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Arbuscular mycorrhizal fungi regulate plant mineral nutrient uptake and partitioning in iron ore tailings undergoing eco-engineered pedogenesis

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Pedosphere 2024年第2期34卷 385-398页

作者： Zhen LI Songlin WU Yunjia LIU Qing YI Merinda HALL Narottam SAHA Junjian WANG Yuanfang huang Longbin huang college of Land Science and Technology China Agricultural UniversityBeijing 100193China centre for Mined Land Rehabilitation Sustainable Minerals InstituteThe University of QueenslandBrisbaneQLD 4072Australia Guangdong Provincial Key Laboratory of Soil and Groundwater Pollution control School of Environmental Science and EngineeringSouthern University of Science and TechnologyShenzhen 518055China

Excess available K and Fe in Fe ore tailings with organic matter amendment and water-deficiencies may restrain plant colonization and growth,which hinders the formation of eco-engineered soil from these tailings for sustainable and cost-effective mine site *** mycorrhizal(AM)fungi are widely demonstrated to assist plant growth under various unfavorable ***,it is still unclear whether AM symbiosis in tailings amended with different types of plant biomass and under different water conditions could overcome the surplus K and Fe stress for plants in Fe ore tailings,and if so,by what ***,host plants(Sorghum *** ***),either colonized or noncolonized by the AM fungi(Glomus spp.),were cultivated in lucerne hay(LH,c:N ratio of 18)-or sugarcane mulch(SM,c:N ratio of 78)-amended Fe ore tailings under well-watered(55%water-holding capacity(WHc)of tailings)or water-deficient(30%WHc of tailings)*** mycorrhizal colonization,plant growth,and mineral elemental uptake and partitioning were *** indicated that AM fungal colonization improved plant growth in tailings amended with plant biomass under water-deficient *** mycorrhizal fungal colonization enhanced plant mineral element uptake,especially P,both in the LH-and SM-amended tailings regardless of water ***,AM symbiosis development restrained the translocation of excess elements(i.e.,K and Fe)from plant roots to shoots,thereby relieving their *** AM fungal roles in P uptake and excess elemental partitioning were greater in LH-amended tailings than in SM-amended *** deficiency weakened AM fungal colonization and functions in terms of mineral element uptake and *** findings highlighted the vital role AM fungi played in regulating plant growth and nutrition status in Fe ore tailings technosol,providing an important basis for involvement of AM fungi in the eco-engineered pedo

关键词： Fe stress fungal symbiosis K stress mine site rehabilitation mycorrhizal colonization plant biomass amendment plant nutrition water deficiency

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Weakly Polarized Organic cation-Modified Hydrated Vanadium Oxides for High-Energy Efficiency Aqueous Zinc-Ion Batteries

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Nano-Micro Letters 2024年第7期16卷 169-186页

作者： Xiaoxiao Jia chaofeng Liu Zhi Wang Di huang Guozhong cao Department of Materials Science and Engineering University of WashingtonSeattleWA 98195USA School of Materials Science and Engineering Tongji UniversityShanghai 201804People’s Republic of China

Vanadium oxides,par-ticularly hydrated forms like V_(2)O_(5)·nH_(2)O(VOH),stand out as promising cathode candidates for aqueous zinc ion batteries due to their adjustable layered structure,unique electronic characteristics,and high theoretical ***,challenges such as vanadium dissolution,sluggish Zn^(2+)diffusion kinetics,and low operating voltage still hinder their direct *** this study,we present a novel vanadium oxide([c_(6)H_(6)N(cH_(3))_(3)]_(1.08)V_(8)O_(20)·0.06H_(2)O,TMPA-VOH),developed by pre-inserting trimethylphenylammonium(TMPA+)cations into *** incorporation of weakly polarized organic cations capitalizes on both ionic pre-intercalation and molecular pre-intercalation effects,resulting in a phase and morphology transition,an expansion of the interlayer distance,extrusion of weakly bonded interlayer water,and a substantial increase in V^(4+)*** modifications synergistically reduce the electrostatic interactions between Zn^(2+)and the V-O lattice,enhancing structural stability and reaction kinetics during *** a result,TMPA-VOH achieves an elevated open circuit voltage and operation voltage,exhibits a large specific capacity(451 mAh g^(-1)at 0.1 A g^(-1))coupled with high energy efficiency(89%),the significantly-reduced battery polarization,and outstanding rate capability and cycling *** concept introduced in this study holds great promise for the development of high-performance oxide-based energy storage materials.

