase,and theβphase grew in steps when it was precipitated.A special transition structure of three atomic layer thicknesses was first observed at the edge of theβphase and the structure of this interface is probably as theβ/Mg_(1) interface for the analysis of thermodynamic characterization and electronic ***β'phase and theβ_(H) structure were precipitated only at the edge of the length directions of theβ***β'phase continues to grow into aβphase directly without the formation ofβ_(1) phase,resulting in an increase in the length of theβphase,which is discovered for the first time.

关键词： HAADF-STEM First-principles study Mg-Gd-Y-Ni alloy βphase Growth Interface

The Implications of Artificial Intelligence on Infection Prevention and Control: Current Progress and Future Perspectives

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China CDC weekly 2024年第35期6卷 901-904页

作者： Lin Yang Shuya Lu lei zhou School of Nursing The Hong Kong Polytechnic UniversityHong Kong Special Administrative RegionChina Chinese Center for Disease Control and Prevention BeijingChina

The rapid advancement of artificial intelligence(AI)has significantly impacted infection prevention and control,particularly amid the coronavirus disease 2019(COVID-19)pandemic(1).AI techniques such as machine learning(ML),deep learning,and natural language processing(NLP)have successfully transformed infection prevention and control strategies(1).These technologies have enhanced our understanding of infectious diseases,facilitated disease transmission prediction,and improved public health emergency responses(2).

关键词： has such prevention

Controlled fluorescent switch based on a cation grease/brake rotor system of pillar[5]arene

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Chinese Chemical Letters 2024年第3期35卷 5-7页

作者： Wei-lei zhou Siwei Wang Yong Chen College of Chemistry and Material Science Inner Mongolia Key Laboratory of Chemistry for Nature Products and Synthesis for Functional MoleculesInnovation Team of Optical Functional Molecular DevicesInner Mongolia Minzu UniversityTongliao 028000China College of Chemistry Nankai UniversityTianjin 300071China

In recent years,molecular shuttles,motors,pumps,and elevators,*** specifically respond external physical or chemical stimuli including light,temperature,pH,redox,solvent and chemical additive to change the structure a... 详细信息

关键词： additive system showing