关键词： Zinc-ion battery Vanadium oxide V_(2)O_(5)·nH_(2)O Pre-intercalation Interlayer engineering

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conversion of Lignin into Porous carbons for High-Performance Supercapacitors via Spray Drying and KOH Activation: Structure-Properties Relationship and Reaction Mechanism

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Journal of Renewable Materials 2024年第7期12卷 1207-1218页

作者： Shihao Feng Qin Ouyang Jing huang Xilin Zhang Zhongjun Ma Kun Liang Qing huang Zhejiang Key Laboratory of Data-Driven High-Safety Energy Materials and Applications Ningbo Key Laboratory of Special Energy Materials and ChemistryNingbo Institute of Materials Technology and EngineeringChinese Academy of SciencesNingbo315201China Engineering Laboratory of Advanced Energy Materials Qianwan Institute of CNITECHNingbo315336China School of Physics Henan Normal UniversityXinxiang453007China School of Environment Henan Normal UniversityXinxiang453007China

Lignin-derived porous carbons have emerged as promising electrode materials for ***,the challenge remains in designing and controlling their structure to achieve ideal electrochemical performance due to the complex molecular structure of lignin and its intricate chemical reactions during the activation *** this study,three porous carbons were synthesized from lignin by spray drying and chemical activation with vary-ing KOH *** speciﬁc surface area and structural order of the prepared porous carbon continued to increase with the increase of the KOH ***-mass spectrometry(TG-MS)was employed to track the molecular fragments generated during the pyrolysis of KOH-activated lignin,and the mechanism of the thermochemical conversion was *** the thermochemical conversion of lignin,KOH facili-tated the removal of H2 and cO,leading to the formation of not only more micropores and mesopores,but also more ordered carbon *** pore structure exhibited a greater impact than the carbon structure on the electrochemical performance of porous *** optimized porous carbon exhibited a capacitance of 256 F g-1 at a current density of 0.2 A g-1,making it an ideal electrode material for high-performance supercapacitors.

关键词： Lignin porous carbon KOH activation mechanism supercapacitor

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Realization of nonreciprocal acoustic energy transfer using an asymmetric strong nonlinear vibroacoustic system

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International Journal of Mechanical System Dynamics 2024年第1期4卷 99-114页

作者： Jiangming Jin Jingxiao huang Yuepeng Xiao Sound and Vibration Laboratory College of Mechanical EngineeringZhejiang University of TechnologyHangzhouChina

In this paper,an asymmetric vibroacoustic system that can passively realize nonreciprocal transmission of acoustic energy is *** experimental system consists of a waveguide,a strongly nonlinear membrane,and three acoustic cavities with different *** theoretical modeling of the system is verified by experiments,and parametric analysis is also carried *** intensive studies reveal the nonreciprocal transmission of acoustic energy in this prototype *** forward excitation,internal resonance between the two nonlinear normal modes of the vibroacoustic system occurs,and acoustic energy is irreversibly transferred from the waveguide to the nonlinear ***,under backward excitation,there is no internal resonance in the *** spectra and wavelet analysis are used to highlight the mechanism of nonreciprocal transfer of acoustic ***,nearly unidirectional(preferential)transmission of acoustic energy transfer is shown by this *** nonreciprocal acoustic energy transfer method illustrated in this paper provides a new way to design the odd acoustic element.

关键词： vibroacoustic system acoustic nonreciprocity nonlinear normal mode transient resonance capture

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Diamond-Like carbon Depositing on the Surface of Polylactide Membrane for Prevention of Adhesion Formation During Tendon Repair

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Nano-Micro Letters 2024年第9期16卷 478-499页

作者： Yao Xiao Zaijin Tao Yufeng Ju Xiaolu huang Xinshu Zhang Xiaonan Liu Pavel A.Volotovski chao huang Hongqi chen Yaozhong Zhang Shen Liu Department of Orthopaedics Shanghai Jiao Tong University School of Medicine Affiliated Sixth People’s Hospital600 Yishan RdShanghai 200233People’s Republic of China Shanghai Tongji Hospital 389 Xincun RdShanghai 200065People’s Republic of China Key Laboratory for Thin Film and Microfabrication of Ministry of Education Research Institute of Micro/Nano Science and TechnologyShanghai Jiao Tong UniversityShanghai 200240People’s Republic of China Orthopedic Trauma Department Belarus Republic Scientific and Practical Center for Traumatology and OrthopedicsKizhevatova str.60/4220024 MinskBelarus Shanghai Haohai Biological Technology Limited Liability company 1386 Hongqiao RdShanghai 200336People’s Republic of China Department of General Surgery Shanghai Jiao Tong University School of Medicine Affiliated Sixth People’s Hospital600 Yishan RdShanghai 200233People’s Republic of China Shanghai Key Laboratory for High Temperature Materials and Precision Forming School of Materials Science and EngineeringShanghai Jiao Tong UniversityShanghai 200240People’s Republic of China

Post-traumatic peritendinous adhesion presents a significant challenge in clinical *** study proposes the use of diamond-like carbon(DLc)deposited on polylactic acid(PLA)membranes as a biophysical mechanism for anti-adhesion barrier to encase ruptured tendons in tendon-injured *** results indicate that PLA/DLc composite membrane exhibits more efficient anti-adhesion effect than PLA membrane,with histological score decreasing from 3.12±0.27 to 2.20±0.22 and anti-adhesion effectiveness increasing from 21.61%to 44.72%.Mechanistically,the abundant c=O bond functional groups on the surface of DLc can reduce reactive oxygen species level effectively;thus,the phosphorylation of NF-κB and M1 polarization of macrophages are ***,excessive inflammatory response augmented by M1 macrophage-originated cytokines including interleukin-6(IL-6),interleukin-1β(IL-1β),and tumor necrosis factor-α(TNF-α)is largely *** biocompatibility evaluation,PLA/DLc membrane is slowly absorbed within tissue and displays prolonged barrier effects compared to traditional PLA *** studies show the DLc depositing decelerates the release of degradation product lactic acid and its induction of macrophage M2 polarization by interfering esterase and PLA ester bonds,which further delays the fibrosis *** was found that the PLA/DLc membrane possess an efficient biophysical mechanism for treatment of peritendinous adhesion.

关键词： Diamond-like carbon Reactive oxygen species scavenging Foreign body reaction Biodegradation Antioxidant Peritendinous adhesion

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Estimation of unfrozen water content of saturated sandstones using nuclear magnetic resonance, mercury intrusion porosimetry, and ultrasonic tests

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Journal of Rock Mechanics and Geotechnical Engineering 2024年第9期16卷 3465-3484页

作者： Fei Liu Shibing huang Gang Liu Shilin Yu School of Resources and Environmental Engineering Wuhan University of Science and TechnologyWuhan430081China Hubei Key Laboratory for Efficient Utilization and Agglomeration of Metallurgic Mineral Resources Wuhan University of Science and TechnologyWuhan430081China

The unfrozenwater content(UWc)is a crucial parameter that affects the strength and thermal properties of rocks in relation to engineering construction and geological disasters in cold *** this study,three different methods were employed to test and estimate the UWc of saturated sandstones,including nuclear magnetic resonance(NMR),mercury intrusion porosimetry(MIP),and ultrasonic *** NMR method enabled the direct measurement of the UWc of sandstones using the free induction decay(FID).The MIP method was used to analyze the pore structures of sandstones,with the UWc subsequently calculated based on pore ice ***,the MIP test constituted an indirect measurement ***,a correlation was established between the P-wave velocity and the UWc of these sandstones based on the mixture theory,which could be employed to estimate the UWc as an empirical *** methods demonstrated that the UWc initially exhibited a rapid decrease from 0c to5c and then generally became constant beyond20***,these test methods had different *** NMR method was used to directly and accurately calculate the UWc in the ***,the cost and complexity of NMR equipment have precluded its use in the *** UWc can be effectively estimated by the MIP test,but the estimation accuracy is influenced by the ice crystallization process and the pore size *** P-wave velocity has been demonstrated to be a straightforward and practical empirical parameter and was utilized to estimate the UWc based on the mixture *** method may be more suitable in the *** methods confirmed the existence of a hysteresis phenomenon in the freezing-thawing *** average hysteresis coefficient was approximately 0.538,thus validating the GibbseThomson *** study not only presents alternative methodologies for estimating the UWc of saturated sandstones but also contribute to our understanding of the freezin

关键词： Unfrozen water content(UWc) Nuclear magnetic resonance(NMR) Mercury intrusion porosimetry(MIP) Pore structures P-wave velocity Sandstone

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copper catalyzed Enantioconvergent Nucleophilic Substitutions

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chinese Journal of chemistry 2024年第10期42卷 1161-1174页

作者： chunxi huang Zilong Wan Aoping Zhu caiyou chen college of chemistry and Molecular Sciences Wuhan UniversityWuhanHubei 430072China Ministry of Education Key Laboratory for the Synthesis and Application of Organic Functional Molecules and college of chemistry and chemical Engineering Hubei UniversityWuhanHubei 430062China

As a versatile earth-abundant transition metal,cu has long been widely applied in the c—c and c—X bond forming *** for now,low-valent cu(Ⅰ)is known to reduce the redox active electrophiles via an SET pathway to give the corresponding radical and cu(Ⅱ)*** resulting cu(Ⅱ)species can interact with the radical via the out-sphere pathway,affording the coupling ***,cu(Ⅱ)can trap the radical through the inner-sphere process to generate cu(Ⅲ)species and then realize challenging bond formations due to the facile reductive elimination of cu(Ⅲ)*** copper catalysis has been widely applied in arylations of various nucleophiles,copper-catalyzed enantioconvergent nucleophilic substitutions of racemic alkyl electrophiles have been less explored,likely due to the difficulties in overcoming the reduction potential of alkyl electrophiles,elimination of side reactions,and enantiomeric *** order to overcome the high reduction potential of alkyl electrophiles,the photo-induced strategy has been developed under mild *** alternative strategy with new anionic tridentate ligands has also been reported in this *** review summarizes recent developments in copper-catalyzed enantioconvergent nucleophilic substitutions of alkyl electrophiles by various nucleophiles to realize c—N,c—c,c—B,c—P and c—O bond formations and their brief mechanistic studies.

关键词： Enantioconvergent Nucleophilic substitution copper Radical reactions Photocatalysis Asymmetric catalysis

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“co-coordination force”assisted rigid-flexible coupling crystalline polymer for high-performance aqueous zinc-organic batteries

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chinese chemical Letters 2024年第9期35卷 501-506页

作者： Jun Guo Zhenbang Zhuang Wanqiang Liu Gang huang School of Materials Science and Engineering Changchun University of Science and TechnologyChangchun 130022China State Key Laboratory of Rare Earth Resource Utilization Changchun Institute of Applied ChemistryChinese Academy of SciencesChangchun 130022China Key Laboratory of Automobile Materials Ministry of EducationDepartment of Materials Science and EngineeringJilin UniversityChangchun 130022China

Organic electrode materials(OEMs)have attracted substantial attention for aqueous zinc-ion batteries(AZIBs)due to their advantages in relieving resource and environmental ***,the potential of OEMs is plagued by their low achievable capacity and high ***,we have proposed a new concept of“co-coordination force”and designed a rigid-flexible coupling crystalline polymer that can overcome the abovementioned *** obtained crystalline polymer(BQSPNs)with multiredox centres makes the BQSPNs exist intermolecular hydrogen bonds(HB)among-c=O,-c=N,and-NH and consequently exhibits transverse two-dimensional arrays and longitudinalπ-πstacking ***,in-situ FTIR,Raman,variable temperature FTIR spectra,and 2D nuclear overhauser effect spectroscopy(NOESY)well capture the existence and evolution process of HB during the electrochemistry reaction process of BQSPNs,uncovering the effect of HB in stabilizing the structure and promoting the reaction *** a result,the BQSPNs with rationally designed“co-coordination force”deliver a high capacity of 459.6 m Ah/g and a stable cycling lifetime for more than 100,000 cycles at 10 A/g in *** results disclose the HB effect and provide a brand-new strategy for high-performance OEMs design.

关键词： co-coordination force crystalline polymer Hydrogen bonds Organic electrode materials Aqueous zinc-ion batteries

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Dynamic Multi-Physics Behaviors and Performance Loss of cylindrical Batteries Upon Low-Velocity Impact Loading

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Energy & Environmental Materials 2024年第6期7卷 184-192页

作者： Qingdan huang Yang Bai Han Luo Yikai Jia chao Zhang School of civil Aviation Northwestern Polytechnical UniversityXi’an 710072China Key Laboratory on the Impact Protection and Safety Assessment of civil Aviation Vehicle Taicang 215400China School of Aeronautics Northwestern Polytechnical UniversityXi’an 710072China EVE Energy co. Ltd.Huizhou 516006C

In challenging operational environments,Lithium-ion batteries(LIBs)inevitably experience mechanical stresses,including impacts and extrusion,which can lead to battery damage,failure,and even the occurrence of fire and explosion ***,it is imperative to investigate the safety performance of LIBs under mechanical *** study is grounded in a more realistic coupling scenario consisting of electrochemical cycling and low-velocity *** systematically and experimentally uncovered the mechanical,electrochemical,and thermal responses,damage behavior,and corresponding mechanisms under various *** study demonstrates that higher impact energy results in increased structural stiffness,maximum temperature,and maximum voltage ***,heightened impact energy significantly influences the electrical resistance parameters within the internal *** also examined the effects of State of charge(SOc)and *** methodology and experimental findings will offer insights for enhancing the safety design,conducting risk assessments,and enabling the cascading utilization of energy storage systems based on LIBs.

关键词： cycling performance damaged battery lithium-ion battery low-velocity impact mechanical safety

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Fe-Induced Electronic Transfer and Structural Evolution of Lotus Pod-Like coNiFePx@P,N-c Heterostructure for Sustainable Oxygen Evolution

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Energy & Environmental Materials 2024年第3期7卷 186-193页

作者： Xiaojun Zeng Qingqing Zhang chulong Jin Hui huang Yanfeng Gao Advanced ceramic Materials Research Institute School of Materials Science and EngineeringJingdezhen Ceramic University Singapore Institute of Technology School of Materials Science and Engineering Shanghai University

Transition metal phosphides with metallic properties are a promising candidate for electrocatalytic water oxidation,and developing highly active and stable metal phosphide-based oxygen evolution reaction catalysts is still ***,we present a facile ion exchange and phosphating processes to transform intestine-like coNiPx@P,N-c into lotus pod-like coNiFePx@P,N-c heterostructure in which numerous P,N-codoped carboncoated coNiFePxnanoparticles tightly anchors on the 2D carbon ***,the as-prepared coNiFePx@P,N-c enables a core-shell structure,high specific surface area,and hierarchical pore structure,which present abundant heterointerfaces and fully exposed active ***,the incorporation of Fe can also induce electron transfer in coNiPx@P,IM-c,thereby promoting the oxygen evolution ***,coNiFePx@P,IM-c delivers a low overpotential of 278 mV （vs RHE） at a current density of10 mA cm-1and inherits excellent long-term stability with no observable current density decay after 30 h of chronoamperometry *** work not only highlights heteroatom induction to tune the electronic structure but also provides a facile approach for developing advanced and stable oxygen evolution reaction electrocatalysts with abundant heterointerfaces.

关键词： electronic transfer Fe exchange multi-metal phosphides OER electrocatalysts structural evolution

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